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Daniel Loss

Publications and source records attributed to Daniel Loss.

At least 433 records · Page 24Linked to original sources

Spin Decay in a Quantum Dot Coupled to a Quantum Point Contact

We consider a mechanism of spin decay for an electron spin in a quantum dot due to coupling to a nearby quantum point contact (QPC) with and without an applied bias voltage. The coupling of spin to charge is induced by the spin-orbit interaction in the presence of a magnetic field. We perform a microscopic calculation of the effective Hamiltonian coupling constants to obtain the QPC-induced spin relaxation and decoherence rates in a realistic system. This rate is shown to be proportional to the shot noise of the QPC in the regime of large bias voltage and scales as $a^{-6}$ where $a$ is the distance between the quantum dot and the QPC. We find that, for some specific orientations of the setup with respect to the crystallographic axes, the QPC-induced spin relaxation and decoherence rates vanish, while the charge sensitivity of the QPC is not changed. This result can be used in experiments to minimize QPC-induced spin decay in read-out schemes.

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Entanglement transfer from electron spins to photons in spin light-emitting diodes containing quantum dots

We show that electron recombination using positively charged excitons in single quantum dots provides an efficient method to transfer entanglement from electron spins onto photon polarizations. We propose a scheme for the production of entangled four-photon states of GHZ type. From the GHZ state, two fully entangled photons can be obtained by a measurement of two photons in the linear polarization basis, even for quantum dots with observable fine structure splitting for neutral excitons and significant exciton spin decoherence. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.

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Shot noise and spin-orbit coherent control of entangled and spin polarized electrons

We extend our previous work on shot noise for entangled and spin polarized electrons in a beam-splitter geometry with spin-orbit (\textit{s-o}) interaction in one of the incoming leads (lead 1). Besides accounting for both the Dresselhaus and the Rashba spin-orbit terms, we present general formulas for the shot noise of singlet and triplets states derived within the scattering approach. We determine the full scattering matrix of the system for the case of leads with \textit{two} orbital channels coupled via weak \textit{s-o} interactions inducing channel anticrossings. We show that this interband coupling coherently transfers electrons between the channels and gives rise to an additional modulation angle -- dependent on both the Rashba and Dresselhaus interaction strengths -- which allows for further independent coherent control of the electrons traversing the incoming leads. We derive explicit shot noise formulas for a variety of correlated pairs (e.g., Bell states) and lead spin polarizations. Interestingly, the singlet and \textit{each} of the triplets defined along the quantization axis perpendicular to lead 1 (with the local \textit{s-o} interaction) and in the plane of the beam splitter display distinctive shot noise for injection energies near the channel anticrossings; hence, one can tell apart all the triplets, in addition to the singlet, through noise measurements. We also find that spin-orbit induced backscattering within lead 1 reduces the visibility of the noise oscillations, due to the additional partition noise in this lead. Finally, we consider injection of two-particle wavepackets into leads with multiple discrete states and find that two-particle entanglement can still be observed via noise bunching and antibunching.

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Fermi liquid parameters in 2D with spin-orbit interaction

We derive analytical expressions for the quasiparticle lifetime tau, the effective mass m*, and the Green's function renormalization factor Z for a 2D Fermi liquid with electron-electron interaction in the presence of the Rashba spin-orbit interaction. We find that the modifications are independent of the Rashba band index rho, and occur in second order of the spin-orbit coupling alpha. In the derivation of these results, we also discuss the screening of the Coulomb interaction, as well as the susceptibility and the self-energy in small alpha.

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Spin relaxation and anticrossing in quantum dots: Rashba versus Dresselhaus spin-orbit coupling

The spin-orbit splitting of the electron levels in a two-dimensional quantum dot in a perpendicular magnetic field is studied. It is shown that at the point of an accidental degeneracy of the two lowest levels above the ground state the Rashba spin-orbit coupling leads to a level anticrossing and to mixing of spin-up and spin-down states, whereas there is no mixing of these levels due to the Dresselhaus term. We calculate the relaxation and decoherence times of the three lowest levels due to phonons. We find that the spin relaxation rate as a function of a magnetic field exhibits a cusp-like structure for Rashba but not for Dresselhaus spin-orbit interaction.

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Singlet-triplet decoherence due to nuclear spins in a double quantum dot

We have evaluated hyperfine-induced electron spin dynamics for two electrons confined to a double quantum dot. Our quantum solution accounts for decay of a singlet-triplet correlator even in the presence of a fully static nuclear spin system, with no ensemble averaging over initial conditions. In contrast to an earlier semiclassical calculation, which neglects the exchange interaction, we find that the singlet-triplet correlator shows a long-time saturation value that differs from 1/2, even in the presence of a strong magnetic field. Furthermore, we find that the form of the long-time decay undergoes a transition from a rapid Gaussian to a slow power law ($\sim 1/t^{3/2}$) when the exchange interaction becomes nonzero and the singlet-triplet correlator acquires a phase shift given by a universal (parameter independent) value of $3π/4$ at long times. The oscillation frequency and time-dependent phase shift of the singlet-triplet correlator can be used to perform a precision measurement of the exchange interaction and Overhauser field fluctuations in an experimentally accessible system. We also address the effect of orbital dephasing on singlet-triplet decoherence, and find that there is an optimal operating point where orbital dephasing becomes negligible.

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Spin-Hall conductivity due to Rashba spin-orbit interaction in disordered systems

We consider the spin-Hall current in a disordered two-dimensional electron gas in the presence of Rashba spin-orbit interaction. We derive a generalized Kubo-Greenwood formula for the spin-Hall conductivity $σ$ and evaluate it in an systematic way using standard diagrammatic techniques for disordered systems. We find that in the diffusive regime both Boltzmann and the weak localization contributions to $σ$ are of the same order and vanish in the zero frequency limit. We show that the uniform spin current is given by the total time derivative of the magnetization from which we can conclude that the spin current vanishes exactly in the stationary limit. This conclusion is valid for arbitrary spin-independent disorder, external electric field strength, and also for interacting electrons.

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Zitterbewegung of electronic wave packets in semiconductor nanostructures

We study the zitterbewegung of electronic wave packets in III-V zinc-blende semiconductor quantum wells due to spin-orbit coupling. Our results suggest a direct experimental proof of this fundamental effect, confirming a long-standing theoretical prediction. For electron motion in a harmonic quantum wire, we numerically and analytically find a resonance condition maximizing the zitterbewegung.

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Cluster States From Heisenberg Interaction

We show that a special type of entangled states, cluster states, can be created with Heisenberg interactions and local rotations in 2d steps where d is the dimension of the lattice. We find that, by tuning the coupling strengths, anisotropic exchange interactions can also be employed to create cluster states. Finally, we propose electron spins in quantum dots as a possible realization of a one-way quantum computer based on cluster states.

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Determining the spin Hall conductance via charge transport

We propose a scheme where transport measurements of charge current and its noise can be used to determine the spin Hall conductance in a four-terminal setup. Starting from the scattering formalism we express the spin current and spin Hall conductance in terms of spin-dependent transmission coefficients. These coefficients are then expressed in terms of charge current and noise. We use the scheme to characterize the spin injection efficiency of a ferromagnetic/semiconductor interface.

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Spin relaxation and decoherence of holes in quantum dots

We investigate heavy-hole spin relaxation and decoherence in quantum dots in perpendicular magnetic fields. We show that at low temperatures the spin decoherence time is two times longer than the spin relaxation time. We find that the spin relaxation time for heavy holes can be comparable to or even longer than that for electrons in strongly two-dimensional quantum dots. We discuss the difference in the magnetic-field dependence of the spin relaxation rate due to Rashba or Dresselhaus spin-orbit coupling for systems with positive (i.e., GaAs quantum dots) or negative (i.e., InAs quantum dots) $g$-factor.

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Recipes for spin-based quantum computing

Technological growth in the electronics industry has historically been measured by the number of transistors that can be crammed onto a single microchip. Unfortunately, all good things must come to an end; spectacular growth in the number of transistors on a chip requires spectacular reduction of the transistor size. For electrons in semiconductors, the laws of quantum mechanics take over at the nanometre scale, and the conventional wisdom for progress (transistor cramming) must be abandoned. This realization has stimulated extensive research on ways to exploit the spin (in addition to the orbital) degree of freedom of the electron, giving birth to the field of spintronics. Perhaps the most ambitious goal of spintronics is to realize complete control over the quantum mechanical nature of the relevant spins. This prospect has motivated a race to design and build a spintronic device capable of complete control over its quantum mechanical state, and ultimately, performing computations: a quantum computer. In this tutorial we summarize past and very recent developments which point the way to spin-based quantum computing in the solid-state. After introducing a set of basic requirements for any quantum computer proposal, we offer a brief summary of some of the many theoretical proposals for solid-state quantum computers. We then focus on the Loss-DiVincenzo proposal for quantum computing with the spins of electrons confined to quantum dots. There are many obstacles to building such a quantum device. We address these, and survey recent theoretical, and then experimental progress in the field. To conclude the tutorial, we list some as-yet unrealized experiments, which would be crucial for the development of a quantum-dot quantum computer.

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Phonon Bottleneck Effect Leads to Observation of Quantum Tunneling of the Magnetization and Butterfly Hysteresis Loops in (Et4N)3Fe2F9

A detailed investigation of the unusual dynamics of the magnetization of (Et4N)3Fe2F9 (Fe2), containing isolated [Fe2F9]3- dimers, is presented and discussed. Fe2 possesses an S=5 ground state with an energy barrier of 2.40 K due to an axial anisotropy. Poor thermal contact between sample and bath leads to a phonon bottleneck situation, giving rise to butterfly-shaped hysteresis loops below 5 K concomitant with slow decay of the magnetization for magnetic fields Hz applied along the Fe--Fe axis. The butterfly curves are reproduced using a microscopic model based on the interaction of the spins with resonant phonons. The phonon bottleneck allows for the observation of resonant quantum tunneling of the magnetization at 1.8 K, far above the blocking temperature for spin-phonon relaxation. The latter relaxation is probed by AC magnetic susceptibility experiments at various temperatures and bias fields. At H=0, no out-of-phase signal is detected, indicating that at T smaller than 1.8 K Fe2 does not behave as a single-molecule magnet. At 1 kG, relaxation is observed, occurring over the barrier of the thermally accessible S=4 first excited state that forms a combined system with the S=5 state.

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Spin susceptibilities, spin densities and their connection to spin-currents

We calculate the frequency dependent spin susceptibilities for a two-dimensional electron gas with both Rashba and Dresselhaus spin-orbit interaction. The resonances of the susceptibilities depends on the relative values of the Rashba and Dresselhaus spin-orbit constants, which could be manipulated by gate voltages. We derive exact continuity equations, with source terms, for the spin density and use those to connect the spin current to the spin density. In the free electron model the susceptibilities play a central role in the spin dynamics since both the spin density and the spin current are proportional to them.

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Spin injection across magnetic/non-magnetic interfaces with finite magnetic layers

We have reconsidered the problem of spin injection across ferromagnet/non-magnetic-semiconductor (FM/NMS) and dilute-magnetic-semiconductor/non-magnetic-semiconductor interfaces, for structures with \textit{finite} magnetic layers (FM or DMS). By using appropriate physical boundary conditions, we find expressions for the resistances of these structures which are in general different from previous results in the literature. When the magnetoresistance of the contacts is negligible, we find that the spin-accumulation effect alone cannot account for the $d$ dependence observed in recent magnetoresistance data. In a limited parameter range, our formulas predict a strong $d$ dependence arising from the magnetic contacts in systems where their magnetoresistances are sizable.

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Spin-Hall transport of heavy holes in III-V semiconductor quantum wells

We investigate spin transport of heavy holes in III-V semiconductor quantum wells in the presence of spin-orbit coupling of the Rashba type due to structure-inversion asymmetry. Similarly to the case of electrons, the longitudinal spin conductivity vanishes, whereas the off-diagonal elements of the spin-conductivity tensor are finite giving rise to an intrinsic spin-Hall effect. For a clean system we find a closed expression for the spin-Hall conductivity depending on the length scale of the Rashba coupling and the hole density. In this limit the spin-Hall conductivity is enhanced compared to its value for electron systems, and it vanishes with increasing strength of the impurity scattering. As an aside, we also derive explicit expressions for the Fermi momenta and the densities of holes in the different dispersion branches as a function of the spin-orbit coupling parameter and the total hole density. These results are of relevance for the interpretation of possible Shubnikov-de Haas measurements detecting the Rashba spin splitting.

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Non-Markovian dynamics of a localized electron spin due to the hyperfine interaction

We review our theoretical work on the dynamics of a localized electron spin interacting with an environment of nuclear spins. Our perturbative calculation is valid for arbitrary polarization p of the nuclear spin system and arbitrary nuclear spin I in a sufficiently large magnetic field. In general, the electron spin shows rich dynamics, described by a sum of contributions with exponential decay, non-exponential decay, and undamped oscillations. We have found an abrupt crossover in the long-time spin dynamics at a critical shape and dimensionality of the electron envelope wave function. We conclude with a discussion of our proposed scheme to measure the relevant dynamics using a standard spin-echo technique.

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Controlling Spin Qubits in Quantum Dots

We review progress on the spintronics proposal for quantum computing where the quantum bits (qubits) are implemented with electron spins. We calculate the exchange interaction of coupled quantum dots and present experiments, where the exchange coupling is measured via transport. Then, experiments on single spins on dots are described, where long spin relaxation times, on the order of a millisecond, are observed. We consider spin-orbit interaction as sources of spin decoherence and find theoretically that also long decoherence times are expected. Further, we describe the concept of spin filtering using quantum dots and show data of successful experiments. We also show an implementation of a read out scheme for spin qubits and define how qubits can be measured with high precision. Then, we propose new experiments, where the spin decoherence time and the Rabi oscillations of single electrons can be measured via charge transport through quantum dots. Finally, all these achievements have promising applications both in conventional and quantum information processing.

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