arXiv subjects

Chenglin Shang

Publications and source records attributed to Chenglin Shang.

10 recordsLinked to original sources

arXiv2026

Vacancy Order and Physical Properties of a Ternary Compound Fe0.68Pd0.80Te with an {\alpha}-Fe1+xTe-Type Structure

We report the identification and characterization of a new compound Fe0.68Pd0.80Te with an {\alpha}-Fe1+xTe prototype structure. Different from the Fe-square net and minor occupancy of interstitial Fe-sites in Fe1+xTe, Fe0.68Pd0.80Te is featured by a Pdsquare net and near 68% occupancy of the corresponding interstitial Fe-sites. Furthermore, noncontact atomic force microscopy and X-ray diffraction provide evidence for the existence of a 3*3*3 Pd-vacancy order in this layered material. A spin-glass ground state below Tg 40 K is identified via magnetic characterization. Electrical transport measurements show that Fe0.68Pd0.80Te is a semiconductor with a very small band gap below 10 meV. It has weak negative magnetoresistance and holelike charge carriers below room temperature. Our results demonstrate its potentials for further exploring various quantum phenomena.

cond-mat.mtrl-sci↗

arXiv2026

Complex Temperature-dependent Thermal Conductivity in a Sawtooth Chain Magnet Fe$_\mathrm{2}$SiSe$_\mathrm{4}$

Geometrically frustrated magnets provide an ideal platform for exploring the interplay between lattice geometry and spin degrees of freedom. Here, we investigate the interactions between lattice and spin via thermal-transport measurements on the triangular sawtooth-lattice olivine magnet Fe$_\mathrm{2}$SiSe$_\mathrm{4}$, which exhibits successive magnetic transitions at $T_1 = 110$ K (antiferromagnetic) and $T_2 = 50$ K (ferrimagnetic). Although phonons dominate the thermal conductivity, its temperature dependence displays a pronounced double-peak structure arising from spin-phonon coupling. In the intermediate temperature range between $T_1$ and $T_2$ , resonant scattering of phonons by magnetic excitations around 5 meV produces a broad maximum around 60 K. Below $T_2$, the resonant spin-phonon scattering is strongly suppressed, leading to a rapid increase in thermal conductivity upon cooling and a pronounced low-temperature peak near 11 K, characteristic of heat transport governed by conventional phonon scattering mechanisms. Notably, this low-temperature peak is enhanced by a factor of $\sim 5$ compared to the broad maximum at higher temperatures. These results demonstrate the strong sensitivity of thermal transport to spin-lattice interactions and highlight spin-phonon scattering as an effective mechanism for tailoring thermal conductivity in geometrically frustrated magnets.

cond-mat.str-el↗

arXiv2026

Noncollinear antiferromagnetic structure and physical properties of CrRhAs with distorted kagome lattice

CrRhAs was theoretically proposed to be a kagome metal with unusual magnetic ground states; however, little is known about its magnetic structure and physical properties experimentally. Here, we present an experimental investigation of CrRhAs with ZrNiAl-type structure and a distorted Cr kagome lattice. CrRhAs is an antiferromagnet with TN = 149 K. Powder neutron diffraction analysis reveals a noncollinear antiferromagnetic structure with propagation vector k = (1/3, 1/3, 1/2), which features a ferromagnetic second nearest neighbor coupling in the kagome plane that is different from the prediction in previous density functional theory calculations. Furthermore, CrRhAs exhibits anomalous electrical transport properties which are possibly related to multiband effects and strong spin fluctuations. For the temperature-dependent longitudinal resistivity \r{ho}xx, it is semiconductinglike above TN and becomes metallic below TN . The Hall coefficients exhibit two sign changes near 70 and 300 K. Combined with the results of heat capacity measurements, a large Kadowaki-Woods ratio {\alpha} = 33.9 {\mu}{\Omega} cm mol2 K2/J2 is obtained. The above results suggest CrRhAs is a strongly correlated kagome metal with multiband and noncollinear magnetic structure features.

cond-mat.str-el↗

arXiv2025

Field-induced magnetic order in DyTa$_7$O$_{19}$ with two-dimensional pseudospin-$\frac{1}{2}$ triangular lattice

The magnetic ground state of geometrically frustrated antiferromagnet attracts great research interests due to the possibility to realize novel quantum magnetic state such as a quantum spin liquid. Here we present a comprehensive magnetic characterization of DyTa$_7$O$_{19}$ with ideal two-dimensional triangular lattice. DyTa$_7$O$_{19}$ exhibits $c$-axis single-ion magnetic anisotropy. Although long-range magnetic order is not observed down to 100 mK under zero field, by applying a small magnetic field ($\sim$0.1 T), a magnetically ordered state with net magnetization of $M_s$/3 below $T_m$=0.14 K is identified ($M_s$ denotes the saturated magnetization). We argue that this state is an up-up-down magnetic structure phase driven by the dipole-dipole interactions between Ising-like spins of Dy$^{3+}$ in a two-dimensional triangular lattice, since its ordering temperature and temperature-field phase diagram can be well explained by the theoretical calculations based on dipolar interactions. DyTa$_7$O$_{19}$ could be viewed as a rare material platform that realizing pure Ising-like dipolar interaction in a geometrically frustrated lattice.

cond-mat.str-el↗

arXiv2024

Structural and magnetic characterization of CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$ with two-dimensional pseudospin-1/2 triangular lattice

Triangular lattice antiferromagnets are prototypes for frustrated magnetism and may potentially realize novel quantum magnetic states such as a quantum spin liquid ground state. A recent work suggests NdTa$_7$O$_{19}$ with rare-earth triangular lattice is a quantum spin liquid candidate and highlights the large family of rare-earth heptatantalates as a framework for quantum magnetism investigation. In this paper, we report the structural and magnetic characterization of CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$. Both compounds are isostructural to NdTa$_7$O$_{19}$ with no detectable structural disorder. For CeTa$_7$O$_{19}$, the crystal field energy levels and parameters are determined by inelastic neutron scattering measurements. Based on the crystal field result, the magnetic susceptibility data could be well fitted and explained, which reveals that CeTa$_7$O$_{19}$ is a highly anisotropic Ising triangular-lattice antiferromagnet ($g_z$/$g_{xy}$$\sim$3) with very weak exchange interaction (J$\sim$0.22~K). For YbTa$_7$O$_{19}$, millimeter sized single crystals could be grown. The anisotropic magnetization and electron spin resonance data show that YbTa$_7$O$_{19}$ has a contrasting in-plane magnetic anisotropy with $g_z$/$g_{xy}$$\sim$0.67 similar as that of YbMgGaO$_4$. The above results indicate that CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$ with pseudospin-1/2 ground states might either be quantum spin liquid candidate materials or find applications in adiabatic demagnetization refrigeration due to the weak exchange interaction.

cond-mat.str-el↗

arXiv2024

FePd2Te2: An Anisotropic Two-Dimensional Ferromagnet with One-Dimensional Fe Chains

Two-dimensional (2D) magnets have attracted significant attentions in recent years due to their importance in the research on both fundamental physics and spintronic applications. Here, we report the discovery of a new ternary compound FePd2Te2. It features a layered quasi-2D crystal structure with one-dimensional Fe zigzag chains extending along the b-axis in the cleavage plane. Single crystals of FePd2Te2 with centimeter-size could be grown. Density functional theory calculations, mechanical exfoliation and atomic force microscopy on these crystals reveal that they are 2D materialsthat can be thinned down to 5 nm. Magnetic characterization shows that FePd2Te2 is an easy-plane ferromagnet with Tc 183 K and strong in-plane uniaxial magnetic anisotropy. Magnetoresistance and anomalous Hall effect demonstrate that ferromagnetism could maintain in FePd2Te2 flakes with large coercivity. A crystal twinning effect is observed by scanning tunneling microscopy which makes the Fe chains right-angle bent in the cleavage plane and creates an intriguing spin texture. Our results show that FePd2Te2 is a correlated anisotropic 2D magnets that may attract multidisciplinary research interests.

cond-mat.mtrl-sci↗

arXiv2024

Magnetic properties of van der Waals layered single crystals DyOBr and SmOCl

Two-dimensional van der Waals single crystals DyOBr and SmOCl have been grown by flux method and their anisotropic magnetic properties are reported. DyOBr orders antiferromagnetically at T$_{N}$=9.5 K with magnetic moments lying along $a$-axis, similar as DyOCl. Its magnetic susceptibility shows an anomaly at T$^{*}$=30 K possibly due to the crystal field effect. Furthermore a 1/3 magnetization plateau is clearly observed under H$\parallel$a and H$\parallel$[110], which might be a field-induced spin-flop phase or some exotic quantum magnetic state. On the other hand, isostructural SmOCl undergoes an antiferromagnetic transition at T$_{N}$=7.1 K and exhibits a contrasting Ising-like perpendicular $c$-axis magnetic anisotropy, which could be well explained by our crystal field calculations. Both DyOBr and SmOCl are insulators with band gap of $\sim$5 eV, our results suggest they are promising in building van der Waals heterostructures and applications in multifunctional devices.

cond-mat.mtrl-sci↗

arXiv2023

High Performance Thin-film Lithium Niobate Modulator Applied ITO Composite Electrode with Modulation Efficiency of 1V*cm

Thin film lithium niobate (TFLN) based electro-optic modulator is widely applied in the field of broadband optical communications due to its advantages such as large bandwidth, high extinction ratio, and low optical loss, bringing new possibilities for the next generation of high-performance electro-optic modulators. However, the modulation efficiency of TFLN modulators is still relatively low when compared with Silicon and Indium-Phosphide (InP) based competitors. Due to the restriction of the trade-off between half-wave voltage and modulation length, it is difficult to simultaneously obtain low driving voltage and large modulating bandwidth. Here, we break this limitation by introducing Transparent Conductive Oxide (TCO) film, resulting in an ultra-high modulation efficiency of 1.02 V*cm in O-Band. The fabricated composite electrode not only achieves high modulation efficiency but also maintains a high electro-optic bandwidth, as demonstrated by the 3 dB roll-off at 108 GHz and the transmission of PAM-4 signals at 224 Gbit/s. Our device presents new solutions for the next generation of low-cost high-performance electro-optic modulators. Additionally, it paves the way for downsizing TFLN-based multi-channel optical transmitter chips.

physics.optics↗

arXiv2023

FeGe1-xSbx:a series of novel kagome metals with noncollinear antiferromagnetism

Kagome metals are important for exploring emergent phenomena due to the interplay between band topology and electron correlation.Motivated by the recent discovery of charge density wave in a kagome lattice antiferromagnetic FeGe,we investigate the impact of Sb doping on the structural,charge and magnetic order of FeGe.The charge density wave is rapidly suppressed by Sb doping(~1.5%) and the antiferromagnetic ordering temperature gradually shifts to 280K for FeGe0.7Sb0.3.For FeGe1-xSbx with x>0.1,crystal structures with slightly distorted Fe kagome lattice are formed.Their magnetic anisotropy has significant change,temperature driven spin-reorientation and field-induced spin-flop transition are identified from magnetization measurement.Interestingly,neutron diffraction reveals noncollinear antiferromagnetic structures widely exist below TN for all sample with x>0.1.This noncollinear magnetic orders could possibly be unconventional and resulted from onsite repulsion and filling condition of kagome flat band,as predicted by a recent theoretical work.

cond-mat.str-el↗

arXiv2022

Thin-Film Lithium Niobate based Dual-Polarization IQ modulator for Single-Carrier 1.6 Tb/s Transmission

We successfully demonstrate a monolithic integrated dual-polarization (DP) IQ modulator based on thin-film lithium niobate (TFLN) platform with a silicon substrate, which consists of IQ modulators, spot-size converters (SSCs) and a polarization rotator combiner (PRC). After coupled with polarization maintaining fibers, the measured insertion loss of the modulator is 12 dB. In addition, we experimentally achieve a single-carrier 1.6 Tb/s net bitrate transmission.

physics.app-ph↗