arXiv subjects

Chao-Xing Liu

Publications and source records attributed to Chao-Xing Liu.

At least 19 recordsLinked to original sources

arXiv2026

Lifshitz-Kosevich Theory of Anomalous Landau Levels in Topological Flat Bands

In conventional metals, quantum oscillations arise from Landau quantization of Fermi-surface cyclotron orbits, whose dynamics are governed by the Fermi velocity and cyclotron effective mass within Lifshitz-Kosevich (LK) theory. A perfectly flat band, by contrast, has vanishing group velocity, which would naively imply an infinite cyclotron mass and complete thermal suppression of quantum oscillations. Yet topological flat bands can support anomalous Landau levels (LLs) whose finite-field spacing is generated by quantum geometry rather than band curvature, allowing quantum oscillations to persist. This work addresses how such anomalous flat-band LLs behave within the LK framework and whether their thermal damping can reveal quantum geometric information. Using a minimal model with exactly flat topological bands, we derive an LK theory for these anomalous LLs and analyze fixed-density magnetization oscillations. The resulting oscillations exhibit a finite LK effective mass that is substantially larger than the normal-band value and possesses a strong magnetic-field dependence. In the weak-field limit, this anomalous mass reflects the quantum geometric origin of the LL spacing and scales inversely with both the magnetic field and the trace of the quantum metric. Thus, thermal damping of flat-band quantum oscillations directly measures the quantum metric, establishing quantum oscillations as a probe to flat-band quantum geometry.

cond-mat.mes-hall↗

arXiv2026

Engineering Tunable Kagome Moiré Superlattices in Twisted Transition Metal Dichalcogenides

Kagome systems are an ideal platform for exploring strongly correlated phases due to their unique electronic structure and geometric frustration. While recent solid-state realizations have uncovered a wealth of correlated states, they suffer from key limitations, including limited tunability of carrier density and interaction strength. Here, we propose an experimentally viable scheme to realize a breathing kagome moiré superlattice using a twisted trilayer of transition metal dichalcogenides (TMDs). By twisting the top and bottom layers relative to the middle by small angles $θ$ and $2θ$, respectively, we generate a kagome-like moiré potential on the central layer. Continuum model calculations reveal isolated kagome bands featuring flat bands, Dirac points with tunable gaps, and van Hove singularities. Crucially, this platform offers unprecedented control over band structure, carrier density, and interactions, achievable via twist angle and electrostatic gating. Our work opens a new route to realizing clean, tunable kagome metals and provides a versatile platform for studying strongly correlated and topological phenomena.

cond-mat.mes-hall↗

arXiv2026

Residual orbital magnetization governs the anomalous Hall effect in altermagnets

In altermagnets that exhibit anomalous Hall effect, the small remanent magnetization exists but has been treated as too small to be relevant to the Hall response. In this work, we point out that this dismissal is incomplete because the generalized Středa relation ties the intrinsic anomalous Hall conductivity ($σ_{xy}$) to the orbital magnetization ($M_z$, the topological component from the modern orbital magnetization) by $σ_{xy}=-e\frac{\partial M_z}{\partial μ}$. We reveal a microscopic mechanism to generate net orbital moment from the interplay of local crystal field and spin-orbit coupling for MnTe-type altermagnets, in which the magnetic anisotropy generates weak net magnetization without invoking exchange between neighboring spins (e.g., Dzyaloshinskii-Moriya interaction). Our work indicates that residual orbital and spin magnetization is an intrinsic thermodynamic property that governs anomalous transport in unconventional antiferromagnets, including altermagnets and noncollinear antiferromagnets.

cond-mat.mes-hall↗

arXiv2026

Perfect Nonreciprocal Axion-polaritons

Dynamical axion describes a massive axion quasiparticle that arises from fluctuations of the magnetic order parameter. These fluctuations couple to electromagnetic fields, forming axion-polaritons -- collective modes that are physically magnon-polaritons. We show that under appropriate static external electric and magnetic fields, axion-polaritons acquire a nonreciprocal dispersion, $ω(\textbf{k}) \neq ω(-\textbf{k})$, arising intrinsically from direction-dependent axion-photon coupling. Strikingly, we identify a regime of \textit{perfect nonreciprocity} in which the photon propagating in one direction is completely decoupled from the axion while the counter-propagating photon hybridizes strongly. Furthermore, the nonreciprocal dispersion manifests as an optical isolator -- a device transmitting light preferentially in one direction. Our results establish nonreciprocal axion-polaritons as a powerful probe of axion quasiparticles and suggest experimentally accessible routes for their detection.

cond-mat.mes-hall↗

arXiv2026

Imaging Surface Magnetization in Altermagnetic MnTe Films

Altermagnets with pronounced spin-splitting band structure, unconventional magnetic and crystal symmetries, and exotic magneto-transport properties have received immense interest in cutting-edge spintronics, materials science, and condensed matter physics research. Microscopic imaging of spontaneous magnetic domains and phases in altermagnets constitutes an important step for investigating their underlying material properties, mechanisms, and spin behaviors. Taking advantage of scanning-probe quantum microscopy, here we report nanoscale quantum sensing of a prototypical altermagnet candidate $α$-MnTe. We visualize evanescent magnetization and the associated magnetic domains in epitaxial MnTe films, which allows external magnetic fields to control the intrinsic altermagnetic order and configurations. By evaluating a series of MnTe films with different thicknesses down to the atomic scale, we further present evidence for the interfacial origin of the observed weak magnetization and show its correlation with the anomalous Hall effect in MnTe film. Our results advance the current understanding of emergent altermagnetism, providing insights into future material design of altermagnet-integrated spintronic devices.

cond-mat.mtrl-sci↗

arXiv2026

Phonon circular birefringence and polarization-filter in Magnetic Topological Insulators

The surface phonon Hall viscosity (PHV)-an acoustic analog of axion electrodynamics-emerges from the strain response of magnetic topological insulators and gives rise to novel acoustic phenomena. In this work, we propose a previously unexplored effect: a phonon polarization-filter mechanism induced by the surface PHV, which generates an interface phonon mode with its frequency below the bulk mode frequency. This interface mode possesses a specific circular polarization and therefore acts as a polarization filter, confining only phonons with the matching polarization at the interface. Magnetic topological insulators can thus selectively transmit one type of circularly polarized phonon mode, enabling the manipulation of phonon polarization and angular momentum. In addition, we further develop a generalized scattering framework to study the effect of an injected acoustic wave from a trivial insulator to a magnetic topological insulator with both normal and oblique incidence, and discuss the phenomena of surface acoustic Faraday rotation and longitudinal-transverse mode conversion. Our results establish surface Hall viscosity as a powerful mechanism for engineering axial phonon states and open new avenues for topological phononic devices based on phonon angular momentum.

cond-mat.mes-hall↗

arXiv2026

Millimeter-Scale, Atomically Controlled 2D Topological Insulators Revealed by Multimodal Spectroscopy

Quantum spin Hall insulators, or synonymously known as 2D topological insulators, are crucial 2D systems hosting topologically protected edge states. The working temperature of this topological quantum phase is dictated by the inverted bandgap. However, the previously identified large-gap 2D topological insulators are either extremely chemically unstable, or cannot be made with atomistic precision over macroscopic scales. Here, we establish two-quintuple-layer Bi2Te3 and MnBi2Te4/Bi2Te3 heterostructures as atomically controlled, millimeter-scale 2D topological insulators, enabled by precision layer-by-layer growth that yields a carpet-like morphology extending coherently over macroscopic distances. This carpet-like growth mode renders the films amenable to mechanical exfoliation and subsequent wet or dry transfer. Multimodal spectroscopies and microscopies reveal the integer-layer tuned electronic structure of (Bi2Te3)n with excellent agreement to theory. Photon-energy-dependent photoemission and time-resolved photoemission identify band inversion and band dynamics, respectively, while scanning tunneling spectroscopy resolves topological edge states, characteristic of the 2D topological insulator phase. Thickness- and photon-energy-dependent photoemission further validates MnBi2Te4/Bi2Te3 as a robust 2D topological insulator. The large inverted gaps of ~100 meV in (Bi2Te3)2 and ~150 meV in MnBi2Te4/Bi2Te3 suggest operation near ambient temperature. These results define a scalable materials platform for next-generation, low-loss quantum and energy-efficient devices.

cond-mat.mtrl-sci↗

arXiv2026

Emergent Anomalous Hall Effect from Surface States in the Altermagnet MnTe Thin Films

Transport measurements on thin films of the prototypical altermagnet MnTe have reported conflicting phenomena of anomalous Hall effects (AHE), including opposite signs and thickness-independent resistivity. Here we resolve these discrepancies by separating bulk and surface contributions to the AHE for different crystal terminations. Using first-principles calculations and symmetry-based effective models, we show that although the bulk hosts a characteristic $g$-wave Fermi surface, surface states within the bulk gap acquire a ferromagnet-like spin polarization and dominate the AHE at experimentally relevant Fermi energies. While the surface magnetization follows the surface spin sublattice, the resulting AHE is uniquely determined by the bulk Néel order for a given termination. Both bulk and surface contributions are closely linked to a small but finite out-of-plane orbital magnetization. Incorporating realistic interfacial chemistry further reveals that a Te capping layer can reverse the surface AHE sign relative to that on an InP substrate. Our results establish a microscopic framework for interpreting and engineering AHE responses in altermagnetic thin films through interface design.

cond-mat.mtrl-sci↗

arXiv2026

Current Induced Switching of Superconducting Order and Enhancement of Superconducting Diode Efficiency

We propose that the superconducting diode (SD) efficiency can be significantly enhanced near the transition between two superconducting states by choosing parameters where, before the system goes normal with increasing supercurrent, it switches into a different superconducting order for one direction of the current but not for the other. This mechanism for producing high SD efficiency relies on the expectation that the critical current depends sensitively on the superconducting order. We demonstrate this explicitly by performing detailed calculations for a bilayer superconductor with an in-plane magnetic field, which admits the standard Bardeen-Cooper-Schrieffer (BCS) and the orbital Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) orders as a function of the strength of the magnetic field. We predict a sharp peak in the SD efficiency in the FFLO state close to the transition, which arises from a complex interplay between the two superconducting orders. An implication of our study is that the measurement of the SD efficiency can provide fundamental insight into the nature of the BCS-FFLO transition both as a function of the magnetic field and the supercurrent.

cond-mat.supr-con↗

arXiv2026

Surface-State-Driven Anomalous Hall Effect in Altermagnetic MnTe Films

Altermagnets have recently emerged as a new class of magnetic materials that combine compensated magnetic order with spin-split electronic band structures. In this work, we employ molecular beam epitaxy to grow MnTe thin films with controlled thickness on InP(111)A substrates. By performing angle-resolved photoemission spectroscopy measurements, we observe a large spin splitting of ~230 meV for bulk bands well below the Fermi level and identify surface states that cross the Fermi level. Electrical transport measurements reveal that a robust anomalous Hall (AH) effect persists down to 2 K and an AH sign reversal occurs near 175 K. By systematically tuning film thickness, growth conditions, and interfacial structure, we demonstrate that the AH response in MnTe films originates from the Berry curvature of surface states rather than from bulk bands. Our first-principles calculations reveal that this surface-state-driven AH effect is imprinted by the bulk altermagnetic order and remains unchanged for terminations with opposite Mn magnetic orientations. Our results establish a unique surface transport probe of bulk altermagnetism, demonstrate interface engineering as an effective route to generate and control the AH effect in altermagnets, and provide a unified understanding of the AH response in altermagentic MnTe films.

cond-mat.mtrl-sci↗

arXiv2026

Surface Phonon Hall Viscosity Induced Phonon Chirality and Nonreciprocity in Magnetic Topological Insulator Films

The surface half-quantum Hall effect, a hallmark consequence of axion electrodynamics, can be induced by gapping out the surface states of topological insulators through surface magnetization, and has led to a variety of topological response phenomena observed in experiments. In this work, we investigate phonon dynamics originating from an acoustic analog - the surface phonon Hall viscosity - that can also occur at the surface of magnetic topological insulators. This surface phonon Hall viscosity stems from the Nieh-Yan action in the strain response of topological insulators, where strain acts as the effective vierbein field for the bulk low-energy massive Dirac fermions. Crucially, this viscosity term entangles phonon dynamics with surface magnetization. In magnetic topological insulator films, we find that this interaction causes acoustic phonons to become chiral when the magnetization at the top and bottom surfaces is parallel, and nonreciprocal when it is anti-parallel. We further discuss potential experimental signatures of phonon dynamics induced by surface phonon Hall viscosity, specifically the phonon thermal Hall effect and magnon-polarons.

cond-mat.mes-hall↗

arXiv2025

QMBench: A Research Level Benchmark for Quantum Materials Research

We introduce QMBench, a comprehensive benchmark designed to evaluate the capability of large language model agents in quantum materials research. This specialized benchmark assesses the model's ability to apply condensed matter physics knowledge and computational techniques such as density functional theory to solve research problems in quantum materials science. QMBench encompasses different domains of the quantum material research, including structural properties, electronic properties, thermodynamic and other properties, symmetry principle and computational methodologies. By providing a standardized evaluation framework, QMBench aims to accelerate the development of an AI scientist capable of making creative contributions to quantum materials research. We expect QMBench to be developed and constantly improved by the research community.

cond-mat.mtrl-sci↗

arXiv2025

Boundary-Bulk Interplay in Nonlinear Topological Transport

Nonlinear transport has emerged as a powerful approach to probe the quantum geometry of electronic wavefunctions, such as Berry curvature and quantum metric, in topological materials. While nonlinear responses governed by bulk quantum geometry and band topology are well understood, the role of boundary modes (e.g., edge, surface, and hinge states) in nonlinear transport of topological materials remains largely unexplored. In this work, we demonstrate boundary-bulk interplay in nonlinear transport, including second-harmonic Hall and nonreciprocal longitudinal responses, in molecular beam epitaxy-grown magnetic topological insulator heterostructures. We find that the nonlinear transport is maximized when the sample is tuned slightly away from the well-quantized states, including the quantum anomalous Hall and axion insulator states. The sign and amplitude of the nonlinear transport depend on electrode configuration, magnetic order, and carrier type, establishing boundary mode transport as the dominant contributor. These findings, supported by symmetry analysis and nonlinear Landauer-Büttiker formalism, demonstrate that nonlinear transport in topological materials is governed by the interplay between boundary and bulk states. We further derive a universal relation between different lead voltages from electrode geometry symmetry, which allows us to distinguish nonlinear boundary transport from bulk contributions. Our work highlights the critical role of electrodes in nonlinear transport, which is absent in nonlinear optics, and establishes boundary modes as a key origin of the giant nonlinear response in nearly bulk-insulating topological materials. This insight opens new opportunities for engineering nonlinear transport through boundary-bulk interplay in future device applications of topological materials.

cond-mat.mes-hall↗

arXiv2025

Symmetry-enforced Moiré Topology

Topological flat bands in two-dimensional (2D) moiré materials have emerged as promising platforms for exploring the interplay between topology and correlation effects. However, realistic calculations of moiré band topology using density functional theory (DFT) are computationally inefficient due to the large number of atoms in a single moiré unit cell. In this work, we propose a systematic scheme to predict the topology of moiré bands from atomic symmetry data and moiré symmetry group, both of which can be efficiently extracted from DFT. Specifically, for $Γ$-valley electron gases, we find that certain combinations of atomic symmetry data and moiré symmetry groups can enforce nontrivial band topology in the low-energy moiré bands, as long as the moiré band gap is smaller than the atomic band splitting at the moiré Brillouin zone boundary. This symmetry-enforced nontrivial moiré topology, including both topological insulators and topological semimetals, is robust against various material-specific details such as the precise form and strength of the moiré potential or the exact twist angle. By exhaustively scanning all 2D atomic symmetry data and moiré symmetry groups, we identify 197 combinations that can yield symmetry-enforced nontrivial moiré topology, and we verify one such combination using a moiré model with cubic Rashba spin-orbit coupling. By screening the existing 2D material database, we currently identify 92 monolayer materials with (i) the low-energy bands near $Γ$ and (ii) the atomic symmetry data that belong to those combinations. Our approach is generalizable to other valleys and provides a useful guideline for experimental efforts to discover and design new topologically nontrivial moiré materials.

cond-mat.mes-hall↗

arXiv2025

Pair-mixing induced Time-reversal-breaking superconductivity

Experimental evidences of spontaneous time-reversal (TR) symmetry breaking have been reported for the superconducting ground state in the transition metal dichalcogenide (TMD) superconductor 4H$_b$-TaS$_2$ or chiral molecule intercalated TaS$_2$ hybrid superlattices, and is regarded as evidence of emergent chiral superconductivity. However, the $T_c$ of these TMD superconductors is of the same order as pristine 1H or 2H-TaS$_2$, which do not show any signature of TR breaking and are believed to be conventional Bardeen-Cooper-Schrieffer superconductors. To resolve this puzzle, we propose a new type of pair-mixing state that mixes the dominant conventional s-wave pairing channel with the subdominant chiral p-wave pairing channel via a finite Cooper-pair momentum, based on symmetry analysis within the Ginzburg-Landau theory. Our analysis shows that the fourth-order terms in the chiral p-wave channel can lead to a variety of pair-mixing states with spontaneous TR breaking. These TR-breaking superconducting states also reveal a zero-field, junction-free superconducting diode effect that is observed in chiral molecule intercalated TaS$_2$ superlattices.

cond-mat.supr-con↗

arXiv2025

Gate-Tunable Ambipolar Josephson Current in a Topological Insulator

Dirac surface states in a topological insulator (TI) with proximity-induced superconductivity offer a promising platform for realizing topological superconductivity and Majorana physics. However, in TIs, the Josephson effect is usually observed in regimes where transport is dominated by either substantial bulk conduction channels or unipolar surface states. In this work, we demonstrate gate-tunable ambipolar Josephson current in lateral Josephson junction (JJ) devices based on bulk-insulating (Bi,Sb)2Te3 thin films grown by molecular beam epitaxy (MBE). For thinner films, the supercurrent exhibits pronounced gate-tunable ambipolar behavior and is significantly suppressed as the chemical potential approaches the Dirac point, yet persists across it. In contrast, thicker films exhibit a much weaker ambipolar response. Moreover, we find that the supercurrent becomes significantly less resilient to external magnetic fields when the chemical potential is tuned near the Dirac point in both thickness regimes. Our numerical simulations demonstrate the ambipolar behavior of these TI JJ devices and attribute the asymmetric supercurrent observed in thicker TI films to the coexistence of Dirac surface states and bulk conduction channels. The demonstration of gate-tunable ambipolar Josephson transport in MBE-grown TI films paves the way for realizing Dirac-surface-state-mediated topological superconductivity and establishes a foundation for future exploration of electrically tunable Majorana modes.

cond-mat.mes-hall↗

arXiv2025

Orbital Hybridization-Induced Ising-Type Superconductivity in a Confined Gallium Layer

In low-dimensional superconductors, the interplay between quantum confinement and interfacial hybridization effects can reshape Cooper pair wavefunctions and induce novel forms of unconventional superconductivity. In this work, we employ a plasma-free, carbon buffer layer-assisted confinement epitaxy method to synthesize trilayer gallium (Ga) sandwiched between a graphene layer and a 6H-SiC(0001) substrate, forming an air-stable graphene/trilayer Ga/SiC heterostructure. In this confined light-element Ga layer, we demonstrate interfacial Ising-type superconductivity driven by atomic orbital hybridization between the Ga layer and the SiC substrate. Electrical transport measurements reveal that the in-plane upper critical magnetic field u0Hc2,|| reaches ~21.98T at T=400 mK, approximately 3.38 times the Pauli paramagnetic limit (~6.51T). Angle-resolved photoemission spectroscopy (ARPES) measurements combined with theoretical calculations confirm the presence of split Fermi surfaces with Ising-type spin textures at the K and K' valleys of the confined Ga layer strongly hybridized with SiC. Moreover, by incorporating finite relaxation time induced by impurity scattering into an Ising-type superconductivity model, we reproduce the entire temperature-dependent u0Hc2,|| phase diagram. This work establishes a new strategy to realize unconventional pairing wavefunctions by combining quantum confinement and interfacial hybridization effects in superconducting thin films. It also opens new avenues for designing scalable superconducting quantum electronic and spintronic devices through interfacial engineering.

cond-mat.mes-hall↗

arXiv2025

Interlayer Exchange Coupling-Induced Critical-Metal-to-Insulator Phase Transition in Quantum Anomalous Hall Insulators

Interlayer exchange coupling (IEC) between two magnetic layers sandwiched by a nonmagnetic spacer layer plays a critical role in shaping the magnetic properties of such heterostructures. The quantum anomalous Hall (QAH) effect has been realized in a structure composed of two magnetically doped topological insulator (TI) layers separated by an undoped TI layer. In this work, we employ molecular beam epitaxy to synthesize a series of magnetic TI sandwiches with varying thicknesses of the middle TI spacer layer. The well-quantized QAH effect is observed in all these samples, and the IEC modulates its critical behavior between the top and bottom magnetic TI layers. Near the plateau phase transition (PPT), thinner QAH samples exhibit a two-dimensional critical metal behavior with nearly temperature-independent longitudinal resistance. In contrast, thicker QAH samples behave as a three-dimensional insulator with reduced longitudinal resistance at higher temperatures. We employ a magnetic TI Hamiltonian with random magnetic domains to understand the IEC-induced critical-metal-to-insulator transition observed near QAH PPT.

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