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D. Das

Publications and source records attributed to D. Das.

At least 19 recordsLinked to original sources

Dimensional Crossover of Mass Anisotropy in Ta-doped WTe2

The observation of extremely large magnetoresistance in WTe2 has attracted considerable attention towards understanding its underlying origin. With its layered van der Waals structure, the question that remains largely unexplored is whether the three-dimensional anisotropic transport characteristics of WTe2 persists under chemical substitution. Here, we present a systematic angle-dependent magneto-transport study of single-crystalline TaxW1-xTe2 (x = 0, 0.05, 0.1). The results are analysed within a mass anisotropy scaling framework to extract the mass anisotropy parameter {\gamma} as a function of temperature and doping. It is observed that Ta substitution leads to monotonic increase of {\gamma} across all temperatures, indicating a progressive deepening of quasi-two-dimensional Fermi surface character. Ta doping also leads to a substantial improvement in crystalline quality, reflected in a pronounced increase in the residual resistivity ratio. Despite weakening electron-hole compensation, the magnetoresistance rises sharply to ~58,211% at x = 0.1, which is assigned to a substantial enhancement in carrier mobility. Rietveld refinement confirms a systematic c-axis contraction with Ta content, identifying the structural origin of the enhanced anisotropy. The mass anisotropy scaling that holds for x = 0 and x = 0.05 breaks down for x = 0.1, where the angular magneto-resistance anisotropy substantially exceeds single-ellipsoid predictions, pointing to a multi-pocket Fermi surface with distinct anisotropies. Nonlinear Hall resistivity provides independent evidence for the underlying multiband character of transport in this system. These findings demonstrate that Fermi surface anisotropy, carrier compensation, and mobility are independent parameters that can lead to tuneable control of large magnetoresistance in topological semimetal WTe2.

cond-mat.mtrl-sci

Demonstrating CBM Capabilities by $\Lambda$ Baryon Reconstruction in Ni+Ni Collisions with the mCBM Experiment at SIS18 of GSI/FAIR

The Compressed Baryonic Matter (CBM) experiment at the upcoming Facility for Antiproton and Ion Research (FAIR) is a high-rate fixed-target experiment designed to investigate nuclear matter at extreme baryon densities in relativistic nucleus-nucleus collisions. To enable high-statistics measurements of rare probes, CBM is designed to operate at event rates up to 10 MHz. This necessitates the development of fast and radiation-tolerant detectors, self-triggered front-end electronics, a free-streaming data acquisition architecture, and real-time event reconstruction capabilities. Prototype versions and pre-series productions of the CBM detector systems have been deployed in the mini-CBM demonstrator setup mCBM - an experimental precursor comprising sub-components of all major CBM systems, installed at the SIS18 facility of GSI/FAIR within the FAIR Phase-0 program. In 2024, Ni+Ni collisions at a kinetic beam energy of 1.93 AGeV and an average interaction rate of about 250 kHz were successfully recorded. This dataset enables a detailed evaluation of the operational performance of the detector systems as well as the complete CBM data chain, while the reconstruction of rare $\Lambda$ baryons serves as a natural benchmark. This paper presents the first results on $\Lambda$ signal reconstruction with the mCBM experiment, demonstrating the readiness of the detector technologies and the data chain for the upcoming full-scale CBM experiment.

physics.ins-det

Single-particle strength toward N = 32: Spectroscopy of 51 Ca via the 50 Ca(d, p) reaction

States in the neutron-rich isotope 51 Ca were populated via the 50 Ca(d, p) transfer reaction in inverse kinematics at a beam energy of about 14 AMeV. The experiment was performed using a decelerated radioactive 50 Ca beam from the OEDO facility and the TiNA2 silicon array in combination with the SHARAQ magnetic spectrometer at RIBF/RIKEN. The energies of excited states in 51 Ca were reconstructed via missing mass spectroscopy, and angular distributions of protons were measured to extract differential cross sections. From a comparison with adiabatic distorted wave approximation (ADWA) calculations, spectroscopic factors were deduced for several states, including the ground state and excited states up to 4.2 MeV. These results are compared with shell-model calculations, as well as ab initio valence-space in-medium similarity renormalization group (VS-IMSRG) predictions. The data support the assignment of the 1/2- and 5/2- single-particle states and provide evidence for a candidate 9/2+ state with a structure consistent with neutron excitation into the 0g9/2 orbital. These findings contribute new constraints on the single-particle structure and shell evolution in neutron-rich calcium isotopes.

nucl-ex

Microscopic origin of hard-plane antiferromagnetism in the Kondo lattice Ce2Rh3Ge5

Hard plane antiferromagnetic order where ordered moments lie perpendicular to the single-ion crystal electric field easy axis is rare in Ce-based Kondo lattices and is a subject of active interest. Here we show that Ce$_2$Rh$_3$Ge$_5$ realizes a hard-plane antiferromagnetic state in which partial delocalization of the local moment gives rise to an RKKY exchange that overturns the single-ion easy-axis preference. Neutron diffraction reveals moments in the $ab$ plane, while inelastic neutron scattering and susceptibility establish a magnetic easy axis along $c$ in the paramagnetic regime, highlighting a clear inversion between single-ion and ordered-state anisotropies. In this work, we establish a unified microscopic framework to consistently account for partial $4f$-moment delocalization, enhanced in-plane RKKY exchange, and the resulting hard-plane antiferromagnetic order. Ce$_2$Rh$_3$Ge$_5$ thus provides a benchmark system in which single-ion anisotropy, Kondo screening, and RKKY exchange compete on comparable energy scales, revealing a cooperative route to hard-axis ordering in strongly hybridized Kondo lattices.

cond-mat.str-el

Isoscalar Giant Resonances in Highly-Deformed $^{172}$Yb

To study the isoscalar giant resonances in a deformed case, background-free $\alpha$-particle inelastic scattering measurements using a 386 MeV $\alpha$ beam were performed on the highly-deformed $^{172}$Yb nucleus using the Grand Raiden spectrometer at the Research Center for Nuclear Physics (RCNP) at very forward angles, including $0^\circ$. The strength distributions for the isoscalar giant resonances up to $L \leq 3$ were obtained using multipole decomposition analysis. The isoscalar giant monopole resonance (ISGMR) strength exhibits a splitting into two components, interpreted as the coupling of the ISGMR with the $K=0$ component of the isoscalar giant quadrupole resonance (ISGQR). A \textit{bimodal} structure is observed in the strength distribution of the isoscalar giant dipole resonance. The ISGQR strength shows an enhancement near 25 MeV, attributed to the excitation of an overtone mode, while the broadening of the main-tone peak is associated with nuclear deformation. The experimental results are well reproduced by theoretical strength distributions calculated using the quasiparticle finite amplitude method for $L \leq 3$.

nucl-ex

Distinct Uniaxial Stress and Pressure Fingerprint of Superconductivity in the 3D Kagome Lattice Compound CeRu2

The exploration of tunable superconductivity in strongly correlated electron systems is a central pursuit in condensed matter physics, with implications for both fundamental understanding and potential applications. The Laves phase CeRu$_{2}$, a pyrochlore compound, exhibits a three-dimensional (3D) Kagome lattice type geometry giving rise to flat bands and degenerate Dirac points, where band structure features intertwine with strong multi-orbital interaction effects deriving from its correlated electronic structure. Here, we combine muon spin rotation ($\mu$SR), uniaxial in-plane stress, and hydrostatic pressure to probe the superconducting state of CeRu$_{2}$. Uniaxial stress up to 0.22 GPa induces a dome-shaped evolution of the critical temperature $T_{\rm c}$, with an initial plateau, successively followed by enhancement and suppression without any structural phase transition. Stress is further found to drive a crossover from anisotropic to isotropic $s$-wave pairing. In contrast, hydrostatic pressure up to 2.2 GPa leaves $T_{\rm c}$ largely unchanged but alters the superfluid density from exponential to linear behavior at low temperatures, indicative of nodal superconductivity under hydrostatic pressure. Taken together, these results indicate that CeRu$_{2}$ occupies an ideal position in parameter space, enabling highly responsive and multifold tunability of superconductivity in this three-dimensional correlated electronic system. This warrants further quantitative analysis of the interplay between lattice geometry, electronic correlations, and pairing symmetry.

cond-mat.supr-con

Effect of ground-state deformation on the Isoscalar Giant Monopole Resonance and the first observation of overtones of the Isoscalar Giant Quadrupole Resonance in rare-earth Nd isotopes

The strength distributions of the Isoscalar Giant Monopole Resonance (ISGMR) and Isoscalar Giant Quadrupole Resonance (ISGQR) in 142,146-150Nd have been determined via inelastic alpha-particle scattering with the Grand Raiden (GR) Spectrometer at the Research Center for Nuclear Physics (RCNP), Japan. In the deformed nuclei 146-150Nd, the ISGMR strength distributions exhibit a splitting into two components, while the nearly spherical nucleus 142Nd displays a single peak in the ISGMR strength distribution. A noteworthy achievement in this study is the first-time detection of overtones in the Isoscalar Giant Quadrupole Resonance (ISGQR) strength distributions within Nd isotopes at an excitation energy around 25 MeV obtained through Multipole Decomposition Analysis (MDA).

nucl-ex

Charge orders with distinct magnetic response in a prototypical kagome superconductor LaRu$_{3}$Si$_{2}$

The kagome lattice has emerged as a promising platform for hosting unconventional chiral charge order at high temperatures. Notably, in LaRu$_{3}$Si$_{2}$, a room-temperature charge-ordered state with a propagation vector of ($\frac{1}{4}$,~0,~0) has been recently identified. However, understanding the interplay between this charge order and superconductivity, particularly with respect to time-reversal-symmetry breaking, remains elusive. In this study, we employ single crystal X-ray diffraction, magnetotransport, and muon-spin rotation experiments to investigate the charge order and its electronic and magnetic responses in LaRu$_{3}$Si$_{2}$ across a wide temperature range down to the superconducting state. Our findings reveal the emergence of a charge order with a propagation vector of ($\frac{1}{6}$,~0,~0) below $T_{\rm CO,2}$ ${\simeq}$ 80 K, coexisting with the previously identified room-temperature primary charge order ($\frac{1}{4}$,~0,~0). The primary charge-ordered state exhibits zero magnetoresistance. In contrast, the appearance of the secondary charge order at $T_{\rm CO,2}$ is accompanied by a notable magnetoresistance response and a pronounced temperature-dependent Hall effect, which experiences a sign reversal, switching from positive to negative below $T^{*}$ ${\simeq}$ 35 K. Intriguingly, we observe an enhancement in the internal field width sensed by the muon ensemble below $T^{*}$ ${\simeq}$ 35 K. Moreover, the muon spin relaxation rate exhibits a substantial increase upon the application of an external magnetic field below $T_{\rm CO,2}$ ${\simeq}$ 80 K. Our results highlight the coexistence of two distinct types of charge order in LaRu$_{3}$Si$_{2}$ within the correlated kagome lattice, namely a non-magnetic charge order ($\frac{1}{4}$,~0,~0) below $T_{\rm co,1}$ ${\simeq}$ 400 K and a time-reversal-symmetry-breaking charge order below $T_{\rm CO,2}$.

cond-mat.supr-con

Depth-dependent study of time-reversal symmetry-breaking in the kagome superconductor $A$V$_{3}$Sb$_{5}$

The breaking of time-reversal symmetry (TRS) in the normal state of kagome superconductors $A$V$_{3}$Sb$_{5}$ stands out as a significant feature. Yet the extent to which this effect can be tuned remains uncertain, a crucial aspect to grasp in light of the varying details of TRS breaking observed through different techniques. Here, we employ the unique low-energy muon spin rotation technique combined with local field numerical analysis to study the TRS breaking response as a function of depth from the surface in single crystals of RbV$_{3}$Sb$_{5}$ with charge order and Cs(V$_{0.86}$Ta$_{0.14}$)$_{3}$Sb$_{5}$ without charge order. In the bulk (i.e., > 33 nm from the surface) of RbV$_{3}$Sb$_{5}$, we have detected a notable increase in the internal magnetic field width experienced by the muon ensemble. This increase occurs only within the charge ordered state. Intriguingly, the muon spin relaxation rate is significantly enhanced near the surface (i.e., < 33 nm from the surface) of RbV$_{3}$Sb$_{5}$, and this effect commences at temperatures significantly higher than the onset of charge order. Conversely, in Cs(V$_{0.86}$Ta$_{0.14}$)$_{3}$Sb$_{5}$, we do not observe a similar enhancement in the internal field width, neither in the bulk nor near the surface. These observations indicate a strong connection between charge order and TRS breaking on one hand, and on the other hand, suggest that TRS breaking can occur prior to long-range charge order. This research offers compelling evidence for depth-dependent magnetism in $A$V$_{3}$Sb$_{5}$ superconductors in the presence of charge order. Such findings are likely to elucidate the intricate microscopic mechanisms that underpin the TRS breaking phenomena in these materials.

cond-mat.supr-con

Ir-Sb Binary System: Unveiling Nodeless Unconventional Superconductivity Proximate to Honeycomb-Vacancy Ordering

Vacancies play a crucial role in solid-state physics, but their impact on materials with strong electron-electron correlations has been underexplored. A recent study on the Ir-Sb binary system, Ir$_{16}$Sb$_{18}$ revealed a novel extended buckled-honeycomb vacancy (BHV) order. Superconductivity is induced by suppressing the BHV ordering through high-pressure growth with excess Ir atoms or isovalent Rh substitution, although the nature of superconducting pairing has remained unexplored. Here, we conduct muon spin rotation experiments probing the temperature-dependence of the effective magnetic penetration depth $\lambda_{eff}\left(T\right)$ in Ir$_{1-{\delta}}$Sb (synthesized at 5.5 GPa with $T_{\rm c}$ = 4.2 K) and ambient pressure synthesized optimally Rh-doped Ir$_{1-x}$Rh$_{x}$Sb ($x$=0.3, $T_{\rm c}$ = 2.7 K). The exponential temperature dependence of the superfluid density $n_{\rm s}$/m$^{*}$ at low temperatures indicates a fully gapped superconducting state in both samples. Notably, the ratio of $T_{\rm c}$ to the superfluid density is comparable to previously measured unconventional superconductors. A significant increase in $n_{\rm s}$/m$^{*}$ in the high-pressure synthesized sample correlates with $T_{\rm c}$, a hallmark feature of unconventional superconductivity. We further demonstrate a similar effect induced by chemical pressure (Rh substitution) and hydrostatic pressure in Ir$_{1-x}$Rh$_{x}$Sb, highlighting that the dome-shaped phase diagram is a fundamental feature of the material. These findings underscore the unconventional nature of the observed superconductivity, and classifies IrSb as the first unconventional superconducting parent phase with ordered vacancies.

cond-mat.supr-con

First (calibration) experiment using proton beam from FRENA at SINP

This work presents the first calibration experiment of a 3 MV Tandetron accelerator, FRENA, performed in May 2022. The $^7$Li(p,n) reaction threshold was measured to calibrate the terminal voltage measuring device. A LiF target of thickness 175 $\mu$g/cm$^2$ was used in the experiment. The measured threshold was 1872$\pm$2.7 keV, indicating 6$-$10 keV energy shift.

physics.ins-det

Microscopic study of the impurity effect in the kagome superconductor La(Ru$_{1-x}$Fe$_{x}$)$_{3}$Si$_{2}$

We report on the effect of magnetic impurities on the microscopic superconducting (SC) properties of the kagome-lattice superconductor La(Ru$_{1-x}$Fe$_{x}$)$_{3}$Si$_{2}$ using muon spin relaxation/rotation. A strong suppression of the superconducting critical temperature $T_{\rm c}$, the SC volume fraction, and the superfluid density was observed. We further find a correlation between the superfluid density and $T_{\rm c}$ which is considered a hallmark feature of unconventional superconductivity. Most remarkably, measurements of the temperature-dependent magnetic penetration depth ${\lambda}$ reveal a change in the low-temperature behavior from exponential saturation to a linear increase, which indicates that Fe doping introduces nodes in the superconducting gap structure at concentrations as low as $x=$~0.015. Our results point to a rare example of unconventional superconductivity in the correlated kagome lattice and accessible tunability of the superconducting gap structure, offering new insights into the microscopic mechanisms involved in superconducting order.

cond-mat.supr-con

Hidden magnetism uncovered in charge ordered bilayer kagome material ScV_6Sn_6

Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV_6Sn_6 does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe a striking enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More remarkably, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AV_3Sb_5 (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices.

cond-mat.str-el

Designing the stripe-ordered cuprate phase diagram through uniaxial-stress

The ability to efficiently control charge and spin in the cuprate high-temperature superconductors is crucial for fundamental research and underpins technological development. Here, we explore the tunability of magnetism, superconductivity and crystal structure in the stripe phase of the cuprate La_2-xBa_xCuO_4, with x = 0.115 and 0.135, by employing temperature-dependent (down to 400 mK) muon-spin rotation and AC susceptibility, as well as X-ray scattering experiments under compressive uniaxial stress in the CuO_2 plane. A sixfold increase of the 3-dimensional (3D) superconducting critical temperature T_c and a full recovery of the 3D phase coherence is observed in both samples with the application of extremely low uniaxial stress of 0.1 GPa. This finding demonstrates the removal of the well-known 1/8-anomaly of cuprates by uniaxial stress. On the other hand, the spin-stripe order temperature as well as the magnetic fraction at 400 mK show only a modest decrease under stress. Moreover, the onset temperatures of 3D superconductivity and spin-stripe order are very similar in the large stress regime. However, a substantial decrease of the magnetic volume fraction and a full suppression of the low-temperature tetragonal structure is found at elevated temperatures, which is a necessary condition for the development of the 3D superconducting phase with optimal T_c. Our results evidence a remarkable cooperation between the long-range static spin-stripe order and the underlying crystalline order with the three-dimensional fully coherent superconductivity. Overall, these results suggest that the stripe- and the SC order may have a common physical mechanism.

cond-mat.supr-con

In-situ uniaxial pressure cell for X-ray and neutron scattering experiments

We present an in-situ uniaxial pressure device optimized for small angle X-ray and neutron scattering experiments at low-temperatures and high magnetic fields. A stepper motor generates force, which is transmitted to the sample via a rod with integrated transducer that continuously monitors the force. The device has been designed to generate forces up to 200 N in both compressive and tensile configurations and a feedback control allows operating the system in a continuous-pressure mode as the temperature is changed. The uniaxial pressure device can be used for various instruments and multiple cryostats through simple and exchangeable adapters. It is compatible with multiple sample holders, which can be easily changed depending on the sample properties and the desired experiment and allow rapid sample changes.

physics.ins-det

Local spectroscopic evidence for a nodeless magnetic kagome superconductor CeRu$_2$

We report muon spin rotation (${\mu}$SR) experiments on the microscopic properties of superconductivity and magnetism in the kagome superconductor CeRu$_{2}$ with $T_{\rm c}$~${\simeq}$~5~K. From the measurements of the temperature-dependent magnetic penetration depth ${\lambda}$, the superconducting order parameter exhibits nodeless pairing, which fits best to an anisotropic $s$-wave gap symmetry. We further show that the $T_{\rm c}$/$\lambda^{-2}$ ratio is comparable to that of unconventional superconductors. Furthermore, the powerful combination of zero-field (ZF)-${\mu}$SR and high-field ${\mu}$SR has been used to uncover magnetic responses across three characteristic temperatures, identified as $T_1^*$~${\simeq}$~110~K, $T_2^*$~${\simeq}$~65~K, and $T_3^*$~${\simeq}$~40~K. Our experiments classify CeRu$_{2}$ as an exceedingly rare nodeless magnetic kagome superconductor.

cond-mat.supr-con

{\mu}SR investigation of the Fe-doped Ca$_{3}$Ru$_{2}$O$_{7}$ polar metal

Ca$_{3}$Ru$_{2}$O$_{7}$ is a polar metal that belongs to the class of multiferroic magnetic materials. Here, tiny amounts of Fe doping in the Ru sites bring about dramatic changes in the electronic and magnetic properties and generate a complex H-T phase diagram. To date, not much is known about the ground state of such a system in the absence of magnetic field. By performing muon-spin spectroscopy (${\mu}$SR) measurements in 5% Fe-doped Ca$_{3}$Ru$_{2}$O$_{7}$ single crystals, we investigate its electronic properties at a local level. Transverse-field ${\mu}$SR results indicate a very sharp normal-to-antiferromagnetic transition at T$_{N}$ = 79.7(1) K, with a width of only 1 K. Zero-field ${\mu}$SR measurements in the magnetically ordered state allow us to determine the local fields B$_{i}$ at the muon implantation sites. By symmetry, muons stopping close to the RuO$_{2}$ planes detect only the weak nuclear dipolar fields, while those stopping next to apical oxygens sense magnetic fields as high as 150 mT. In remarkable agreement with the nominal Fe-doping, a $\sim$ 6% minority of the these muons feel slightly lower fields, reflecting a local magnetic frustration induced by iron ions. Finally, B$_{i}$ shows no significant changes across the metal-to-insulator transition, close to 40 K. We ascribe this surprising lack of sensitivity to the presence of crystal twinning.

cond-mat.str-el