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Christine Silberhorn

Publications and source records attributed to Christine Silberhorn.

At least 37 records · Page 2Linked to original sources
arXiv2026

High-gain effects in broadband continuous-wave parametric down conversion sources and measurements with undetected photons

We study theoretically how high-gain effects affect the measurement outcome of visible signal spectra in undetected photon measurement schemes. We consider two interferometric configurations: firstly, the SU(1,1) interferometer where the idler incurs loss and additional dispersion in between two identical, lossless, squeezers; secondly, the induced coherence interferometer where the idler incurs loss and additional dispersion in between two identical, lossless, squeezers and where the second squeezer is seeded by the idler and a vacuum ancilla mode. Furthermore, we consider a distributed loss configuration where the idler incurs loss as it propagates in the nonlinear medium. Motivated by experimental evidence and due to the fact that broadband sources are ideal for these measurement schemes, we use the dispersive data of a third-order dispersion engineered integrated waveguide parametric down conversion (PDC) source presented in New Journal of Physics 26, 123025 (2024) to model the PDC spectra in the three configurations. For each configuration we consider the case of idler-only (i) absorption, (ii) additional dispersion, and (iii) the combined effects. We obtain results which outline the strength and weaknesses of the different configurations at different operation points.

quant-ph↗
arXiv2026

Photorefraction Management in Lithium Niobate Waveguides: High-Temperature vs. Cryogenic Solutions

Lithium niobate sees widespread use in nonlinear and quantum optical devices, such as for sum- and difference-frequency generation or spontaneous parametric down-conversion. In lithium niobate waveguides, nonlinear optical processes are often limited by the so-called photorefractive effect, which limits the maximum input or output powers and impacts the nonlinear spectral response. Therefore, strategies for the management of photorefractive damage are a key consideration in device design. Usually, the photorefractive damage threshold, i.e. the maximal permissible operating power, can be increased by high temperature operation of devices. This approach, however, is not applicable in cryogenic environments, which may be required for specialized applications. To better understand the impact of photorefraction in nonlinear optical applications, we study the impact of photorefraction on the phase-matching spectra of two nonlinear-optical sum-frequency generation experiments at 1) high temperatures and 2) cryogenic temperatures. Furthermore, we present an approach to reduce the impact of photorefraction which is compatible with cryogenic operation. This comprises an auxiliary light source, propagating in the same waveguide, which is used to restore phase-matching spectra impacted by photorefraction, as well as reduce pyroelectric effects. Our work provides an alternative route to photorefraction management applicable to cryogenic environments, as well as in situations with tight energy budgets like space applications.

physics.optics↗
arXiv2025

Limitations of Entangled Two-Photon Absorption detection

We introduce a method for determining the sensitivity of any given Entangled Two-Photon Absorption (ETPA) measurement. By modeling all signal and noise contributions to the measurement, we derive a single numerical value that describes the sensitivity of the ETPA measurement in Göppert-Mayer units. This allows us to directly compare vastly different experimental approaches and, determine whether ETPA will be detectable under the given conditions. Therefore, we can quantify the effect of any change to a given experimental apparatus and identify the ideal optimization pathway.

quant-ph↗
arXiv2025

Two Photon Tripartite Entanglement Transfer via Time-Multiplexed Quantum Walks

Photonic multidimensional quantum networks (MDQN), where individual subsystems are encoded using multiple degrees of freedom and photons, are an emerging platform for quantum algorithms because they offer high scalability. The distribution of non-classical and non-local correlations between the individual subsystems in an MDQN is of fundamental interest for many quantum protocols. Interestingly in an MDQN, the inseparability of two subsystems underlying entanglement can occur both between multiple distinct photons as well as between individual degrees of freedom associated with a single photon. In this work, we investigate the entanglement transfer enabled by the interplay of both entanglement between two distinct photons as well as inseparability between multiple degrees of freedom. For this purpose, we subject one photon of a polarization entangled two-photon pair to a discrete-time quantum walk introducing the position subsystem of the quantum walk as a third subsystem with qudit encoding. Here we study the resulting transfer of entanglement from the polarization degree of freedom, representing qubit encoding, towards the position degree of freedom, representing quidt encoding, via partial state tomography and correlation measurements.

quant-ph↗
arXiv2025

Spectro-temporally tailored Non-Gaussian Quantum Operations in Thin-Film Waveguides

Advancements in photonic platforms have enabled the precise control of light's spectral and temporal degrees of freedom, a capability crucial for the development of scalable quantum information systems. In this work, we address the challenge of implementing spectro-temporal mode-selective non-Gaussian quantum operations, specifically single-photon subtraction (SPS) and addition (SPA), in the telecom wavelength regime. Building on prior experimental demonstrations of mode-selective near-infrared SPS, we present the first design framework for achieving mode-selective SPA and SPS using thin-film lithium niobate nonlinear waveguide platforms. We introduce an inverse-design optimization scheme by modeling the quantum-optical response via the Joint Spectral Amplitude and Transfer Function, in order to identify optimal waveguide and pump parameters that maximize mode selectivity and state purity. This approach is first tested on a metallic waveguide design. We then exploit the dispersion engineering capabilities of thin-film waveguides, which offer enhanced nonlinear interactions through tighter light confinement. Our findings demonstrate that tailored nonlinear processes, particularly parametric down-conversion and frequency up-conversion, can support high-fidelity non-Gaussian operations essential for next-generation quantum photonic networks.

quant-ph↗
arXiv2025

Complementarity-based complementarity: the choice of mutually unbiased observables shapes quantum uncertainty relations

Quantum uncertainty relations impose fundamental limits on the joint knowledge that can be acquired from complementary observables: perfect knowledge of a quantum state in one basis implies maximal indetermination in all other mutually unbiased bases (MUBs). Uncertainty relations derived from joint properties of the MUBs are generally assumed to be uniform, irrespective of the specific observables chosen within a set. In this work, we demonstrate instead that the uncertainty relations can depend on the choice of observables. Through both experimental observation and numerical methods, we show that selecting different sets of three MUBs in a 5-dimensional quantum system results in distinct uncertainty bounds, i.e. in varying degrees of complementarity, in terms of both entropy and variance.

quant-ph↗
arXiv2025

Practical considerations for assignment of photon numbers with SNSPDs

Superconducting nanowire single-photon detectors (SNSPDs) can enable photon-number resolution (PNR) based on accurate measurements of the detector's response time to few-photon optical pulses. In this work we investigate the impact of the optical pulse shape and duration on the accuracy of this method. We find that Gaussian temporal pulse shapes yield cleaner arrival-time histograms, and thus more accurate PNR, compared to bandpass-filtered pulses of equal bandwidth. For low system jitter and an optical pulse duration comparable to the other jitter contributions, photon numbers can be discriminated in our system with a commercial SNSPD. At 60 ps optical pulse duration, photon-number discrimination is significantly reduced. Furthermore, we highlight the importance of using the correct arrival-time histogram model when analyzing photon-number assignment. Using exponentially-modified Gaussian (EMG) distributions, instead of the commonly used Gaussian distributions, we can more accurately determine photon-number misidentification probabilities. Finally, we reconstruct the positive operator-valued measures (POVMs) of the detector, revealing sharp features which indicate the intrinsic PNR capabilities.

quant-ph↗
arXiv2025

Optimizing Ultra-Long Continuous Wafer-Scale Periodic Poling in Thin-Film Lithium Niobate

Periodically poled thin-film lithium niobate (TFLN) crystals are the fundamental building block for highly-efficient quantum light sources and frequency converters. The efficiency of these devices is strongly dependent on the interaction length between the light and the nonlinear material, scaling quadratically with this parameter. Nevertheless, the fabrication of long, continuously poled areas in TFLN remains challenging, the length of continuously poled areas rarely exceeds 10 mm. In this work, we demonstrate a significant progress in this field achieving the periodic poling of continuous poled areas of 70 mm length with a 3 microns poling period and a close to 50 % duty cycle. We compare two poling electrode design approaches to fabricate long, continuous poled areas. The first approach involves the poling of a single, continuous 70 mm long electrode. The second utilize a segmented approach including the poling of more than 20 individual sections forming together a 70 mm long poling area with no stitching errors. While the continuous electrode allows for faster fabrication, the segmented approach allows to individually optimize the poling resulting in less duty cycle variation. A detailed analysis of the periodic poling results reveals that the results of both are consistent with previously reported poling outcomes for shorter devices. Thus, we demonstrate wafer-scale periodic poling exceeding chiplet-size without any loss in the periodic poling quality. Our work presents a key step towards highly-efficient, narrowbandwidth and low-pump power nonlinear optical devices.

physics.app-ph↗
arXiv2025

Widely non-degenerate nonlinear frequency conversion in cryogenic titanium in-diffused lithium niobate waveguides

The titanium in-diffused lithium niobate waveguide platform is well-established for reliable prototyping and packaging of many quantum photonic components at room temperature. Nevertheless, compatibility with certain quantum light sources and superconducting detectors requires operation under cryogenic conditions. We characterize alterations in phase-matching and mode guiding of a non-degenerate spontaneous parametric down-conversion process emitting around 1556 nm and 950 nm, under cryogenic conditions. Despite the effects of pyroelectricity and photorefraction, the spectral properties match our theoretical model. Nevertheless, these effects cause small but significant variations within and between cooling cycles. These measurements provide a first benchmark against which other nonlinear photonic integration platforms, such as thin-film lithium niobate, can be compared.

quant-ph↗
arXiv2025

Towards integrated sensors for optimized OCT with undetected photons

The development of practical sensors for optical coherence tomography (OCT) with undetected photons requires miniaturization via integration. To be practical, these sensors must exhibit a large spectral bandwidth and a high brightness, which are linked to a high axial resolution and a sufficient signal to noise ratio, respectively. Here, we combine these requirements in a scheme for OCT-measurements with undetected photons based on nonlinear Ti:LiNbO$_3$ waveguides. We investigate the performance benchmarks of the commonly used SU(1,1) scheme in comparison to an induced coherence scheme and find that the latter is actually better suited when implementing measurements with undetected photons in integrated systems. In both schemes, we perform pump gain optimization and OCT measurements with undetected photons with an axial resolution as low as 28 $\mathrmμ$m.

quant-ph↗
arXiv2025

Observing High-dimensional Bell Inequality Violations using Multi-Outcome Spectral Measurements

Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify and violate a Bell inequality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or Bell-nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing Bell-nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.

quant-ph↗
arXiv2025

Experimental entropic uncertainty relations in dimensions three to five

We provide experimental validation of tight entropic uncertainty relations for the Shannon entropies of observables with mutually unbiased eigenstates in high dimensions. In particular, we address the cases of dimensions $d = 3$, $4$ and $5$ and consider from $2$ to $d+1$ mutually unbiased bases. The experiment is based on pulsed frequency bins measured with a multi-output quantum pulse gate, which can perform projective measurements on a complete high-dimensional basis in the time-frequency domain. Our results fit the theoretical predictions: the bound on the sum of the entropies is never violated and is saturated by the states that minimize the uncertainty relations.

quant-ph↗
arXiv2025

A ultrabright, two-colour photon pair source based on thin-film lithium niobate for bridging visible and telecom wavelengths

We present the design and characterisation of a guided-wave, bright and highly frequency non-degenerate parametric down-conversion source in thin-film lithium niobate. The source generates photon pairs with wavelengths of 815$\,\mathrm{nm}$ and 1550$\,\mathrm{nm}$ linking the visible wavelength regime with telecommunication wavelengths. We confirm the high quality of the generated single photons by determining a value for the heralded second-order correlation function as low as $g^{(2)}_h(0) = (6.7\pm1.1)\cdot10^{-3}$. Furthermore, we achieve a high spectral brightness of 0.44$\cdot$10$^{7}$$\frac{\text{pairs}}{\text{s} \cdot \text{mW} \cdot \text{GHz}}$ which is two orders of magnitude higher than sources based on weakly guiding waveguides. The almost perfect sinc-shape and the strong agreement between the effective and nominal bandwidth highlights the success of our integrated workflow, which begins with device design and continues through precise fabrication to detailed quantum-state characterization. This comprehensive approach enables targeted optimization of the source, resulting in excellent quantum state generation. Our results set a new standard for on-chip, non-degenerate photon-pair sources and represent a crucial step towards practical, scalable quantum communication networks and photonic quantum computing.

quant-ph↗
arXiv2025

Frequency-bin interferometry for reconstructing electric fields with low intensity

Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate characterization of such pulses, including spectral coherence, remains challenging because current methods require substantial experimental resources and complex reconstruction algorithms. Here, we introduce frequency-bin interferometry for reconstructing electric fields with low intensity (FIREFLY), a technique that directly provides spectral amplitude, phase, and coherence profiles of single-photon pulses without requiring intensive reconstruction algorithms. Our approach measures the two-point spectral correlation function of the pulse by interfering its different frequency components using a quantum pulse gate (QPG) driven by a reference pump pulse. We demonstrate its compatibility with quantum light by characterizing partially coherent pulses generated by a type-0 parametric down-conversion process. We also overcome this requirement of a known pump pulse by introducing spectral shear into our interferometric scheme using a multi-output QPG (mQPG). This enables simultaneous characterization of a single-photon-level input pulse alongside an unknown pump pulse. Notably, our method achieves theory-experiment similarity above 95\% across all retrieved profiles, which demonstrates the reliability of this scheme for quantum information applications based on time-frequency encodings.

physics.optics↗
arXiv2025

Jitter in photon-number-resolved detection by superconducting nanowires

By analyzing the physics of multi-photon absorption in superconducting nanowire single-photon detectors (SNSPDs), we identify physical components of jitter. From this, we formulate a quantitative physical model of the multi-photon detector response which combines local detection mechanism and local fluctuations (hotspot formation and intrinsic jitter) with thermoelectric dynamics of resistive domains. Our model provides an excellent description of the arrival-time histogram of a commercial SNSPD across several orders of magnitude, both in arrival-time probability and across mean photon number. This is achieved with just three fitting parameters: the scaling of the mean arrival time of voltage response pulses, as well as the Gaussian and exponential jitter components. Our findings have important implications for photon-number-resolving detector design, as well as applications requiring low jitter such as light detection and ranging (LIDAR).

quant-ph↗
arXiv2025

Harnessing of temporal dispersion for integrated pump filtering in spontaneous heralded single-photon generation processes

Cointegration of heralded single-photon generation and on-chip detection requires the ability to differentiate between pump light and single photons. We explored the dispersion-induced temporal separation of optical pulses to reach this goal. Our method exploits the distinct group velocities of pump light and single photons, as well as single-photon detectors with high timing resolution. We simulate the propagation for photon pair generation by spontaneous parametric down-conversion in titanium in-diffused waveguides in lithium niobate and thin-film lithium niobate, and spontaneous four-wave mixing in silicon on insulator and silicon nitride. For the different integration platforms, we show the propagation distance required to sufficiently distinguish between pump and single photons for different timing resolutions, and demonstrate that this should be feasible with current superconducting nanowire single-photon detector technologies. Finally, we experimentally simulate our approach using the dispersion in the optical fiber.

quant-ph↗
arXiv2025

Spectral and temporal properties of type-II parametric down-conversion: The impact of losses during state generation

In this paper, we theoretically study spectral and temporal properties of pulsed spontaneous parametric down-conversion (SPDC) generated in lossy waveguides. Our theoretical approach is based on the formalism of Gaussian states and the Langevin equation, which is elaborated for weak parametric down-conversion and photon-number-unresolved click detection. Using the example of frequency-degenerate type-II SPDC generated under pump-idler group-velocity-matching condition, we show how the joint-spectral intensity, mode structure, normalized second-order correlation function, and Hong-Ou-Mandel interference pattern depend on internal losses of the SPDC process. In addition, we propose a new method for the experimental determination of internal losses of nonlinear waveguides which is based on the measurement of the normalized second-order correlation functions.

quant-ph↗