arXiv subjects

Chunlei Wang

Publications and source records attributed to Chunlei Wang.

42 records · Page 3Linked to original sources

arXiv2011

Direct observation of nanometer-scale amorphous layers and oxide crystallites at grain boundaries in polycrystalline Sr1-xKxFe2As2 superconductors

We report here an atomic resolution study of the structure and composition of the grain boundaries in polycrystalline Sr0.6K0.4Fe2As2 superconductor. A large fraction of grain boundaries contain amorphous layers larger than the coherence length, while some others contain nanometer-scale particles sandwiched in between amorphous layers. We also find that there is significant oxygen enrichment at the grain boundaries. Such results explain the relatively low transport critical current density (Jc) of polycrystalline samples with respect to that of bicrystal films.

cond-mat.supr-con↗

arXiv2011

Superconductivity induced by doping Rh in CaFe2-xRhxAs2

In this paper we report the synthesis of iron-based superconductors CaFe2-xRhxAs2 using one-step solid state reaction method, which crystallizes in the ThCr2Si2-type structure with a space group I4/mmm. The systematic evolution of the lattice constants demonstrates that the Fe ions are successfully replaced by the Rh. By increasing the doping content of Rh, the spin-density-wave (SDW) transition in the parent compound is suppressed and superconductivity emerges. The maximum superconducting transition temperature is found at 18.5 K with the doping level of x = 0.15. The temperature dependence of DC magnetization confirms superconducting transitions at around 15 K. The general phase diagram was obtained and found to be similar to the case of Rh-doping Sr122 system. Our results explicitly demonstrate the feasibility of inducing superconductivity in Ca122 compounds by higher d-orbital electrons doping, however, different Rh-doping effect between FeAs122 compounds and FeAs1111 systems still remains an open question.

cond-mat.supr-con↗

arXiv2011

Enhanced critical current properties in Ba0.6K0.4+xFe2As2 superconductor by over-doping of potassium

Phase-pure polycrystalline Ba0.6K0.4+xFe2As2 with were prepared using a one-step solid-state reaction method. We found that over-doping of potassium can improve critical current density (Jc). High-field Jc for samples with x = 0.1 is three times higher than that for samples with x = 0. Over-doping of K has minimal effect on the critical transition temperature (Tc). Less than 0.5 K degradations in Tc was measured for samples with x = 0.1. TEM revealed high concentration of dislocations in samples with x = 0.1, resulting in enhanced flux pining. Further analyses on magnetization loops for powder samples confirm that K over-doping can promote intra-grain Jc. Our results indicate that slight excess of K in Ba0.6K0.4Fe2As2 samples is beneficial to high-field applications.

cond-mat.supr-con↗

arXiv2010

One-step method to grow Ba0.6K0.4Fe2As2 single crystals without fluxing agent

Single crystals of Ba0.6K0.4Fe2As2 with excellent quality have been successfully grown without fluxing agent through a simple one-step method for the first time. X-ray diffraction patterns demonstrate that the samples have high crystalline quality and c-axis orientation. The onset transition temperature is up to 38 K with the zero resistivity temperature about 36.7 K. Both the R-T and M-T data show a very sharp superconducting transition with transition width 0.4 K. We also found that the samples possess very large current carrying ability and high upper critical fields, indicating potential applications requiring very high field. The above simple and safe one-step technique of single crystal growth can be effective in other systems of Fe-based superconductors.

cond-mat.supr-con↗

arXiv2010

Low-temperature synthesis of SmO0.8F0.2FeAs superconductor with Tc = 56.1K

We report a systematic study on the effect of sintering temperature on the structural and superconducting properties of nominal SmO0.8F0.2FeAs fabricated by simple one-step solid state reaction method. A detailed correlation between the sintering temperature, structure, onset transition temperature (Tc) and critical current density (Jc) has been found in all samples of each batch. Most importantly, samples sintered at a low temperature clearly shows high Tc, for example the Tc of the samples sintered at 850C is even above 53 K, and the samples prepared at 1000C display the highest Tc of 56.1 K reported so far. Furthermore, the samples sintered at 1000C also show the highest RRR and the lowest resistivity(57K), indicating the low impurity scattering and enhanced carrier density. However, the maximum Jc of 10510 A/cm^2 at 5 K in self field was achieved in the samples sintered at 1100oC. The dependence of Tc on a-axis lattice constant indicates that the sintering temperature has strong influence on the effective substitution level of F for O. This result suggests that annealing at a temperature of ~1000C seems much better for obtaining high quality 1111 phase oxypnictides, compared to commonly used temperatures of around 1200C.

cond-mat.supr-con↗

arXiv2010

Low-temperature synthesis of SmFeAsO0.7F0.3 wires with high transport critical current density

Ag-sheathed SmFeAsO0.7F0.3 (Sm-1111) superconducting wires were prepared by a one-step solid state reaction at temperatures as low as 850~900C, instead of commonly used temperatures of 1150~1250C. The X-ray diffraction pattern of the as-sintered samples is well indexed on the basis of tetragonal ZrCuSiAs-type structure. We characterized transport critical current density Jc of the SmFeAsO0.7F0.3 wires in increasing and subsequently decreasing fields, by a resistive four-probe method. A transport Jc as high as ~1300 A/cm^2 at 4.2 K and self field has been observed for the first time in Sm-1111 type polycrystalline superconductors. The Jc also shows a rapid depression in small applied fields as well as a magnetic-history dependence, indicating weak-linked grain boundaries. The low-temperature synthesis method can be very beneficial to fabricating the RE-1111 iron oxynictides in a convenient and safe way.

cond-mat.supr-con↗