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Connor Roncaioli

Publications and source records attributed to Connor Roncaioli.

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Resilient $j$=3/2 superconductivity in topological semimetal YPtBi

Cooper pairing in most of the known fermionic superfluids occurs via spin-1/2 quasiparticle interactions that lead to spin-singlet or spin-triplet pairing. In the topological semimetal YPtBi, strong spin-orbit coupling results in a band inversion between highly symmetric $s$- and $p$-like electronic bands and a degeneracy at the $\Gamma$ point that ensures the manifold of $j$=3/2 quasiparticle states thrive near the Fermi level, where superconducting pairing occurs. Here we study the effects of magnetic and nonmagnetic disorder and carrier density on this exotic superconducting pairing state. By varying levels of disorder and carrier densities by nearly two and three orders of magnitude, respectively, we show that the superconducting critical temperature of YPtBi has a remarkable robustness, with little variation across this span. Our results suggest that superconductivity in YPtBi may reside in a regime where phase stiffness, rather than pair formation, governs the transition temperature. The insensitivity of Cooper pairing to dramatic changes in quasiparticle environment in a $j$=3/2 superconductor highlights a new form of protection realized in topological high-spin superconductors.

cond-mat.supr-con

All-in-one Quantum Diamond Microscope for Sensor Characterization

Nitrogen-vacancy (NV) centers in diamond are a leading modality for magnetic sensing and imaging under ambient conditions. However, these sensors suffer from degraded performance due to paramagnetic impurities and regions of stress in the diamond crystal lattice. This work demonstrates a quantum diamond microscope (QDM) for simultaneous mapping and spatial correlation of key properties of a millimeter-scale NV-diamond sensor chip, including: NV ensemble photoluminescence (PL) amplitude, spin-lattice relaxation time (T$_1$), and homogeneous and inhomogeneous spin coherence lifetimes (T$_2$ and T$_2^*$), as well as lattice stress/strain, birefringence magnitude, and birefringence angle of the diamond crystal.

quant-ph

Pressure-Driven Valence Increase and Metallization in Kondo Insulator Ce$_3$Bi$_4$Pt$_3$

We report the results of high pressure x-ray diffraction, x-ray absorption, and electrical transport measurements of Kondo insulator Ce$_3$Bi$_4$Pt$_3$ up to 42 GPa, the highest pressure reached in the study of any Ce-based KI. We observe a smooth decrease in volume and movement toward intermediate Ce valence with pressure, both of which point to increased electron correlations. Despite this, temperature-dependent resistance data show the suppression of the interaction-driven ambient pressure insulating ground state. We also discuss potential ramifications of these results for the predicted topological KI state.

cond-mat.str-el

Influence of growth flux solvent on anneal-tuning of ground states in CaFe2As2

The effects of anneal-tuning of single-crystalline samples of CaFe$_2$As$_2$ synthesized via a molten Sn flux method are investigated using x-ray diffraction, chemical composition, electrical transport and magnetic susceptibility measurements in order to understand the role of growth conditions on the resultant phase diagram. Previous studies of CaFe$_2$As$_2$ crystals synthesized using a self-flux (FeAs) method revealed an ability to tune the structural and magnetic properties of this system by control of post-synthesis annealing conditions, resulting in an ambient pressure phase diagram that spans from tetragonal/orthorhombic antiferromagnetism to the collapsed tetragonal phase of this system. In this work, we compare previous results to those obtained on crystals synthesized via Sn flux, finding similar tunability in both self- and Sn-flux cases, but less sensitivity to annealing temperatures in the latter case, resulting in a temperature-shifted phase diagram.

cond-mat.supr-con

High Fidelity Detection of the Orbital Angular Momentum of Light by Time Mapping

We demonstrate high-fidelity detection of the orbital angular momentum (OAM) of light using a compact and practical OAM spectrometer that maps the OAM spectrum to time. The spectrometer consists of a single optical delay loop to achieve timing mapping, a vortex phase plate that iteratively decreases the OAM value, and a single mode fibre to distinguish zero from non-zero OAM states. Light with arbitrarily OAM compositions can be measured. For light with OAM up to 4hbar, we measured an average crosstalk of -21.3 dB, which is mainly limited by the purity of the input states and optical alignment.

physics.optics