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Cristiano Nisoli

Publications and source records attributed to Cristiano Nisoli.

At least 55 records · Page 3Linked to original sources

Classical topological order of the Rys F-model and its breakdown in realistic spin ice: Topological sectors of Faraday loops

Both the Rys F-model and antiferromagnetic square ice posses the same ordered, antiferromagnetic ground state, but the ordering transition is of second order in the latter, and of infinite order in the former. To tie this difference to topological properties and their breakdown, we introduce a Faraday line representation where loops carry the energy and magnetization of the system. Because of the absence of monopoles in the F-model, its loops have distinct topological properties, absent in square ice, and which allow for a natural partition of its phase space into topological sectors. Then the Néel temperature corresponds to a transition from trivial to non-trivial topological sectors. Moreover, its zero susceptibility below a critical field is explained by the homotopy invariance of its magnetization. In spin ices, instead, monopoles destroy the homotopy invariance of the magnetization, and thus erase this rich topological structure. Consequently, even trivial loops can be magnetized, and their susceptibility is never zero.

cond-mat.stat-mech↗

Field Theory for Magnetic Monopoles in (Square, Artificial) Spin Ice

Proceeding from the more general to the more concrete, we propose an equilibrium field theory describing spin ice systems in terms of topological charges and magnetic monopoles. We show that for a spin ice on a graph, the entropic interaction in a Gaussian approximation is the inverse of the graph Laplacian matrix, while the screening function for external charges is the inverse of the screened laplacian. We particularize the treatment to square and pyrochlore ice. For square ice we highlight the gauge-free duality between direct and perpendicular structure in terms of symmetry between charges and currents, typical of magnetic fragmentation in a two-dimensional setting. We derive structure factors, correlations, correlation lengths, and susceptibilities for spins, topological charges, and currents. We show that the divergence of the correlation length at low temperature is exponential and inversely proportional to the mean square charge. While in three dimension real and entropic interactions among monopoles are both 3D-Coulomb, in two dimension the former is a 3D-Coulomb and the latter 2D-Coulomb, or logarithmic, leading to weak singularities in correspondence of the pinch points and destroying charge screening. This suggests that the monopole plasma of square ice is a magnetic charge insulator.

cond-mat.mes-hall↗

Understanding Thermal Annealing of Artificial Spin Ice

We have performed a detailed study of thermal annealing of the moment configuration in artificial spin ice. Permalloy (Ni$_{80}$Fe$_{20}$) artificial spin ice samples were examined in the prototypical square ice geometry, studying annealing as a function of island thickness, island shape, and annealing temperature and duration. We also measured the Curie temperature as a function of film thickness, finding that thickness has a strong effect on the Curie temperature in regimes of relevance to many studies of the dynamics of artificial spin ice systems. Increasing the interaction energy between island moments and reducing the energy barrier to flipping the island moments allows the system to more closely approach the collective low energy state of the moments upon annealing, suggesting new channels for understanding the thermalization processes in these important model systems.

cond-mat.mes-hall↗

Ice Rule and Emergent Frustration in Particle Ice and Beyond

Geometric frustration and the ice rule are two concepts that are intimately connected and widespread across condensed matter. The first refers to the inability of a system to satisfy competing interactions in the presence of spatial constraints. The second, in its more general sense, represents a prescription for the minimization of the topological charges in a constrained system. Both can lead to manifolds of high susceptibility and non-trivial, constrained disorder where exotic behaviors can appear and even be designed deliberately. In this Colloquium, we describe the emergence of geometric frustration and the ice rule in soft condensed matter. This Review excludes the extensive developments of mathematical physics within the field of geometric frustration, but rather focuses on systems of confined micro- or mesoscopic particles that emerge as a novel paradigm exhibiting spin degrees of freedom. In such systems, geometric frustration can be engineered artificially by controlling the spatial topology and geometry of the lattice, the position of the individual particle units, or their relative filling fraction. These capabilities enable the creation of novel and exotic phases of matter, and also potentially lead towards technological applications related to memory and logic devices that are based on the motion of topological defects. We review the rapid progress in theory and experiments and discuss the intimate physical connections with other frustrated systems at different length scales.

cond-mat.soft↗

Artificial Spin Ice Phase-Change Memory Resistors

We study the implications of the anisotropic magnetic resistance on permalloy nanowires, and in particular on the property of the resistance depending on the type of lattice. We discuss how the internal spin configuration of artificial spin ice nanowires can affect their effective resistive state, and which mechanisms can introduce a current-dependent effect dynamic resistive state. We discuss a spin-induced thermal phase-change mechanism, and an athermal domain-wall spin inversion. In both cases we observe memory behavior reminiscent of a memristor, with an I-V hysteretic pinched behavior.

cond-mat.mes-hall↗

Ice Rule Fragility via Topological Charge Transfer in Artificial Colloidal Ice

Artificial particle ices are model systems of constrained, interacting particles. They have been introduced theoretically to study ice-manifolds emergent from frustration, along with domain wall and grain boundary dynamics, doping, pinning-depinning, controlled transport of topological defects, avalanches, and memory effects. Recently such particle-based ices have been experimentally realized with vortices in nano-patterned superconductors or gravitationally trapped colloids. Here we demonstrate that, although these ices are generally considered equivalent to magnetic spin ices, they can access a novel spectrum of phenomenologies that are inaccessible to the latter. With experiments, theory and simulations we demonstrate that in mixed coordination geometries, entropy-driven negative monopoles spontaneously appear at a density determined by the vertex-mixture ratio. Unlike its spin-based analogue, the colloidal system displays a "fragile ice" manifold, where local energetics oppose the ice rule, which is instead enforced through conservation of the global topological charge. The fragile colloidal ice, stabilized by topology, can be spontaneously broken by topological charge transfer.

cond-mat.stat-mech↗

Topology by Design in Magnetic nano-Materials: Artificial Spin Ice

Artificial Spin Ices are two dimensional arrays of magnetic, interacting nano-structures whose geometry can be chosen at will, and whose elementary degrees of freedom can be characterized directly. They were introduced at first to study frustration in a controllable setting, to mimic the behavior of spin ice rare earth pyrochlores, but at more useful temperature and field ranges and with direct characterization, and to provide practical implementation to celebrated, exactly solvable models of statistical mechanics previously devised to gain an understanding of degenerate ensembles with residual entropy. With the evolution of nano--fabrication and of experimental protocols it is now possible to characterize the material in real-time, real-space, and to realize virtually any geometry, for direct control over the collective dynamics. This has recently opened a path toward the deliberate design of novel, exotic states, not found in natural materials, and often characterized by topological properties. Without any pretense of exhaustiveness, we will provide an introduction to the material, the early works, and then, by reporting on more recent results, we will proceed to describe the new direction, which includes the design of desired topological states and their implications to kinetics.

cond-mat.mes-hall↗

Understanding magnetotransport signatures in networks of connected permalloy nanowires

The change in electrical resistance associated with the application of an external magnetic field is known as the magnetoresistance (MR). The measured MR is quite complex in the class of connected networks of single-domain ferromagnetic nanowires, known as "artificial spin ice", due to the geometrically-induced collective behavior of the nanowire moments. We have conducted a thorough experimental study of the MR of a connected honeycomb artificial spin ice, and we present a simulation methodology for understanding the detailed behavior of this complex correlated magnetic system. Our results demonstrate that the behavior, even at low magnetic fields, can be well-described only by including significant contributions from the vertices at which the legs meet, opening the door to new geometrically-induced MR phenomena.

cond-mat.mes-hall↗

Long-time behavior of the $ω\to α$ transition in shocked Zirconium: Interplay of nucleation and plastic deformation

We study the thermally activated, slow conversion of the hysteretically retained $ω$ phase into stable $α$ phase in recovered samples of shocked zirconium. The $ω$-phase decays in time following an algebraic law, unlike the predictions of the nucleation-growth framework for first order transitions, and residual volume fractions of phases and dislocation densities are related by a power law. We propose an explanation for the annealing mechanism through coupled dynamics of dislocations and phase change. We find that the long-time behavior is controlled by the interplay of dislocations, shear fluctuations, and remnant volume fractions of phases, which lead to an algebraic decay in time. For late time, thermally activated quantities such as the dislocation mobility and nucleation rate set the timescale and control the algebraic behavior, respectively. At high enough temperatures this behavior is effectively indistinguishable from standard Avrami kinetics.

cond-mat.mtrl-sci↗

More Opportunities than Wealth: A Network of Power and Frustration

We introduce a minimal agent-based model to qualitatively conceptualize the allocation of limited wealth among more abundant opportunities. We study the interplay of power, satisfaction and frustration in distribution, concentration, and inequality of wealth. Our framework allows us to compare subjective measures of frustration and satisfaction to collective measures of fairness in wealth distribution, such as the Lorenz curve and the Gini index. We find that a completely libertarian, law-of-the-jungle setting, where every agent can acquire wealth from, or lose wealth to, anybody else invariably leads to a complete polarization of the distribution of wealth vs. opportunity. The picture is however dramatically modified when hard constraints are imposed over agents, and they are limited to share wealth with neighbors on a network. We then propose an out of equilibrium dynamics {\it of} the networks, based on a competition between power and frustration in the decision-making of agents that leads to network coevolution. We show that the ratio of power and frustration controls different dynamical regimes separated by kinetic transitions and characterized by drastically different values of the indices of equality. The interplay of power and frustration leads to the emergence of three self-organized social classes, lower, middle, and upper class, whose interactions drive a cyclical regime.

physics.soc-ph↗

Direct Visualization of Memory Effects in Artificial Spin Ice

We experimentally demonstrate that arrays of interacting nanoscale ferromagnetic islands, known as artificial spin ice, develop reproducible microstates upon cycling an applied magnetic field. The onset of this memory effect is determined by the strength of the applied field relative to the array coercivity. Specifically, when the applied field strength is almost exactly equal to the array coercivity, several training cycles are required before the array achieves a nearly completely repeatable microstate, whereas when the applied field strength is stronger or weaker than the array coercivity, a repeatable microstate is achieved after the first minor loop. We show through experiment and simulation that this memory exhibited by artificial spin ice is due to a ratchet effect on interacting, magnetically-charged defects in the island moment configuration and to the complexity of the network of strings of reversed moments that forms during magnetization reversal.

cond-mat.mes-hall↗

Topological Solitons in Helical Strings

The low-energy physics of (quasi)degenerate one-dimensional systems is typically understood as the particle-like dynamics of kinks between stable, ordered structures. Such dynamics, we show, becomes highly non-trivial when the ground states are topologically constrained: a dynamics of the domains rather than on the domains which the kinks separate. Motivated by recently reported observations of charged polymers physisorbed on nanotubes, we study kinks between helical structures of a string wrapping around a cylinder. While their motion cannot be disentangled from domain dynamics, and energy and momentum is not concentrated in the solitons, the dynamics of the domains can be folded back into a one-particle picture.

cond-mat.soft↗

Thermomechanical Stability and Mechanochemical Response of DNA: a Minimal Mesoscale Model

We show that a mesoscale model, with a minimal number of parameters, can well describe the thermomechanical and mechanochemical behavior of homogeneous DNA at thermal equilibrium under tension and torque. We predict critical temperatures for denaturation under torque and stretch, phase diagrams for stable DNA, probe/response profiles under mechanical loads, and the density of dsDNA as a function of stretch and twist. We compare our predictions with available single molecule manipulation experiments and find strong agreement. In particular we elucidate the difference between angularly constrained and unconstrained overstretching. We propose that the smoothness of the angularly constrained overstreching transition is a consequence of the molecule being in the vicinity of criticality for a broad range of values of applied tension.

q-bio.BM↗

Quasi-One-Dimensional Thermal Breakage

Breakage is generally understood in mechanical terms, yet nano-structures can rupture not only under external loads but also via thermal activation. Here we treat in a general framework the statistical mechanics of thermally induced breakage at the nano-scale for one-dimensional systems. We test it on a simple approximation and find that the probability of breakage controls distinct regimes, characterized by sharp crossovers and narrow peaks in the thermal fluctuations and specific heat. Our work provides predictions on clustering of new phases, of relevance in nano-fabrication.

cond-mat.stat-mech↗

Attractive Inverse Square Potential, U(1) Gauge, and Winding Transitions

The inverse square potential arises in a variety of different quantum phenomena, yet notoriously it must be handled with care: it suffers from pathologies rooted in the mathematical foundations of quantum mechanics. We show that its recently studied conformality-breaking corresponds to an infinitely smooth winding-unwinding topological transition for the {\it classical} statistical mechanics of a one-dimensional system: this describes the the tangling/untangling of floppy polymers under a biasing torque. When the ratio between torque and temperature exceeds a critical value the polymer undergoes tangled oscillations, with an extensive winding number. At lower torque or higher temperature the winding number per unit length is zero. Approaching criticality, the correlation length of the order parameter---the extensive winding number---follows a Kosterlitz-Thouless type law. The model is described by the Wilson line of a (0+1) $U(1)$ gauge theory, and applies to the tangling/untangling of floppy polymers and to the winding/diffusing kinetics in diffusion-convection-reactions.

cond-mat.soft↗

Dumping Topological Charges on Neighbors: Ice Manifolds for Colloids and Vortices

We investigate the recently reported analogies between pinned vortices in nano-structured superconductors or colloids in optical traps, and spin ice materials. The frustration of colloids and vortices differs essentially from spin ice. However, their effective energetics is made identical by the contribution of an emergent field associated to the topological charge, thus leading to a (quasi) ice manifold for lattices of even (odd) coordination. The equivalence extends to the local low-energy dynamics of the ice manifold, where the effect of geometric hard constraints can be subsumed into the spatial modulation of the emergent field, which mediates an entropic interaction between topological charges. There, as in spin ice materials, genuine ice manifolds enter a Coulomb phase, whereas quasi-ice manifolds posses a well defined screening length, provided by a plasma of embedded topological charges. The equivalence between the two systems breaks down in lattices of mixed coordination because of topological charge transfer between sub-latices. We discuss extensions to social and economical networks.

cond-mat.stat-mech↗

On the Equivalence of Trapped Colloids, Pinned Vortices, and Spin Ice

We investigate the recently reported analogies between pinned vortices in nano-structured superconductors or colloids in optical traps, and spin ice materials. The frustration of the two models, one describing colloids and vortices, the other describing spin ice, differs essentially. However, their effective energetics is made identical by the contribution of an emergent field associated to a topological charge. This equivalence extends to the local low-energy dynamics of the ice manifold, yet breaks down in lattices of mixed coordination, because of topological charge transfer between sub-latices.

cond-mat.stat-mech↗

Realizing three-dimensional artificial spin ice by stacking planar nanoarrays

Artificial spin ice is a frustrated magnetic two-dimensional nano-material, recently employed to study variety of tailor-designed unusual collective behaviours. Recently proposed extensions to three dimensions are based on self-assembly techniques and allow little control over geometry and disorder. We present a viable design for the realization of a three-dimensional artificial spin ice with the same level of precision and control allowed by lithographic nano-fabrication of the popular two-dimensional case. Our geometry is based on layering already available two-dimensional artificial spin ice and leads to an arrangement of ice-rule-frustrated units which is topologically equivalent to that of the tetrahedra in a pyrochlore lattice. Consequently, we show, it exhibits a genuine ice phase and its excitations are, as in natural spin ice materials, magnetic monopoles interacting via Coulomb law.

cond-mat.mes-hall↗