arXiv subjects

Claire Donnelly

Publications and source records attributed to Claire Donnelly.

At least 19 recordsLinked to original sources

arXiv2026

A Fourier-Space Approach to Physics-Informed Magnetization Reconstruction from Nitrogen-Vacancy Measurements

Reconstructing magnetization textures from nitrogen-vacancy (NV) magnetometry stray-field measurements is a challenging, fundamentally ill-posed inverse problem, further complicated by the unknown effective distance between sensor and magnetic material. Here we show that incorporating a micromagnetic energy functional directly into the inversion filters out unphysical, high-energy configurations, while Fourier-space upward continuation of the stray field allows us to simultaneously fit the distance. Applied to measurements of the van der Waals ferromagnet Fe$_{3-x}$GaTe$_2$, it recovers an effective distance estimate of approximately 81nm and low-energy configurations that reproduce the observed field. More broadly, embedding physics directly into the reconstruction turns ill-posed magnetic inverse problems into transparent, interpretable reconstructions, with applicability well beyond NV magnetometry.

cond-mat.mes-hall↗

arXiv2026

Generation of Bloch Points with Controlled Spin Texture Using Geometrical Boundary Conditions

Bloch points are three-dimensional topological singularities in magnetization that play a key role in topological transformations of spin textures, such as skyrmion creation or annihilation. While topology often enforces the existence of Bloch points in confined geometries like cylindrical nanowires, deterministic control over their position and magnetic configuration remains challenging. Here we demonstrate the generation of Bloch points with controlled spin texture by engineering geometrical boundary conditions in three-dimensional nanomagnets. By introducing a chirality interface between two three-dimensional double-helix nanowires of opposite handedness, forming a kinked, non-collinear structure, we impose competing topological constraints that uniquely define the magnetization configuration surrounding the Bloch point. A saturating magnetic field nucleates head-to-head or tail-to-tail domain configurations at the chirality interface, producing a Bloch-point domain wall with deterministic polarity, circulation and helicity. This geometrical approach enables full three-dimensional control of Bloch point domain walls allowing deterministic engineering of their spin texture and its selective coupling to current-induced Oersted fields.

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arXiv2026

The 2026 Skyrmionics Roadmap

Magnetic skyrmions and related topological spin textures have emerged as a central topic in condensed-matter physics, combining fundamental significance with potential for transformative applications in spintronics, magnonics, and beyond. Over the past decade, advances in material platforms, imaging techniques, theoretical modeling, and device concepts have established skyrmionics as a rapidly expanding field. At the same time, challenges remain in stabilizing, controlling, and integrating such textures into functional architectures, while novel phenomena such as antiskyrmions, higher-order skyrmions, hopfions, and antiferromagnetic textures arise. The 2026 Skyrmionics Roadmap represents a collective effort of many authors, providing a comprehensive perspective on the current state-of-the-art and the outlook for the coming years. In 33 focused sections, each co-authored by two researchers, we chart progress in theory and modeling, material systems, skyrmion dynamics, and skyrmion technologies. By offering a consolidated vision, this Roadmap aims to guide both fundamental research and application-driven efforts, accelerating the transition of skyrmionics from conceptual breakthroughs toward practical technologies.

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arXiv2026

3D tomographic imaging of skyrmionic cocoons using HERALDO

Uncovering the rich and intricate characteristics of three-dimensional (3D) magnetic textures is essential for functional materials such as magnetic multilayers, where the delicate balance of various magnetic interactions leads to complex 3D spin arrangements. Among these textures, skyrmionic cocoons-tubular 3D magnetic structures characterized by a closed magnetization surface wrapping around a core-have emerged as particularly intriguing. Stabilized by competing magnetic interactions, these textures reside within a fraction of the thickness of the magnetic material and exhibit a typical lateral size of approximately 100 nm. Here, we present a vector tomographic reconstruction of the 3D magnetization in aperiodic Pt/Co/Al chiral multilayers, where skyrmionic cocoons have been recently reported. Using soft X-ray Holography with Extended Reference by Autocorrelation Linear Differential Operator (HERALDO), we acquire tomographic projections of the magnetic configuration and reconstruct the full 3D magnetization vector field with a spatial resolution of approximately 30 nm, as determined by Fourier shell correlation (FSC). This resolution allows us to observe critical features of the cocoons, such as their vertical misalignment and their overall chirality. Our findings demonstrate that HERALDO-based vector tomography is a powerful approach for revealing the internal structure and vertical extent of these nanoscale magnetic textures, offering new experimental insights into their intrinsic behavior.

cond-mat.mtrl-sci↗

arXiv2026

Magnetization reversal mechanism of double-helix nanowires probed by dark-field magneto-optical Kerr effect

Double-helix (DH) nanowires provide a platform to study the influence of geometric chirality on spin chirality. Their three-dimensional (3D) helical architecture and tunable inter-strand coupling enable control of spin chirality, including the stabilization of topological 3D magnetic states such as helical domains and domain walls, topological stray fields, and extended helical vortex/skyrmion tubes. So far, the study of these and other 3D nanostructures is usually confined to a limited number of magnetic microscopy experiments in large facilities. Here, we investigate the reversal mechanism of a single DH nanowire using Dark-Field magneto-optical Kerr effect (DF-MOKE) magnetometry under external 3D magnetic fields. By analyzing the angular dependence of the DF-MOKE signal, we fit the reversal process using established models for domain-wall nucleation and propagation, finding a characteristic behavior similar to that reported for cylindrical nanowires. Micromagnetic simulations indicate that the reversal process goes through nucleation of the helical vortex tube in a curling manner while ptychographic X-ray magnetic circular dichroism data reveal that this helical vortex tube state forms through a mixed nucleation-propagation process. These observations provide a consistent microscopic picture of reversal mediated by a helical vortex tube extending along the nanowire. Our work provides a comprehensive characterization of magnetization reversal in DH nanowires and demonstrates that DF-MOKE magnetometry is effective for probing reversal mechanisms in single 3D nanostructures. This lab-based approach expands the range of accessible experiments beyond large-scale facilities, enabling extensive exploration of the rich spin states supported by 3D nano-geometries.

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arXiv2025

Interlinking helical spin textures in nanopatterned chiral magnets

Nanoscale topologically non-trivial magnetization configurations generate significant interest due to both the fundamental properties of their knotted structures and their potential applications in ultra-efficient computing devices. While such textures have been widely studied in two dimensions, three-dimensional (3D) systems can yield more complex configurations, resulting in richer topologies and dynamic behaviors. However, reliably nucleating these 3D textures has proven challenging, and so far, 3D configurations such as vortex rings and hopfions can often only be observed forming spontaneously in relatively uncontrolled manners. Here, we demonstrate that through the 3D nanopatterning of chiral single crystal helimagnets into nano-tori, the controlled formation of a magnetic double helix can be achieved. This surface-localized topological state is stabilized by the interplay of intrinsic exchange interactions of the single crystal with the extrinsic emergent effects of the patterned geometry. These double helices host magnetic defects akin to supercoiling in circular DNA and climbing vines. We expect this study to serve as a foundation for future research combining single crystal systems with 3D nanopatterning, offering a new degree of control over emergent phenomena in nanoscale magnets and wider quantum material systems.

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arXiv2025

X-ray linear dichroic orientation tomography: reconstruction of nanoscale three-dimensional orientation fields

Properties in crystalline and ordered materials tend to be anisotropic, with their orientation affecting the macroscopic behavior and functionality of materials. The ability to image the orientation of anisotropic material properties in three dimensions (3D) is fundamental for the understanding and functionality-driven development of novel materials. With the development of X ray linear dichroic orientation tomography (XL DOT), it is now possible to non-destructively map three-dimensional (3D) orientation fields in micrometer-sized samples. In this work, we present the iterative, gradient-based reconstruction algorithm behind XL DOT that can be used to map orientations based on linear dichroism in 3D. As linear dichroism can be exhibited by a broad spectrum of materials, XL DOT can be used to map, for example, crystal orientations as well as ferroic alignment, such as ferroelectric and antiferromagnetic order. We demonstrate the robustness of this technique for orientation fields that exhibit smoothly varying and granular configurations, and subsequently identify and discuss optimal geometries for experimental data acquisition and optimal conditions for the reconstruction. We anticipate that this technique will be instrumental in enabling a deeper understanding of the relationship between material structures and their functionality, quantifying, for example, the orientation of charge distributions and magnetic anisotropies at the nanoscale in a wide variety of systems - from functional to energy materials.

cond-mat.mtrl-sci↗

arXiv2025

Altermagnetic nanotextures revealed in bulk MnTe

With many candidate altermagnetic materials, MnTe has emerged as one of the most promising systems, with growing experimental evidence for altermagnetic phenomena. So far, the majority of measurements have been performed on thin-films, or have involved surface measurements. However, the question of altermagnetic order in the bulk system - in the absence of substrate or surface effects - remains. Here we show evidence for bulk altermagnetism in single crystal MnTe, through spectroscopic X-ray microscopy. By performing nanoscale X-ray magnetic circular dichroic (XMCD) imaging in transmission on a 200 nm thick lamella, we observe domains and magnetic textures with a spectroscopic signature characteristic of altermagnetic order, thereby confirming the intrinsic nature of altermagnetism in MnTe. Quantitative analysis of the XMCD signal reveals an excellent agreement with predicted signals, establishing that the altermagnetic order exists throughout the thickness of the lamella and confirming the intrinsic, bulk nature of the state. With these results, we demonstrate that transmission XMCD spectroscopic imaging is a robust, quantitative technique to probe altermagnetic order, providing a means to probe individual altermagnetic domains within complex configurations. This ability to investigate, and characterise altermagnetic order in bulk crystals represents an important tool for the exploration of altermagnetism across a wide range of candidate materials, of key importance for the development of future technologies.

cond-mat.mtrl-sci↗

arXiv2025

Nanoscale Mapping of Magnetic Orientations with Complex X-ray Magnetic Linear Dichroism

Compensated magnets are of increasing interest for both fundamental research and applications, with their net-zero magnetization leading to ultrafast dynamics and robust order. To understand and control this order, nanoscale mapping of local domain structures is necessary. One of the main routes to mapping antiferromagnetic order is X-ray magnetic linear dichroism (XMLD), which probes the local orientation of the Néel vector. However, XMLD imaging typically suffers from weak contrast and has mainly been limited to surface-sensitive techniques. Here, we harness coherent diffractive imaging to map the complex XMLD spectroscopically, and identify the phase linear dichroism as a high-contrast, high-resolution mechanism for imaging magnetic order. By applying X-ray spectroptychography to a model sample, we retrieve the full complex XMLD spectrum. Combining this with hierarchical clustering, we resolve the spatial distribution of probed domains by their distinct spectral signatures, providing a robust method for analyzing magnetic configurations with weak signals. Our results show that phase contrast is significantly stronger than the corresponding absorption contrast, offering higher spatial-resolution magnetic imaging. This approach establishes a reliable, element- and orbital-sensitive tool for studying compensated magnets.

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arXiv2025

Unidirectional motion of topological defects mediating continuous rotation processes

Topological defects play a critical role across many fields, mediating phase transitions and macroscopic behaviors as they move through space. Their role as robust information carriers has also generated much attention. However, controlling their motion remains challenging, especially towards achieving motion along well-defined paths which typically require predefined structural patterning. Here we demonstrate the tunable, unidirectional motion of topological defects, specifically magnetic dislocations in a weak magnetic stripe pattern, induced by external magnetic field in a laterally unconfined thin film. This motion is shown to mediate the overall continuous rotation of the stripe pattern. We determine the connection between the unidirectional motion of dislocations and the underlying three-dimensional (3D) magnetic structure by performing 3D magnetic vectorial imaging with in situ magnetic fields. A minimal model for dislocations in stripe patterns that encodes the symmetry breaking induced by the external magnetic field reproduces the motion of dislocations that facilitate the 2D rotation of the stripes, highlighting the universality of the phenomenon. This work establishes a framework for studying the field-driven behavior of topological textures and designing materials that enable well defined, controlled motion of defects in unconfined systems, paving the way to manipulate information carriers in higher-dimensional systems.

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arXiv2024

Fractional Skyrmion Tubes in Chiral-Interfaced Three-Dimensional Magnetic Nanowires

Magnetic skyrmions are chiral spin textures with rich physics and great potential for unconventional computing. Typically, skyrmions form in bulk crystals with reduced symmetry or ultrathin film multilayers involving heavy metals. Here, we demonstrate the formation of fractional Bloch skyrmion tubes at room temperature by 3D printing ferromagnetic double-helix nanowires with two regions of opposite chirality. Using X-ray microscopy and micromagnetic simulations, we show that the coexistence of vortex and anti-parallel spin states induces the formation of fractional skyrmion tubes at zero magnetic fields, minimising the energy cost of breaking the coupling between geometric and magnetic chirality. We also demonstrate control over zero-field states, including pure vortex, or mixed skyrmion-vortex states, highlighting the magnetic reconfigurability of these 3D nanowires. This work shows how interfacing chiral geometries at the nanoscale can enable advanced forms of topological spintronics.

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arXiv2024

Vortex motion in reconfigurable three-dimensional superconducting nanoarchitectures

When materials are patterned in three dimensions, there exist opportunities to tailor and create functionalities associated with an increase in complexity, the breaking of symmetries, and the introduction of curvature and non-trivial topologies. For superconducting nanostructures, the extension to the third dimension may trigger the emergence of new physical phenomena, as well as advances in technologies. Here, we harness three-dimensional (3D) nanopatterning to fabricate and control the emergent properties of a 3D superconducting nanostructure. Not only are we able to demonstrate the existence and motion of superconducting vortices in 3D but, with simulations, we show that the confinement leads to a well-defined bending of the vortices within the volume of the structure. Moreover, we experimentally observe a strong geometrical anisotropy of the critical field, through which we achieve the reconfigurable coexistence of superconducting and normal states in our 3D superconducting architecture, and the local definition of weak links. In this way, we uncover an intermediate regime of nanosuperconductivity, where the vortex state is truly three-dimensional and can be designed and manipulated by geometrical confinement. This insight into the influence of 3D geometries on superconducting properties offers a route to local reconfigurable control for future computing devices, sensors, and quantum technologies.

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arXiv2024

Three-dimensional spin-wave dynamics, localization and interference in a synthetic antiferromagnet

Spin waves are collective perturbations in the orientation of the magnetic moments in magnetically ordered materials. Their rich phenomenology is intrinsically three-dimensional; however, the three-dimensional imaging of spin waves has so far not been possible. Here, we image the three-dimensional dynamics of spin waves excited in a synthetic antiferromagnet, with nanoscale spatial resolution and sub-ns temporal resolution, using time-resolved magnetic laminography. In this way, we map the distribution of the spin-wave modes throughout the volume of the structure, revealing unexpected depth-dependent profiles originating from the interlayer dipolar interaction. We experimentally demonstrate the existence of complex three-dimensional interference patterns and analyze them via micromagnetic modelling. We find that these patterns are generated by the superposition of spin waves with non-uniform amplitude profiles, and that their features can be controlled by tuning the composition and structure of the magnetic system. Our results open unforeseen possibilities for the study and manipulation of complex spin-wave modes within nanostructures and magnonic devices.

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arXiv2024

Tailoring the energy landscape of a Bloch point singularity with curvature

Topological defects, or singularities, play a key role in the statics and dynamics of complex systems. In magnetism, Bloch point singularities represent point defects that mediate the nucleation of textures such as skyrmions and hopfions. However, while the textures are typically stabilised in chiral magnets, the influence of chirality on the Bloch point singularities remains relatively unexplored. Here we harness advanced three-dimensional nanofabrication to explore the influence of chirality on Bloch point singularities by introducing curvature-induced symmetry breaking in a ferromagnetic nanowire. Combining X-ray magnetic microscopy with the application of in situ magnetic fields, we demonstrate that Bloch point singularity-containing domain walls are stabilised in straight regions of the sample, and determine that curvature can be used to tune the energy landscape of the Bloch points. Not only are we able to pattern pinning points but, by controlling the gradient of curvature, we define asymmetric potential wells to realise a robust Bloch point shift-register with non-reciprocal behaviour. These insights into the influence of symmetry and chirality on singularities offers a route to the controlled nucleation and propagation of topological textures, providing opportunities for logic and computing devices.

cond-mat.mes-hall↗

arXiv2024

X-ray Linear Dichroic Tomography of Crystallographic and Topological Defects

The functionality of materials is determined by their composition and microstructure, that is, the distribution and orientation of crystalline grains, grain boundaries and the defects within them. The characterisation of the material's microstructure is therefore critical for materials applications such as catalysis, energy storage and buildings. Until now, characterization techniques that map the distribution of grains, their orientation, and the presence of defects have either been limited to surface investigations, to spatial resolutions of a few hundred nanometres, or to systems of thickness around one hundred nanometres, thus requiring destructive sample preparation for measurements and preventing the study of system-representative volumes or the investigation of materials under operational conditions. Here, we present X-ray linear dichroic orientation tomography, a quantitative, non-invasive technique that allows for an intra- and inter-granular characterisation of extended polycrystalline and amorphous materials in three dimensions (3D). We present the detailed characterisation of a polycrystalline sample of vanadium pentoxide (V2O5), a key catalyst in the production of sulfuric acid. In addition to determining the nanoscale composition, we map the crystal orientation throughout the polycrystalline sample with 73 nm spatial resolution. We identify grains, as well as twist, tilt, and twin grain boundaries. We further observe the creation and annihilation of topological defects promoted by the presence of volume crystallographic defects in 3D. Our method's non-destructive and spectroscopic nature opens the door to in-operando combined chemical and microstructural investigations of functional materials, including energy and mechanical materials in existing industries, as well as quantum materials for future technologies.

cond-mat.mtrl-sci↗

arXiv2023

Soft X-ray phase nano-microscopy of micrometre-thick magnets

Imaging of nanoscale magnetic textures within extended material systems is of critical importance both to fundamental research and technological applications. Whilst high resolution magnetic imaging of thin nanoscale samples is well-established with electron and soft X-ray microscopy, the extension to micrometer-thick systems with hard X-rays currently limits high resolution imaging to rare-earth magnets. Here we overcome this limitation by establishing soft X-ray magnetic imaging of micrometer-thick systems using the pre-edge phase X-ray Magnetic Circular Dichroism signal, thus making possible the study of a wide range of magnetic materials. By performing dichroic spectro-ptychography, we demonstrate high spatial resolution imaging of magnetic samples up to 1.7 μm thick, an order of magnitude higher than conventionally possible with absorption-based techniques. This new regime of magnetic imaging makes possible the study of extended non rare-earth systems that have until now been inaccessible, from magnetic textures for future spintronic applications to non-rare-earth permanent magnets.

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arXiv2023

X-ray nanotomography reveals formation of single diamonds by block copolymer self-assembly

Block copolymers are recognised as a valuable platform for creating nanostructured materials with unique properties. Morphologies formed by block copolymer self-assembly can be transferred into a wide range of inorganic materials, enabling applications including energy storage and metamaterials. However, imaging of the underlying, often complex, nanostructures in large volumes has remained a challenge, limiting progress in materials development. Taking advantage of recent advances in X-ray nanotomography, we non-invasively imaged exceptionally large volumes of nanostructured soft materials at high resolution, revealing a single diamond morphology in a triblock terpolymer composite network. This morphology, which is ubiquitous in nature, has so far remained elusive in block copolymers, despite its potential to create materials with large photonic bandgaps. The discovery was made possible by the precise analysis of distortions in a large volume of the self-assembled diamond network, which are difficult to unambiguously assess using traditional characterisation tools. We anticipate that high-resolution X-ray nanotomography, which allows imaging of much larger sample volumes than electron-based tomography, will become a powerful tool for the quantitative analysis of complex nanostructures and that structures such as the triblock terpolymer-directed single diamond will enable the generation of advanced multicomponent composites with hitherto unknown property profiles.

cond-mat.soft↗

arXiv2023

High-resolution three-dimensional imaging of topological textures in single-diamond networks

Highly periodic structures are often said to convey the beauty of nature. However, most material properties are strongly influenced by the defects they contain. On the mesoscopic scale, molecular self-assembly exemplifies this interplay; thermodynamic principles determine short-range order, but long-range order is mainly impeded by the kinetic history of the material and by thermal fluctuations. For the development of self-assembly technologies, it is imperative to characterise and understand the interplay between self-assembled order and defect-induced disorder. Here we used synchrotron-based hard X-ray nanotomography to reveal a pair of extended topological defects within a self-assembled single-diamond network morphology. These defects are morphologically similar to the comet and trefoil patterns of equal and opposite half-integer topological charges observed in liquid crystals and appear to maintain a constant separation across the thickness of the sample, resembling pairs of full vortices in superconductors and other hard condensed matter systems. These results are expected to open new windows to study defect formation in soft condensed matter, particularly in biological systems where most structures are formed by self-assembly.

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