arXiv subjects

D. Vretenar

Publications and source records attributed to D. Vretenar.

At least 37 records · Page 2Linked to original sources

arXiv2022

Model for collective motion

Collective motion is a manifestation of emergent phenomena in medium-heavy and heavy nuclei. A relatively large number of constituent nucleons contribute coherently to nuclear excitations (vibrations, rotations) that are characterized by large electromagnetic moments and transition rates. Basic features of collective excitations are reviewed, and a simple model introduced that describes large-amplitude quadrupole and octupole shape dynamics, as well as the dynamics of induced fission. Modern implementations of the collective Hamiltonian model are based on the microscopic framework of energy density functionals, that provide an accurate global description of nuclear ground states and collective excitations. Results of illustrative calculations are discussed in comparison with available data.

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arXiv2021

Interplay between pairing and triaxial shape degrees of freedom in Os and Pt nuclei

The effect of coupling between pairing and quadrupole triaxial shape vibrations on the low-energy collective states of $γ$-soft nuclei is investigated using a model based on the framework of nuclear energy density functionals (EDFs). Employing a constrained self-consistent mean-field (SCMF) method that uses universal EDFs and pairing interactions, potential energy surfaces of characteristic $γ$-soft Os and Pt nuclei with $A\approx190$ are calculated as functions of the pairing and triaxial quadrupole deformations. Collective spectroscopic properties are computed using a number-nonconserving interacting boson model (IBM) Hamiltonian, with parameters determined by mapping the SCMF energy surface onto the expectation value of the Hamiltonian in the boson condensate state. It is shown that, by simultaneously considering both the shape and pairing collective degrees of freedom, the EDF-based IBM successfully reproduces data on collective structures based on low-energy $0^{+}$ states, as well as $γ$-vibrational bands.

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arXiv2021

Coupling of pairing and triaxial shape vibrations in collective states of $γ$-soft nuclei

In addition to shape oscillations, low-energy excitation spectra of deformed nuclei are also influenced by pairing vibrations. The simultaneous description of these collective modes and their coupling has been a long-standing problem in nuclear structure theory. Here we address the problem in terms of self-consistent mean-field calculations of collective deformation energy surfaces, and the framework of the interacting boson approximation. In addition to quadrupole shape vibrations and rotations, the explicit coupling to pairing vibrations is taken into account by a boson-number non-conserving Hamiltonian, specified by a choice of a universal density functional and pairing interaction. An illustrative calculation for $^{128}$Xe and $^{130}$Xe shows the importance of dynamical pairing degrees of freedom, especially for structures built on low-energy $0^+$ excited states, in $γ$-soft and triaxial nuclei.

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arXiv2021

Microscopic description of octupole collective excitations near $N=56$ and $N=88$

Octupole deformations and related collective excitations are analyzed using the framework of nuclear density functional theory. Axially-symmetric quadrupole-octupole constrained self-consistent mean-field (SCMF) calculations with a choice of universal energy density functional and a pairing interaction are performed for Xe, Ba, and Ce isotopes from proton-rich to neutron-rich regions, and neutron-rich Se, Kr, and Sr isotopes, in which enhanced octupole correlations are expected to occur. Low-energy positive- and negative-parity spectra and transition strengths are computed by solving the quadrupole-octupole collective Hamiltonian, with the inertia parameters and collective potential determined by the constrained SCMF calculations. Octupole-deformed equilibrium states are found in the potential energy surfaces of the Ba and Ce isotopes with $N\approx 56$ and 88. The evolution of spectroscopic properties indicates enhanced octupole correlations in the regions corresponding to $N\approx Z\approx 56$, $Z\approx 88$ and $Z\approx 56$, and $N\approx 56$ and $Z\approx 34$. The average $β_{30}$ deformation parameter and its fluctuation exhibit signatures of octupole shape phase transition around $N=56$ and 88.

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arXiv2020

Pairing vibrations in the interacting boson model based on density functional theory

We propose a method to incorporate the coupling between shape and pairing collective degrees of freedom in the framework of the interacting boson model (IBM), based on the nuclear density functional theory. To account for pairing vibrations, a boson-number non-conserving IBM Hamiltonian is introduced. The Hamiltonian is constructed by using solutions of self-consistent mean-field calculations based on a universal energy density functional and pairing force, with constraints on the axially-symmetric quadrupole and pairing intrinsic deformations. By mapping the resulting quadrupole-pairing potential energy surface onto the expectation value of the bosonic Hamiltonian in the boson condensate state, the strength parameters of the boson Hamiltonian are determined. An illustrative calculation is performed for $^{122}$Xe, and the method is further explored in a more systematic study of rare-earth $N=92$ isotones. The inclusion of the dynamical pairing degree of freedom significantly lowers the energies of bands based on excited $0^+$ states. The results are in quantitative agreement with spectroscopic data, and are consistent with those obtained using the collective Hamiltonian approach.

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arXiv2020

Shape phase transitions in odd-A Zr isotopes

Spectroscopic properties that characterize shape phase transitions in neutron-rich odd-A Zr isotopes are investigated using the framework of nuclear density functional theory and particle-core coupling. The interacting-boson Hamiltonian of the even-even core nuclei, and the single-particle energies and occupation probabilities of the unpaired neutron are completely determined by deformation constrained self-consistent mean-field calculations based on the relativistic Hartree-Bogoliubov model with a choice of a universal energy density functional and pairing interaction. The triaxial $(β,γ)$ deformation energy surfaces for even-even $^{94-102}$Zr indicates transition from triaxial or $γ$-soft ($^{94,96}$Zr) to prolate ($^{98}$Zr), and triaxial ($^{100,102}$Zr) shapes. The corresponding low-energy excitation spectra of the odd-A Zr isotopes are in very good agreement with recent experimental results. Consistent with the structural evolution of the neighboring even-even Zr nuclei, the state-dependent effective deformations and their fluctuations in the odd-A isotopes indicate a pronounced discontinuity around the transitional nucleus $^{99}$Zr.

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arXiv2020

Low-energy cluster vibrations in N = Z nuclei

Significant transition strength in light $α$-conjugate nuclei at low energy, typically below 10 MeV, has been observed in many experiments. In this work the isoscalar low-energy response of N=Z nuclei is explored using the Finite Amplitude Method (FAM) based on the microscopic framework of nuclear energy density functionals. Depending on the multipolarity of the excitation and the equilibrium deformation of a particular isotope, the low-energy strength functions display prominent peaks that can be attributed to vibration of cluster structures: $α$+$^{12}$C+$α$ and $α$+$^{16}$O in $^{20}$Ne, $^{12}$C+$^{12}$C in $^{24}$Mg, 4$α$+$^{12}$C in $^{28}$Si, etc. Such cluster excitations are favored in light nuclei with large deformation.

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arXiv2020

Microscopic description of the self-conjugate $^{108}$Xe and $^{104}$Te $α$-decay chain

A microscopic calculation of half-lives for the recently observed $^{108}$Xe $\to$ $^{104}$Te $\to$ $^{100}$Sn $α$-decay chain is performed using a self-consistent framework based on energy density functionals. The relativistic density functional DD-PC1 and a separable pairing interaction of finite range are used to compute axially-symmetric deformation energy surfaces of $^{104}$Te and $^{108}$Xe as functions of quadrupole, octupole and hexadecupole collective coordinates. Dynamic least-action paths are determined that trace the $α$-particle emission from the equilibrium deformation to the point of scission. The calculated half-lives: 197 ns for $^{104}$Te and 50 $μ$s for $^{108}$Xe, are compared to recent experimental values of the half-lives of superallowed $α$-decay of $^{104}$Te: $< 18$ ns, and $^{108}$Xe: 58$^{+106}_{-23}$ $μ$s.

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arXiv2020

Coupling of shape and pairing vibrations in a collective Hamiltonian based on nuclear energy density functionals

The quadrupole collective Hamiltonian, based on relativistic energy density functionals, is extended to include a pairing collective coordinate. In addition to quadrupole shape vibrations and rotations, the model describes pairing vibrations and the coupling between shape and pairing degrees of freedom. The parameters of the collective Hamiltonian are determined by constrained self-consistent relativistic mean-field plus Bardeen-Cooper-Schrieffer (RMF+BCS) calculations in the space of intrinsic shape and pairing deformations. The effect of coupling between shape and pairing degrees of freedom is analyzed in a study of low-energy spectra and transition rates of four axially symmetric $N=92$ rare-earth isotones. When compared to results obtained with the standard quadrupole collective Hamiltonian, the inclusion of dynamical pairing increases the moment of inertia, lowers the energies of excited $0^+$ states and reduces the E0-transition strengths, in better agreement with data.

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arXiv2019

Microscopic core-quasiparticle coupling model for spectroscopy of odd-mass nuclei with octupole correlations

[Background] Predictions of spectroscopic properties of low-lying states are critical for nuclear structure studies. Theoretical methods can be particularly involved for odd-mass nuclei because of the interplay between the unpaired nucleon and collective degrees of freedom. Only a few models have been developed for systems in which octupole collective degrees of freedom play a role. [Purpose] We aim to predict spectroscopic properties of odd-mass nuclei characterized by octupole shape deformation, employing a model that describes single-particle and collective degrees of freedom within the same microscopic framework. [Method] A microscopic core-quasiparticle coupling (CQC) model based on the covariant density functional theory is developed, which includes collective excitations of even-mass core nuclei and single-particle states of the odd nucleon, calculated using a quadrupole-octupole collective Hamiltonian combined with a constrained reflection-asymmetric relativistic Hartree-Bogoliubov model. [Results] Model predictions for low-energy excitation spectra and transition rates of odd-mass radium isotopes $^{223, 225, 227}$Ra are shown to be in good agreement with available data. [Conclusions] A microscopic CQC model based on covariant density functional theory has been developed for odd-mass nuclei characterized by both quadrupole and octupole shape deformations. Theoretical results reproduce data in odd-mass Ra isotopes and provide useful predictions for future studies of octupole correlations in nuclei and related phenomena.

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arXiv2018

Shape evolution and coexistence in neutron-deficient Nd and Sm nuclei

The evolution of shapes and low-energy shape coexistence is analyzed in neutron-deficient Nd and Sm nuclei, using a five-dimensional quadrupole collective Hamiltonian (5DCH). Deformation energy surfaces, calculated with the relativistic energy density functional PC-PK1 and a separable finite-range pairing interaction, exhibit a transition from spherical shapes near $N=80$, to $γ-$soft shapes, and to prolate deformed minima in lighter isotopes. The corresponding 5DCH model calculation, based on the self-consistent mean-field potentials, reproduces the empirical isotopic trend of characteristic collective observables, and predicts significantly different deformations for the first two $0^+$ states in the $N=74$ isotones $^{134}$Nd and $^{136}$Sm. In addition to bands based on the triaxial $γ-$soft ground state, in excellent agreement with data, the occurrence of a low-energy rotational band is predicted, built on the prolate deformed ($β\sim0.4$) excited state $0^+_2$.

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arXiv2018

Single-particle spatial dispersion and clusters in nuclei

The spatial dispersion of the single-nucleon wave functions is analyzed using the self-consistent mean-field framework based on nuclear energy density functionals, and with the harmonic oscillator approximation for the nuclear potential. It is shown that the dispersion depends on the radial quantum number n, but displays only a very weak dependence on the orbital angular momentum. An analytic expression is derived for the localization parameter that explicitly takes into account the radial quantum number of occupied single-nucleon states. The conditions for single-nucleon localization and formation of cluster structures are fulfilled in relatively light nuclei with $A \leq 30$ and $n=1$ states occupied. Heavier nuclei exhibit the quantum liquid phase of nucleonic matter because occupied levels that originate from $n > 1$ spherical states are largely delocalized. Nevertheless, individual $α$-like clusters can be formed from valence nucleons filling single-particle levels originating from $n=1$ spherical mean-field states.

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arXiv2018

Nuclear quantum shape-phase transitions in odd-mass systems

Microscopic signatures of nuclear ground-state shape phase transitions in odd-mass Eu isotopes are explored starting from excitation spectra and collective wave functions obtained by diagonalization of a core-quasiparticle coupling Hamiltonian based on energy density functionals. As functions of the physical control parameter -- the number of nucleons -- theoretical low-energy spectra, two-neutron separation energies, charge isotope shifts, spectroscopic quadrupole moments, and $E2$ reduced transition matrix elements accurately reproduce available data, and exhibit more pronounced discontinuities at neutron number $N=90$, compared to the adjacent even-even Sm and Gd isotopes. The enhancement of the first-order quantum phase transition in odd-mass systems can be attributed to a shape polarization effect of the unpaired proton which, at the critical neutron number, starts predominantly coupling to Gd core nuclei that are characterized by larger quadrupole deformation and weaker proton pairing correlations compared to the corresponding Sm isotopes.

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arXiv2018

Signatures of octupole correlations in neutron-rich odd-mass barium isotopes

Octupole deformation and the relevant spectroscopic properties of neutron-rich odd-mass barium isotopes are investigated in a theoretical framework based on nuclear density functional theory and the particle-core coupling scheme. The interacting-boson Hamiltonian that describes the octupole-deformed even-even core nucleus, as well as the single-particle energies and occupation probabilities of an unpaired nucleon, are completely determined by microscopic axially-symmetric $(β_{2},β_{3})$-deformation constrained self-consistent mean-field calculations for a specific choice of the energy density functional and pairing interaction. A boson-fermion interaction that involves both quadrupole and octupole degrees of freedom is introduced, and their strength parameters are determined to reproduce selected spectroscopic data for the odd-mass nuclei. The model reproduces recent experimental results both for the even-even and odd-mass Ba isotopes. In particular, for $^{145,147}$Ba our results indicate, in agreement with recent data, that octupole deformation does not determine the structure of the lowest states in the vicinity of the ground state, and only becomes relevant at higher excitation energies.

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arXiv2018

Quadrupole and octupole collectivity and cluster structures in neon isotopes

The lowest positive- and negative-parity bands of $^{20}$Ne and neutron-rich even-even Ne isotopes are investigated using a theoretical framework based on energy density functionals. Starting from a self-consistent relativistic Hartree-Bogoliubov calculation of axially-symmetric and reflection-asymmetric deformation energy surfaces, the collective symmetry-conserving states are built using projection techniques and the generator coordinate method. Overall a good agreement with the experimental excitation energies and transition rates is obtained. In particular, the model provides an accurate description of the excitation spectra and transition probabilities in $^{20}$Ne. The contribution of cluster configurations to the low-energy states is discussed, as well as the transitional character of the ground state. The analysis is extended to $^{22}$Ne and the shape-coexisting isotope $^{24}$Ne, and to the drip-line nuclei $^{32}$Ne and $^{34}$Ne. The role of valence neutrons in the formation of molecular-type bonds between clusters is discussed.

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arXiv2017

Spectroscopy of reflection-asymmetric nuclei with relativistic energy density functionals

Quadrupole and octupole deformation energy surfaces, low-energy excitation spectra and transition rates in fourteen isotopic chains: Xe, Ba, Ce, Nd, Sm, Gd, Rn, Ra, Th, U, Pu, Cm, Cf, and Fm, are systematically analyzed using a theoretical framework based on a quadrupole-octupole collective Hamiltonian (QOCH), with parameters determined by constrained reflection-asymmetric and axially-symmetric relativistic mean-field calculations. The microscopic QOCH model based on the PC-PK1 energy density functional and $δ$-interaction pairing is shown to accurately describe the empirical trend of low-energy quadrupole and octupole collective states, and predicted spectroscopic properties are consistent with recent microscopic calculations based on both relativistic and non-relativistic energy density functionals. Low-energy negative-parity bands, average octupole deformations, and transition rates show evidence for octupole collectivity in both mass regions, for which a microscopic mechanism is discussed in terms of evolution of single-nucleon orbitals with deformation.

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arXiv2017

Microscopic study of induced fission dynamics of $^{226}$Th with covariant energy density functionals

Static and dynamic aspects of the fission process of $^{226}$Th are analyzed in a self-consistent framework based on relativistic energy density functionals. Constrained relativistic mean-field (RMF) calculations in the collective space of axially symmetric quadrupole and octupole deformations, based on the energy density functional PC-PK1 and a $δ$-force pairing, are performed to determine the potential energy surface of the fissioning nucleus, the scission line, the single-nucleon wave functions, energies and occupation probabilities, as functions of deformation parameters. Induced fission dynamics is described using the time-dependent generator coordinate method in the Gaussian overlap approximation. A collective Schrödinger equation, determined entirely by the microscopic single-nucleon degrees of freedom, propagates adiabatically in time the initial wave packet built by boosting the ground-state solution of the collective Hamiltonian for $^{226}$Th. The position of the scission line and the microscopic input for the collective Hamiltonian are analyzed as functions of the strength of the pairing interaction. The effect of static pairing correlations on the pre-neutron emission charge yields and total kinetic energy of fission fragments is examined in comparison with available data, and the distribution of fission fragments is analyzed for different values of the initial excitation energy.

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arXiv2017

Shape-phase transitions in odd-mass $γ$-soft nuclei with mass $A\approx 130$

Quantum phase transitions between competing equilibrium shapes of nuclei with an odd number of nucleons are explored using a microscopic framework of nuclear energy density functionals and a particle-boson core coupling model. The boson Hamiltonian for the even-even core nucleus, as well as the spherical single-particle energies and occupation probabilities of unpaired nucleons, are completely determined by a constrained self-consistent mean-field calculation for a specific choice of the energy density functional and pairing interaction. Only the strength parameters of the particle-core coupling have to be adjusted to reproduce a few empirical low-energy spectroscopic properties of the corresponding odd-mass system. The model is applied to the odd-A Ba, Xe, La and Cs isotopes with mass $A\approx 130$, for which the corresponding even-even Ba and Xe nuclei present a typical case of $γ$-soft nuclear potential. The theoretical results reproduce the experimental low-energy excitation spectra and electromagnetic properties, and confirm that a phase transition between nearly spherical and $γ$-soft nuclear shapes occurs also in the odd-A systems.

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