arXiv subjects

Daniel D. Hickstein

Publications and source records attributed to Daniel D. Hickstein.

At least 19 recordsLinked to original sources

arXiv2024

Propagation of pulsed light in an optical cavity in a gravitational field

All modern theories of gravitation, starting with Newton's, predict that gravity will affect the speed of light propagation. Einstein's theory of General Relativity famously predicted that the effect is twice the Newtonian value, a prediction that was verified during the 1919 solar eclipse. Recent theories of vector gravity can be interpreted to imply that gravity will have a different effect on pulsed light versus continuous-wave (CW) light propagating between the two mirrors of an optical cavity. Interestingly, we are not aware of any previous experiments to determine the relative effect of gravity on the propagation of pulsed versus CW light. In order to observe if there are small differences, we use a 6 GHz electro-optic frequency comb and low-noise CW laser to make careful measurements of the resonance frequencies of a high-finesse optical cavity. Once correcting for the effects of mirror dispersion, we determine that the cavity resonance frequencies for pulsed and CW light are the same to within our experimental error, which is on the order of $10^{-12}$ of the optical frequency, and one part in 700 of the expected gravitational shift.

physics.optics↗

arXiv2024

High-resolution MHz time- and angle-resolved photoemission spectroscopy based on a tunable vacuum ultraviolet source

Time and angle-resolved photoemission spectroscopy (trARPES) allows direct mapping of the electronic band structure and its dynamic response on femtosecond timescales. Here, we present a new ARPES system, powered by a new fiber-based femtosecond light source in the vacuum ultraviolet (VUV) range, accessing the complete first Brillouin zone for most materials. We present trARPES data on Au(111), polycrystalline Au, Bi2Se3 and TaTe2, demonstrating an energy resolution of 21 meV with a time resolution of <360 fs, at a high repetition rate of 1 MHz. The system is integrated with an extreme ultraviolet (EUV) high harmonic generation (HHG) beamline, enabling excellent tunability of the time-bandwidth resolution.

physics.ins-det↗

arXiv2022

Direct observation of enhanced electron-phonon coupling in copper nanoparticles in the warm-dense matter regime

Warm-dense matter (WDM) is a highly-excited state that lies at the confluence of solids, plasmas, and liquids and that cannot be described by equilibrium theories. The transient nature of this state when created in a laboratory, as well as the difficulties in probing the strongly-coupled interactions between the electrons and the ions, make it challenging to develop a complete understanding of matter in this regime. In this work, by exciting isolated ~8 nm nanoparticles with a femtosecond laser below the ablation threshold, we create uniformly-excited WDM. We then use photoelectron spectroscopy to track the instantaneous electron temperature and directly extract the strongest electron-ion coupling observed experimentally to date. By directly comparing with state-of-the-art theories, we confirm that the superheated nanoparticles lie at the boundary between hot solids and plasmas, with associated strong electron-ion coupling. This is evidenced both by the fast energy loss of electrons to ions, as well as a strong modulation of the electron temperature by acoustic oscillations in the nanoparticle. This work demonstrates a new route for experimental exploration and theoretical validation of the exotic properties of WDM.

physics.plasm-ph↗

arXiv2021

Broadband ultraviolet-visible frequency combs from cascaded high-harmonic generation in quasi-phase-matched waveguides

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped periodically poled lithium niobate waveguides driven by phase-stable $\leq$12-nJ, 100 fs pulses at 3 $μ$m with 100 MHz repetition rate. A mid-infrared to ultraviolet-visible conversion efficiency as high as 10% is observed, amongst an overall 23% conversion of the fundamental to all harmonics. We verify the coherence of the harmonic frequency combs despite the complex highly nonlinear process. Numerical simulations based on a single broadband envelope equation with quadratic nonlinearity give estimates for the conversion efficiency within approximately 1 order of magnitude over a wide range of experimental parameters. From this comparison we identify a dimensionless parameter capturing the competition between three-wave mixing and group-velocity walk-off of the harmonics that governs the cascaded HHG physics. These results can inform cascaded HHG in a range of different platforms.

physics.optics↗

arXiv2020

Ultrafast 1 MHz vacuum-ultraviolet source via highly cascaded harmonic generation in negative-curvature hollow-core fibers

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of VUV light at MHz repetition rates using highly cascaded four-wave mixing processes in a negative-curvature hollow-core fiber. Both even and odd order harmonics are generated up to the 15th harmonic (69 nm, 18.0 eV), with high energy resolution of ~40 meV. In contrast to direct high harmonic generation, this highly cascaded harmonic generation process requires lower peak intensity and therefore can operate at higher repetition rates, driven by a robust ~10 W fiber-laser system in a compact setup. Additionally, we present numerical simulations that explore the fundamental capabilities and spatiotemporal dynamics of highly cascaded harmonic generation. This VUV source can enhance the capabilities of spectroscopies of molecular and quantum materials, such as photoionization mass spectrometry and time , angle , and spin-resolved photoemission.

physics.optics↗

arXiv2019

Generating few-cycle pulses with integrated nonlinear photonics

Ultrashort laser pulses that last only a few optical cycles have been transformative tools for studying and manipulating light--matter interactions. Few-cycle pulses are typically produced from high-peak-power lasers, either directly from a laser oscillator, or through nonlinear effects in bulk or fiber materials. Now, an opportunity exists to explore the few-cycle regime with the emergence of fully integrated nonlinear photonics. Here, we experimentally and numerically demonstrate how lithographically patterned waveguides can be used to generate few-cycle laser pulses from an input seed pulse. Moreover, our work explores a design principle in which lithographically varying the group-velocity dispersion in a waveguide enables the creation of highly constant-intensity supercontinuum spectra across an octave of bandwidth. An integrated source of few-cycle pulses could broaden the range of applications for ultrafast light sources, including supporting new lab-on-a-chip systems in a scalable form factor.

physics.optics↗

arXiv2019

A direct comparison of high-speed methods for the numerical Abel transform

The Abel transform is a mathematical operation that transforms a cylindrically symmetric three-dimensional (3D) object into its two-dimensional (2D) projection. The inverse Abel transform reconstructs the 3D object from the 2D projection. Abel transforms have wide application across numerous fields of science, especially chemical physics, astronomy, and the study of laser-plasma plumes. Consequently, many numerical methods for the Abel transform have been developed, which makes it challenging to select the ideal method for a specific application. In this work eight transform methods have been incorporated into a single, open-source Python software package (PyAbel) to provide a direct comparison of the capabilities, advantages, and relative computational efficiency of each transform method. Most of the tested methods provide similar, high-quality results. However, the computational efficiency varies across several orders of magnitude. By optimizing the algorithms, we find that some transform methods are sufficiently fast to transform 1-megapixel images at more than 100 frames per second on a desktop personal computer. In addition, we demonstrate the transform of gigapixel images.

physics.chem-ph↗

arXiv2018

Dual-comb spectroscopy with tailored spectral broadening in Si$_3$N$_4$ nanophotonics

Si$_3$N$_4$ waveguides, pumped at 1550 nm, can provide spectrally smooth, broadband light for gas spectroscopy in the important 2 ${\mathrmμ}$m to 2.5 ${\mathrmμ}$m atmospheric water window, which is only partially accessible with silica-fiber based systems. By combining Er+:fiber frequency combs and supercontinuum generation in tailored Si$_3$N$_4$ waveguides, high signal-to-noise dual-comb spectroscopy (DCS) spanning 2 ${\mathrmμ}$m to 2.5 ${\mathrmμ}$m is demonstrated. Acquired broadband dual-comb spectra of CO and CO$_2$ agree well with database line shape models and have a spectral-signal-to-noise as high as 48$/\sqrt{\mathrm{s}}$, showing that the high coherence between the two combs is retained in the Si$_3$N$_4$ supercontinuum generation. The DCS figure of merit is 6$\times 10^6/\sqrt{\mathrm{s}}$, equivalent to that of all-fiber DCS systems in the 1.6 ${\mathrmμ}$m band. Based on these results, future DCS can combine fiber comb technology with Si$_3$N$_4$ waveguides to access new spectral windows in a robust non-laboratory platform.

physics.optics↗

arXiv2018

A Kerr-microresonator optical clockwork

Kerr microresonators generate interesting and useful fundamental states of electromagnetic radiation through nonlinear interactions of continuous-wave (CW) laser light. Using photonic-integration techniques, functional devices with low noise, small size, low-power consumption, scalable fabrication, and heterogeneous combinations of photonics and electronics can be realized. Kerr solitons, which stably circulate in a Kerr microresonator, have emerged as a source of coherent, ultrafast pulse trains and ultra-broadband optical-frequency combs. Using the f-2f technique, Kerr combs support carrier-envelope-offset phase stabilization for optical synthesis and metrology. In this paper, we introduce a Kerr-microresonator optical clockwork based on optical-frequency division (OFD), which is a powerful technique to transfer the fractional-frequency stability of an optical clock to a lower frequency electronic clock signal. The clockwork presented here is based on a silicon-nitride (Si$_3$N$_4$) microresonator that supports an optical-frequency comb composed of soliton pulses at 1 THz repetition rate. By electro-optic phase modulation of the entire Si$_3$N$_4$ comb, we arbitrarily generate additional CW modes between the Si$_3$N$_4$ comb modes; operationally, this reduces the pulse train repetition frequency and can be used to implement OFD to the microwave domain. Our experiments characterize the residual frequency noise of this Kerr-microresonator clockwork to one part in $10^{17}$, which opens the possibility of using Kerr combs with high performance optical clocks. In addition, the photonic integration and 1 THz resolution of the Si$_3$N$_4$ frequency comb makes it appealing for broadband, low-resolution liquid-phase absorption spectroscopy, which we demonstrate with near infrared measurements of water, lipids, and organic solvents.

physics.optics↗

arXiv2018

Fully self-referenced frequency comb consuming 5 Watts of electrical power

We present a hybrid fiber/waveguide design for a 100-MHz frequency comb that is fully self-referenced and temperature controlled with less than 5 W of electrical power. Self-referencing is achieved by supercontinuum generation in a silicon nitride waveguide, which requires much lower pulse energies (~200 pJ) than with highly nonlinear fiber. These low-energy pulses are achieved with an erbium fiber oscillator/amplifier pumped by two 250-mW passively-cooled pump diodes that consume less than 5 W of electrical power. The temperature tuning of the oscillator, necessary to stabilize the repetition rate in the presence of environmental temperature changes, is achieved by resistive heating of a section of gold-palladium-coated fiber within the laser cavity. By heating only the small thermal mass of the fiber, the repetition rate is tuned over 4.2 kHz (corresponding to an effective temperature change of 4.2 °C) with a fast time constant of 0.5 s, at a low power consumption of 0.077 W/°C, compared to 2.5 W/°C in the conventional 200-MHz comb design.

physics.ins-det↗

arXiv2018

Rapid, accurate, and precise concentration measurements of a methanol-water mixture using Raman spectroscopy

Here we design, construct, and characterize a compact Raman-spectroscopy-based sensor that measures the concentration of a water-methanol mixture. The sensor measures the concentration with an accuracy of 0.5% and a precision of 0.2% with a 1 second measuring time. With longer measurement times, the precision reaches as low as 0.006%. We characterize the long-term stability of the instrument over an 11-day period of constant measurement, and confirm that systematic drifts are on the level of 0.02%. We describe methods to improve the sensor performance, providing a path towards accurate, precise, and reliable concentration measurements in harsh environments. This sensor should be adaptable to other water-alcohol mixtures, or other small-molecule liquid mixtures.

physics.ins-det↗

arXiv2018

Self-organized nonlinear gratings for ultrafast nanophotonics

Modern nonlinear optical materials allow light of one wavelength be efficiently converted into light at another wavelength. However, designing nonlinear optical materials to operate with ultrashort pulses is difficult, because it is necessary to match both the phase velocities and group velocities of the light. Here we show that self-organized nonlinear gratings can be formed with femtosecond pulses propagating through nanophotonic waveguides, providing simultaneous group-velocity matching and quasi-phase-matching for second harmonic generation. We record the first direct microscopy images of photo-induced nonlinear gratings, and demonstrate how these waveguides enable simultaneous $χ^{(2)}$ and $χ^{(3)}$ nonlinear processes, which we utilize to stabilize a laser frequency comb. Finally, we derive the equations that govern self-organized grating formation for femtosecond pulses and explain the crucial role of group-velocity matching. In the future, such nanophotonic waveguides could enable scalable, reconfigurable nonlinear optical systems.

physics.optics↗

arXiv2018

Dual-comb interferometry via repetition-rate switching of a single frequency comb

We experimentally demonstrate a versatile technique for performing dual-comb interferometry using a single frequency comb. By rapid switching of the repetition rate, the output pulse train can be delayed and heterodyned with itself to produce interferograms. The full speed and resolution of standard dual-comb interferometry is preserved while simultaneously offering a significant experimental simplification and cost savings. We show that this approach is particularly suited for absolute distance metrology due to an extension of the non-ambiguity range as a result of the continuous repetition-rate switching.

physics.ins-det↗

arXiv2018

Heterogeneously integrated GaAs waveguides on insulator for efficient frequency conversion

Tremendous scientific progress has been achieved through the development of nonlinear integrated photonics. Prominent examples are Kerr-frequency-comb generation in micro-resonators, and supercontinuum generation and frequency conversion in nonlinear photonic waveguides. High conversion efficiency is enabling for applications of nonlinear optics, including such broad directions as high-speed optical signal processing, metrology, and quantum communication and computation. In this work, we demonstrate a gallium-arsenide-on-insulator (GaAs) platform for nonlinear photonics. GaAs has among the highest second- and third-order nonlinear optical coefficients, and use of a silica cladding results in waveguides with a large refractive index contrast and low propagation loss for expanded design of nonlinear processes. By harnessing these properties and developing nanofabrication with GaAs, we report a record normalized second-harmonic efficiency of 13,000% W-1cm-2 at a fundamental wavelength of 2 um. This work paves the way for high performance nonlinear photonic integrated circuits (PICs), which not only can transition advanced functionalities outside the lab through fundamentally reduced power consumption and footprint, but also enables future optical sources and detectors.

physics.optics↗

arXiv2018

Deuterated silicon nitride photonic devices for broadband optical frequency comb generation

We report and characterize low-temperature, plasma-deposited deuterated silicon nitride thin films for nonlinear integrated photonics. With a peak processing temperature less than 300$^\circ$C, it is back-end compatible with pre-processed CMOS substrates. We achieve microresonators with a quality factor of up to $1.6\times 10^6 $ at 1552 nm, and $>1.2\times 10^6$ throughout $λ$ = 1510 -- 1600 nm, without annealing or stress management. We then demonstrate the immediate utility of this platform in nonlinear photonics by generating a 1 THz free spectral range, 900-nm-bandwidth modulation-instability microresonator Kerr comb and octave-spanning, supercontinuum-broadened spectra.

physics.optics↗

arXiv2018

Mid-infrared frequency comb generation via cascaded quadratic nonlinearities in quasi-phase-matched waveguides

We experimentally demonstrate a simple configuration for mid-infrared (MIR) frequency comb generation in quasi-phase-matched lithium niobate waveguides using the cascaded-$χ^{(2)}$ nonlinearity. With nanojoule-scale pulses from an Er:fiber laser, we observe octave-spanning supercontinuum in the near-infrared with dispersive-wave generation in the 2.5--3 $\textμ$m region and intra-pulse difference-frequency generation in the 4--5 $\textμ$m region. By engineering the quasi-phase-matched grating profiles, tunable, narrow-band MIR and broadband MIR spectra are both observed in this geometry. Finally, we perform numerical modeling using a nonlinear envelope equation, which shows good quantitative agreement with the experiment---and can be used to inform waveguide designs to tailor the MIR frequency combs. Our results identify a path to a simple single-branch approach to mid-infrared frequency comb generation in a compact platform using commercial Er:fiber technology.

physics.optics↗

arXiv2017

Quasi-phase-matched supercontinuum-generation in photonic waveguides

Supercontinuum generation in integrated photonic waveguides is a versatile source of broadband light, and the generated spectrum is largely determined by the phase-matching conditions. Here we show that quasi-phase-matching via periodic modulations of the waveguide structure provides a useful mechanism to control the evolution of ultrafast pulses and the supercontinuum spectrum. We experimentally demonstrate quasi-phase-matched supercontinuum to the TE20 and TE00 waveguide modes, which enhances the intensity of the SCG in specific spectral regions by as much as 20 dB. We utilize higher-order quasi-phase-matching (up to the 16th order) to enhance the intensity in numerous locations across the spectrum. Quasi-phase-matching adds a unique dimension to the design-space for SCG waveguides, allowing the spectrum to be engineered for specific applications.

physics.optics↗

arXiv2017

An ultrafast electro-optic light source with sub-cycle precision

Controlling femtosecond optical pulses with temporal precision better than one cycle of the carrier field has a profound impact on measuring and manipulating interactions between light and matter. We explore pulses that are carved from a continuous-wave laser via electro-optic modulation and realize the regime of sub-cycle optical control without a mode-locked resonator. Our ultrafast source, with a repetition rate of 10 GHz, is derived from an optical-cavity-stabilized laser and a microwave-cavity-stabilized electronic oscillator. Sub-cycle timing jitter of the pulse train is achieved by coherently linking the laser and oscillator through carrier-envelope phase stabilization enabled by a photonic-chip supercontinuum that spans up to 1.9 octaves across the near infrared. Moreover, the techniques we report are relevant for other ultrafast lasers with repetition rates up to 30 GHz and may allow stable few-cycle pulses to be produced by a wider range of sources.

physics.optics↗