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D. S. Leonard

Publications and source records attributed to D. S. Leonard.

At least 19 recordsLinked to original sources

Characterization of CRYO ASIC for charge readout in the nEXO experiment

nEXO is a proposed next-generation experiment searching for the neutrinoless double beta decay of $^{136}$Xe using a tonne-scale liquid xenon (LXe) time projection chamber (TPC). To image the ionization signals from events in the liquid xenon, the detector will employ metallized fused-silica charge collection tiles instrumented with cryogenic application-specific integrated circuits (ASICs), referred to as CRYO ASIC, which are designed to operate directly in LXe to minimize input capacitance and pick-up noise. Here we present the performance of the CRYO ASIC mounted on an auxiliary printed circuit board and evaluated both in a cryogenic environmental chamber and in a dedicated LXe test stand. We demonstrate that the ASICs achieve the desired performance at liquid xenon temperatures, showing a gain stability better than 0.2% over 24-hour operation and reliable in-situ calibration using an on-chip pulser. In the LXe test stand, we show that boiling caused by the chip heat dissipation can be mitigated by operating the system above ~0.1 MPa. The in-LXe noise measured agrees with simulation, which indicates it the $150~e^-$ design requirement can be satisfied. These results establish CRYO ASIC as a viable low-noise in-LXe charge readout solution for nEXO.

physics.ins-det

Pushing the Limits of Pulse Shape Discrimination in a Large Liquid Xenon Detector

The LUX-ZEPLIN (LZ) experiment is a direct-detection dark matter experiment, optimized to search for weakly interacting massive particles (WIMPs) through WIMP-nucleon interactions. The main challenge in dark matter detection is differentiating between WIMP signals and background events. In LZ, the ratio of ionization to scintillation signals (charge-to-light) is the primary method for rejecting electronic recoil (ER) background. Pulse shape discrimination (PSD) offers a method for additional ER backgrounds rejection in liquid xenon detectors. In this paper, the discrimination power of PSD with the LZ experiment is discussed. To precisely characterize the scintillation pulse shape, an analysis framework is developed to reconstruct the detection time of individual photons. Using LZ calibration data, the photon-timing prompt fraction discriminator is optimized and achieves ER leakage as low as $15\%$. For specific background processes such as $^{124}$Xe double electron capture, the leakage is reduced further to about $5\%$. PSD is combined with charge-to-light to form two-factor discrimination (TFD). The optimized TFD performance is compared with the performance of the charge-to-light method, with the corresponding false positive rate reduced by up to a factor of two for large scintillation pulses. Finally, PSD and TFD are applied to data from LZ's WS2024 run and their performance is summarized.

physics.ins-det

Flow-dependent tagging of $^{214}$Pb decays in the LZ dark matter detector

The LUX-ZEPLIN (LZ) experiment is searching for dark matter interactions in a liquid xenon time projection chamber (LXe-TPC). This article demonstrates how control of the flow state in the LXe-TPC enables the identification of pairs of sequential alpha-decays, which are used to map fluid flow and ion drift in the liquid target. The resulting transport model is used to tag \UChPb~ beta-decays, a leading background to dark matter signals in LZ. Temporally evolving volume selections, at a cost of 9.0\% of exposure, target the decay of each \UChPb~ atom up to 81 minutes after production, resulting in (63~$\pm$~6$_{(\mathrm{stat})}$~$\pm$~7$_{(\mathrm{sys})}$)\% identification of \UChPb~decays to ground state. We also demonstrate how flow-based tagging techniques enable a novel calibration side band that is concurrent with science data. Finally we report updated estimates of radon-chain charge branching fractions in liquid xenon, finding branching to $^{218}$Po$^+$ at $0.49 \pm 0.01$, $^{214}$Pb$^+$ at $0.48 \pm 0.12$, and $^{214}$Bi$^+$ at $0.74 \pm 0.05$, with a mean charged ion lifetime in the LZ TPC of $49 \pm 4$ min.

physics.ins-det

Search for New Physics via Low-Energy Electron Recoils with a 4.2 Tonne\times Year Exposure from the LZ Experiment

We report results from searches for new physics models through electron recoils using data collected by the LUX-ZEPLIN (LZ) experiment during its first two science runs, with a total exposure of 4.2 tonne-years. The observed data are consistent with a background-only hypothesis. Constraints are derived for electromagnetic interactions of solar neutrinos, solar axion-like particles (ALPs), mirror dark matter, and the absorption of bosonic dark matter candidates. The inverse Primakoff process for 57Fe de-excitation solar ALPs is considered for the first time. These results represent the most stringent constraints to date on keV-scale Primakoff and 57Fe solar ALPs, bosonic dark matter, mirror dark matter, and neutrino millicharge, while remaining competitive for the other signal models investigated.

hep-ex

Probing unexplored spin-dependent dark matter-proton coupling with few-photoelectron threshold in COSINE-100

We report new constraints on the spin-dependent scattering cross section between low-mass dark matter and protons using data collected by the COSINE-100 experiment. By implementing a specialized event selection process using a multi-layer perceptron and robust noise mitigation, this analysis pioneers a detection threshold of 3 and 4 isolated peaks, corresponding to the reconstructed photoelectrons, which are significantly lower than the 8 photoelectron threshold used in previous analyses. In this unstudied few-photoelectron regime, where instrumental noise and phosphorescence are prevalent, we utilize a phenomenological background model to search for the annual modulation signal expected from the Standard Halo Model. No statistically significant annual modulation is observed in our data. We derive new 90% confidence level (C.L.) upper limits for the spin-dependent DM-proton cross section, establishing the world's most stringent constraints in the 1.75-2.25 GeV/c$^2$ mass range. Furthermore, by incorporating the Migdal effect, we extend the experimental sensitivity to the sub-GeV/c$^2$ regime, setting world-leading limits in the 15-58 MeV/c$^2$ range. These results demonstrate the capability of NaI(Tl) target materials to probe previously unexplored regions of the dark matter parameter space.

hep-ex

A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0ν\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0ν\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0ν}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0νββ$ search program.

nucl-ex

Precision measurement of positron decay modes of Xe-125 in the LUX-ZEPLIN experiment

The radioisotope $^{125}\text{Xe}$ is a short-lived ($T_{1/2}\sim16.9 h$) activation product of the neutron calibrations performed in the LUX-ZEPLIN experiment. Subsequently, $^{125}$Xe decays primarily ($>99\%$) via electron capture, but positron emission has been confirmed by direct measurement to at least the 243 keV level of $^{125}\text{I}$. An additional decay to the 188keV level is expected from triple-coincident measurements of the annihilation and relaxation $γ$ rays, but has not been directly confirmed. By utilizing multiple-scatter event analysis and the pre-activation data to constrain backgrounds, this work reports positron emission with a statistical significance of 5.5$σ$. This corresponds to a total branching ratio of $0.29\pm0.08_{\text{stat.}}\pm0.04_{\text{sys.}}$ %, and is the first constraint to the individual branching levels of $^{125}\text{I}$.

hep-ex

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det

Constraints on sub-GeV dark matter scattering on electrons with COSINE-100

We present results of the search for sub-GeV dark matter interaction with electrons in the NaI(Tl) crystals of the COSINE-100 experiment. The two benchmark scenarios of a heavy and a light vector boson as mediator of the interaction were studied. We found no excess events over the expected background in a data-set of 2.82 years, with a total exposure of 172.9 kg-year. The derived 90% confidence level upper limits exclude a DM-electron scattering cross section above 6.4 $\times$ 10$^{-33}$ cm$^2$ for a DM mass of 0.25 GeV, assuming a light mediator; and above 3.4 $\times$ 10$^{-37}$ cm$^2$ for a 0.4 GeV DM, assuming a heavy mediator, and represent the most stringent constraints for a NaI(Tl) target to date. We also briefly discuss a planned analysis using an annual modulation method below the current 0.7 keV threshold of COSINE-100, down to few photoelectrons yield.

hep-ex

Study of few-electron backgrounds in the LUX-ZEPLIN detector

The LUX-ZEPLIN (LZ) experiment aims to detect rare interactions between dark matter particles and xenon. Although the detector is designed to be the most sensitive to GeV/$c^2$--TeV/$c^2$ Weakly Interacting Massive Particles (WIMPs), it is also capable of measuring low-energy ionization signals down to a single electron that may be produced by scatters of sub-GeV/$c^2$ dark matter. The major challenge in exploiting this sensitivity is to understand and suppress the ionization background in the few-electron regime. We report a characterization of the delayed electron backgrounds following energy depositions in the LZ detector under different detector conditions. In addition, we quantify the probability for photons to be emitted in coincidence with electron emission from the high voltage grids. We then demonstrate that spontaneous grid electron emission can be identified and rejected with a high efficiency using a coincident photon tag, which provides a tool to improve the sensitivity of future dark matter searches.

physics.ins-det

Measurement of the Muon Flux at the Sanford Underground Research Facility with the LUX-ZEPLIN Dark Matter Detector

High-energy cosmic-ray muons reaching deep underground laboratories can cause events in detectors that mimic signals expected from dark matter particles, neutrinos, or rare decays. Knowledge of the muon flux and energy spectrum is important for evaluating the background rate caused by muons and their secondaries. In this paper, we report the measurement of the cosmic-ray muon flux in the Davis Campus of the Sanford Underground Research Facility with the LUX-ZEPLIN detector. Using 366.4~days of exposure, the muon rate through the detector was measured as $10.94\pm0.17_\textrm{stat.}~\textrm{day}^{-1}$ with energy thresholds of 20~MeV in the inner xenon detector and 8 MeV in the outer liquid scintillator detector. This rate corresponds to a muon flux of $(5.09\pm0.08_\textrm{stat.}\pm0.10_\textrm{sys.})\times10^{-9}~\textrm{cm}^{-2}\textrm{s}^{-1}$ in the Davis Cavern.

hep-ex

Search for Double Beta Decays of $^{134}$Xe with EXO-200 Phase II

EXO-200 was a leading double beta decay experiment consisting of a single-phase, enriched liquid xenon time projection chamber filled with an admixture of 80.672% $^{136}$Xe and 19.098% $^{134}$Xe. The detector operated at WIPP between 2010 and 2018 and was designed to search for double beta decay of $^{136}$Xe. Data was acquired in two phases separated by a period of detector upgrades. We report on the search for $0νββ$ and $2νββ$ decay of $^{134}$Xe with Phase II EXO-200 data, with median 90% C.L. exclusion sensitivity $T_{1/2}^{0ν} \geq 3.7\times 10^{23}$ yr and $T_{1/2}^{2ν} \geq 2.6 \times 10^{21}$ yr, respectively. No statistically significant signal is observed for either decay mode. We set a world-leading lower limit on the half-life of the neutrinoless decay mode of $^{134}$Xe of $T_{1/2}^{0ν} \geq 8.7\times10^{23}$ (90% C.L.) and the second strongest constraint on the two-neutrino decay of $T_{1/2}^{2ν} \geq 2.9\times10^{21}$ (90% C.L.), a 3-fold improvement over the EXO-200 Phase I measurement. New constraints are also set for the $2νββ$ and $0νββ$ decays of $^{134}$Xe to the lowest excited state of $^{134}$Ba.

nucl-ex

Limits on WIMP dark matter with NaI(Tl) crystals in three years of COSINE-100 data

We report limits on WIMP dark matter derived from three years of data collected by the COSINE-100 experiment with NaI(Tl) crystals, achieving an improved energy threshold of 0.7 keV. This lowered threshold enhances sensitivity in the sub-GeV mass range, extending the reach for direct detection of low-mass dark matter. Although no excess of WIMP-like events was observed, the increased sensitivity enabled a model-insensitive comparison between the expected WIMP signal rate-based on mass limits from our data-and DAMA's reported modulation amplitude. Our findings strongly disfavor the DAMA signal as originating from WIMP interactions, fully excluding DAMA/LIBRA 3$σ$ allowed regions and providing enhanced WIMP mass limits by an order of magnitude in the spin-independent model compared to previous results. In the spin-dependent model, cross-section upper limits were obtained in the mass range [0.1-5.0] GeV/c$^2$, with additional sensitivity to sub-GeV WIMPs through the inclusion of the Migdal effect. These results represent substantial progress in low-mass dark matter exploration and reinforce constraints on the longstanding DAMA claim.

hep-ex

Combined Annual Modulation Dark Matter Search with COSINE-100 and ANAIS-112

The annual modulation signal, claimed to be consistent with dark matter as observed by DAMA/LIBRA in a sodium-iodide based detector, has persisted for over two decades. COSINE-100 and ANAIS-112 were designed to test the claim directly using the same target material. COSINE-100, located at Yangyang Underground Laboratory in South Korea, and ANAIS-112, located at Canfranc Underground Laboratory in Spain, have been taking data since 2016 and 2017, respectively. Each experiment published its respective results independently. In this paper, we present the results of an annual modulation search as a test of the signal observed by DAMA/LIBRA with the first three respective years of data from COSINE-100 and ANAIS-112. Using a Markov Chain Monte Carlo method, we find best fit values for modulation amplitude of $-0.0002 {\pm} 0.0026$ cpd/kg/keV in the 1-6 keV and $0.0021 {\pm} 0.0028$ cpd/kg/keV in the 2-6 keV energy regions. These results are not compatible with DAMA/LIBRA's assertion for their observation of annual modulation at $3.7σ$ and $2.6σ$, respectively. Performing a simple combination of the newly released 6-years datasets from both experiments find values consistent with no modulation at $0.0005 {\pm} 0.0019$ cpd/kg/keV in the 1-6 keV and $0.0027 {\pm} 0.0021$ cpd/kg/keV in the 2-6 keV energy regions with $4.68σ$ and $3.53σ$ respective exclusions of the DAMA/LIBRA signal.

astro-ph.IM

Low-energy nuclear recoil calibration of the LUX-ZEPLIN experiment with a photoneutron source

The LZ experiment is a liquid xenon time-projection chamber (TPC) searching for evidence of particle dark matter interactions. In the simplest assumption of elastic scattering, many dark matter models predict an energy spectrum which rises quasi-exponentially with decreasing energy transfer to a target atom. LZ expects to detect coherent neutrino-nucleus scattering of $^{8}$B solar neutrinos, the signal from which is very similar to a dark matter particle with mass of about 5.5 GeV/$c^{2}$, which result in typical nuclear recoil energies of $<$5 keV$_{\text{nr}}$. Therefore, it is of crucial importance to calibrate the response of recoiling xenon nuclei to keV-energy recoils. This analysis details the first in situ photoneutron calibration of the LZ detector and probes its response in this energy regime.

physics.ins-det

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $μ$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

COSINE-100 Full Dataset Challenges the Annual Modulation Signal of DAMA/LIBRA

For over 25 years, the DAMA/LIBRA collaboration has claimed to observe an annual modulation signal, suggesting the existence of dark matter interactions. However, no experiment employing different target materials has observed a dark matter signal consistent with their result. To address this puzzle, the COSINE-100 collaboration conducted a model-independent test using sodium iodide crystal detectors, the same target material as DAMA/LIBRA. Analyzing data collected over 6.4 years by the effective mass of 61.3 kg, with improved energy calibration and time-dependent background modeling, we found no evidence of an annual modulation signal, challenging the DAMA/LIBRA result with a confidence level greater than 3$σ$. This finding represents a substantial step toward resolving the long-standing debate surrounding DAMA/LIBRA's dark matter claim, indicating that the observed modulation is unlikely to be caused by dark matter interactions.

hep-ex