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Chengbao Jiang

Publications and source records attributed to Chengbao Jiang.

13 recordsLinked to original sources

Saturated and Anisotropic Magnetostriction in an Altermagnet

Magnetostriction, a fundamental phenomenon bridging magnetism and mechanics, has enabled a broad spectrum of applications. For almost two centuries, it has been mainly investigated for ferromagnets. Regarding the magnetostriction of antiferromagnets (AFMs), limitedly known examples for both conventional collinear AFMs and noncollinear AFMs predominantly exhibit non-saturating magnetic-field dependence. Herein, we report an easily saturated magnetostriction effect in a prototypical altermagnet - MnTe, which is an emerging class of collinear AFMs with special crystal symmetries. For high-quality MnTe single crystals, the magnetostriction saturates under a moderate field of ~0.7 T with an intriguing two-fold-symmetry anisotropy. First-principles calculations reveal that the saturated and anisotropic magnetostriction originates from symmetry-allowed coupling between elastic strain and its N\'eel order parameter. These findings break the traditional wisdom on antiferromagnetic magnetostriction.

cond-mat.mtrl-sci

Giant Room-Temperature Third-Order Electrical Transport in a Thin-Film Altermagnet Candidate

Quantum geometry, a quantum mechanical quantity comprised of Berry curvature and quantum metric, describes the geometric structure of the electronic bands in solids. The correlation between nontrivial quantum geometry and quantum materials leads to new findings in condensed matter systems. Here we demonstrate that altermagnets, with spontaneously broken time-reversal (T)- half-lattice-translation and parity-time symmetry, host both T-odd and T-even quantum geometric quantities that simultaneously manifest themselves despite the vanishing net magnetization. Consequently, giant room-temperature third-order electrical transport responses with sizable quantum geometric contributions are observed in (101)-oriented RuO2 thin films, an altermagnetic candidate; in particular, the third-order Hall effect is intimately correlated with altermagnetic order and can serve as a promising tool for detecting the Neel vector. Our work not only supports the existence of altermagnetism in 8-nm-thick RuO2 thin films, but also shows altermagnets as a versatile platform for exploring quantum geometry and constructing quantum electronic and spintronic devices.

cond-mat.mes-hall

Spin-Splitting Magnetoresistance in Altermagnetic RuO2 Thin Films

The recently discovered altermagnets, featured by the exotic correlation of magnetic exchange interaction and alternating crystal environments, have offered exciting cutting-edge opportunities for spintronics. Nevertheless, the altermagnetism of RuO2, one of the earliest-discovered altermagnets, is currently under intense debate. Here we try to resolve this controversy by demonstrating an altermagnetic spin-splitting magnetoresistance (SSMR) effect that is driven by a spin current associated with the giant nonrelativistic spin splitting of an altermagnet. Compared to the spin Hall magnetoresistance induced by a conventional relativistic spin current, the SSMR is characterized by unusual angular dependence with a phase-shift feature underpinned by the Neel-vector orientation and pronounced temperature dependence caused by its susceptibility to electron scattering. Through systematical investigations on the magnetoresistance of (101)-RuO2/Co bilayers, we disentangle a sizable SSMR and hence unveil a Neel vector along [001] direction. Our work not only demonstrates a simple electric avenue to probing the Neel vector of altermagnets, but also indicates long-range magnetic order in thin films of RuO2.

cond-mat.mes-hall

Antiferromagnetism in Ni-Based Superconductors

Due to the lack of any magnetic order down to 1.7 K in the parent bulk compound NdNiO2, the recently discovered 9-15 K superconductivity in the infinite-layer Nd0.8Sr0.2NiO2 thin films has provided an exciting playground for unearthing new superconductivity mechanisms. In this letter, we report the successful synthesis of a series of superconducting Nd0.8Sr0.2NiO2 thin films ranging from 8 to 40 nm. We observe the large exchange bias effect between the superconducting Nd0.8Sr0.2NiO2 films and a thin ferromagnetic layer, which suggests the existence of the antiferromagnetic order. Furthermore, the existence of the antiferromagnetic order is evidenced by X-ray magnetic linear dichroism measurements. These experimental results are fundamentally critical for the current field.

cond-mat.supr-con

Electric-Field-Controlled Antiferromagnetic Spintronic Devices

In recent years, the field of antiferromagnetic spintronics has been substantially advanced. Electric-field control is a promising approach to achieving ultra-low power spintronic devices via suppressing Joule heating. In this article, cutting-edge research, including electric-field modulation of antiferromagnetic spintronic devices using strain, ionic liquids, dielectric materials, and electrochemical ionic migration, are comprehensively reviewed. Various emergent topics such as the Neel spin-orbit torque, chiral spintronics, topological antiferromagnetic spintronics, anisotropic magnetoresistance, memory devices, two-dimensional magnetism, and magneto-ionic modulation with respect to antiferromagnets are examined. In conclusion, we envision the possibility of realizing high-quality room-temperature antiferromagnetic tunnel junctions, antiferromagnetic spin logic devices, and artificial antiferromagnetic neurons. It is expected that this work provides an appropriate and forward-looking perspective that will promote the rapid development of this field.

cond-mat.mes-hall

Giant Piezospintronic Effect in a Noncollinear Antiferromagnetic Metal

One of the main bottleneck issues for room-temperature antiferromagnetic spintronic devices is the small signal read-out owing to the limited anisotropic magnetoresistance in antiferromagnets. However, this could be overcome by either utilizing the Berry-curvature-induced anomalous Hall resistance in noncollinear antiferromagnets or establishing tunnel junction devices based on effective manipulation of antiferromagnetic spins. In this work, we demonstrate the giant piezoelectric strain control of the spin structure and the anomalous Hall resistance in a noncollinear antiferromagnetic metal - D019 hexagonal Mn3Ga. Furthermore, we built tunnel junction devices with a diameter of 200 nm to amplify the maximum tunneling resistance ratio to more than 10% at room-temperature, which thus implies significant potential of noncollinear antiferromagnets for large signal-output and high-density antiferromagnetic spintronic device applications.

cond-mat.mes-hall

Observation of the Anomalous Hall Effect in a Collinear Antiferromagnet

Time-reversal symmetry breaking is the basic physics concept underpinning many magnetic topological phenomena such as the anomalous Hall effect (AHE) and its quantized variant. The AHE has been primarily accompanied by a ferromagnetic dipole moment, which hinders the topological quantum states and limits data density in memory devices, or by a delicate noncollinear magnetic order with strong spin decoherence, both limiting their applicability. A potential breakthrough is the recent theoretical prediction of the AHE arising from collinear antiferromagnetism in an anisotropic crystal environment. This new mechanism does not require magnetic dipolar or noncollinear fields. However, it has not been experimentally observed to date. Here we demonstrate this unconventional mechanism by measuring the AHE in an epilayer of a rutile collinear antiferromagnet RuO$_2$. The observed anomalous Hall conductivity is large, exceeding 300 S/cm, and is in agreement with the Berry phase topological transport contribution. Our results open a new unexplored chapter of time-reversal symmetry breaking phenomena in the abundant class of collinear antiferromagnetic materials.

cond-mat.mtrl-sci

A two-dimensional electron gas based on a 5s oxide with high room-temperature mobility and strain sensitivity

The coupling of optical and electronic degrees of freedom together with quantum confinement in low-dimensional electron systems is particularly interesting for achieving exotic functionalities in strongly correlated oxide electronics. Recently, high room-temperature mobility has been achieved for a large bandgap transparent oxide - BaSnO$_3$ upon extrinsic La or Sb doping, which has excited significant research attention. In this work, we report the observation of room-temperature ferromagnetism in BaSnO$_3$ thin films and the realization of a two-dimensional electron gas (2DEG) on the surface of transparent BaSnO$_3$ via oxygen vacancy creation, which exhibits a high carrier density of $\sim 7.72*10^{14} /{\rm cm}^2$ and a high room-temperature mobility of ~18 cm$^2$/V/s. Such a 2DEG is rather sensitive to strain and a less than 0.1% in-plane biaxial compressive strain leads to a giant resistance enhancement of 350% (more than 540 kOhm/Square) at room temperature. Thus, this work creates a new path to exploring the physics of low-dimensional oxide electronics and devices applicable at room temperature.

cond-mat.str-el

Integration of the Noncollinear Antiferromagnetic Metal Mn3Sn onto Ferroelectric Oxides for Electric-Field Control

Non-collinear antiferromagnetic materials have received dramatically increasing attention in the field of spintronics as their exotic topological features such as the Berry-curvature-induced anomalous Hall effect and possible magnetic Weyl states could be utilized in future topological antiferromagnetic spintronic devices. In this work, we report the successful integration of the antiferromagnetic metal Mn3Sn thin films onto ferroelectric oxide PMN-PT. By optimizing growth, we realized the large anomalous Hall effect with small switching magnetic fields of several tens mT fully comparable to those of bulk Mn3Sn single crystals, anisotropic magnetoresistance and negative parallel magnetoresistance in Mn3Sn thin films with antiferromagnetic order, which are similar to the signatures of the Weyl state in bulk Mn3Sn single crystals. More importantly, we found that the anomalous Hall effect in antiferromagnetic Mn3Sn thin films can be manipulated by electric fields applied onto the ferroelectric materials, thus demonstrating the feasibility of Mn3Sn-based topological spintronic devices operated in an ultralow power manner.

cond-mat.mtrl-sci

Antiferromagnetic Piezospintronics

Antiferromagnets naturally exhibit three obvious advantages over ferromagnets for memory device applications: insensitivity to external magnetic fields, much faster spin dynamics (~THz) and higher packing density due to the absence of any stray field. Recently, antiferromagnetic spintronics emerges as a cutting-edge field in the magnetic community. The key mission of this rapidly rising field is to steer the spins or spin axes of antiferromagnets via external stimuli and then realize advanced devices based on their physical property changes. Herein, the state of the art of antiferromagnetic spintronics is presented. Subsequently, the history of ferromagnetic/ferroelectric multiferroic composites is briefly revisited. Finally, we introduce an ultralow-power, long-range, and magnetic-field-insensitive approach for harnessing antiferromagnetic spins based on our recent experimental progress, i.e., piezoelectric strain control. Relevant theoretical and experimental studies have formed an attractive new branch in antiferromagnetic spintronics, which we coin as antiferromagnetic piezospintronics.

cond-mat.mes-hall

A Piezoelectric, Strain-Controlled Antiferromagnetic Memory Insensitive to Magnetic Fields

Spintronic devices based on antiferromagnetic (AFM) materials hold the promise of fast switching speeds and robustness against magnetic fields. Different device concepts have been predicted and experimentally demonstrated, such as low-temperature AFM tunnel junctions that operate as spin-valves, or room-temperature AFM memory, for which either thermal heating in combination with magnetic fields, or Néel spin-orbit torque is used for the information writing process. On the other hand, piezoelectric materials were employed to control magnetism by electric fields in multiferroic heterostructures, which suppresses Joule heating caused by switching currents and may enable low energy-consuming electronic devices. Here, we combine the two material classes to explore changes of the resistance of the high-Néel-temperature antiferromagnet MnPt induced by piezoelectric strain. We find two non-volatile resistance states at room temperature and zero electric field, which are stable in magnetic fields up to 60 T. Furthermore, the strain-induced resistance switching process is insensitive to magnetic fields. Integration in a tunnel junction can further amplify the electroresistance. The tunneling anisotropic magnetoresistance reaches ~11.2% at room temperature. Overall, we demonstrate a piezoelectric, strain-controlled AFM memory which is fully operational in strong magnetic fields and has potential for low-energy and high-density memory applications.

cond-mat.mtrl-sci

Giant magnetostriction in Tb-doped Fe83Ga17 melt-spun ribbons

Giant magnetostriction is achieved in the slightly Tb-doped Fe83Ga17 melt-spun ribbons. The tested average perpendicular magnetostriction is -886 ppm along the melt-spun ribbon direction in the Fe82.89Ga16.88Tb0.23 alloy. The calculated parallel magnetostriction is 1772 ppm, more than 4 times as large as that of binary Fe83Ga17 alloy. The enhanced magnetostriction should be attributed to a small amount of Tb solution into the A2 matrix phase during rapid solidification. The localized strong magnetocrystalline anisotropy of Tb element is suggested to cause the giant magnetostriction.

cond-mat.mtrl-sci

Stable magnetostructural coupling with tunable magnetoresponsive effects in hexagonal phase-transition ferromagnets

The magnetostructural coupling between the structural and the magnetic transition plays a crucial role in magnetoresponsive effects in a martensitic-transition system. A combination of various magnetoresponsive effects based on this coupling may facilitate the multifunctional applications of a host material. Here, we demonstrate a possibility to obtain a stable magnetostructural coupling in a broad temperature window from 350 to 70 K, showing tunable magnetoresponsive effects, based on simultaneous manipulation of the phase stability and the magnetic structure by suitable chemical substitution of iron in MnNiGe. The resultant MnNiGe:Fe exhibits a magnetic-field-induced martensitic transition from paramagnetic austenite to ferromagnetic martensite, featuring (i) a large volume increase, (ii) a distinct magnetization change, (iii) small thermal hysteresis and (iv) a giant negative magnetocaloric effect. The results indicate that stable magnetostructural coupling is accessible in hexagonal phase-transition systems to attain the magnetoresponsive effects with broad tunability.

cond-mat.mtrl-sci