arXiv subjects

D. Quang To

Publications and source records attributed to D. Quang To.

11 recordsLinked to original sources

arXiv2026

Resonance-enhanced super-superexchange yields giant chiral magnon splitting in rutile altermagnets

Altermagnets host momentum-selective spin splitting and chiral-split magnonic excitations despite vanishing net magnetization, enabling spin transport without ferromagnetism. In rutile structures, establishing altermagnetism spectroscopically has been challenging, motivating the search for a rutile platform with a resolvable exchange-driven chiral magnon splitting. Here we combine hybrid-functional first-principles calculations with linear spin-wave theory to show that rutile CuF$_2$ exhibits a meV-scale splitting between magnon modes of opposite chirality along momentum directions dictated by its $d$-wave altermagnetic symmetry. The splitting originates from an anomalously strong long-range super-superexchange channel Cu--F$\cdots$F--Cu, which enhances the symmetry-allowed difference between seventh-neighbour exchanges, $J_{7b} - J_{7a}$, controlling the chiral-mode splitting. We identify an orbital-resonance mechanism: energetic alignment between Cu $3d_{z^2}$ and F $2p_z$ states strengthens virtual hopping along the Cu--F$\cdots$F--Cu path and amplifies the anisotropic long-range exchange. Rutile CuF$_2$ therefore provides an ideal platform to validate rutile altermagnetism and suggests an orbital-energy description for engineering large chiral magnon splittings in insulating altermagnets.

cond-mat.mtrl-sci↗

arXiv2025

Quantum geometric origins of the orbital degrees of freedom of hybrid bosonic quasiparticles in magnetic systems

The orbital degree of freedom has recently attracted significant attention due to the novel phenomena it enables in condensed matter systems. However, the interpretation of the orbital degree of freedom in bosonic quasiparticles remains conceptually ambiguous and the mechanisms governing the transfer of orbital angular moment (OAM) between distinct quasiparticles, such as magnons and phonons, are not yet fully understood. We investigate orbital dynamics in bosonic systems and identify two origins of OAM: (i) global rotational motion of the system, and (ii) the quantum geometry of wavefunctions. Focusing on the latter, we study strongly coupled magnon-phonon systems in two-dimensional antiferromagnets as a test case. We uncover finite OAM arising from quantum geometric effects via two mechanisms: (a) time-parity symmetry breaking, yielding intra band OAM, and (b) interband coupling, generating interband OAM. We propose that an electrical detection scheme based on the transverse voltage generated by hybrid magnon phonon modes can be used to experimentally probe the bosonic orbital degree of freedom. Our results establish a foundation for the emerging field of phonon orbitronics, providing both a conceptual bridge between phonon and magnon orbitronics and a tool for better understanding magnon-polarons. They also advance a unified framework for harnessing orbital degrees of freedom in bosonic systems and pave the way toward electrical control of magnetization and phononic transport.

cond-mat.mes-hall↗

arXiv2025

Probing Magnetic Properties of RuO$_{2}$ Heterostructures Through the Ferromagnetic Layer

RuO$_{2}$ has been proposed as the prototypical altermagnetic material. However, several reports have recently questioned its intrinsic magnetic ordering, leading to conflicting findings, especially in thin film heterostructures pointing to possible interface effects being convoluted with supposed antiferromagnetic/altermagnetic signatures. Here, extensive magnetometry measurements were performed on two independently grown thin film heterostructures of RuO$_{2}$ interfaced with either NiFe or Fe acting as the ferromagnetic layer. Below about 15 K, both samples exhibit exchange bias fields when cooled to approximately 2 K in a $+$1 T field, and a spin transitional feature is observed around 31 K. Magneto-Raman measurements on RuO$_{2}$ thin films only reveal a magnon mode when there is a NiFe layer, suggesting that RuO$_{2}$ does not intrinsically possess long range magnetic ordering.. When in contact with a ferromagnet, RuO$_2$ displays effects that could be ascribed to antiferromagnetism. However, the lack of intrinsic magnon modes points toward possible diffusion between the layers or spin disorder at the interface as seen by density functional theory (DFT) calculations.

cond-mat.mtrl-sci↗

arXiv2025

Tunable magnon band topology and magnon orbital Nernst effect in noncollinear antiferromagnets

We theoretically investigate the intrinsic magnon orbital Nernst effect (ONE) in noncollinear antiferromagnets with Kagom\'e spin systems. Our analysis reveals that an externally applied magnetic field induces topological phase transitions in the magnonic system, characterized by the closing and reopening of the band gap between distinct magnon bands. These transitions enable tunable control of the magnon orbital Nernst effect with applied magnetic field, with a pronounced enhancement in magnon orbital Nernst conductivity near the phase transition points. This tunability presents a promising direction for experimental detection of the magnon ONE.

cond-mat.mtrl-sci↗

arXiv2025

Symmetry-breaking induced surface magnetization in non-magnetic RuO$_2$

Altermagnetism is a newly identified phase of magnetism distinct from ferromagnetism and antiferromagnetism. RuO$_2$ has been considered a prototypical metallic altermagnet with a critical temperature higher than room temperature. Previous interpretations of the unusual magnetic properties of RuO$_2$ relied on the theoretical prediction that local moments on two Ru sublattices, which are connected by four-fold rotational symmetry, are quite significant (approximately 1 $\mu_B$), leading to long-range antiferromagnetic order. However, accumulated experimental data suggest that local moments on Ru in RuO$_2$ are vanishingly small, indicating that the bulk material is likely non-magnetic. This observation is consistent with the delocalized nature of the 4$d$ electrons of Ru and the strong screening effect in the metallic state. In this work, we show that despite the non-magnetic bulk, the RuO$_2$(110) surface exhibits spontaneous magnetization. We attribute this effect to the breaking of local symmetry, which results in electronic redistribution and magnetic moment enhancement. The emergence of surface magnetism gives rise to interesting spectroscopic phenomena, including spin-polarized surface states, spin-polarized scanning probe microscopy images, and potentially spin-dependent transport effects. These findings highlight the important role of surface magnetic structures in the otherwise non-magnetic bulk RuO$_2$.

cond-mat.mtrl-sci↗

arXiv2024

Electric polarization induced by magnons and magnon Nernst effects

Magnons offer a promising path toward energy-efficient information transmission and the development of next-generation classical and quantum computing technologies. However, methods to efficiently excite, manipulate, and detect magnons remain a critical need. Here, we show that magnons, despite their charge-neutrality, can induce electric polarization as a result of both their spin and orbital moments. We demonstrate this by calculating the electric polarization induced by magnons in two-dimensional (2D) honeycomb antiferromagnets. The electric polarization becomes finite when the Dzyaloshinskii-Moriya Interaction (DMI) is present and its magnitude can be increased by symmetries of the system. We illustrate this by computing and comparing the electric polarizations induced by the magnon Nernst effects in 2D materials with N\'eel and Zigzag ordering. Our findings show that in the Zigzag order, where the effect is dominated by the magnon orbital moment, the induced electric polarization is approximately three orders of magnitude greater than in the N\'eel phase. These findings reveal that electric fields could enable both detection and manipulation of magnons under certain conditions by leveraging their spin and orbital angular moment. They also suggest that the discovery or engineering of materials with substantial magnon orbital moments could lead to more practical use of magnons for future computing and information transmission device applications.

cond-mat.mes-hall↗

arXiv2023

Non-trivial topology in rare-earth monopnictides from dimensionality reduction

Thin films of rare-earth monopnictide semimetals are expected to turn into semiconductors due to quantum confinement effect, which lifts the overlap between electron pockets at Brillouin zone edges and hole pockets at the zone center. Instead, taking non-magnetic LaSb as an example, we find the emergence of a quantum spin Hall insulator phase in LaSb(001) films as the thickness is reduced to 7, 5, or 3 monolayers. This is attributed to a strong quantum confinement effect on the in-plane electron pockets, and the lack of quantum confinement on the out-of-plane pocket in reciprocal space projected onto zone center, leading to a band inversion. Spin-orbit coupling opens a sizeable non-trivial gap in the band structure of the thin films. Such effect is shown to be general in rare-earth monopnictides and may lead to interesting phenomena when coupled with the 4f magnetic moments present in other members of this family of materials.

cond-mat.mtrl-sci↗

arXiv2022

Phonon-mediated strong coupling between a three-dimensional topological insulator and a two-dimensional antiferromagnetic material

Van der Waals antiferromagnetic and topological insulator materials provide powerful platforms for modern optical, electronic, and spintronic devices applications. The interaction between an antiferromagnet (AFM) and a topological insulator (TI), if sufficiently strong, could offer emergent hybrid material properties that enable new functionality exceeding what is possible in any individual material constituent. In this work, we study strong coupling between THz excitations in a three dimensional (3D) topological insulator and a quasi-two dimensional (2D) antiferromagnetic material resulting in a new hybridized mode, namely a surface Dirac plasmon-phonon-magnon polariton. We find that the interaction between a surface Dirac plasmon polariton in the 3D TI and a magnon polariton in the 2D AFM is mediated by the phonon coupling in the 3D TI material. The coupling of phonons with an electromagnetic wave propagating in the 3D TI enhances the permittivity of the TI thin film in a way that results in a strong correlation between the dispersion of Dirac plasmon polaritons on the surfaces of the TI with the thickness of the TI. As a result, the dispersion of surface Dirac plasmon polaritons in the TI can be tuned toward resonance with the magnon polariton in the AFM material by varying the TI's thickness, thereby enhancing the strength of the coupling between the excitations in the two materials. The strength of this coupling, which results in the surface Dirac plasmon-phonon-magnon polariton, can be parameterized by the amplitude of the avoided-crossing splitting between the two polariton branches at the magnon resonance frequency...

cond-mat.mes-hall↗

arXiv2022

Surface plasmon-phonon-magnon polariton in a topological insulator-antiferromagnetic bilayer structure

We present a robust technique for computationally studying surface polariton modes in hybrid materials. We use a semi-classical model that allows us to understand the physics behind the interactions between collective excitations of the hybrid system and develop a scattering and transfer matrix method that imposes the proper boundary conditions to solve Maxwell equations and derive a general equation describing the surface polariton in a heterostructure consisting of N constituent materials. We apply this method to a test structure composed of a topological insulator (TI) and an antiferromagnetic material (AFM) to study the resulting surface Dirac plasmon-phonon-magnon polariton (DPPMP). We find that interactions between the excitations of the two constituents result in the formation of hybridized modes and the emergence of avoided-crossing points in the dispersion relations for the DPPMP. For the specific case of a Bi2Se3 TI material, the polariton branch with low frequency below 2 THz redshifts upon increasing the thickness of TI thin film, which leads to an upper bound on the thickness of the TI layer that will allow an observable signature of strong coupling and the emergence of hybridized states. We also find that the strength of the coupling between the TI and the AFM, which is parameterized by the amplitude of the avoided-crossing splitting between the two polariton branches at the magnon resonance frequency, depends on the magnitude of the magnetic dipole and the line width of the magnon in the AFM material as well as on the Fermi energy of Dirac plasmon in the TI. Finally, we predict that materials with extremely high quality, i.e. low scattering loss rate, are essential to achieve an experimentally-observable strong coupling between a TI and AFM.

cond-mat.mtrl-sci↗

arXiv2022

Strong coupling between a topological insulator and a III-V heterostructure at terahertz frequency

We probe theoretically the emergence of strong coupling in a system consisting of a topological insulator (TI) and a III-V heterostructure using a numerical approach based on the scattering matrix formalism. Specifically, we investigate the interactions between terahertz excitations in a structure composed of Bi$_{2}$Se$_{3}$ and GaAs materials. We find that the interaction between the Bi$_{2}$Se$_{3}$ layer and AlGaAs/GaAs quantum wells with intersubband transitions (ISBTs) in the terahertz frequency regime creates new hybrid modes, namely Dirac plasmon-phonon-ISBT polaritons. The formation of these hybrid modes results in anti-crossings (spectral mode splitting) whose magnitude is an indication of the strength of the coupling. By varying the structural parameters of the constituent materials, our numerical calculations reveal that the magnitude of splitting depends strongly on the doping level and the scattering rate in the AlGaAs/GaAs quantum wells, as well as on the thickness of the GaAs spacer layer that separates the quantum-well structure from the TI layer. Our results reveal the material and device parameters required to obtain experimentally-observable signatures of strong coupling. Our model includes the contribution of an extra two-dimensional hole gas (2DHG) that is predicted to arise at the Bi$_{2}$Se$_{3}$/GaAs interface, based on density functional theory (DFT) calculations that explicitly account for details of the atomic terminations at the interface. The presence of this massive 2DHG at the TI/III-V interface shifts the dispersion of the Dirac plasmon-ISBT polaritons to higher frequencies. The damping rate at this interface, in contrast, compensates the effect of the 2DHG. Finally, we observe that the phonon resonances in the TI layer are crucial to the coupling between the THz excitations in the TI and III-V materials.

cond-mat.mtrl-sci↗

arXiv2017

Theory of the Anomalous Tunnel Hall Effect at Ferromagnet-Semiconductor Junctions

We report on theoretical investigations of carrier scattering asymmetry at ferromagnet-semiconductor junctions. By an analytical $2\times 2$ spin model, we show that, when Dresselhaus interactions is included in the conduction band of III-V $T_d$ symmetry group semiconductors, the electrons may undergo a difference of transmission vs. the sign of their incident parallel wavevector normal to the in-plane magnetization. This asymmetry is universally scaled by a unique function independent of the spin-orbit strength. This particular feature is reproduced by a multiband $\mathbf{k}\cdot \mathbf{p}$ tunneling transport model. Astonishingly, the asymmetry of transmission persists in the valence band of semiconductors owing to the inner atomic spin-orbit strength and free of asymmetric potentials . We present multiband $14\times 14$ and $30\times 30$ $\mathbf{k}\cdot \mathbf{p}$ tunneling models together with tunneling transport perturbation calculations corroborating these results. Those demonstrate that a tunnel spin-current normal to the interface can generate a surface transverse charge current, the so-called Anomalous Tunnel Hall Effect.

cond-mat.mtrl-sci↗