arXiv subjects

Craig Holliman

Publications and source records attributed to Craig Holliman.

5 recordsLinked to original sources

arXiv2026

Quantum-HPC hybrid computation of biomolecular excited-state energies

We develop a workflow within the ONIOM framework and demonstrate it on the hybrid computing system consisting of the supercomputer Fugaku and the Quantinuum Reimei trapped-ion quantum computer. This hybrid platform extends the layered approach for biomolecular chemical reactions to accurately treat the active site, such as a protein, and the large and often weakly correlated molecular environment. Our result marks a significant milestone in enabling scalable and accurate simulation of complex biomolecular reactions

quant-ph↗

arXiv2025

Helios: A 98-qubit trapped-ion quantum computer

We report on Quantinuum Helios, a 98-qubit trapped-ion quantum processor based on the quantum charge-coupled device (QCCD) architecture. Helios features $^{137}$Ba$^{+}$ hyperfine qubits, all-to-all connectivity enabled by a rotatable ion storage ring connecting two quantum operation regions by a junction, speed improvements from parallelized operations, and a new software stack with real-time compilation of dynamic programs. Averaged over all operational zones in the system, we achieve average infidelities of $2.5(1)\times10^{-5}$ for single-qubit gates, $7.9(2)\times10^{-4}$ for two-qubit gates, and $4.8(6)\times10^{-4}$ for state preparation and measurement, none of which are fundamentally limited and likely able to be improved. These component infidelities are predictive of system-level performance in both random Clifford circuits and random circuit sampling, the latter demonstrating that Helios operates well beyond the reach of classical simulation and establishes a new frontier of fidelity and complexity for quantum computers.

quant-ph↗

arXiv2025

Lifetimes of the Metastable $6\mathrm{d}\, ^{2}\mathrm{D}_{5/2}$ and $6\mathrm{d}\, ^{2}\mathrm{D}_{3/2}$ States of Ra$^+$

We report lifetime measurements of the metastable $6\mathrm{d}\, ^{2}\mathrm{D}_{5/2}$ and $6\mathrm{d}\, ^{2}\mathrm{D}_{3/2}$ states of Ra$^+$. The measured lifetimes, $\tau_{5} = $ 303.8(1.5) ms and $\tau_{3} = $ 642(9) ms, are important for optical frequency standards and for benchmarking high-precision relativistic atomic theory. Independent of the reported measurements, the D state lifetimes were calculated using the coupled-cluster single double triple method, in which the coupled-cluster equations for both core and valence triple excitations were solved iteratively. The method was designed for precise prediction of atomic properties, especially for heavy elements, where relativistic and correlation corrections become large, making their treatment more challenging. This Letter presents the first tests of the method for transition properties. Our prediction agrees with experimental values within the uncertainties. The ability to accurately predict the atomic properties of heavy elements is important for many applications, from tests of fundamental symmetries to the development of optical clocks.

physics.atom-ph↗

arXiv2024

Laser Cooling and Hyperfine Measurements of Radium-225 Ions

$^{225}$Ra$^+$ ions (nuclear spin $I=1/2$) have transitions that are first-order insensitive to magnetic field noise, which is advantageous for optical clocks and quantum information science. We report on laser cooling and trapping of $^{225}$Ra$^+$ ions and hyperfine splitting measurements of the ion's $\mathrm{7s}$ $^2\mathrm{S}_{1/2}$, $\mathrm{7p}$ $^2\mathrm{P}_{1/2}$, and $\mathrm{6d}$ $^2\mathrm{D}_{3/2}$ states. We measured the ground state hyperfine constant, $A(\mathrm{S}_{1/2}) =$ $-27.684511052(5)$ $\mathrm{GHz}$, and the quadratic Zeeman coefficient, $C_2 =$ $142.3(1.0)$ $\mathrm{Hz\ G}^{-2}$, of the $^2\mathrm{S}_{1/2} (F=0, m_F = 0) \leftrightarrow~^2\mathrm{S}_{1/2} (F=1, m_{F} = 0)$ transition. Our result addresses a discrepancy in the literature for the ground state hyperfine splitting. We measured the hyperfine constants of the $^2\mathrm{P}_{1/2}$ state, $A(\mathrm{P}_{1/2}) =$ $-5.447(4)$ $\mathrm{GHz}$, and the $^2\mathrm{D}_{3/2}$ state, $A(\mathrm{D}_{3/2}) =$ $-619.7(1.1)$ $\mathrm{MHz}$. We also performed state preparation and measurement using the ground state hyperfine levels and realized a fidelity of $0.9951(9)$.

physics.atom-ph↗

arXiv2024

The computational power of random quantum circuits in arbitrary geometries

Empirical evidence for a gap between the computational powers of classical and quantum computers has been provided by experiments that sample the output distributions of two-dimensional quantum circuits. Many attempts to close this gap have utilized classical simulations based on tensor network techniques, and their limitations shed light on the improvements to quantum hardware required to frustrate classical simulability. In particular, quantum computers having in excess of $\sim 50$ qubits are primarily vulnerable to classical simulation due to restrictions on their gate fidelity and their connectivity, the latter determining how many gates are required (and therefore how much infidelity is suffered) in generating highly-entangled states. Here, we describe recent hardware upgrades to Quantinuum's H2 quantum computer enabling it to operate on up to $56$ qubits with arbitrary connectivity and $99.843(5)\%$ two-qubit gate fidelity. Utilizing the flexible connectivity of H2, we present data from random circuit sampling in highly connected geometries, doing so at unprecedented fidelities and a scale that appears to be beyond the capabilities of state-of-the-art classical algorithms. The considerable difficulty of classically simulating H2 is likely limited only by qubit number, demonstrating the promise and scalability of the QCCD architecture as continued progress is made towards building larger machines.

quant-ph↗