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Daniel Loss

Publications and source records attributed to Daniel Loss.

At least 415 records · Page 23Linked to original sources

Exchange-controlled single-electron-spin rotations in quantum dots

We show theoretically that arbitrary coherent rotations can be performed quickly (with a gating time ~1 ns) and with high fidelity on the spin of a single confined electron using control of exchange only, without the need for spin-orbit coupling or ac fields. We expect that implementations of this scheme would achieve gate error rates on the order of η~ 10^{-3} in GaAs quantum dots, within reach of several known error-correction protocols

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Spin qubits with electrically gated polyoxometalate molecules

Spin qubits offer one of the most promising routes to the implementation of quantum computers. Very recent results in semiconductor quantum dots show that electrically-controlled gating schemes are particularly well-suited for the realization of a universal set of quantum logical gates. Scalability to a larger number of qubits, however, remains an issue for such semiconductor quantum dots. In contrast, a chemical bottom-up approach allows one to produce identical units in which localized spins represent the qubits. Molecular magnetism has produced a wide range of systems with tailored properties, but molecules permitting electrical gating have been lacking. Here we propose to use the polyoxometalate [PMo12O40(VO)2]q-, where two localized spins-1/2 can be coupled through the electrons of the central core. Via electrical manipulation of the molecular redox potential, the charge of the core can be changed. With this setup, two-qubit gates and qubit readout can be implemented.

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Sequential Tunneling through Molecular Spin Rings

We consider electrical transport through molecules with Heisenberg-coupled spins arranged in a ring structure in the presence of an easy-axis anisotropy. The molecules are coupled to two metallic leads and a gate. In the charged state of the ring, a Zener double-exchange mechanism links transport properties to the underlying spin structure. This leads to a remarkable contact-site dependence of the current, which for an antiferromagnetic coupling of the spins can lead to a total suppression of the zero-bias conductance when the molecule is contacted at adjacent sites.

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Spin qubits in graphene quantum dots

We propose how to form spin qubits in graphene. A crucial requirement to achieve this goal is to find quantum dot states where the usual valley degeneracy in bulk graphene is lifted. We show that this problem can be avoided in quantum dots based on ribbons of graphene with semiconducting armchair boundaries. For such a setup, we find the energies and the exact wave functions of bound states, which are required for localized qubits. Additionally, we show that spin qubits in graphene can not only be coupled between nearest neighbor quantum dots via Heisenberg exchange interaction but also over long distances. This remarkable feature is a direct consequence of the quasi-relativistic spectrum of graphene.

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Direct Measurement of the Spin-Orbit Interaction in a Two-Electron InAs Nanowire Quantum Dot

We demonstrate control of the electron number down to the last electron in tunable few-electron quantum dots defined in catalytically grown InAs nanowires. Using low temperature transport spectroscopy in the Coulomb blockade regime we propose a simple method to directly determine the magnitude of the spin-orbit interaction in a two-electron artificial atom with strong spin-orbit coupling. Due to a large effective g-factor |g*|=8+/-1 the transition from singlet S to triplet T+ groundstate with increasing magnetic field is dominated by the Zeeman energy rather than by orbital effects. We find that the spin-orbit coupling mixes the T+ and S states and thus induces an avoided crossing with magnitude $Δ_{SO}$=0.25+/-0.05 meV. This allows us to calculate the spin-orbit length $λ_{SO}\approx$127 nm in such systems using a simple model.

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Nuclear spin ferromagnetic phase transition in an interacting 2D electron gas

Electrons in a two-dimensional semiconducting heterostructure interact with nuclear spins via the hyperfine interaction. Using a a Kondo lattice formulation of the electron-nuclear spin interaction, we show that the nuclear spin system within an interacting two-dimensional electron gas undergoes a ferromagnetic phase transition at finite temperatures. We find that electron-electron interactions and non-Fermi liquid behavior substantially enhance the nuclear spin Curie temperature into the $mK$ range with decreasing electron density.

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Measurement, control, and decay of quantum-dot spins

In this review we discuss a recent proposal to perform partial Bell-state (parity) measurements on two-electron spin states for electrons confined to quantum dots. The realization of this proposal would allow for a physical implementation of measurement-based quantum computing. In addition, we consider the primary sources of energy relaxation and decoherence which provide the ultimate limit to all proposals for quantum information processing using electron spins in quantum dots. We give an account of the Hamiltonians used for the most important interactions (spin-orbit and hyperfine) and survey some of the recent work done to understand dynamics, control, and decoherence under the action of these Hamiltonians. We conclude the review with a table of important decay times found in experiment, and relate these time scales to the potential viability of measurement-based quantum computing.

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Electric Dipole Induced Spin Resonance in Quantum Dots

An alternating electric field, applied to a quantum dot, couples to the electron spin via the spin-orbit interaction. We analyze different types of spin-orbit coupling known in the literature and find two efficient mechanisms of spin control in quantum dots. The linear in momentum Dresselhaus and Rashba spin-orbit couplings give rise to a fully transverse effective magnetic field in the presence of a Zeeman splitting at lowest order in the spin-orbit interaction. The cubic in momentum Dresselhaus terms are efficient in a quantum dot with non-harmonic confining potential and give rise to a spin-electric coupling proportional to the orbital magnetic field. We derive an effective spin Hamiltonian, which can be used to implement spin manipulation on a timescale of $10 {\rm ns}$ with the current experimental setups.

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Spin-spin coupling in electrostatically coupled quantum dots

We study the spin-spin coupling between two single-electron quantum dots due to the Coulomb and spin-orbit interactions, in the absence of tunneling between the dots. We find an anisotropic XY spin-spin interaction that is proportional to the Zeeman splitting produced by the external magnetic field. This interaction is studied both in the limit of weak and strong Coulomb repulsion with respect to the level spacing of the dot. The interaction is found to be a non-monotonic function of inter-dot distance $a_0$ and external magnetic field, and, moreover, vanishes for some special values of $a_0$ and/or magnetic field orientation. This mechanism thus provides a new way to generate and tune spin interaction between quantum dots. We propose a scheme to measure this spin-spin interaction based on the spin-relaxation-measurement technique.

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Electric Dipole Spin Resonance for Heavy Holes in Quantum Dots

We propose and analyze a new method for manipulation of a heavy hole spin in a quantum dot. Due to spin-orbit coupling between states with different orbital momenta and opposite spin orientations, an applied rf electric field induces transitions between spin-up and spin-down states. This scheme can be used for detection of heavy-hole spin resonance signals, for the control of the spin dynamics in two-dimensional systems, and for determining important parameters of heavy-holes such as the effective $g$-factor, mass, spin-orbit coupling constants, spin relaxation and decoherence times.

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Quantum computing with spins in solids

The ability to perform high-precision one- and two-qubit operations is sufficient for universal quantum computation. For the Loss-DiVincenzo proposal to use single electron spins confned to quantum dots as qubits, it is therefore sufficient to analyze only single- and coupled double-dot structures, since the strong Heisenberg exchange coupling between spins in this proposal falls off exponentially with distance and long-ranged dipolar coupling mechanisms can be made significantly weaker. This scalability of the Loss-DiVincenzo design is both a practical necessity for eventual applications of multi-qubit quantum computing and a great conceptual advantage, making analysis of the relevant components relatively transparent and systematic. We review the Loss-DiVincenzo proposal for quantum-dot-confned electron spin qubits, and survey the current state of experiment and theory regarding the relevant single- and double- quantum dots, with a brief look at some related alternative schemes for quantum computing.

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Electric Dipole Induced Spin Resonance in Disordered Semiconductors

One of the hallmarks of spintronics is the control of magnetic moments by electric fields enabled by strong spin-orbit interaction (SOI) in semiconductors. A powerful way of manipulating spins in such structures is electric dipole induced spin resonance (EDSR), where the radio-frequency fields driving the spins are electric, and not magnetic like in standard paramagnetic resonance. Here, we present a theoretical study of EDSR for a two-dimensional electron gas in the presence of disorder where random impurities not only determine the electric resistance but also the spin dynamics via SOI. Considering a specific geometry with the electric and magnetic fields parallel and in-plane, we show that the magnetization develops an out-of-plane component at resonance which survives the presence of disorder. We also discuss the spin Hall current generated by EDSR. These results are derived in a diagrammatic approach with the dominant effects coming from the spin vertex correction, and the optimal parameter regime for observation is identified.

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Quantum-dot spin qubit and hyperfine interaction

We review our investigation of the spin dynamics for two electrons confined to a double quantum dot under the influence of the hyperfine interaction between the electron spins and the surrounding nuclei. Further we propose a scheme to narrow the distribution of difference in polarization between the two dots in order to suppress hyperfine induced decoherence.

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Dynamics of Coupled Qubits Interacting with an Off-Resonant Cavity

We study a model for a pair of qubits which interact with a single off-resonant cavity mode and, in addition, exhibit a direct inter-qubit coupling. Possible realizations for such a system include coupled superconducting qubits in a line resonator as well as exciton states or electron spin states of quantum dots in a cavity. The emergent dynamical phenomena are strongly dependent on the relative energy scales of the inter-qubit coupling strength, the coupling strength between qubits and cavity mode, and the cavity mode detuning. We show that the cavity mode dispersion enables a measurement of the state of the coupled-qubit system in the perturbative regime. We discuss the effect of the direct inter-qubit interaction on a cavity-mediated two-qubit gate. Further, we show that for asymmetric coupling of the two qubits to the cavity, the direct inter-qubit coupling can be controlled optically via the ac Stark effect.

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Nuclear spin state narrowing via gate--controlled Rabi oscillations in a double quantum dot

We study spin dynamics for two electrons confined to a double quantum dot under the influence of an oscillating exchange interaction. This leads to driven Rabi oscillations between the $\ket{\uparrow\downarrow}$--state and the $\ket{\downarrow\uparrow}$--state of the two--electron system. The width of the Rabi resonance is proportional to the amplitude of the oscillating exchange. A measurement of the Rabi resonance allows one to narrow the distribution of nuclear spin states and thereby to prolong the spin decoherence time. Further, we study decoherence of the two-electron states due to the hyperfine interaction and give requirements on the parameters of the system in order to initialize in the $\ket{\uparrow\downarrow}$--state and to perform a $\sqrt{\mathrm{SWAP}}$ operation with unit fidelity.

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A Mesoscopic Resonating Valence Bond system on a triple dot

We introduce a mesoscopic pendulum from a triple dot. The pendulum is fastened through a singly-occupied dot (spin qubit). Two other strongly capacitively islands form a double-dot charge qubit with one electron in excess oscillating between the two low-energy charge states (1,0) and (0,1); this embodies the weight of the pendulum. The triple dot is placed between two superconducting leads as shown in Fig. 1. Under well-defined conditions, the main proximity effect stems from the injection of resonating singlet (valence) bonds on the triple dot. This gives rise to a Josephson current that is charge- and spin-dependent. Consequences in a SQUID-geometry are carefully investigated.

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Cotunneling current through quantum dots with phonon-assisted spin-flip processes

We consider cotunneling through a quantum dot in the presence of spin-flip processes induced by the coupling to acoustic phonons of the surrounding. An expression for the phonon-assisted cotunneling current is derived by means of a generalized Schrieffer-Wolff transformation. The influence of the spin-phonon coupling on the heating of the dot is considered. The result is evaluated for the case of a parabolic semiconductor quantum dot with Rashba and Dresselhaus spin-orbit coupling and a method for the determination of the spin-phonon relaxation rate is proposed.

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Zitterbewegung of electrons and holes in III-V semiconductor quantum wells

The notion of zitterbewegung is a long-standing prediction of relativistic quantum mechanics. Here we extend earlier theoretical studies on this phenomenon for the case of III-V zinc-blende semiconductors which exhibit particularly strong spin-orbit coupling. This property makes nanostructures made of these materials very favorable systems for possible experimental observations of zitterbewegung. Our investigations include electrons in n-doped quantum wells under the influence of both Rashba and Dresselhaus spin-orbit interaction, and also the two-dimensional hole gas. Moreover, we give a detailed anaysis of electron zitterbewegung in quantum wires which appear to be particularly suited for experimentally observing this effect.

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