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Charles Roques-Carmes

Publications and source records attributed to Charles Roques-Carmes.

At least 37 records · Page 2Linked to original sources

Variational processing of multimode squeezed light

Integrated multimode quantum optics is a promising platform for scalable continuous-variable quantum technologies leveraging multimode squeezing in both the spatial and spectral domains. However, on-chip measurement, routing and processing the relevant ``supermodes'' over which the squeezing resource is distributed still scales quadratically with the number of modes $N$, causing rapid increase in photonic circuit size and number of required measurements. Here, we introduce a variational scheme, relying on self-configuring photonic networks (SCN) that learns and extracts the most-squeezed supermodes sequentially, reducing both the circuit size and the experimental overhead. Using homodyne measurement as a cost function, a sparse SCN discovers the $l\ll N$ most significant supermodes using $O(lN)$ physical elements and optimization steps. We analyze and numerically simulate these architectures for both real-space and frequency-domain implementations, showing a fidelity close to unity between the learned circuit and the supermode decomposition, even in the presence of optical losses and detection noise. In the frequency domain, we show that circuit size can be further reduced by using inverse-designed surrogate networks, which emulate the layers learned thus far. Using two different frequency encoding schemes -- uniformly- and non-uniformly-spaced frequency bins -- we reduce an entire network (learning all $N$ supermodes) to $O(N)$ and even $O(1)$ modulated cavities. Our results point toward chip-scale, resource-efficient quantum processing units and demultiplexers for continuous variable processing in multimode quantum optics, with applications ranging from quantum communication, metrology, and computation.

quant-ph↗

Quantum sensing of electron beams using solid-state spins

Scattering experiments with energetic particles, such as free electrons, have been historically used to reveal the quantum structure of matter. However, realizing coherent interactions between free-electron beams and solid-state quantum systems has remained out of reach, owing to their intrinsically weak coupling. Realizing such coherent control would open up opportunities for hybrid quantum platforms combining free electrons and solid-state qubits for coincident quantum information processing and nanoscale sensing. Here, we present a framework that employs negatively charged nitrogen-vacancy centers (NV-) in diamond as quantum sensors of a bunched electron beam. We develop a Lindblad master equation description of the magnetic free-electron--qubit interactions and identify spin relaxometry as a sensitive probe of the interaction. Experimentally, we integrate a confocal fluorescence microscopy setup into a microwave-bunched electron beam line. We monitor charge-state dynamics and assess their impact on key sensing performance metrics (such as spin readout contrast), defining safe operating parameters for quantum sensing experiments. By performing $T_1$ relaxometry under controlled electron beam exposure, we establish an upper bound on the free-electron--spin coupling strength. Our results establish NV- centers as quantitative probes of free electrons, providing a metrological benchmark for free-electron--qubit coupling under realistic conditions, and chart a route toward solid-state quantum control with electron beams.

quant-ph↗

On-Chip Laser-Driven Free-Electron Spin Polarizer

Spin-polarized electron beam sources enable studies of spin-dependent electric and magnetic effects at the nanoscale. We propose a method of creating spin-polarized electrons on an integrated photonics chip by laser driven nanophotonic fields. A two-stage interaction separated by a free space drift length is proposed, where the first stage and drift length introduces spin-dependent characteristics into the probability distribution of the electron wavefunction. The second stage uses an adjusted optical near-field to rotate the spin states utilizing the spin-dependent wavepacket distribution to produce electrons with high ensemble average spin expectation values. This platform provides an integrated and compact method to generate spin-polarized electrons, implementable with millimeter scale chips and table-top lasers.

quant-ph↗

End-to-end design of multicolor scintillators for enhanced energy resolution in X-ray imaging

Scintillators have been widely used in X-ray imaging due to their ability to convert high-energy radiation into visible light, making them essential for applications such as medical imaging and high-energy physics. Recent advances in the artificial structuring of scintillators offer new opportunities for improving the energy resolution of scintillator-based X-ray detectors. Here, we present a three-bin energy-resolved X-ray imaging framework based on a three-layer multicolor scintillator used in conjunction with a physics-aware image postprocessing algorithm. The multicolor scintillator is able to preserve X-ray energy information through the combination of emission wavelength multiplexing and energy-dependent isolation of X-ray absorption in specific layers. The dominant emission color and the radius of the spot measured by the detector are used to infer the incident X-ray energy based on prior knowledge of the energy-dependent absorption profiles of the scintillator stack. Through ab initio Monte Carlo simulations, we show that our approach can achieve an energy reconstruction accuracy of 49.7%, which is only 2% below the maximum accuracy achievable with realistic scintillators. We apply our framework to medical phantom imaging simulations where we demonstrate that it can effectively differentiate iodine and gadolinium-based contrast agents from bone, muscle, and soft tissue.

physics.ins-det↗

Nanophotonic thermal management in X-ray tubes

In X-ray tubes, more than 99% of the kilowatts of power supplied to generate X-rays via bremsstrahlung are lost in the form of heat generation in the anode. Therefore, thermal management is a critical barrier to the development of more powerful X-ray tubes with higher brightness and spatial coherence, which are needed to translate imaging modalities such as phase-contrast imaging to the clinic. In rotating anode X-ray tubes, the most common design, thermal radiation is a bottleneck that prevents efficient cooling of the anode$\unicode{x2014}$the hottest part of the device by far. We predict that nanophotonically patterning the anode of an X-ray tube enhances heat dissipation via thermal radiation, enabling it to operate at higher powers without increasing in temperature. The focal spot size, which is related to the spatial coherence of generated X-rays, can also be made smaller at a constant temperature. A major advantage of our "nanophotonic thermal management" approach is that in principle, it allows for complete control over the spectrum and direction of thermal radiation, which can lead to optimal thermal routing and improved performance.

physics.optics↗

Creating high-dimensional topological physics using a single ring resonator

In spaces of three or more dimensions, there exists topological physics of significant richness that has no lower-dimensional counterparts. To experimentally explore high-dimensional physics, it is advantageous to augment the physical space with synthetic dimensions. An emerging approach is to use a single modulated photonic ring resonator to form multiple synthetic frequency dimensions. However, all the high-dimensional Hamiltonians experimentally demonstrated in this approach are topologically trivial. Here we propose a general scheme to create high-dimensional topological physics using multiple synthetic frequency dimensions in a single ring resonator. This scheme utilizes specifically designed mode-selective modulations and mode conversions to create non-trivial topology. As examples, we numerically demonstrate a three-dimensional, two-band model exhibiting Weyl points and topological insulator phases, and a five-dimensional, four-band model exhibiting Yang monopoles and Weyl surfaces. Our results will facilitate the experimental studies and future applications of topological physics in high dimensions.

physics.optics↗

Noise-immune quantum correlations of intense light

Lasers with high intensity generally exhibit strong intensity fluctuations far above the shot-noise level. Taming this noise is pivotal to a wide range of applications, both classical and quantum. Here, we demonstrate the creation of intense light with quantum levels of noise even when starting from inputs with large amounts of excess noise. In particular, we demonstrate how intense squeezed light with intensities approaching 0.1 TW/cm^2, but noise at or below the shot noise level, can be produced from noisy inputs associated with high-power amplified laser sources (an overall noise-reduction of 30-fold). Based on a new theory of quantum noise in multimode systems, we show that the ability to generate quantum light from noisy inputs results from multimode quantum correlations, which maximally decouple the output light from the dominant noise channels in the input light. As an example, we demonstrate this effect for femtosecond pulses in nonlinear fibers, but the noise-immune correlations that enable our results are generic to many other nonlinear systems in optics and beyond.

quant-ph↗

Universal programmable and self-configuring optical filter

We propose an approach to integrated optical spectral filtering that allows arbitrary programmability, can compensate automatically for imperfections in filter fabrication, allows multiple simultaneous and separately programmable filter functions on the same input, and can configure itself automatically to the problem of interest, for example to filter or reject multiple arbitrarily chosen frequencies. The approach exploits splitting the input light into an array of multiple waveguides of different lengths that then feed a programmable interferometer array that can also self-configure. It can give spectral response similar to arrayed waveguide gratings but offers many other filtering functions, as well as supporting other structures based on non-redundant arrays for precise spectral filtering. Simultaneous filtering also allows, for the first time to our knowledge, an automatic measurement of the temporal coherency matrix and physical separation into the Karhunen-Loève expansion of temporally partially coherent light fields.

physics.optics↗

Superfluorescent scintillation from coupled perovskite quantum dots

Scintillation, the process of converting high-energy radiation to detectable visible light, is pivotal in advanced technologies spanning from medical diagnostics to fundamental scientific research. Despite significant advancements toward faster and more efficient scintillators, there remains a fundamental limit arising from the intrinsic properties of scintillating materials. The scintillation process culminates in spontaneous emission of visible light, which is restricted in rate by the oscillator strength of individual emission centers. Here, we observe a novel collective emission phenomenon under X-ray excitation, breaking this limit and accelerating the emission. Our observation reveals that strong interactions between simultaneously excited coupled perovskite quantum dots can create collective radioluminescence. This effect is characterized by a spectral shift and an enhanced rate of emission, with an average lifetime of 230 ps, 14 times faster than their room temperature spontaneous emission. It has been established that such quantum dots exhibit superfluorescence under UV excitation. However, X-ray superfluorescence is inherently different, as each high-energy photon creates multiple synchronized excitation events, triggered by a photoelectron and resulting in even faster emission rates, a larger spectral shift, and a broader spectrum. This observation is consistent with a quantum-optical analysis explaining both the UV-driven and X-ray-driven effects. We use a Hanbury-Brown-Twiss g^(2) (τ) setup to analyze the temperature-dependent temporal response of these scintillators. Collective radioluminescence breaks the limit of scintillation lifetime based on spontaneous emission and could dramatically improve time-of-flight detector performance, introducing quantum enhancements to scintillation science.

physics.optics↗

X-Ray-Driven Photon Bunching

Hanbury Brown and Twiss (HBT) interferometry is a milestone experiment that transformed our understanding of the nature of light. The concept was demonstrated in 1956 to measure the radii of stars through photon coincidence detection. This form of coincidence detection later became a cornerstone of modern quantum optics. Here we connect HBT interferometry to the physics of scintillation, the process of spontaneous light emission upon excitation by high-energy particles, such as x-rays. Our work reveals intrinsic photon bunching in the scintillation process, which we utilize to elucidate its underlying light emission mechanisms. Specifically, g^((2) ) (τ) enables the quantitative extraction of scintillation lifetime and light yield, showing their dependence on temperature and X-ray flux as well. This approach provides a characterization method that we benchmark on a wide gamut of scintillators, including rare-earth-doped garnets and perovskite nanocrystals. Our method is particularly important for nano- and micro-scale scintillators, whose properties are challenging to quantify by conventional means: We extract the scintillation properties in perovskite nanocrystals of only a few hundreds of nanometers, observing strong photon bunching (g^((2) ) (0)>50). Our research paves the way for broader use of photon-coincidence measurement and methods from quantum optics in studying materials with complex optical properties in extremes regions of the electromagnetic spectrum.

physics.optics↗

Cavity Quantum Electrodynamics in Finite-Bandwidth Squeezed Reservoir

Light-matter interaction with squeezed vacuum has received much interest for the ability to enhance the native interaction strength between an atom and a photon with a reservoir assumed to have an infinite bandwidth. Here, we study a model of parametrically driven cavity quantum electrodynamics (cavity QED) for enhancing light-matter interaction while subjected to a finite-bandwidth squeezed vacuum drive. Our method is capable of unveiling the effect of relative bandwidth as well as squeezing required to observe the anticipated anti-crossing spectrum and enhanced cooperativity without the ideal squeezed bath assumption. Furthermore, we analyze the practicality of said models when including intrinsic photon loss due to resonators imperfection. With these results, we outline the requirements for experimentally implementing an effectively squeezed bath in solid-state platforms such as InAs quantum dot cavity QED such that \textit{in situ} control and enhancement of light-matter interaction could be realized.

quant-ph↗

Quantum sensitivity of parametric oscillators

Many quantum systems exhibit high sensitivity to their initial conditions, where microscopic quantum fluctuations can significantly influence macroscopic observables. Understanding how quantum states may influence the behavior of nonlinear dynamic systems may open new avenues in controlling light-matter interactions. To explore this issue, we analyze the sensitivity of a fundamental quantum optical process - parametric oscillation - to quantum initializations. Focusing on optical parametric oscillators (OPOs), we demonstrate that the quantum statistics of arbitrary initial states are imprinted in the early-stage dynamics and can persist in the steady-state probabilities. We derive the "quantum sensitivity" of parametric oscillators, linking the initial quantum state to the system's steady-state outcomes, highlighting how losses and parametric gain govern the system's quantum sensitivity. Moreover, we show that these findings extend beyond OPOs to a broader class of nonlinear systems, including Josephson junction based superconducting circuits. Our work opens the way to a new class of experiments that can test the sensitivity of macroscopic systems to quantum initial conditions and offers a pathway for controlling systems with quantum degrees of freedom.

quant-ph↗

Observing the dynamics of quantum states generated inside nonlinear optical cavities

Quantum states at optical frequencies are often generated inside cavities to facilitate strong nonlinear interactions. However, measuring these quantum states with traditional homodyne techniques poses a challenge, as outcoupling from the cavity disturbs the state's quantum properties. Here, we propose a framework for reconstructing quantum states generated inside nonlinear optical cavities and observing their dynamics. Our approach directly imprints the field distribution of the cavity quantum state onto the statistics of bistable cavity steady-states. We propose a protocol to fully reconstruct the cavity quantum state, visualized in 2D phase-space, by measuring the changes in the steady-state statistics induced by a probe signal injected into the cavity under different condition. We experimentally demonstrate our approach in a degenerate optical parametric oscillator, generating and reconstructing the quasi-probability distribution of different quantum states. As a validation, we reconstruct the Husimi Q function of the cavity squeezed vacuum state. In addition, we observe the evolution of the quantum vacuum state inside the cavity as it undergoes phase-sensitive amplification. By enabling generation and measurement of quantum states in a single nonlinear optical cavity, our method realizes an "end-to-end" approach to intracavity quantum tomography, facilitating studies of quantum optical phenomena in nonlinear driven-dissipative systems.

quant-ph↗

Computational metaoptics for imaging

Metasurfaces -- ultrathin structures composed of subwavelength optical elements -- have revolutionized light manipulation by enabling precise control over electromagnetic waves' amplitude, phase, polarization, and spectral properties. Concurrently, computational imaging leverages algorithms to reconstruct images from optically processed signals, overcoming limitations of traditional imaging systems. This review explores the synergistic integration of metaoptics and computational imaging, "computational metaoptics," which combines the physical wavefront shaping ability of metasurfaces with advanced computational algorithms to enhance imaging performance beyond conventional limits. We discuss how computational metaoptics addresses the inherent limitations of single-layer metasurfaces in achieving multifunctionality without compromising efficiency. By treating metasurfaces as physical preconditioners and co-designing them with reconstruction algorithms through end-to-end (inverse) design, it is possible to jointly optimize the optical hardware and computational software. This holistic approach allows for the automatic discovery of optimal metasurface designs and reconstruction methods that significantly improve imaging capabilities. Advanced applications enabled by computational metaoptics are highlighted, including phase imaging and quantum state measurement, which benefit from the metasurfaces' ability to manipulate complex light fields and the computational algorithms' capacity to reconstruct high-dimensional information. We also examine performance evaluation challenges, emphasizing the need for new metrics that account for the combined optical and computational nature of these systems. Finally, we identify new frontiers in computational metaoptics which point toward a future where computational metaoptics may play a central role in advancing imaging science and technology.

physics.optics↗

Automated modal analysis of entanglement with bipartite self-configuring optics

Entanglement is a unique feature of quantum mechanics. In coupled systems of light and matter, entanglement manifests itself in the linear superposition of multipartite quantum states (e.g., parametrized by the multiple spatial, spectral, or temporal degrees of freedom of a light field). In bipartite systems, the Schmidt decomposition provides a modal decomposition of the entanglement structure over independent, separable states. Although ubiquitous as a mathematical tool to describe and measure entanglement, there exists no general efficient experimental method to decompose a bipartite quantum state onto its Schmidt modes. Here, we propose a method that relies on bipartite self-configuring optics that automatically ``learns'' the Schmidt decomposition of an arbitrary pure quantum state. Our method is agnostic to the degrees of freedom over which quantum entanglement is distributed and can reconstruct the Schmidt modes and values by variational optimization of the network's output powers or coincidences. We illustrate our method with numerical examples of spectral entanglement analysis for biphotons generated via spontaneous parametric down conversion and provide experimental guidelines for its realization, including the influence of losses and impurities. Our method provides a versatile and scalable way of analyzing entanglement in bipartite integrated quantum photonic systems.

quant-ph↗

Large-scale self-assembled nanophotonic scintillators for X-ray imaging

Scintillators are essential for converting X-ray energy into visible light in imaging technologies. Their widespread application in imaging technologies has been enabled by scalable, high-quality, and affordable manufacturing methods. Nanophotonic scintillators, which feature nanostructures at the scale of their emission wavelength, provide a promising approach to enhance emission properties like light yield, decay time, and directionality. However, scalable fabrication of such nanostructured scintillators has been a significant challenge, impeding their widespread adoption. Here, we present a scalable fabrication method for large-area nanophotonic scintillators based on the self-assembly of chalcogenide glass photonic crystals. This technique enables the production of nanophotonic scintillators over wafer-scale areas, achieving a six-fold enhancement in light yield compared to unpatterned scintillators. We demonstrate this approach using a conventional X-ray scintillator material, cerium-doped yttrium aluminum garnet (YAG:Ce). By analyzing the influence of surface nanofabrication disorder, we establish its effect on imaging performance and provide a route towards large-scale scintillation enhancements without decrease in spatial resolution. Finally, we demonstrate the practical applicability of our nanophotonic scintillators through X-ray imaging of biological and inorganic specimens. Our results indicate that this scalable fabrication technique could enable the industrial implementation of a new generation of nanophotonic-enhanced scintillators, with significant implications for advancements in medical imaging, security screening, and nondestructive testing.

physics.optics↗

Nonreciprocal scintillation using one-dimensional magneto-optical photonic crystals

Scintillation describes the conversion of high-energy particles into light in transparent media and finds diverse applications such as high-energy particle detection and industrial and medical imaging. This process operates on multiple timescales, with the final radiative step consisting of spontaneous emission, which can be modeled within the framework of quasi-equilibrium fluctuational electrodynamics. Scintillation can therefore be controlled and enhanced via nanophotonic effects, which has been proposed and experimentally demonstrated. Such designs have thus far obeyed Lorentz reciprocity, meaning there is a direct equivalence between scintillation emission and absorption by the scintillator. However, scintillators that do not obey Lorentz reciprocity have not been explored, even though they represent a novel platform for probing emission which is both nonequilibrium and nonreciprocal in nature. In this work, we propose to harness nonreciprocity to achieve directional control of scintillation emission, granting an additional degree of control over scintillation. Such directionality of light output is important in improving collection efficiencies along the directions where detectors are located. We present the design of a nonreciprocal scintillator using a one-dimensional magnetophotonic crystal in the Voigt configuration. Our work demonstrates the potential of controlling nonequilibrium emission such as scintillation by breaking reciprocity and expands the space of nanophotonic design for achieving such control.

physics.optics↗

Non-reciprocal frequency conversion in a multimode nonlinear system

Nonlinear optics has become the workhorse for countless applications in classical and quantum optics, from optical bistability to single photon pair generation. However, the intrinsic weakness of optical nonlinearity has meant that large input powers and weak output powers are often a necessity in nonlinear frequency conversion. Here, motivated by recent advances in using non-Hermitian photonics and gain/loss engineering to enable non-reciprocal light transport, we explore how the interplay between non-Hermiticity and optical nonlinearity leads to a fundamentally new regime of nonlinear frequency conversion. We show how non-Hermitian coupling between discrete frequency modes can result in non-reciprocal flow of energy in the frequency dimension, closely resembling the non-Hermitian skin effect (NHSE). Applying our theory to a multimode nonlinear cavity supporting cascaded nonlinear processes, we create an asymmetric infrared (IR) comb that features a ``skin'' frequency mode populated with efficiency exceeding 85\%. Furthermore, we demonstrate how three-wave mixing processes in the non-reciprocal infrared comb we generate enables terahertz (THz) generation exceeding the Manley-Rowe limit. We then show how the non-reciprocal frequency conversion is robust against cavity defects and disorder that cause random fluctuations in the dissipation rate for different modes. Moreover, in certain regimes, the nonlinear, non-Hermitian system supports stable limit cycles that can enable multimode pulsing with picosecond pulse widths and GHz repetition rates. Finally, we explore how the system can be applied to generate simultaneous IR and THz frequency combs, potentially unlocking novel applications in spectroscopy and metrology.

physics.optics↗