arXiv subjects

Charles Santori

Publications and source records attributed to Charles Santori.

31 records · Page 2Linked to original sources

arXiv2007

Coherent Population Trapping of Electron Spins in a Semiconductor

In high-purity n-type GaAs under strong magnetic field, we are able to isolate a lambda system composed of two Zeeman states of neutral-donor bound electrons and the lowest Zeeman state of bound excitons. When the two-photon detuning of this system is zero, we observe a pronounced dip in the excited-state photoluminescence indicating the creation of the coherent population-trapped state. Our data are consistent with a steady-state three-level density-matrix model. The observation of coherent population trapping in GaAs indicates that this and similar semiconductor systems could be used for various EIT-type experiments.

cond-mat.mes-hall↗

arXiv2006

Coherent Population Trapping of Single Spins in Diamond Under Optical Excitation

Coherent population trapping is demonstrated in single nitrogen-vacancy centers in diamond under optical excitation. For sufficient excitation power, the fluorescence intensity drops almost to the background level when the laser modulation frequency matches the 2.88 GHz splitting of the ground states. The results are well described theoretically by a four-level model, allowing the relative transition strengths to be determined for individual centers. The results show that all-optical control of single spins is possible in diamond.

quant-ph↗

arXiv2006

Millisecond spin-flip times of donor-bound electrons in GaAs

We observe millisecond spin-flip relaxation times of donor-bound electrons in high-purity n-GaAs . This is three orders of magnitude larger than previously reported lifetimes in n-GaAs . Spin-flip times are measured as a function of magnetic field and exhibit a strong power-law dependence for fields greater than 4 T . This result is in qualitative agreement with previously reported theory and measurements of electrons in quantum dots.

cond-mat.mes-hall↗

arXiv2006

Coherent Population Trapping in Diamond N-V Centers at Zero Magnetic Field

Coherent population trapping at zero magnetic field was observed for nitrogen-vacancy centers in diamond under optical excitation. This was measured as a reduction in photoluminescence when the detuning between two excitation lasers matched the 2.88 GHz crystal-field splitting of the color center ground states. This behavior is highly sensitive to strain, which modifies the excited states, and was unexpected following recent experiments demonstrating optical readout of single nitrogen-vacancy electron spins based on cycling transitions. These results demonstrate for the first time that three-level Lambda configurations suitable for proposed quantum information applications can be realized simultaneously for all four orientations of nitrogen-vacancy centers at zero magnetic field.

cond-mat.mes-hall↗

arXiv2005

Photon correlation studies of single GaN quantum dots

We present measurements of the second-order coherence function on emission from single GaN quantum dots. In some cases a large degree of photon antibunching is observed, demonstrating isolation of a single quantum system. For a selected quantum dot, we study the dependence of photon antibunching on excitation power and temperature. Using pulsed excitation, we demonstrate an ultraviolet triggered single-photon source operating at a wavelength of 358 nm.

cond-mat.mes-hall↗

arXiv2003

Sub-microsecond correlations in photoluminescence from InAs quantum dots

Photon correlation measurements reveal memory effects in the optical emission of single InAs quantum dots with timescales from 10 to 800 ns. With above-band optical excitation, a long-timescale negative correlation (antibunching) is observed, while with quasi-resonant excitation, a positive correlation (blinking) is observed. A simple model based on long-lived charged states is presented that approximately explains the observed behavior, providing insight into the excitation process. Such memory effects can limit the internal efficiency of light emitters based on single quantum dots, and could also be problematic for proposed quantum-computation schemes.

cond-mat.mes-hall↗

arXiv2003

Enhanced single-photon emission from a quantum dot in a micropost microcavity

We demonstrate a single-photon source based on a quantum dot in a micropost microcavity that exhibits a large Purcell factor together with a small multi-photon probability. For a quantum dot on resonance with the cavity, the spontaneous emission rate is increased by a factor of five, while the probability to emit two or more photons in the same pulse is reduced to 2% compared to a Poisson-distributed source of the same intensity. In addition to the small multi-photon probability, such a strong Purcell effect is important in a single-photon source for improving the photon outcoupling efficiency and the single-photon generation rate, and for bringing the emitted photon pulses closer to the Fourier transform limit.

quant-ph↗

arXiv2003

Entanglement formation and violation of Bell's inequality with a semiconductor single photon source

We report the generation of polarization-entangled photons, using a quantum dot single photon source, linear optics and photodetectors. Two photons created independently are observed to violate Bell's inequality. The density matrix describing the polarization state of the postselected photon pairs is also reconstructed, and agrees well with a simple model predicting the quality of entanglement from the known parameters of the single photon source. Our scheme provides a method to generate no more than one entangled photon pair per cycle, a feature useful to enhance quantum cryptography protocols using entangled photons.

quant-ph↗

arXiv2002

An Efficient Source of Single Photons: A Single Quantum Dot in a Micropost Microcavity

We have demonstrated efficient production of triggered single photons by coupling a single semiconductor quantum dot to a three-dimensionally confined optical mode in a micropost microcavity. The efficiency of emitting single photons into a single-mode travelling wave is approximately 38%, which is nearly two orders of magnitude higher than for a quantum dot in bulk semiconductor material. At the same time, the probability of having more than one photon in a given pulse is reduced by a factor of seven as compared to light with Poissonian photon statistics.

quant-ph↗

arXiv2002

Polarization-Correlated Photon Pairs from a Single Quantum Dot

Polarization correlation in a linear basis, but not entanglement, is observed between the biexciton and single-exciton photons emitted by a single InAs quantum dot in a two-photon cascade. The results are well described quantitatively by a probabilistic model that includes two decay paths for a biexciton through a non-degenerate pair of one-exciton states, with the polarization of the emitted photons depending on the decay path. The results show that spin non-degeneracy due to quantum-dot asymmetry is a significant obstacle to the realization of an entangled-photon generation device.

cond-mat.mes-hall↗

arXiv2001

Time-resolved spectroscopy of multi-excitonic decay in an InAs quantum dot

The multi-excitonic decay process in a single InAs quantum dot is studied through high-resolution time-resolved spectroscopy. A cascaded emission sequence involving three spectral lines is seen that is described well over a wide range of pump powers by a simple model. The measured biexcitonic decay rate is about 1.5 times the single-exciton decay rate. This ratio suggests the presence of selection rules, as well as a significant effect of the Coulomb interaction on the biexcitonic wavefunction.

cond-mat.mes-hall↗

arXiv2001

Electrostatic force spectroscopy of a single InAs quantum dot

Electrostatic force microscopy at cryogenic temperatures was used to probe the electrostatic interaction between a conductive atomic force microscopy tip and electronic charges trapped in an InAs quantum dot. Measurement of the self-oscillation frequency shift of the cantilever as a function of tip-sample bias voltage revealed discrete jumps at certain voltages when the tip was positioned above a quantum dot. These jumps are attributed to single-electron filling of the electronic states of the quantum dot. The estimated resonant energies of two s-states and four p-states are compared with the experimental data obtained for an ensemble of quantum dots by the capacitance measurement technique.

cond-mat↗

arXiv2000

Triggered single photons from a quantum dot

We demonstrate a new method for generating triggered single photons. After a laser pulse generates excitons inside of a single quantum dot, electrostatic interactions between them and the resulting spectral shifts allow a single emitted photon to be isolated. Autocorrelation measurements show a reduction of the two-photon probability to 0.12 times the value for Poisson light. Strong anti-bunching persists when the emission is saturated. The emitted photons are also polarized.

cond-mat.mes-hall↗