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D. V. Poda

Publications and source records attributed to D. V. Poda.

90 records · Page 5Linked to original sources

Search for 2β decay of 116Cd with the help of enriched 116CdWO4 crystal scintillators

Cadmium tungstate crystal scintillators enriched in $^{116}$Cd to 82% ($^{116}$CdWO$_4$, total mass of $\approx$1.2 kg) are used to search for 2$β$ decay of $^{116}$Cd deep underground at the Gran Sasso National Laboratory of the INFN (Italy). The radioactive contamination of the $^{116}$CdWO$_4$ crystals has been studied carefully to reconstruct the background of the detector. The measured half-life of $^{116}$Cd relatively to 2$ν$2$β$ decay is $T^{2\nu2β}_{1/2}$ = [2.8 $\pm$ 0.05(stat.) $\pm$ 0.4(syst.)] $\times$ 10$^{19}$ yr, in agreement with the results of previous experiments. The obtained limit on the 0$ν$2$β$ decay of $^{116}$Cd (considering the data of the last 8696 h run with an advanced background 0.12(2) counts/yr/kg/keV in the energy interval 2.7-2.9 MeV) is $T_{1/2} \ge 1.0 \times 10^{23}$ yr at 90% C.L. The sensitivity of the experiment to the $0\nu2β$ process is $\lim T_{1/2} = 3 \times 10^{23}$ yr at 90% C.L. over 5 years of the measurements and it can be advanced (by further reduction of the background by a factor 3-30) to the level of $\lim T_{1/2} = (0.5-1.5) \times 10^{24}$ yr for the same period of the data taking.

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Search for Rare Nuclear Decays with HPGe Detectors at the STELLA Facility of the LNGS

Results on the search for rare nuclear decays with the ultra low background facility STELLA at the LNGS using gamma ray spectrometry are presented. In particular, the best T1/2 limits were obtained for double beta processes in 96Ru and 104Ru. Several isotopes, which potentially decay through different double beta decay channels, including also possible resonant double electron captures, were investigated for the first time (156Dy, 158Dy, 184Os, 192Os, 190Pt, 198Pt). Search for resonant absorption of solar 7Li axions in a LiF crystal gave the best limit for the mass of 7Li axions (< 8.6 keV). Rare alpha decay of 190Pt to the first excited level of 186Os (Eexc = 137.2 keV) was observed for the first time.

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Astrophysical and cosmological problems of invisible mass and dark energy in the Universe

The Workshop on results of the Project Kosmomikrofizyka-2 (Astroparticle Physics) of the National Academy of Sciences (NAS) of Ukraine "Astrophysical and cosmological problems of invisible mass and dark energy in the Universe" was held on November 21-22, 2012 in the Institute for Nuclear Research, Kyiv, Ukraine (http://lpd.kinr.kiev.ua/kmf12). This Project was carried out during three years (2010-2012) by scientists from various universities and institutes of the National Academy of Sciences of Ukraine; it was a logical continuation of the previous scientific program of the NAS of Ukraine "Researches of structure and composition of the Universe, hidden mass and dark energy (Kosmomikrofizyka)" in 2007-2009. These programs were devoted to theoretical and experimental investigations in astronomy, astrophysics, cosmology, physics of atomic nuclei and particle physics, which are related with the problems of dark matter and dark energy in the Universe.

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Search for 2β decays of 96Ru and 104Ru by ultra-low background HPGe gamma spectrometry at LNGS: final results

An experiment to search for double beta decay processes in 96Ru and 104Ru, which are accompanied by gamma rays, has been realized in the underground Gran Sasso National Laboratories of the I.N.F.N. (Italy). Ruthenium samples with masses of about (0.5-0.7) kg were measured with the help of ultra-low background high purity Ge gamma ray spectrometry. After 2162 h of data taking the samples were deeply purified to reduce the internal contamination of 40K. The last part of the data has been accumulated over 5479 h. New improved half life limits on 2β+/εβ+/2ε processes in 96Ru have been established on the level of 10^{20} yr, in particular for decays to the ground state of 96Mo: T1/2(2ν2β+) > 1.4 10^{20} yr, T1/2(2νεβ+) > 8.0 10^{19} yr and T1/2(0ν2K) > 1.0 10^{21} yr (all limits are at 90% C.L.). The resonant neutrinoless double electron captures to the 2700.2 keV and 2712.7 keV excited states of 96Mo are restricted as: T1/2(0νKL) > 2.0 10^{20} yr and T1/2(0ν2L) > 3.6 10^{20} yr, respectively. Various two neutrino and neutrinoless 2β half lives of 96Ru have been estimated in the framework of the QRPA approach. In addition, the T1/2 limit for 0ν2β- transitions of 104Ru to the first excited state of 104Pd has been set as > 6.5 10^{20} yr.

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CdWO4 crystal scintillators from enriched isotopes for double beta decay experiments

Cadmium tungstate crystal scintillators enriched in 106Cd and 116Cd were developed. The produced scintillators exhibit good optical and scintillation properties, and a low level of radioactive contamination. Experiments to search for double beta decay of 106Cd and 116Cd are in progress at the Gran Sasso National Laboratories of the INFN (Italy). Prospects to further improve the radiopurity of the detectors by recrystallization are discussed.

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First search for double-beta decay of 184Os and 192Os

A search for double-beta decay of osmium has been realized for the first time with the help of an ultra-low background HPGe gamma detector at the underground Gran Sasso National Laboratories of the INFN (Italy). After 2741 h of data taking with a 173 g ultra-pure osmium sample limits on double-beta processes in 184Os have been established at the level of T_{1/2} about 10^{14}-10^{17} yr. Possible resonant double-electron captures in 184Os were searched for with a sensitivity T_{1/2} about 10^{16} yr. A half-life limit T_{1/2} > 5.3 10^{19} yr was set for the double-beta decay of 192Os to the first excited level of 192Pt. The radiopurity of the osmium sample has been investigated and radionuclides 137Cs, 185Os and 207Bi were detected in the sample, while activities of 40K, 60Co, 226Ra and 232Th were limited at the mBq/kg level.

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Search for double beta decay processes in 106Cd with the help of 106CdWO4 crystal scintillator

A search for the double beta processes in 106Cd was carried out at the Gran Sasso National Laboratories of the INFN (Italy) with the help of a 106CdWO4 crystal scintillator (215 g) enriched in 106Cd up to 66%. After 6590 h of data taking, new improved half-life limits on the double beta processes in 106Cd were established at the level of 10^{19}-10^{21} yr; in particular, T_{1/2}(2νεβ^+) > 2.1 10^{20} yr, T_{1/2}(2ν2β^+) > 4.3 10^{20} yr, and T_{1/2}(0ν2ε) > 1.0 10^{21} yr. The resonant neutrinoless double electron captures to the 2718 keV, 2741 keV and 2748 keV excited states of 106Pd are restricted to T_{1/2}(0ν2K) > 4.3 10^{20} yr, T_{1/2}(0νKL1) > 9.5 10^{20} yr and T_{1/2}(0νKL3) > 4.3 10^{20} yr, respectively (all limits at 90% C.L.). A possible resonant enhancement of the 0ν2εprocesses is estimated in the framework of the QRPA approach. The radioactive contamination of the 106CdWO4 crystal scintillator is reported.

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Searches for neutrinoless resonant double electron captures at LNGS

Several experiments were performed during last years at underground (3600 m w.e.) Laboratori Nazionali del Gran Sasso (LNGS) of the INFN (Italy) to search for resonant 2$\varepsilon0ν$ captures in 96Ru, 106Cd, 136Ce, 156Dy, 158Dy, 180W, 184Os, 190Pt with the help of HP Ge semiconductor detectors, and ZnWO4 and 106CdWO4 crystal scintillators. No evidence for r-2$\varepsilon0ν$ decays was found, and only T_{1/2} limits were established in the range of 10^{14}-10^{21} yr.

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Double beta decay of ^{64,70}Zn and ^{180,186}W isotopes

The results of the experimental investigations of double beta processes in Zinc and Tungsten isotopes with the help of middle volume (117 g, 168 g and 699 g) low-background ZnWO_4 crystal scintillators are presented. The experiment was carried out in the low-background "DAMA/R&D" set-up at the Gran Sasso National Laboratories of the INFN (Italy) at a depth of \approx3600 m w.e. The total measurement time exceeds ten thousand hours. New improved half-life limits on double electron capture and electron capture with positron emission in ^{64}Zn have been set: T^{2ν2K}_{1/2}(^{64}Zn) \geq 6.2(6.3) \times 10^{18} yr, T^{0ν2ε}_{1/2} (^{64}Zn) \geq 1.1(2.8) \times 10^{20} yr, T^{2νεβ^+}_{1/2}(^{64}Zn) \geq 0.7(2.1) \times 10^{21} yr, and T^{0νεβ^+}_{1/2}(^{64}Zn) \geq 4.3(5.7) \times 10^{20} yr, all the limits are at 90% (68%) C.L. The positive indication on the εβ^+ decay of ^{64}Zn with T^{(2ν+ 0ν) εβ^+}_{1/2} (^{64}Zn) = (1.1 \pm 0.9) \times 10^{19} yr suggested in [Appl. Radiat. Isot. 46 (1995) 455-456] is fully discarded by the present experiment. The half-life limits on the 2βprocesses in ^{70}Zn, ^{180}W, and two neutrino mode of 2β^- decay in ^{186}W established in the present work on the level of 10^{17}-10^{20} yr are one order of magnitude higher than those set in previous experiments. Energy resolution, relative light output, α/βratio, decay time, pulse-shape discrimination between αparticles and γrays (βparticles), and radioactive contamination of CdWO_4, PbWO_4 (undoped, and doped by F, Eu, Mo, Gd, S), and ZnWO_4 crystal scintillators were studied. Applicability of these scintillators to search for double beta decay was proved.

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Final results of an experiment to search for 2beta processes in zinc and tungsten with the help of radiopure ZnWO4 crystal scintillators

A search for the double beta decay of zinc and tungsten isotopes has been performed with the help of radiopure ZnWO4 crystal scintillators (0.1-0.7 kg) at the Gran Sasso National Laboratories of the INFN. The total exposure of the low background measurements is 0.529 kg yr. New improved half-life limits on the double beta decay modes of 64Zn, 70Zn, 180W, and 186W have been established at the level of 10^{18}-10^{21} yr. In particular, limits on double electron capture and electron capture with positron emission in 64Zn have been set: T_{1/2}(2ν2K) > 1.1 10^{19} yr, T_{1/2} (0ν2ε) > 3.2 10^{20} yr, T_{1/2} (2νεβ^+) > 9.4 10^{20} yr, and T_{1/2} (0νεβ^+) > 8.5 10^{20} yr, all at 90% C.L. Resonant neutrinoless double electron capture in 180W has been restricted on the level of T_{1/2} (0ν2ε) > 1.3 10^{18} yr. A new half-life limit on alpha transition of 183W to the metastable excited level 1/2^- 375 keV of 179Hf has been established: T_{1/2} > 6.7 10^{20} yr.

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Low background detector with enriched 116CdWO4 crystal scintillators to search for double beta decay of 116Cd

A cadmium tungstate crystal boule enriched in $^{116}$Cd to 82% with mass of 1868 g was grown by the low-thermal-gradient Czochralski technique. The isotopic composition of cadmium and the trace contamination of the crystal were estimated by High Resolution Inductively Coupled Plasma Mass-Spectrometry. The crystal scintillators produced from the boule were subjected to characterization that included measurements of transmittance and energy resolution. A low background scintillation detector with two $^{116}$CdWO$_4$ crystal scintillators (586 g and 589 g) was developed. The detector was running over 1727 h deep underground at the Gran Sasso National Laboratories of the INFN (Italy), which allowed to estimate the radioactive contamination of the enriched crystal scintillators. The radiopurity of a third $^{116}$CdWO$_4$ sample (326 g) was tested with the help of ultra-low background high purity germanium $γ$ detector. Monte Carlo simulations of double $β$ processes in $^{116}$Cd were used to estimate the sensitivity of an experiment to search for double $β$ decay of $^{116}$Cd.

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Radioactive contamination of ZnWO4 crystal scintillators

The radioactive contamination of ZnWO4 crystal scintillators has been measured deep underground at the Gran Sasso National Laboratory (LNGS) of the INFN in Italy with a total exposure 3197 kg x h. Monte Carlo simulation, time-amplitude and pulse-shape analyses of the data have been applied to estimate the radioactive contamination of the ZnWO4 samples. One of the ZnWO4 crystals has also been tested by ultra-low background gamma spectrometry. The radioactive contaminations of the ZnWO4 samples do not exceed 0.002 -- 0.8 mBq/kg (depending on the radionuclide), the total alpha activity is in the range: 0.2 - 2 mBq/kg. Particular radioactivity, beta active 65Zn and alpha active 180W, has been detected. The effect of the re-crystallization on the radiopurity of the ZnWO4 crystal has been studied. The radioactive contamination of samples of the ceramic details of the set-ups used in the crystals growth has been checked by low background gamma spectrometry. A project scheme on further improvement of the radiopurity level of the ZnWO4 crystal scintillators is briefly addressed.

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Search for double beta decay of Zinc and Tungsten with the help of low-background ZnWO4 crystal scintillators

Double beta processes in 64-Zn, 70-Zn, 180-W, and 186-W have been searched for with the help of large volume (0.1-0.7 kg) low background ZnWO4 crystal scintillators at the Gran Sasso National Laboratories of the INFN. Total time of measurements exceeds 10 thousands hours. New improved half-life limits on double electron capture and electron capture with positron emission in 64-Zn have been set, in particular (all the limits are at 90% C.L.): T1/2(0nu2EC)> 1.1e20 yr, T1/2(2nuECbeta+)>7.0e20 yr, and T1/2(0nuECbeta+)>4.3e20 yr. The different modes of double beta processes in 70-Zn, 180-W, and 186-W have been restricted at the level of 1e17-1e20 yr.

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Development of CaMoO4 crystal scintillators for double beta decay experiment with 100-Mo

Energy resolution, alpha/beta ratio, pulse-shape discrimination for gamma rays and alpha particles, temperature dependence of scintillation properties, and radioactive contamination were studied with CaMoO4 crystal scintillators. A high sensitivity experiment to search for neutrinoless double beta decay of 100-Mo by using CaMoO4 scintillators is discussed.

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Pulse-shape discrimination with PbWO$_4$ crystal scintillators

The light output, $α/β$ ratio, and pulse shape have been investigated at $-25^\circ$ C with PbWO$_4$ crystal scintillators undoped, and doped by F, Eu, Mo, Gd and S. The fast $0.01-0.06 μ$s and middle $0.1-0.5 μ$s components of scintillation decay were observed for all the samples. Slow components of scintillation signal with the decay times $1-3 μ$s and $13-28 μ$s with the total intensity up to $\approx50%$ have been recognized for several samples doped by Molybdenum. We found some indications of a pulse-shape discrimination between $α$ particles and $γ$ quanta with PbWO$_4$ (Mo doped) crystal scintillators.

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Further study of CdWO4 crystal scintillators as detectors for high sensitivity double beta experiments: scintillation properties and pulse-shape discrimination

Energy resolution, light yield, non-proportionality in the scintillation response, alpha/beta ratio, pulse shape for gamma rays and alpha particles were studied with CdWO4 crystal scintillators. Some indication for a difference in the emission spectra for gamma rays and alpha particles was observed. No dependence of CdWO4 pulse shape on emission spectrum wavelengths under laser, alpha particles and gamma ray excitation was observed. Dependence of scintillation pulse shape for gamma quanta and alpha particles and pulse-shape discrimination ability on temperature was measured in the range of 0-24 degrees.

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Application of PbWO4 crystal scintillators in experiment to search for double beta decay of 116Cd

PbWO4 crystal scintillators are discussed as an active shield and light-guides in 116Cd double beta decay experiment with CdWO4 scintillators. Scintillation properties and radioactive contamination of PbWO4 scintillators were investigated. Energy resolution of CdWO4 detector, coupled to PbWO4 crystal as a light-guide, was tested. Efficiency of PbWO4-based active shield to suppress background from the internal contamination of PbWO4 crystals was calculated. Using of lead tungstate crystal scintillators as high efficiency 4-pi active shield could allow to build sensitive double beta experiment with 116CdWO4 crystal scintillators.

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ZnWO_4 crystals as detectors for double beta decay and dark matter experiments

Energy resolution, alpha/beta ratio, and the pulse shape discrimination ability of the ZnWO_4 crystal scintillators were studied. The radioactive contamination of a ZnWO_4 crystal was investigated in the Solotvina Underground Laboratory. Possibilities to apply ZnWO_4 crystals for the dark matter and double beta decay searches are discussed. New improved half-life limits on double beta decay in zinc isotopes were established, in particular, for ECβ^+ decay of 64-Zn as: T_1/2^2nu > 8.9 10^18 yr and T_1/2^0nu > 3.6 10^18 yr, both at 68% CL.

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