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D. Vretenar

Publications and source records attributed to D. Vretenar.

At least 55 records · Page 3Linked to original sources

Global analysis of quadrupole shape invariants based on covariant energy density functionals

Coexistence of different geometric shapes at low energies presents a universal structure phenomenon that occurs over the entire chart of nuclides. Studies of the shape coexistence are important for understanding the microscopic origin of collectivity and modifications of shell structure in exotic nuclei far from stability. The aim of this work is to provide a systematic analysis of characteristic signatures of coexisting nuclear shapes in different mass regions, using a global self-consistent theoretical method based on universal energy density functionals and the quadrupole collective model. The low-energy excitation spectrum and quadrupole shape invariants of the two lowest $0^{+}$ states of even-even nuclei are obtained as solutions of a five-dimensional collective Hamiltonian (5DCH) model, with parameters determined by constrained self-consistent mean-field calculations based on the relativistic energy density functional PC-PK1, and a finite-range pairing interaction. The theoretical excitation energies of the states: $2^+_1$, $4^+_1$, $0^+_2$, $2^+_2$, $2^+_3$, as well as the $B(E2; 0^+_1\to 2^+_1)$ values, are in very good agreement with the corresponding experimental values for 621 even-even nuclei. Quadrupole shape invariants have been implemented to investigate shape coexistence, and the distribution of possible shape-coexisting nuclei is consistent with results obtained in recent theoretical studies and available data. The present analysis has shown that, when based on a universal and consistent microscopic framework of nuclear density functionals, shape invariants provide distinct indicators and reliable predictions for the occurrence of low-energy coexisting shapes. This method is particularly useful for studies of shape coexistence in regions far from stability where few data are available.

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Signatures of shape phase transitions in odd-mass nuclei

Quantum phase transitions between competing ground-state shapes of atomic nuclei with an odd number of protons or neutrons are investigated in a microscopic framework based on nuclear energy density functional theory and the particle-plus-boson-core coupling scheme. The boson-core Hamiltonian, as well as the single-particle energies and occupation probabilities of the unpaired nucleon, are completely determined by constrained self-consistent mean-field calculations for a specific choice of the energy density functional and paring interaction, and only the strength parameters of the particle-core coupling are adjusted to reproduce selected spectroscopic properties of the odd-mass system. We apply this method to odd-A Eu and Sm isotopes with neutron number $N \approx 90$, and explore the influence of the single unpaired fermion on the occurrence of a shape phase transition. Collective wave functions of low-energy states are used to compute quantities that can be related to quantum order parameters: deformations, excitation energies, E2 transition rates and separation energies, and their evolution with the control parameter (neutron number) is analysed.

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Spin-orbit interaction in relativistic nuclear structure models

Relativistic self-consistent mean-field (SCMF) models naturally account for the coupling of the nucleon spin to its orbital motion, whereas non-relativistic SCMF methods necessitate a phenomenological ansatz for the effective spin-orbit potential. Recent experimental studies aim to explore the isospin properties of the effective spin-orbit interaction in nuclei. SCMF models are very useful in the interpretation of the corresponding data, however standard relativistic mean-field and non-relativistic Hartree-Fock models use effective spin-orbit potentials with different isovector properties, mainly because exchange contributions are not treated explicitly in the former. The impact of exchange terms on the effective spin-orbit potential in relativistic mean-field models is analysed, and it is shown that it leads to an isovector structure similar to the one used in standard non-relativistic Hartree-Fock. Data on the isospin dependence of spin-orbit splittings in spherical nuclei could be used to constrain the isovector-scalar channel of relativistic mean-field models. The reproduction of the empirical kink in the isotope shifts of even Pb nuclei by relativistic effective interactions points to the occurrence of pseudospin symmetry in the single-neutron spectra in these nuclei.

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Beyond mean-field boson-fermion model for odd-mass nuclei

A novel method for calculating spectroscopic properties of medium-mass and heavy atomic nuclei with an odd number of nucleons is introduced, based on the framework of nuclear energy density functional theory and the particle-core coupling scheme. The deformation energy surface of the even-even core, as well as the spherical single-particle energies and occupation probabilities of the odd particle(s), are obtained in a self-consistent mean-field calculation determined by the choice of the energy density functional and pairing interaction. This method uniquely determines the parameters of the Hamiltonian of the boson core, and only the strength of the particle-core coupling is specifically adjusted to selected data for a particular nucleus. The approach is illustrated in a systematic study of low-energy excitation spectra and transition rates of axially deformed odd-mass Eu isotopes.

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The neutron skin thickness from the measured electric dipole polarizability in $^{68}$Ni, $^{120}$Sn, and $^{208}$Pb

The information on the symmetry energy and its density dependence is deduced by comparing the available data on the electric dipole polarizability $α_D$ of ${}^{68}$Ni, ${}^{120}$Sn, and ${}^{208}$Pb with the predictions of the Random Phase Approximation, using a representative set of nuclear energy density functionals. The calculated values of $α_D$ are used to validate different correlations involving $α_D$, the symmetry energy at the saturation density $J$, the corresponding slope parameter $L$ and the neutron skin thickness $Δr_{\!np}$, as suggested by the Droplet Model. A subset of models that reproduce simultaneously the measured polarizabilities in ${}^{68}$Ni, ${}^{120}$Sn, and ${}^{208}$Pb are employed to predict the values of the symmetry energy parameters at saturation density and $Δr_{\!np}$. The resulting intervals are: $J\!=\!30 \text{-}35$ MeV, $L\!=\!20 \text{-} 66$ MeV; and the values for $Δr_{\!np}$ in ${}^{68}$Ni, ${}^{120}$Sn, and ${}^{208}$Pb are in the ranges: 0.15\text{-}0.19 fm, 0.12\text{-}0.16 fm, and 0.13\text{-}0.19 fm, respectively. The strong correlation between the electric dipole polarizabilities of two nuclei is instrumental to predict the values of electric dipole polarizabilities in other nuclei.

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Spin-orbit coupling rule in bound fermions systems

Spin-orbit coupling characterizes quantum systems such as atoms, nuclei, hypernuclei, quarkonia, etc., and is essential for understanding their spectroscopic properties. Depending on the system, the effect of spin-orbit coupling on shell structure is large in nuclei, small in quarkonia, perturbative in atoms. In the standard non-relativistic reduction of the single-particle Dirac equation, we derive a universal rule for the relative magnitude of the spin-orbit effect that applies to very different quantum systems, regardless of whether the spin-orbit coupling originates from the strong or electromagnetic interaction. It is shown that in nuclei the near equality of the mass of the nucleon and the difference between the large repulsive and attractive potentials explains the fact that spin-orbit splittings are comparable to the energy spacing between major shells. For a specific ratio between the particle mass and the effective potential whose gradient determines the spin-orbit force, we predict the occurrence of giant spin-orbit energy splittings that dominate the single-particle excitation spectrum.

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Modeling nuclear weak-interaction processes with relativistic energy density functionals

Relativistic energy density functionals have become a standard framework for nuclear structure studies of ground-state properties and collective excitations over the entire nuclide chart. We review recent developments in modeling nuclear weak-interaction processes: charge-exchange excitations and the role of isoscalar proton-neutron pairing, charged-current neutrino-nucleus reactions relevant for supernova evolution and neutrino detectors, and calculation of beta-decay rates for r-process nucleosynthesis.

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Density Functional Theory studies of cluster states in nuclei

The framework of nuclear energy density functionals is applied to a study of the formation and evolution of cluster states in nuclei. The relativistic functional DD-ME2 is used in triaxial and reflection-asymmetric relativistic Hartree-Bogoliubov calculations of relatively light $N = Z$ and neutron-rich nuclei. The role of deformation and degeneracy of single-nucleon states in the formation of clusters is analysed, and interesting cluster structures are predicted in excited configurations of Be, C, O, Ne, Mg, Si, S, Ar and Ca $N = Z$ nuclei. Cluster phenomena in neutron-rich nuclei are discussed, and it is shown that in neutron-rich Be and C nuclei cluster states occur as a result of molecular bonding of $α$-particles by the excess neutrons, and also that proton covalent bonding can occur in $^{10}$C.

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Neutron star structure and collective excitations of finite nuclei

We study relationships between properties of collective excitations in finite nuclei and the phase transition density $n_t$ and pressure $P_t$ at the inner edge separating the liquid core and the solid crust of a neutron star. A theoretical framework that includes the thermodynamic method, relativistic nuclear energy density functionals and the quasiparticle random-phase approximation is employed in a self-consistent calculation of $(n_t,P_t)$ and collective excitations in nuclei. The covariance analysis shows that properties of charge-exchange dipole transitions, isovector giant dipole and quadrupole resonances and pygmy dipole transitions are correlated with the core-crust transition density and pressure. A set of relativistic nuclear energy density functionals, characterized by systematic variation of the density dependence of the symmetry energy of nuclear matter, is used to constrain possible values for $(n_t,P_t)$. By comparing the calculated excitation energies of giant resonances, energy weighted pygmy dipole strength, and dipole polarizability with available data, we obtain the weighted average values: $n_t = 0.0955 \pm 0.0007$ fm$^{-3}$ and $P_t = 0.59 \pm 0.05$ MeV fm$^{-3}$.

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DIRHB -- a relativistic self-consistent mean-field framework for atomic nuclei

The DIRHB package consists of three Fortran computer codes for the calculation of the ground-state properties of even-even atomic nuclei using the framework of relativistic self-consistent mean-field models. Each code corresponds to a particular choice of spatial symmetry: the DIRHBS, DIRHBZ and DIRHBT codes are used to calculate nuclei with spherical symmetry, axially symmetric quadrupole deformation, and triaxial quadrupole shapes, respectively. Reflection symmetry is assumed in all three cases. The latest relativistic nuclear energy density functionals are implemented in the codes, thus enabling efficient and accurate calculations over the entire nuclide chart.

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Microscopic description of octupole shape-phase transitions in light actinides and rare-earth nuclei

A systematic analysis of low-lying quadrupole and octupole collective states is presented, based on the microscopic energy density functional framework. By mapping the deformation constrained self-consistent axially symmetric mean-field energy surfaces onto the equivalent Hamiltonian of the $sdf$ interacting boson model (IBM), that is, onto the energy expectation value in the boson condensate state, the Hamiltonian parameters are determined. The study is based on the global relativistic energy density functional DD-PC1. The resulting IBM Hamiltonian is used to calculate excitation spectra and transition rates for the positive- and negative-parity collective states in four isotopic chains characteristic for two regions of octupole deformation and collectivity: Th, Ra, Sm and Ba. Consistent with the empirical trend, the microscopic calculation based on the systematics of $β_{2}$-$β_{3}$ energy maps, the resulting low-lying negative-parity bands and transition rates show evidence of a shape transition between stable octupole deformation and octupole vibrations characteristic for $β_{3}$-soft potentials.

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Pairing transitions in the finite-temperature relativistic Hartree-Bogoliubov theory

We formulate the finite-temperature relativistic Hartree-Bogoliubov theory for spherical nuclei based on a point-coupling functional, with the Gogny or separable pairing force. Using the functional PC-PK1, the framework is applied to the study of pairing transitions in Ca, Ni, Sn, and Pb isotopic chains. The separable pairing force reproduces the gaps calculated with the Gogny force not only at zero temperature, but also at finite temperatures. By performing a systematic calculation of the even-even Ca, Ni, Sn, and Pb isotopes, it is found that the critical temperature for a pairing transition generally follows the rule $T_c =0.6 Δ_n(0)$, where $Δ_n(0)$ is the neutron pairing gap at zero temperature. This rule is further verified by adjusting the pairing gap at zero temperature with a strength parameter.

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Neutron-skin thickness of $^{208}$Pb, and symmetry-energy constraints from the study of the anti-analog giant dipole resonance

The $^{208}$Pb($p$,$nγ\bar p$) $^{207}$Pb reaction at a beam energy of 30 MeV has been used to excite the anti-analog of the giant dipole resonance (AGDR) and to measure its $γ$-decay to the isobaric analog state in coincidence with proton decay of IAS. The energy of the transition has also been calculated with the self-consistent relativistic random-phase approximation (RRPA), and found to be linearly correlated to the predicted value of the neutron-skin thickness ($ΔR_{pn}$). By comparing the theoretical results with the measured transition energy, the value of 0.190 $\pm$ 0.028 fm has been determined for $ΔR_{pn}$ of $^{208}$Pb, in agreement with previous experimental results. The AGDR excitation energy has also been used to calculate the symmetry energy at saturation ($J=32.7 \pm 0.6$ MeV) and the slope of the symmetry energy ($L=49.7 \pm 4.4$ MeV), resulting in more stringent constraints than most of the previous studies.

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Measurement of the 92,93,94,100Mo(g,n) reactions by Coulomb Dissociation

The Coulomb Dissociation (CD) cross sections of the stable isotopes 92,94,100Mo and of the unstable isotope 93Mo were measured at the LAND/R3B setup at GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. Experimental data on these isotopes may help to explain the problem of the underproduction of 92,94Mo and 96,98Ru in the models of p-process nucleosynthesis. The CD cross sections obtained for the stable Mo isotopes are in good agreement with experiments performed with real photons, thus validating the method of Coulomb Dissociation. The result for the reaction 93Mo(g,n) is especially important since the corresponding cross section has not been measured before. A preliminary integral Coulomb Dissociation cross section of the 94Mo(g,n) reaction is presented. Further analysis will complete the experimental database for the (g,n) production chain of the p-isotopes of molybdenum.

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Simultaneous quadrupole and octupole shape phase transitions in Thorium

The evolution of quadrupole and octupole shapes in Th isotopes is studied in the framework of nuclear Density Functional Theory. Constrained energy maps and observables calculated with microscopic collective Hamiltonians indicate the occurrence of a simultaneous quantum shape phase transition between spherical and quadrupole-deformed prolate shapes, and between non-octupole and octupole-deformed shapes, as functions of the neutron number. The nucleus $^{224}$Th is closest to the critical point of a double phase transition. A microscopic mechanism of this phenomenon is discussed in terms of the evolution of single-nucleon orbitals with deformation.

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Electric Dipole Polarizability in ${}^{208}$Pb: insights from the Droplet Model

We study the electric dipole polarizability $α_D$ in ${}^{208}$Pb based on the predictions of a large and representative set of relativistic and non-relativistic nuclear mean field models. We adopt the droplet model as a guide to better understand the correlations between $α_D$ and other isovector observables. Insights from the droplet model suggest that the product of $α_D$ and the nuclear symmetry energy at saturation density $J$ is much better correlated with the neutron skin thickness $Δr_{np}$ of ${}^{208}$Pb than the polarizability alone. Correlations of $α_D J$ with $Δr_{np}$ and with the symmetry energy slope parameter $L$ suggest that $α_D J$ is a strong isovector indicator. Hence, we explore the possibility of constraining the isovector sector of thenuclear energy density functional by comparing our theoretical predictions against measurements of both $α_D$ and the parity-violating asymmetry in ${}^{208}$Pb. We find that the recent experimental determination of $α_D$ in ${}^{208}$Pb in combination with the range for the symmetry energy at saturation density $J=[31\pm (2)_{\rm est.}]$\,MeV suggests $Δr_{np}({}^{208}{\rm Pb}) = 0.165 \pm (0.009)_{\rm exp.} \pm (0.013)_{\rm theo.} \pm (0.021)_{\rm est.} {\rm fm}$ and $L= 43 \pm(6)_{\rm exp.} \pm (8)_{\rm theo.}\pm(12)_{\rm est.}$ MeV.

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Neutron-skin thickness of 208Pb from the energy of the anti-analog giant dipole resonance

The energy of the charge-exchange Anti-analog Giant Dipole Resonance (AGDR) has been calculated for the 208Pb isotope using the state-of-the-art fully self-consistent relativistic proton-neutron quasiparticle random-phase approximation based on the Relativistic Hartree-Bogoliubov model. It is shown that the AGDR centroid energy is very sensitively related to the corresponding neutron-skin thickness. The neutron-skin thickness of 208Pb has been determined very precisely by comparing the theoretical results with the available experimental data on E(AGDR). The result DR(pn)= 0.161(42) agrees nicely with the previous experimental results.

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Microscopic analysis of the octupole phase transition in Th isotopes

A shape phase transition between stable octupole deformation and octupole vibrations in Th nuclei is analyzed in a microscopic framework based on nuclear density functional theory. The relativistic functional DD-PC1 is used to calculate axially-symmetric quadrupole-octupole constrained energy surfaces. Observables related to order parameters are computed using an interacting-boson Hamiltonian, with parameters determined by mapping the microscopic energy surfaces to the expectation value of the Hamiltonian in the boson condensate. The systematics of constrained energy surfaces and low-energy excitation spectra point to the occurrence of a phase transition between octupole-deformed shapes and shapes characterized by octupole-soft potentials.

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