arXiv subjects

D. van der Marel

Publications and source records attributed to D. van der Marel.

At least 73 records · Page 4Linked to original sources

arXiv2009

Optics clues to pairing glues in high T$_{c}$ cuprates

We analyze optical spectra of high temperature superconductors using a minimal model of electrons coupled to bosons. We consider the marginal Fermi liquid theory and the spin fluctuation theory, as well as a histogram representation of the bosonic spectral density. We find that the two theories can both be used to describe the experimental data provided that we allow for an additional scattering channel with an energy of 55 meV.

cond-mat.supr-con↗

arXiv2009

Doping dependent optical properties of Bi2201

An experimental study of the in-plane optical conductivity of (Pb$_{x}$,Bi$_{2-x}$)(La$_{y}$Sr$_{2-y}$)CuO$_{6+δ}$ (Bi2201) is presented for a broad doping and temperature range. The in-plane conductivity is analyzed within a strong coupling formalism. We address the interrelationship between the optical conductivity ($σ(ω)$), the single particle self energy, and the electron-boson spectral function. We find that the frequency and temperature dependence can be well described within this formalism. We present a universal description of optical, ARPES and tunneling spectra. The full frequency and temperature dependence of the optical spectra and single particle self-energy is shown to result from an electron-boson spectral function, which shows a strong doping dependence and weak temperature dependence.

cond-mat.supr-con↗

arXiv2009

Optical determination of the relation between the electron-boson coupling function and the critical temperature in high T$_c$ cuprates

We take advantage of the connection between the free carrier optical conductivity and the glue function in the normal state, to reconstruct from the infrared optical conductivity the glue-spectrum of ten different high-Tc cuprates revealing a robust peak in the 50-60 meV range and a broad con- tinuum at higher energies for all measured charge carrier concentrations and temperatures up to 290 K. We observe that the strong coupling formalism accounts fully for the known strong temperature dependence of the optical spectra of the high Tc cuprates, except for strongly underdoped samples. We observe a correlation between the doping trend of the experimental glue spectra and the critical temperature. The data obtained on the overdoped side of the phase diagram conclusively excludes the electron-phonon coupling as the main source of superconducting pairing.

cond-mat.supr-con↗

arXiv2008

Infrared spectroscopy of electronic bands in bilayer graphene

We present infrared spectra (0.1-1 eV) of electrostatically gated bilayer graphene as a function of doping and compare it with tight binding calculations. All major spectral features corresponding to the expected interband transitions are identified in the spectra: a strong peak due to transitions between parallel split-off bands and two onset-like features due to transitions between valence and conduction bands. A strong gate voltage dependence of these structures and a significant electron-hole asymmetry is observed that we use to extract several band parameters. Surprisingly, the structures related to the gate-induced bandgap are much less pronounced in the experiment than predicted by the tight binding model.

cond-mat.str-el↗

arXiv2008

Observation of a robust peak in the glue function of the high-Tc cuprates in the 50-60 meV range

cond-mat.supr-con↗

arXiv2008

Optical probes of electron correlations in solids

Classically the interaction between light and matter is given by the Maxwell relations. These are briefly reviewed and will be used as a basis to discuss several techniques that are used in optical spectroscopy. We then discuss the quantum mechanical description of the optical conductivity based on the Kubo formalism. This is used as a basis to understand how strong correlation effects can be observed using optical techniques. We will discuss the use of sum rules in the interpretation of optical experiments. Finally, we describe the effect of including interactions between electronic and collective degrees of freedom on optical spectra.

cond-mat.str-el↗

arXiv2008

On the importance of the electron-phonon coupling function on the superconducting transition temperature in dodecaboride superconductors: A comparison of LuB12 with ZrB12

We report a detailed study of specific heat, electrical resistivity and optical spectroscopy in the superconducting boride LuB12 (Tc = 0.4 K) and compare it to the higher Tc compound ZrB12 (Tc = 6 K). Both compounds have the same structure based on enclosed metallic Lu or Zr ions in oversized boron cages. The infrared reflectivity and ellipsometry in the visible range allow us to extract the optical conductivity from 6 meV to 4 eV in the normal state from 20 to 280 K. By extracting the superconducting properties, phonon density of states and electron-phonon coupling function from these measurements we discuss the important factors governing Tc and explain the difference between the two compounds. The phonon density of states seems to be insignificantly modified by substitution of Zr with Lu. However, the soft vibrations of the metal ions in boron cages, responsible for the relatively high Tc in ZrB12, have almost no contribution to the electron-phonon coupling in LuB12.

cond-mat.supr-con↗

arXiv2008

Far-infrared probe of superconductivity in SmO$_{1-x}$F$_{x}$FeAs}

We report far-infrared reflectance measurements on polycrystalline superconducting samples of SmO$_{1-x}$F$_{x}$FeAs ($x$ = 0.12, 0.15 and 0.2). We clearly observe superconductivity induced changes of reflectivity in a broad range of energies, which resembles earlier optical measurements on high $T_{c}$ cuprates. The superconducting-to-normal reflectivity ratio $R_{s}/R_{n}$ grows for the photon energies below 18 meV and shows a complicated structure due to the presence of a strong infrared-active phonon at about 10 meV.

cond-mat.supr-con↗

arXiv2008

Optical spectra of the heavy fermion uniaxial ferromagnet UGe$_2$

We report a detailed study of UGe$_{2}$ single crystals using infrared reflectivity and spectroscopic ellipsometry. The optical conductivity suggests the presence of a low frequency interband transition and a narrow free-carrier response with strong frequency dependence of the scattering rate and effective mass. We observe sharp changes in the low frequency mass and scattering rate below the upper ferromagnetic transition $T_C = 53 K$. The characteristic changes are exhibited most strongly at an energy scale of around 12 meV (100 cm$^{-1}$). They recover their unrenormalized value above $T_C$ and for $ω>$ 40 meV. In contrast no sign of an anomaly is seen at the lower transition temperature of unknown nature $T_x \sim$ 30 K, observed in transport and thermodynamic experiments. In the ferromagnetic state we find signatures of a strong coupling to the longitudinal magnetic excitations that have been proposed to mediate unconventional superconductivity in this compound.

cond-mat.str-el↗

arXiv2007

Optical Integral in the Cuprates and the Question of Sum Rule Violation

Much attention has been given to a possible violation of the optical sum rule in the cuprates, and the connection this might have to kinetic energy lowering. The optical integral is composed of a cut-off independent term (whose temperature dependence is a measure of the sum rule violation), plus a cut-off dependent term that accounts for the extension of the Drude peak beyond the upper bound of the integral. We find that the temperature dependence of the optical integral in the normal state of the cuprates can be accounted for solely by the latter term, implying that the dominant contribution to the observed sum rule `violation' in the normal state is due to the finite cut-off. This cut-off dependent term is well modeled by a theory of electrons interacting with a broad spectrum of bosons.

cond-mat.supr-con↗

arXiv2007

Electron-phonon interaction and charge carrier mass enhancement in SrTiO3

We report a comprehensive THz, infrared and optical study of Nb doped SrTiO3 as well as DC conductivity and Hall effect measurements. Our THz spectra at 7K show the presence of a very narrow (<2 meV) Drude peak, the spectral weight of which shows approximately a factor of three enhancement of the band mass for all carrier concentrations. The missing spectral weight is regained in a broad 'mid-infrared' band which originates from electron-phonon coupling. We find no evidence of a particularly large electron-phonon coupling that would result in small polaron formation. Analysis of the results yields an electron-phonon coupling parameter of an intermediate strength, $α\approx 4$.

cond-mat.str-el↗

arXiv2007

Universal dynamical conductance in graphite

We find experimentally that the optical sheet conductance of graphite per graphene layer is very close to $(π/2)e^2/h$, which is the theoretically expected value of dynamical conductance of isolated monolayer graphene. Our calculations within the Slonczewski-McClure-Weiss model explain well why the interplane hopping leaves the conductance of graphene sheets in graphite almost unchanged for photon energies between 0.1 and 0.6 eV, even though it significantly affects the band structure on the same energy scale. The f-sum rule analysis shows that the large increase of the Drude spectral weight as a function of temperature is at the expense of the removed low-energy optical spectral weight of transitions between hole and electron bands.

cond-mat.str-el↗

arXiv2007

The Missing Link: Magnetism and Superconductivity

The effect of magnetic moments on superconductivity has long been a controversial subject in condensed matter physics. While Matthias and collaborators experimentally demonstrated the destruction of superconductivity in La by the addition of magnetic moments (Gd), it has since been suggested that magnetic fluctuations are in fact responsible for the development of superconducting order in other systems. Currently this debate is focused on several families of unconventional superconductors including high-Tc cuprates, borocarbides as well as heavy fermion systems where magnetism and superconductivity are known to coexist. Here we report a novel aspect of competition and coexistence of these two competing orders in an interesting class of heavy fermion compounds, namely the 1-1-5 series: CeTIn5 where T=Co, Ir, or Rh. Our optical experiments indicate the existence of regions in momentum space where local moments remain unscreened. The extent of these regions in momentum space appears to control both the normal and superconducting state properties in the 1-1-5 family of heavy fermion (HF) superconductors.

cond-mat.supr-con↗

arXiv2007

Experimental and First principle calculation of Co_xNi_{(1-x)}Si solid solution structural stability

We report the investigation of the structural stability of Co$_{(1-x)}$Ni$_x$Si monosilicides for $0<x<1$. As CoSi crystallizes in the FeSi-type structure (B20) and NiSi is stable in the MnP-type structure (B31), a complete set of samples has been synthesized and a systematic study of phase formation under different annealing conditions were carried out in order to understand the reason of such a structural transition when x goes from 0 to 1. This study has revealed a limit in the solubility of Ni in CoSi B20 structure of about 17.5 at.% and of Co in NiSi B31 phase of about 13 at.%. For $0.35<x<0.74$ both B20 and B31 phases are present in the sample at there respective limits of solubility. The temperature dependence of the magnetic susceptibility has also been measured revealing diamagnetic behaviors. Optimal structural parameters and phase stability of the solid solution have been investigated using self-consistent full-potential linearized augmented plane wave method (FP-LAPW) based on the density functional theory (DFT). This calculation well predicts the structural instability observed experimentally.

cond-mat.mtrl-sci↗

arXiv2007

Model-Independent Sum Rule Analysis Based on Limited-Range Spectral Data

Partial sum rules are widely used in physics to separate low- and high-energy degrees of freedom of complex dynamical systems. Their application, though, is challenged in practice by the always finite spectrometer bandwidth and is often performed using risky model-dependent extrapolations. We show that, given spectra of the real and imaginary parts of any causal frequency-dependent response function (for example, optical conductivity, magnetic susceptibility, acoustical impedance etc.) in a limited range, the sum-rule integral from zero to a certain cutoff frequency inside this range can be safely derived using only the Kramers-Kronig dispersion relations without any extra model assumptions. This implies that experimental techniques providing both active and reactive response components independently, such as spectroscopic ellipsometry in optics, allow an extrapolation-independent determination of spectral weight 'hidden' below the lowest accessible frequency.

cond-mat.other↗

arXiv2007

Optical evidence for heavy charge carriers in FeGe

The optical spectrum of the cubic helimagnetic metal FeGe has been investigated in the frequency range from 0.01 - 3.1 eV for different temperatures from 30 K to 296 K. The optical conductivity shows the evolution of a low energy (0.22 eV) interband transition and the development of a narrow free carrier response with a strong energy and temperature dependence. The frequency dependent effective mass and scattering rate derived from the optical data indicate the formation of dressed quasi-particles with a mass renormalization factor of 12. Similar to FeSi the spectral weight in FeGe is not recovered over a broad frequency range, an effect usually attributed to the influence of the on-site Coulomb interaction.

cond-mat.str-el↗

arXiv2007

Optical properties and electronic structure of ZrB$_{12}$

We report optical (6 meV - 4 eV) properties of a boride superconductor ZrB$_{12}$ ($T_c$ = 6 K) in the normal state from 20 to 300 K measured on high-quality single crystals by a combination of reflectivity and ellipsometry. The Drude plasma frequency and interband optical conductivity calculated by self-consistent full-potential LMTO method agree well with experimental data. The Eliashberg function $α_{tr}^2F(ω)$ extracted from optical spectra features two peaks at about 25 and 80 meV, in agreement with specific heat data. The total coupling constant is $λ_{tr}=1.0\pm0.35$. The low energy peak presumably corresponds to the displacement mode of Zr inside $B_{24}$ cages, while the second one involves largely boron atoms. In addition to the usual narrowing of the Drude peak with cooling down, we observe an unexpected removal of about 10 % of the Drude spectral weight which is partially transferred to the region of the lowest-energy interband transition ($\sim$ 1 eV). This effect may be caused by the delocalization of the metal ion from the center of the $B_{24}$ cluster.

cond-mat.supr-con↗

arXiv2007

Charge carrier interaction with a purely electronic collective mode: Plasmarons and the infrared response of elemental bismuth

We present a detailed optical study of single crystal bismuth using infrared reflectivity and ellipsometry. Colossal changes in the plasmon frequency are observed as a function of temperature due to charge transfer between hole and electron Fermi pockets. In the optical conductivity, an anomalous temperature dependent mid-infrared absorption feature is observed. An extended Drude model analysis reveals that it can be connected to a sharp upturn in the scattering rate, the frequency of which exactly tracks the temperature dependent plasmon frequency. We interpret this absorption and increased scattering as the first direct optical evidence for a charge carrier interaction with a collective mode of purely electronic origin; here electron-plasmon scattering. The observation of a \emph{plasmaron} as such is made possible only by the unique coincidence of various energy scales and exceptional properties of semi-metal bismuth.

cond-mat.str-el↗