Searcharxiv⌕ Search

arXiv subjects

Christine Silberhorn

Publications and source records attributed to Christine Silberhorn.

At least 19 recordsLinked to original sources

Surface Acoustic Wave-Mediated Brillouin Temperature Sensor on Thin-Film Lithium Niobate

The emergence of thin-film lithium niobate (TFLN) has paved the way for realizing strong Brillouin interactions in lithium niobate platforms, enabling new opportunities in integrated photonics. However, fully harnessing stimulated Brillouin scattering (SBS) in TFLN for the plethora of Brillouin applications remains an exciting area of research, with significant opportunities for further exploration and technological advancement. Here, we present the first comprehensive experimental and numerical study of the surface acoustic wave (SAW)-mediated Brillouin temperature sensor on a TFLN-on-insulator chip. The proposed technique directly senses the surrounding environment via SAWs, providing an optical-power-efficient platform compatible with existing integrated photonic architectures. Exploiting the strong intermodal Brillouin interactions in x-cut TFLN waveguides, we report a high Brillouin gain of 24.8$ \pm $1.3\, m$^{-1}$W$^{-1}$ and a temperature coefficient of $-0.73$ $\pm$ 0.02\,MHz/$^\circ$C. Considering the anisotropic nature of lithium niobate, we investigate the temperature dependence of the Brillouin frequency for the propagation directions 0$^\circ$, 10$^\circ$, 20$^\circ$, 30$^\circ$ relative to the crystallographic y-axis.

physics.optics↗

On the temperature dependence of the optical band gap in the material system of lithium niobate and lithium tantalate

Lithium niobate and lithium tantalate see widespread use in optics and electronics, and are increasingly used for cryogenic applications. Despite their broad deployment, their optical band gap and its relation to the crystal stoichiometry are not well characterised as a function of temperature. In this work, we study the optical absorption properties of congruent, stoichiometric, MgO-doped and Er-doped lithium niobate as well as congruent lithium tantalate across the temperature range between 7~K and 1000~K by means of optical transmission spectroscopy. Our results demonstrate that the difference of the optical band gap typically observed at room temperature between different stoichiometries is not primarily attributable to the intrinsic electronic structure, but rather to different electron-phonon couplings and the average phonon energies. Additionally, we exemplarily study the temperature shift of the 523 nm absorption line in Er-doped lithium niobate due to the increased interest in optically active dopants. To facilitate future analyses, we present the open-source software suite PhoQS-Treat (Tauc Regression Edge Analysis Tool), which enables automated Tauc regressions alongside additional analytical capabilities. This work advances the development of high-performance lithium niobate-based devices.

cond-mat.mtrl-sci↗

An ultra-bright, highly-scalable, squeezed light source for hybrid quantum photonics

Hybrid quantum photonics seeks to combine the complementary advantages of continuous- and discrete-variable quantum optics. This typically entails photon-counting measurements on entangled states generated by interfering many single-mode squeezed-vacuum (SMSV) states. However, because conventional photon-counting schemes are mode-insensitive, it is critical that the SMSV states occupy a single, well-defined mode. Achieving this requires careful engineering of the process, which determines both the spatial and spectro-temporal properties of the generated state. In addition, the ideal source must be massively scalable, capable of efficiently generating strong squeezing, and remain compatible with existing detection schemes and fiber networks. Although many platforms address one or more of these requirements, satisfying all of them simultaneously remains challenging. Here, we present a source that meets all of these requirements: a single-pass, periodically poled, Type-II potassium titanyl phosphate (KTP) waveguide optimized for scalable hybrid quantum-photonic architectures. The SMSV state produced by the source has a measured effective mode number of 1.24. Furthermore, the source is extremely bright (producing up to 40 000 photons per pulse) and operates at a central wavelength of 1546nm, optimized for fiber-network compatibility and which, in combination with picosecond duration, also enables intrinsic photon-number resolution in superconducting nanowire single-photon detectors. Although this source constitutes an ideal source in a simplified picture, the ultimate limitations of any source will be governed by complex dynamics that arise when the system is driven at high-gain or due to unavoidable loss during state generation. We have therefore developed a complete theoretical framework that enables a comprehensive photon-counting-based characterization of the source.

quant-ph↗

Coherent temporal filtering of multimode parametric down-conversion using a quantum pulse gate

Spectrally pure and indistinguishable single photons are essential for quantum network platforms, where high-visibility interference underpins many quantum information protocols. However, most practical single-photon sources emit spectrally multimode states with reduced purity. Conventional spectral intensity filtering can partially improve purity but cannot select a well-defined temporal mode (TM). Here, we demonstrate coherent temporal filtering of a multimode parametric down-conversion (PDC) source using a quantum pulse gate (QPG) and benchmark its performance against conventional intensity filtering. The generated PDC photons exhibit strong spectral correlations, rendering extraction of pure heralded photons from the pair a challenge. We demonstrate that QPG filtering consistently generates heralded photons with purities above 0.90 regardless of the filter shape. Contrariwise, using spectral intensity filters yields mixed photons. Photon purities are probed with chronocyclic Q-function tomography. Furthermore, we demonstrate the versatility of QPG filtering by extracting structured TMs, including superposition of picosecond time bins. These results establish the QPG as a practical coherent filtering tool for quantum network applications.

quant-ph↗

A high-performance quantum pulse gate in thin-film lithium niobate

In this work, we demonstrate a quantum pulse gate (QPG) in thin-film lithium niobate. QPGs enable the selective manipulation and detection of temporal modes of quantum light and form the basis of numerous applications in photonic quantum technologies. To date, their widespread adaption is held back by two main limitations: restricted wavelength and polarization combinations of the involved fields and low normalized conversion efficiencies. We overcome these limitations through developing a QPG in thin-film lithium niobate. We design a waveguide geometry that provides the required dispersion properties for a highly efficient type-0 sum-frequency generation.We verify our design through mapping of the phase matching intensity, and demonstrate high-quality QPG operation by measuring a temporal-mode selectivity of (96.8$\pm$1.7)% on par with existing QPGs. Thanks to the strong confinement in thin-film lithium niobate, we succeed in demonstrating an internal conversion efficiency of (89.6$\pm$0.1)% for a pump power of only 20mW in front of our sample. This yields a lower-bound estimate for the normalized conversion efficiency of (1810$\pm$10)$\mathrm{W}^{-1}\mathrm{cm}^{-2}$, three orders of magnitude higher than in previous QPGs. Our results establish thin-film lithium niobate as ideal platform for high-performance QPGs and are a major step towards practical QPGs for photonic quantum technologies.

quant-ph↗

Input phase noise in Gaussian Boson sampling

Gaussian boson sampling is an important protocol for testing the performance of photonic quantum simulators. As such, various noise sources have been investigated that degrade the operation of such devices. In this paper, we examine a situation with phase noise between different modes of the input state leading to dephasing of the system. This models the phase fluctuations which remain even when the mean phase is controlled. We aim to determine whether these phase-noisy input states still form a computationally difficult problem. To do this, we use Matrix Product Operators to model the system, a technique recently used to model boson sampling scenarios. Our investigation finds that the Entanglement entropy grows linearly with the number of input states even for noisy input states. This implies that, unlike boson loss, this form of experimentally relevant noise remains difficult to simulate with tensor networks and may allow for the demonstration of quantum advantage without the need for implementing the challenging task of input-state phase stabilisation.

quant-ph↗

Demonstration of unpartible entanglement

We report on the first experimental verification of mode-independent entanglement. Commonly, the entanglement of a state is firmly based on pre-defined parties that are correlated, and the state might be disentangled when the definition of the parties is changed. Exceeding this party-dependent concept, we realize a type of quantum entanglement that persists even if the parties, in our case modes, are transformed. This safeguards the performance of entanglement in real-world applications, such as quantum communication settings involving noise and untrusted parties. For the state generation, we present an experimental scheme based on a fully reconfigurable temporally multiplexed interferometer with measurement-induced nonlinearities, which generates heralded two-photon states in two modes that are entangled for all choices of orthonormal mode basis. For the certification process, we utilize a tailored quantum-state tomography, achieving fidelities that validate the presence of mode-independent entanglement as a resilient and operationally advantageous quantum correlation.

quant-ph↗

Resource-efficient universal photonic processor based on time-multiplexed hybrid architectures

For the ever-growing field of quantum information processing, large-scale, efficient multi-port interferometers serving as photonic processors are required. In this context, the suitability of quantum walks as the interferometric base for universal computation has been theoretically proven. In this work, we bridge the gap between theoretical proposals and state-of-the-art experimental capabilities by providing the recipe for the implementation of a universal photonic processor in discrete-time quantum walks. Specifically, we present the protocol how to translate arbitrary linear transformations into the coin and step operator of a quantum walk and map these to the experimental parameters of the established time-multiplexed platform. We show that our interface is highly scalable and resource-efficient due to the hybrid encoding consisting of multiple degrees of freedom. Finally, we prove that our system is highly resilient against experimental imperfections and show that it compares favorably against existing architectures.

quant-ph↗

Macroscopic photon counting beating the Poisson noise limit

Photon counting is a cornerstone of quantum optics. Here, we demonstrate precisely counting from 0 to over 9000 photons, beating the Poisson noise limit by at least $4.1~\mathrm{dB}$ across this range. We achieve sub-single-photon precision up to 276 photons per pulse. To do so, we multiplex eight intrinsically photon-number-resolving superconducting nanowire single-photon detectors across 128 temporal modes. We use a model-informed characterization of each of the 1024 detection bins, for optimal precision. We perform quantum detector tomography to reconstruct the positive operator valued measures (POVMs) of the complete device, which consists of $1.38\cdot10^8$ matrix elements. At the repetition rate of our experiment of $80~\mathrm{kHz}$, we can precisely count photons corresponding to an optical power of approximately $71~\mathrm{pW}$, bridging the gap from single-photon measurements to high-sensitivity optical power meters. A photon-number-resolving detector of this size, and the tools used to analyze it, will become increasingly important to characterize large quantum states, as well as tasks in precision metrology and optical power standards.

quant-ph↗

Demonstration of a quantum C-NOT Gate in a Time-Multiplexed fully reconfigurable photonic processor

The two-qubit controlled-not (C-NOT) gate is an essential component for gate-based quantum circuits. In fact, its operation, combined with single qubit rotations allows to realise any quantum circuit. Several strategies have been adopted in order to build quantum gates. Among them, photonics offers the dual advantage of excellent isolation from the environment and ease of manipulation at the single qubit level. Here we adopt a scalable time-multiplexed approach in order to build a fully reconfigurable architecture capable of implementing a post-selected C-NOT gate with a fidelity of $(93.8 \pm 1.4)\%$. We then show how our time-multiplexed platform can be employed to combine a C-NOT and a single qubit gate in order to generate the four Bell states.

quant-ph↗

High-Dimensional Quantum Photonics: Roadmap

The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.

quant-ph↗

Benchmarking Gaussian and non-Gaussian input states with a hybrid sampling platform

The original boson sampling paradigm-consisting of multiple single-photon input states, a large interferometer, and multi-channel click detection-was originally proposed as a photonic route to quantum computational advantage. Its non-Gaussian resources, essential for outperforming any classical system, are provided by single-photon inputs and click detection. Yet the drive toward larger experiments has led to the replacement of experimentally demanding single-photon sources with Gaussian states, thereby diminishing the available non-Gaussianity-a critical quantum resource. As the community broadens its focus from the initial sampling task to possible real-world applications, it becomes crucial to quantify the performance cost associated with reducing non-Gaussian resources and to benchmark sampling platforms that employ different input states. To address this need, we introduce the Paderborn Quantum Sampler (PaQS), a hybrid platform capable of performing sampling experiments with eight Gaussian or non-Gaussian input states in a 12-mode interferometer within a single experimental run. This architecture enables direct, side-by-side benchmarking of distinct sampling regimes under otherwise identical conditions. By employing a semi-device-independent framework, offering certification that does not rely on prior knowledge of the interferometer or the input states, we verify that the observed data cannot be reproduced by any classical model-a prerequisite for demonstrating quantum advantage. Applying this framework, we observe clear performance gains arising from non-Gaussian input states.

quant-ph↗

Quantum-limited detection of arrival time and carrier frequency of time-dependent signals

Precise measurements of both the arrival time and carrier frequency of light pulses are essential for time-frequency-encoded quantum technologies. Quantum mechanics, however, imposes fundamental limits on the simultaneous determination of these quantities. In this work, we derive and experimentally verify the quantum uncertainty bounds governing joint time-frequency measurements. We show that when detection is restricted to finite time windows, the problem is naturally described by a quantum rotor, rendering the commonly used Heisenberg uncertainty relation inapplicable. We further propose an optimal detection scheme that saturates these fundamental limits. By sampling the Q-function, we demonstrate the reconstruction of the Wigner function beyond the harmonic oscillator. Using an experimental implementation based on a quantum pulse gate, we confirm that the proposed scheme approaches the ultimate quantum limit for simultaneous time-frequency measurements. These results provide a new framework for joint time-frequency detection with direct implications for precision measurements and quantum information processing.

quant-ph↗

Bridging chemistry and Gaussian boson sampling: A photonic hierarchy of approximations for molecular vibronic spectra

Simulating vibronic spectra is a central task in physical chemistry, offering insight into important properties of molecules. Recently, it has been experimentally demonstrated that photonic platforms based on Gaussian boson sampling (GBS) are capable of performing these simulations. However, whether an actual GBS approach is required depends on the molecule under investigation. To develop a better understanding on the requirements for simulating vibronic spectra, we explore connections between theoretical approximations in physical chemistry and their photonic counterparts. Mapping these approximations into photonics, we show that for certain molecules the GBS approach is unnecessary. We place special emphasis on the linear coupling approximation, which in photonics corresponds to sampling from multiple coherent states. By implementing this approach in experiments, we demonstrate improved similarities over previously reported GBS results for formic acid and identify the particular attributes that a molecule must exhibit for this, and other approximations, to be valid. These results highlight the importance in forming deeper connections between traditional methods and photonic approaches.

quant-ph↗

Quantum Fisher information analysis for absorption measurements with undetected photons

We theoretically compare the quantum Fisher information (QFI) for three configurations of absorption spectroscopy with undetected idler photons: an SU(1,1) interferometer with inter-source idler loss, an induced-coherence (IC) setup in which the idler partially seeds a second squeezer together with a vacuum ancilla, and a distributed-loss (DL) scheme with in-medium attenuation. We calculate the QFI as a function of parametric gain for both full and signal-only detection access. For losses below 99% and low to moderate gain, the SU(1,1) configuration provides the largest QFI. At high gain and intermediate loss, the IC scheme performs best, while under extreme attenuation (transmission $<$ 1%) the DL model becomes optimal. These results delineate the measurement regimes in which each architecture is optimal in terms of information theory.

quant-ph↗

High-gain effects in broadband continuous-wave parametric down conversion sources and measurements with undetected photons

We study theoretically how high-gain effects affect the measurement outcome of visible signal spectra in undetected photon measurement schemes. We consider two interferometric configurations: firstly, the SU(1,1) interferometer where the idler incurs loss and additional dispersion in between two identical, lossless, squeezers; secondly, the induced coherence interferometer where the idler incurs loss and additional dispersion in between two identical, lossless, squeezers and where the second squeezer is seeded by the idler and a vacuum ancilla mode. Furthermore, we consider a distributed loss configuration where the idler incurs loss as it propagates in the nonlinear medium. Motivated by experimental evidence and due to the fact that broadband sources are ideal for these measurement schemes, we use the dispersive data of a third-order dispersion engineered integrated waveguide parametric down conversion (PDC) source presented in New Journal of Physics 26, 123025 (2024) to model the PDC spectra in the three configurations. For each configuration we consider the case of idler-only (i) absorption, (ii) additional dispersion, and (iii) the combined effects. We obtain results which outline the strength and weaknesses of the different configurations at different operation points.

quant-ph↗

Photorefraction Management in Lithium Niobate Waveguides: High-Temperature vs. Cryogenic Solutions

Lithium niobate sees widespread use in nonlinear and quantum optical devices, such as for sum- and difference-frequency generation or spontaneous parametric down-conversion. In lithium niobate waveguides, nonlinear optical processes are often limited by the so-called photorefractive effect, which limits the maximum input or output powers and impacts the nonlinear spectral response. Therefore, strategies for the management of photorefractive damage are a key consideration in device design. Usually, the photorefractive damage threshold, i.e. the maximal permissible operating power, can be increased by high temperature operation of devices. This approach, however, is not applicable in cryogenic environments, which may be required for specialized applications. To better understand the impact of photorefraction in nonlinear optical applications, we study the impact of photorefraction on the phase-matching spectra of two nonlinear-optical sum-frequency generation experiments at 1) high temperatures and 2) cryogenic temperatures. Furthermore, we present an approach to reduce the impact of photorefraction which is compatible with cryogenic operation. This comprises an auxiliary light source, propagating in the same waveguide, which is used to restore phase-matching spectra impacted by photorefraction, as well as reduce pyroelectric effects. Our work provides an alternative route to photorefraction management applicable to cryogenic environments, as well as in situations with tight energy budgets like space applications.

physics.optics↗

Limitations of Entangled Two-Photon Absorption detection

We introduce a method for determining the sensitivity of any given Entangled Two-Photon Absorption (ETPA) measurement. By modeling all signal and noise contributions to the measurement, we derive a single numerical value that describes the sensitivity of the ETPA measurement in Göppert-Mayer units. This allows us to directly compare vastly different experimental approaches and, determine whether ETPA will be detectable under the given conditions. Therefore, we can quantify the effect of any change to a given experimental apparatus and identify the ideal optimization pathway.

quant-ph↗