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Charles Roques-Carmes

Publications and source records attributed to Charles Roques-Carmes.

At least 19 recordsLinked to original sources

Quantum Skyrmions in Mixed States of Light and Their Nested Topology

Topological quasiparticles of light, such as classical and quantum optical skyrmions, have so far relied on fully coherent or pure quantum states whose topology is encoded in the entanglement between polarization and two-dimensional spatial modes. Here we show that skyrmionic topology can emerge directly within the density matrix of a mixed quantum state. We introduce a framework in which a coherence-Stokes vector defines a topological texture over the density matrix, enabling the realization of quantum skyrmions using only a pseudospin and a real or synthetic one-dimensional space of modes. For a single photon, the density matrix is analogous to the coherence matrix of classical light, and can be encoded using partially coherent electromagnetic fields. We further analyze the topological texture encoded in a bipartite entangled photon pair, showing how skyrmions arise not only in the full bi-photon system, but also in its reduced subspaces with any pseudospin-mode combination simultaneously. We then explore the robustness of such skyrmions to environmental noise, and discover their persistence in mixed-quantum states of multiple photons. Finally, we propose a feasible experimental route to generate and measure such skyrmions using integrated photonic networks, and suggest avenues for similar implementations in other quantum systems. Our work paves the way for robustly encoding classical information on partially coherent light or on mixed quantum states and for encoding topological charges on many-body quantum systems.

quant-ph

Nanophotonic control of spatial information in scintillation detectors

X-rays enable non-invasive imaging across medicine, security, materials science, and beyond, yet modern systems remain constrained by the need to resolve finer structures at lower radiation dose. Scintillators are the dominant materials for detecting X-rays, but face a longstanding compromise: thick scintillators absorb X-rays effectively, whereas optical photons generated throughout their volume spread before detection, degrading spatial information. Existing scintillator architectures largely try to preserve resolution by physically confining light using pixels, columnar crystals, or microstructured channels. Here, we show that high-resolution detection does not require the volumetric confinement of scintillation light. A metalens integrated directly with a bulk scintillator uses nanophotonic wavefront control to preferentially transfer high-spatial-frequency information from volumetrically generated scintillation light to the detector, while retaining the X-ray absorption of a thick scintillator. We experimentally recover fine spatial detail in X-ray images of inorganic and biological specimens. In a detector geometry relevant to computed tomography (CT), the experimentally validated model predicts a fivefold reduction in required X-ray dose and a 25-fold increase in resolution bandwidth relative to a state-of-the-art pixelated scintillator. These results establish wavefront engineering as a route to separating efficient X-ray absorption from optical image formation, with the potential for substantially higher-resolution, lower-dose CT.

physics.optics

Polarization vector conjugation in a photonic integrated circuit

We show how to perform polarization conjugation of light in a simple apparatus without any nonlinear optical materials, based on self-configuring Mach-Zehnder interferometers fed by a polarization splitter. This allows us to completely and automatically remove the polarization variations on a single beam or mode propagating through an optical system with arbitrary birefringence, such as a conventional optical fiber, and compensate polarization variations experienced in the forward direction by propagating the conjugated beam back through the system and recreating the original polarization at the source. We demonstrate this polarization conjugation in an optical fiber setup in different orientations with a measured polarization extinction ratio of -30 dB for the returned beam.

physics.optics

Vacuum Fluctuation-Induced State Switching in Degenerate Optical Parametric Oscillators

Bistable driven-dissipative systems near bifurcations can exhibit noise-activated switching between steady states. Here, we investigate how quantum vacuum fluctuations induce such switching in a biased optical parametric oscillator (OPO), a nonlinear system with intrinsic bistability. We show how microscopic quantum fluctuations driving macroscopic transitions can be controlled with an external bias field that reshapes the OPO steady-state metapotential. We derive analytical expressions for the average switching time and validate them through simulations of the OPO field distribution and inter-state probability flow under bias injection. We further examine how switching depends on bias strength, pump gain, and optical nonlinearity. Our findings clarify how quantum noise can shape macroscopic dynamics and provide a foundation for noise-assisted photonic machine learning and probabilistic quantum gates.

quant-ph

Neural network inverse design of nanophotonic scintillators

Scintillators are materials converting high-energy radiation into optical light, essential in a range of technologies such as medical imaging systems and security scanners. Scintillator development and optimization have remained limited by the complexity of their underlying physics, involving stochastic cascades of electron-electron, electron-phonon, and electron-photon interactions. Such processes are typically modeled by non-differentiable Monte Carlo simulations, limiting the applicability of machine learning for scintillator development. Here we present a physics-informed neural network that learns the scintillation cascade process from the incident high-energy particle to photon emission, substantially accelerating scintillator design and optimization. Combining this neural network with photonic simulations enables end-to-end differentiable optimization of the scintillator geometry. This allows us to optimize for arbitrary figures of merit, such as specific target emission patterns.. We demonstrate the concept and characterize it relative to previous approaches by inverse design of nanophotonic scintillators for X-ray imaging.

physics.optics

Dosimetric characterization of a nanophotonic scintillator and applications to real-time in-vivo total body irradiation dosimetry

Purpose: Recent advances in metasurface photonics and manufacturing have enabled a nanophotonic surface coating to be applied to conventional scintillators, which has been shown to significantly improve light yield. However, the dosimetric properties of such coatings has not been established. We performed the first dosimetric characterization of a nanophotonic scintillator and explored clinical application to real-time in-vivo total body irradiation (TBI) dosimetry. Methods: A 4.5x1.5 cm cerium-doped yttrium aluminum garnet (YAG:Ce) scintillator, half patterned with the nanophotonic structure, half left unpatterned, enabled direct comparison between conventional and nanophotonic surfaces. The scintillator was placed in a 3D-printed light-tight box with an off-axis CMOS camera and irradiated with a clinical linear accelerator. Absolute dosimetry was done with dose-calibrated radiochromic film. For TBI, the scintillator was positioned on an anthropomorphic phantom in a TBI booth, with signal measured by both CMOS and consumer-grade phone cameras under different room lighting conditions. Results: The nanophotonic scintillator showed a 4.1x increase in signal and a 3.7x increase in contrast-to-noise ratio versus the conventional scintillator. Both scintillators exhibited dose-rate independence and linear dose response, with modest energy dependence. For TBI, the nanophotonic scintillator produced a clearly detectable signal with both CMOS and phone cameras, whereas the conventional scintillator signal was undetectable. Conclusions: Nanophotonic structures significantly enhance light output of conventional scintillators without impacting their dosimetric properties. Nanophotonic scintillators may enable real-time in-vivo TBI dosimetry. Future work should investigate this technology for improved dosimetry equipment and X-ray imaging detectors.

physics.med-ph

Diffractive cascades for polychromatic hard X-ray focusing

Diffractive focusing of hard X-rays has traditionally required structures with large aspect ratios due to the limited interaction of most materials with X-rays. This has increased the complexity of fabricating diffractive X- ray lenses, restricting their widespread deployment. Here, we utilize topology optimization to design diffractive cascades to focus X-rays. When restricting the structures to a maximum aspect ratio of 8, a diffractive cascade can achieve a focusing efficiency of 40%, far exceeding the 3% efficiency of a zone plate with the same aspect ratio. Diffractive cascades also allow the focusing of beams with energies beyond 20 keV and bandwidths exceeding 1%, loosening the restrictions on other system components. We characterize the robustness of these cascades to alignment, fabrication, and heating perturbations, demonstrating the ability of our designs to operate under real-world conditions. Finally, we exploit the flexibility of our framework to include multiple depths in the objective function. This enables a depth of focus exceeding that of a zone plate or a cascade designed using single-plane optimization. This work demonstrates the utility of topology optimization in the X-ray regime and the possibility of advancing X-ray manipulation across a range of tasks.

physics.optics

Supercollimating photonic crystal scintillators

Scintillators convert X-ray energy into visible or near-visible photons, enabling applications in high-energy particle detection and X-ray imaging. Increasing scintillator thickness improves X-ray absorption but degrades spatial resolution due to diffraction-induced lateral spreading of emitted light, resulting in a fundamental trade-off between detection efficiency and image resolution. Here, we propose a class of three-dimensional photonic crystal scintillators that overcomes this limitation through supercollimation, in which light propagates with suppressed diffraction. We develop a multiscale modeling framework that integrates nanophotonic band-structure simulations with Monte Carlo particle transport to quantitatively evaluate the performance of such scintillators. Our results show that supercollimating photonic crystal scintillators can enhance spatial resolution by up to an order of magnitude relative to conventional bulk scintillators of equal thickness. This improvement leads to a substantial increase in detector quantum efficiency (DQE), particularly at high spatial frequencies, enabling fine features to be preserved at reduced X-ray dose. We further demonstrate that comparable image quality can be achieved with approximately an order-of-magnitude lower X-ray dose. By directly engineering light transport within the bulk of the scintillator, this work establishes a nanophotonic route to simultaneously improving resolution and dose efficiency in X-ray imaging.

physics.optics

Hybrid Nanophotonic Scintillators for Enhanced X-ray Absorption, Emission, and Time Resolution

Scintillators convert ionizing radiation into visible photons, enabling applications from cosmic ray detection to medical imaging. Two independent strategies for improving scintillator performance via nanoscale patterning have recently been demonstrated: engineering material properties to enhance absorption of ionizing radiation and integrating nanophotonic structures to enhance the spontaneous emission rate ("nanophotonic scintillators"). Here, we propose a nanophotonic scintillator that simultaneously enhances both the initial energy conversion and the spontaneous emission rate, by periodically stacking a fast-emitting scintillator and a visible-light-transparent material with strong X-ray attenuation ("stopping layer") to form a one-dimensional (1D) photonic crystal (PhC) scintillator. Photoelectric absorption in the stopping layer increases the number of photoelectrons that deposit energy in neighboring scintillator layers and contribute to scintillation. At the same time, the spontaneous emission rate is enhanced by the nanophotonic structuring itself. We design a 1D PhC comprising an organic scintillator and indium tin oxide (ITO) as the stopping layer and numerically simulate the enhancement in scintillation yield and decay rate. The total detected light output is enhanced by up to a factor of 700 compared to a bulk organic scintillator of equal thickness. We further investigate a 1D PhC structure integrating inorganic and organic scintillators for time-of-flight positron emission tomography (TOF-PET): replacing the non-scintillating stopping layer with an inorganic scintillator further increases the light yield, and the coincidence time resolution (CTR) is enhanced up to 3.5 times compared to a bulk inorganic scintillator of equal thickness. Our work presents a unified approach to improve key scintillation parameters within a single nanophotonic structure.

physics.optics

Toward nanophotonic platforms for solid-state $^{229}$Th nuclear clocks

While the $^{229}$Th nuclear isomer has recently been observed and laser-excited, converting optical nuclear manipulation into a chip-scale solid-state frequency standard remains an open challenge. Here, we present a nanophotonic platform to realize an all-solid-state nuclear clock based on the low-energy isomeric transition of $^{229}$Th embedded in high-$Q$ fluoride photonic resonators. By coupling ensembles of thorium nuclei to confined optical modes, we show that resonant field build-up in the cavity can substantially enhance the nuclear excitation rate, enabling optical interrogation at practical laser intensities. We model the nuclei-photon interaction dynamics and outline a technological roadmap toward addressing this challenge, including resonator fabrication in fluoride crystals, thorium implantation, nuclear excitation with integrated lasers, and on-chip detection of vacuum-ultraviolet photons. As an initial proof of concept, we implant a crystalline fluoride whispering-gallery-mode resonator with $^{229}$Th and assess the impact of implantation-induced damage on resonator performance. Our platform leverages recent advances in materials integration and nanophotonics to chart a realistic route toward compact and scalable nuclear frequency standards.

physics.optics

Separating partially coherent light

Recent advances in optical imaging and communication increasingly involve high-dimensional, partially coherent light, creating a growing need for scalable tools to measure and manipulate coherence. Here, we demonstrate the automatic separation of spatially partially coherent light into "coherence modes" -- its orthogonal and mutually incoherent components. To make this separation possible, we exploit variational processing in layered self-configuring interferometer architectures in a silicon photonic circuit. This process formally finds and measures the eigenvectors and eigenvalues of the coherency matrix, hence measuring the partially coherent state, while leaving it intact and separated after optimization. Furthermore, we show that mutually incoherent beams, if spatially orthogonal, can be automatically separated even if they are completely overlapped, hence separating unknown laser beams based only on their mutual incoherence. Our experiment finds and separates the two strongest coherence modes starting from a nine-mode sampling of the partially or fully overlapping fields from two independent lasers. The method requires a number of physical components that scales linearly with the rank $r$ of the coherency matrix and operates through a sequence of $r$ in situ gradient-based optimizations enabled by electronic drive frequency multiplexing of interferometer phase shifters. We benchmark its performance against a mixture-based tomographic method, also implemented on chip. These results establish a scalable framework for programmable coherence analysis and control in imaging, communication, and photonic information processing.

physics.optics

Integrated Photonic Polarization Synthesizer and Analyzer

Polarization-resolved control and measurement of the optical field are essential for a wide range of photonic systems, including coherent communication, polarimetric sensing, and quantum information processing. We present a photonic integrated circuit that enables the generation and analysis of arbitrary polarization states. The device provides reconfigurable access to the full polarization degree of freedom of coherent light within a single integrated platform. We experimentally demonstrate arbitrary polarization state generation spanning the Poincare sphere, as well as Stokes vector measurement on chip. Unlike conventional Stokes measurements that rely on direct detection, polarization analysis utilizing this architecture is intrinsically non-destructive, preserving the optical signal for further optical domain processing. The devices are fabricated in a commercial foundry using CMOS-compatible processes, enabling scalable and reproducible integration. By combining polarization generation and analysis in a compact and stable photonic circuit, this work eliminates the need for external polarization optics and provides a foundation for robust, polarization-enabled photonic integrated systems.

physics.optics

A general framework for interactions between electron beams and quantum optical systems

We provide a theoretical framework to describe the dynamics of a free-electron beam interacting with quantized bound systems in arbitrary electromagnetic environments. This expands the quantum optics toolbox to incorporate free-electron beams for applications in highly tunable quantum control, imaging, and spectroscopy at the nanoscale. The framework recovers previously studied results and shows that electromagnetic environments can amplify the intrinsically weak coupling between a free-electron and a bound electron to reach previously inaccessible interaction regimes. We leverage this enhanced coupling for experimentally feasible protocols in coherent qubit control and towards the nondestructive readout and projective control of the electron beam's quantum-number statistics. Our framework is broadly applicable to microwave-frequency qubits, optical nanophotonics, cavity quantum electrodynamics, and emerging platforms at the interface of electron microscopy and quantum information.

quant-ph

Wavefront Engineering for Scintillation-Based Imaging

Recent research in nanophotonics for scintillation-based imaging has demonstrated promising improvements in scintillator performance. In parallel, advances in nanophotonics have enabled wavefront control through metasurfaces, a capability that has transformed fields such as microscopy by allowing tailored control of optical propagation. This naturally raises the following question, which we address in this perspective: can wavefront-control strategies be leveraged to improve scintillation-based imaging? To answer this question, we explore nanophotonic- and metasurface-enabled wavefront control in scintillators to mitigate image blurring arising from their intrinsically diffuse light emission. While depth-of-field extension in scintillation faces fundamental limitations absent in microscopy, this approach reveals promising avenues, including stacked scintillators, selective spatial-frequency enhancement, and X-ray energy-dependent imaging. These results clarify the key distinctions in adapting wavefront engineering to scintillation and its potential to enable tailored detection strategies.

physics.optics

Programmable Optical Filters Based on Feed-Forward Photonic Meshes

We demonstrate an integrated photonic circuit based on feed forward photonic meshes that can be programmed and reconfigured to perform arbitrary spectral filter functions. We investigate a subset of the available filter functions, demonstrating that a N = 4 input triangular mesh with M = 3 layers may be operated via self-configuration algorithms to filter M arbitrary wavelengths from a given input spectrum. The tunable nature of the architecture enables preconfigured filter functions to be swept in the spectral domain continuously over the free spectral range of the device. This removes any strict requirements between the design parameters of the architecture and the center wavelength of a desired filter function. With this architecture, we experimentally demonstrate arbitrary wavelength rejection filters with contrasts as deep as 40 dB. Further, by intentionally selecting the center wavelengths of each filter function to lie along a wavelength grid we demonstrate deep wavelength division demultiplexing (DWDM) with inter-channel crosstalk between -25 dB and -40 dB. Unlike typical DWDM systems, in this architecture the center wavelength of each channel is not fixed at fabrication and instead may be swept or reordered arbitrarily. This device demonstrates advantages over typical methods for DWDM, Raman spectroscopy, and correlation spectroscopy as well as other applications.

physics.optics

Experimental observation of energy-band Riemann surface

Non-Hermiticity naturally arises in many physical systems that exchange energy with their environment. The presence of non-Hermiticity leads to many novel topological physics phenomena and device applications. In the non-Hermitian energy band theory, the foundation of these physics and applications, both energies and wavevectors can take complex values. The energy bands thus become a Riemann surface, and such an energy-band Riemann surface underlies all the important signatures of non-Hermitian topological physics phenomena. Despite a long history and recent theoretical interests, the energy-band Riemann surface has not been experimentally studied. Here we provide a photonic observation of the energy-band Riemann surface of a non-Hermitian system. This is achieved by applying a tunable imaginary gauge transformation on the platform of the photonic synthetic frequency dimension. From the measured topology of the Riemann surface, we reveal the complex-energy winding, the open-boundary-condition spectrum, the generalized Brillouin zone, and the branch points. Our findings demonstrate a unified framework in the studies of diverse effects in non-Hermitian topological physics through an experimental observation of energy-band Riemann surfaces.

physics.optics

Superluminal Correlations in Ensembles of Optical Phase Singularities

Phase singularities are universal features found across diverse wave systems. Their ensembles exhibit distance correlations governing exotic material phases. However, the full correlations in phase-space have remained unexplored and experimentally inaccessible. Here, we directly measure the ultrafast dynamics of optical singularity ensembles, capturing their phase-space correlations. Our observations reveal that phase singularities exhibit acceleration to unbounded velocities before annihilation, indicated by measurements of velocities exceeding the speed of light. These superluminal velocities are paradoxically amplified by the slow group velocity of hyperbolic phonon polaritons in our material platform, hexagonal boron nitride membranes. We demonstrate these phenomena using combined hardware and algorithmic advances in ultrafast electron microscopy, achieving spatial and temporal resolutions each an order of magnitude below the polaritonic wavelength and cycle period. Our findings enable probing topological defect dynamics at previously unattainable timescales, deepening our understanding of phase-singularity universality and suggesting phenomena of ultrafast information flow in polaritonic media.

physics.optics

Variational processing of multimode squeezed light

Integrated multimode quantum optics is a promising platform for scalable continuous-variable quantum technologies leveraging multimode squeezing in both the spatial and spectral domains. However, on-chip measurement, routing and processing the relevant ``supermodes'' over which the squeezing resource is distributed still scales quadratically with the number of modes $N$, causing rapid increase in photonic circuit size and number of required measurements. Here, we introduce a variational scheme, relying on self-configuring photonic networks (SCN) that learns and extracts the most-squeezed supermodes sequentially, reducing both the circuit size and the experimental overhead. Using homodyne measurement as a cost function, a sparse SCN discovers the $l\ll N$ most significant supermodes using $O(lN)$ physical elements and optimization steps. We analyze and numerically simulate these architectures for both real-space and frequency-domain implementations, showing a fidelity close to unity between the learned circuit and the supermode decomposition, even in the presence of optical losses and detection noise. In the frequency domain, we show that circuit size can be further reduced by using inverse-designed surrogate networks, which emulate the layers learned thus far. Using two different frequency encoding schemes -- uniformly- and non-uniformly-spaced frequency bins -- we reduce an entire network (learning all $N$ supermodes) to $O(N)$ and even $O(1)$ modulated cavities. Our results point toward chip-scale, resource-efficient quantum processing units and demultiplexers for continuous variable processing in multimode quantum optics, with applications ranging from quantum communication, metrology, and computation.

quant-ph