arXiv subjects

Dapeng Yu

Publications and source records attributed to Dapeng Yu.

At least 91 records · Page 5Linked to original sources

arXiv2021

$LnCu_3(OH)_6Cl_3 (Ln = Gd, Tb, Dy)$: Heavy Lanthanides on Spin-1/2 Kagome Magnets

The spin-1/2 kagome antiferromagnets are key prototype materials for studying frustrated magnetism. Three isostructural kagome antiferromagnets LnCu$_3$(OH)$_6$Cl$_3$ (Ln = Gd, Tb, Dy) have been successfully synthesized by the hydrothermal method. LnCu$_3$(OH)$_6$Cl$_3$ adopts space group $P\overline{3}m1$ and features the layered Cu-kagome lattice with lanthanide Ln$^{3+}$ cations sitting at the center of the hexagons. Although heavy lanthanides (Ln = Gd, Tb, Dy) in LnCu$_3$(OH)$_6$Cl$_3$ provide a large effective magnetic moment and ferromagnetic-like spin correlations compared to light-lanthanides (Nd, Sm, Eu) analogues, Cu-kagome holds an antiferromagnetically ordered state at around 17 K like YCu$_3$(OH)$_6$Cl$_3$.

cond-mat.str-el↗

arXiv2021

Dzyaloshinskii-Moriya anisotropy effect on field-induced magnon condensation in kagome antiferromagnet $α-Cu_3Mg(OH)_6Br_2$

We performed a comprehensive electron spin resonance, magnetization and heat capacity study on the field-induced magnetic phase transitions in the kagome antiferromagnet $α-Cu_3Mg(OH)_6Br_2$. With the successful preparation of single crystals, we mapped out the magnetic phase diagrams under the $c$-axis and $ab$-plane directional magnetic fields $B$. For $B\|c$, the three-dimensional (3D) magnon Bose-Einstein condensation (BEC) is evidenced by the power law scaling of the transition temperature, $T_c\propto (B_c-B)^{2/3}$. For $B\|ab$, the transition from the canted antiferromagetic (CAFM) state to the fully polarized (FP) state is a crossover rather than phase transition, and the characteristic temperature has a significant deviation from the 3D BEC scaling. The different behaviors of the field-induced magnetic transitions for $B\|c$ and $B\|ab$ could result from the Dzyaloshinkii-Moriya (DM) interaction with the DM vector along the $c$-axis, which preserves the $c$-axis directional spin rotation symmetry and breaks the spin rotation symmetry when $B\|ab$. The 3D magnon BEC scaling for $B\|c$ is immune to the off-stoichiometric disorder in our sample $α-Cu_{3.26}Mg_{0.74}(OH)_6Br_2$. Our findings have the potential to shed light on the investigations of the magnetic anisotropy and disorder effects on the field-induced magnon BEC in the quantum antiferromagnet.

cond-mat.str-el↗

arXiv2021

Measuring phonon dispersion at an interface

The breakdown of translational symmetry at heterointerfaces leads to the emergence of new phonon modes localized near the interface. These interface phonons play an essential role in thermal/electrical transport properties in devices especially in miniature ones wherein the interface may dominate the entire response of the device. Knowledge of phonon dispersion at interfaces is therefore highly desirable for device design and optimization. Although theoretical work has begun decades ago, experimental research is totally absent due to challenges in achieving combined spatial, momentum and spectral resolutions required to probe localized phonon modes. Here we use electron energy loss spectroscopy in an electron microscope to directly measure both the local phonon density of states and the interface phonon dispersion relation for an epitaxial cBN-diamond heterointerface. In addition to bulk phonon modes, we observe acoustic and optical phonon modes localized at the interface, and modes isolated away from the interface. These features only appear within ~ 1 nm around the interface. The experimental results can be nicely reproduced by ab initio calculations. Our findings provide insights into lattice dynamics at heterointerfaces and should be practically useful in thermal/electrical engineering.

cond-mat.mtrl-sci↗

arXiv2021

Atomic-scale imaging of CH3NH3PbI3 structure and its decomposition pathway

Understanding the atomic structure and structural instability of organic-inorganic hybrid perovskites is the key to appreciate their remarkable photoelectric properties and failure mechanism. Here, using low-dose imaging technique by direct-detection electron-counting camera in transmission electron microscope, we investigate the atomic structure and decomposition pathway of CH3NH3PbI3 (MAPbI3) at the atomic scale. We successfully image the atomic structure of perovskite in real space under ultra-low electron dose condition, and observe a two-step decomposition process, i.e. initial loss of MA followed by the collapse of perovskite structure into 6H-PbI2 with their critical threshold dose also determined. Interestingly, an intermediate phase (MA0.5PbI3) with locally ordered vacancies can robustly exist before perovskite collapses, enlightening strategies for prevention and recovery of perovskite structure during degradation. Associated with structure evolution, the bandgap gradually increases from ~1.6 eV to ~2.1 eV, and it is found that both C-N and N-H bonds can be destroyed under irradiation, releasing NH3 and leaving hydrocarbons. These findings enhance our understanding of the photoelectric properties and failure mechanism of MAPbI3, providing potential strategy into material optimization.

physics.app-ph↗

arXiv2021

Simulation of Higher-Order Topological Phases and Related Topological Phase Transitions in a Superconducting Qubit

Higher-order topological phases give rise to new bulk and boundary physics, as well as new classes of topological phase transitions. While the realization of higher-order topological phases has been confirmed in many platforms by detecting the existence of gapless boundary modes, a direct determination of the higher-order topology and related topological phase transitions through the bulk in experiments has still been lacking. To bridge the gap, in this work we carry out the simulation of a two-dimensional second-order topological phase in a superconducting qubit. Owing to the great flexibility and controllability of the quantum simulator, we observe the realization of higher-order topology directly through the measurement of the pseudo-spin texture in momentum space of the bulk for the first time, in sharp contrast to previous experiments based on the detection of gapless boundary modes in real space. Also through the measurement of the evolution of pseudo-spin texture with parameters, we further observe novel topological phase transitions from the second-order topological phase to the trivial phase, as well as to the first-order topological phase with nonzero Chern number. Our work sheds new light on the study of higher-order topological phases and topological phase transitions.

cond-mat.supr-con↗

arXiv2021

Suppressing Coherent Two-Qubit Errors via Dynamical Decoupling

Scalable quantum information processing requires the ability to tune multi-qubit interactions. This makes the precise manipulation of quantum states particularly difficult for multi-qubit interactions because tunability unavoidably introduces sensitivity to fluctuations in the tuned parameters, leading to erroneous multi-qubit gate operations. The performance of quantum algorithms may be severely compromised by coherent multi-qubit errors. It is therefore imperative to understand how these fluctuations affect multi-qubit interactions and, more importantly, to mitigate their influence. In this study, we demonstrate how to implement dynamical-decoupling techniques to suppress the two-qubit analogue of the dephasing on a superconducting quantum device featuring a compact tunable coupler, a trending technology that enables the fast manipulation of qubit--qubit interactions. The pure-dephasing time shows an up to ~14 times enhancement on average when using robust sequences. The results are in good agreement with the noise generated from room-temperature circuits. Our study further reveals the decohering processes associated with tunable couplers and establishes a framework to develop gates and sequences robust against two-qubit errors.

quant-ph↗

arXiv2021

Many-body critical phase: extended and nonthermal

The transition between ergodic phase and many-body localization (MBL) phase lies at the heart in understanding quantum thermalization of many-body systems. Here we predict a many-body critical phase in the one-dimensional extended Aubry-André-Harper-Hubbard model, which is different from both the ergodic phase and MBL phase, implying that the quantum system hosts three different fundamental phases. It is shown that the level statistics in the many-body critical phase are well characterized by the so-called critical statistics, and the wave functions in this phase generally exhibit a multifractal behavior. We further study the half-chain entanglement entropy (EE) and thermalization properties by exact diagonalization, which show that the EE in this critical phase manifest a volume law EE scaling while the many-body states violate the eigenstate thermalization hypothesis. This work unveils a novel many-body phase which is extended but non-ergodic.

cond-mat.dis-nn↗

arXiv2021

Probing quasi-long-range ordering by magnetostriction in monolayer CoPS3

Mermin-Wagner-Coleman theorem predicts no long-range magnetic order at finite temperature in the two-dimensional (2D) isotropic systems, but a quasi-long-range order with a divergent correlation length at the Kosterlitz-Thouless (KT) transition for planar magnets. As a representative of two-dimensional planar antiferromagnets, single-layer CoPS3 carries the promise of monolayer antiferromagnetic platforms for the ultimately thin spintronics. Here, with the aid of magnetostriction which is sensitive to the local magnetic order, we observe the signatured phonon mode splitting of below TKT in monolayer CoPS3, revealing the presence of quasi-long-range ordering in XY-type antiferromagnet. Moreover, the ratio (J'/J) between the interlayer and intralayer interactions, which characterizes the 2D behaviors, is evaluated to be around 0.03 for the first time. Our results provide an efficient method to detect the quasi-long-range antiferromagnetic ordering in the two-dimensional magnets down to monolayer limit.

cond-mat.mes-hall↗

arXiv2020

Measuring the Unique Identifiers of Topological Order Based on Boundary-Bulk Duality and Anyon Condensation

A topological order is a new quantum phase that is beyond Landau's symmetry-breaking paradigm. Its defining features include robust degenerate ground states, long-range entanglement and anyons. It was known that $R$- and $F$-matrices, which characterize the fusion-braiding properties of anyons, can be used to uniquely identify topological order. In this article, we explore an essential question: how can the $R$- and $F$-matrices be experimentally measured? By using quantum simulations based on a toric code model with boundaries and state-of-the-art technology, we show that the braidings, i.e. the $R$-matrices, can be completely determined by the half braidings of boundary excitations due to the boundary-bulk duality and the anyon condensation. The $F$-matrices can also be measured in a scattering quantum circuit involving the fusion of three anyons in two different orders. Thus we provide an experimental protocol for measuring the unique identifiers of topological order.

quant-ph↗

arXiv2020

High-fidelity, high-scalability two-qubit gate scheme for superconducting qubits

High-quality two-qubit gate operations are crucial for scalable quantum information processing. Often, the gate fidelity is compromised when the system becomes more integrated. Therefore, a low-error-rate, easy-to-scale two-qubit gate scheme is highly desirable. Here, we experimentally demonstrate a new two-qubit gate scheme that exploits fixed-frequency qubits and a tunable coupler in a superconducting quantum circuit. The scheme requires less control lines, reduces crosstalk effect, simplifies calibration procedures, yet produces a controlled-Z gate in 30ns with a high fidelity of 99.5%, derived from the interleaved randomized benchmarking method. Error analysis shows that gate errors are mostly coherence limited. Our demonstration paves the way for large-scale implementation of high-fidelity quantum operations.

quant-ph↗

arXiv2020

Theory for the Charge-Density-Wave Mechanism of 3D Quantum Hall Effect

The charge-density-wave (CDW) mechanism of the 3D quantum Hall effect has been observed recently in ZrTe$_5$ [Tang et al., Nature 569, 537 (2019)]. Different from previous cases, the CDW forms on a one-dimensional (1D) band of Landau levels, which strongly depends on the magnetic field. However, its theory is still lacking. We develop a theory for the CDW mechanism of 3D quantum Hall effect. The theory can capture the main features in the experiments. We find a magnetic field induced second-order phase transition to the CDW phase. We find that electron-phonon interactions, rather than electron-electron interactions, dominate the order parameter. We extract the electron-phonon coupling constant from the non-Ohmic I-V relation. We point out a commensurate-incommensurate CDW crossover in the experiment. More importantly, our theory explores a rare case, in which a magnetic field can induce an order-parameter phase transition in one direction but a topological phase transition in other two directions, both depend on one magnetic field.

cond-mat.mes-hall↗

arXiv2020

Dynamic fingerprint of fractionalized excitations in single-crystalline Cu$_3$Zn(OH)$_6$FBr

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized spin excitations. Subject to the strong quantum fluctuations, the spin-1/2 antiferromagnetic system on a kagome lattice is the promising candidate for hosting a QSL ground state, but the structurally ideal realization is rare. Here, we report Raman scattering on the single crystalline Cu$_3$Zn(OH)$_6$FBr, and confirm that the ideal kagome structure remains down to low temperatures without any lattice distortion by the angle-resolved polarized Raman responses and second-harmonic-generation measurements. Furthermore, at low temperatures the Raman scattering reveals a continuum of the spin excitations in Cu$_3$Zn(OH)$_6$FBr, in contrast to the sharp magnon peak in the ordered kagome antiferromagnet EuCu$_3$(OH)$_6$Cl$_3$. Such magnetic Raman continuum, in particular, the substantial low-energy one-pair spinon excitation serves as strong evidence for fractionalized spin excitations in Cu$_3$Zn(OH)$_6$FBr.

cond-mat.str-el↗

arXiv2020

Four-dimensional Vibrational Spectroscopy for Nanoscale Mapping of Phonon Dispersion in BN Nanotubes

Direct measurement of local phonon dispersion in individual nanostructures can greatly advance our understanding of their electrical, thermal, and mechanical properties. However, such experimental measurements require extremely high detection sensitivity and combined spatial, energy and momentum resolutions, thus has been elusive. Here, we develop a four-dimensional electron energy loss spectroscopy (4D-EELS) technique based a monochromated scanning transmission electron microscope (STEM), and present the position-dependent phonon dispersion measurement in individual boron nitride nanotubes (BNNTs). Our measurement shows that the unfolded phonon dispersion of multi-walled BNNTs is close to hexagonal-boron nitride (h-BN) crystals, suggesting that interlayer coupling and curved geometry have no substantial impacts on phonon dispersion. We also find that the acoustic phonons are extremely sensitive to momentum-dependent defect scattering, while optical phonons are much less susceptible. This work not only provides useful insights into vibrational properties of BNNTs, but also demonstrates huge prospects of the developed 4D-EELS technique in nanoscale phonon dispersion measurements.

cond-mat.mes-hall↗

arXiv2020

Creating topological polar structure in a nonpolar matter

Nontrivial topological structures offer rich playground in condensed matter physics including fluid dynamics, superconductivity, and ferromagnetism, and they promise alternative device configurations for post-Moore spintronics and electronics. Indeed, magnetic skyrmions are actively pursued for high-density data storage, while polar vortices with exotic negative capacitance may enable ultralow power consumption in microelectronics. Following extensive investigations on a variety of magnetic textures including vortices, domain walls and skyrmions in the past decades, studies on polar topologies have taken off in recent years, resulting in discoveries of closure domains, vortices, and skyrmions in ferroelectric materials. Nevertheless, the atomic-scale creation of topological polar structures is largely confined in a single ferroelectric system, PbTiO3 (PTO) with large polarization, casting doubt on the generality of polar topologies and limiting their potential applications. In this work, we successfully create previously unrealized atomic-scale polar antivortices in the nominally nonpolar SrTiO3 (STO), expanding the reaches of topological structures and completing an important missing link in polar topologies. The work shed considerable new insight into the formation of topological polar structures, and offers guidance in searching for new polar textures.

cond-mat.mtrl-sci↗

arXiv2020

Experimental realization of phase-controlled dynamics with hybrid digital-analog approach

Quantum simulation can be implemented in pure digital or analog ways, each with their pros and cons. By taking advantage of the universality of a digital route and the efficiency of analog simulation, hybrid digital-analog approaches can enrich the possibilities for quantum simulation. We use a unique hybrid approach to experimentally perform a quantum simulation of phase-controlled dynamics resulting from a closed-contour interaction (CCI) within certain multi-level systems in superconducting quantum circuits. Due to symmetry constraints, such systems cannot host an inherent CCI. Nevertheless, by assembling analog modules corresponding to their natural evolutions and specially designed digital modules constructed from standard quantum logic gates, we can bypass such constraints and realize an effective CCI in these systems. Based on this realization, we demonstrate a variety of related and interesting phenomena, including phase-controlled chiral dynamics, separation of chiral enantiomers, and a new mechanism to generate entangled states based on CCI.

quant-ph↗

arXiv2020

Non-Hermitian coherent coupling of nanomagnets by exchange spin waves

Non-Hermitian physics has recently attracted much attention in optics and photonics. Less explored is non-Hermitian magnonics that provides opportunities to take advantage of the inevitable dissipation of magnons or spin waves in magnetic systems. Here we demonstrate non-Hermitian coherent coupling of two distant nanomagnets by fast spin waves with sub-50 nm wavelengths. Magnons in two nanomagnets are unidirectionally phase-locked with phase shifts controlled by magnon spin torque and spin-wave propagation. Our results are attractive for analog neuromorphic computing that requires unidirectional information transmission.

cond-mat.mes-hall↗

arXiv2020

Pressure-dependent Intermediate Magnetic Phase in Thin Fe$_3$GeTe$_2$ Flakes

We investigated the evolution of ferromagnetism in layered Fe$_3$GeTe$_2$ flakes under different pressures and temperatures using in situ magnetic circular dichroism (MCD) spectroscopy. We found that the rectangle shape of hysteretic loop under an out-of-plane magnetic field sweep can sustain below 7 GPa. Above that pressure, an intermediate state appears at low temperature region signaled by an 8-shaped skew hysteretic loop. Meanwhile, the coercive field and Curie temperature decrease with increasing pressures, implying the decrease of the exchange interaction and the magneto-crystalline anisotropy under pressures. The intermediate phase has a labyrinthine domain structure, which is attributed to the increase of ratio of exchange interaction to magneto-crystalline anisotropy based on Jagla's theory. Moreover, our calculation results reveal a weak structural transition around 6 GPa, which leads to a drop of the magnetic momentum of Fe ions.

cond-mat.mes-hall↗

arXiv2020

Spin wave based tunable switch between superconducting flux qubits

Quantum computing hardware has received world-wide attention and made considerable progress recently. YIG thin film have spin wave (magnon) modes with low dissipation and reliable control for quantum information processing. However, the coherent coupling between a quantum device and YIG thin film has yet been demonstrated. Here, we propose a scheme to achieve strong coupling between superconducting flux qubits and magnon modes in YIG thin film. Unlike the direct $\sqrt{N}$ enhancement factor in coupling to the Kittel mode or other spin ensembles, with N the total number of spins, an additional spatial dependent phase factor needs to be considered when the qubits are magnetically coupled with the magnon modes of finite wavelength. To avoid undesirable cancelation of coupling caused by the symmetrical boundary condition, a CoFeB thin layer is added to one side of the YIG thin film to break the symmetry. Our numerical simulation demonstrates avoided crossing and coherent transfer of quantum information between the flux qubits and the standing spin waves in YIG thin films. We show that the YIG thin film can be used as a tunable switch between two flux qubits, which have modified shape with small direct inductive coupling between them. Our results manifest that it is possible to couple flux qubits while suppressing undesirable cross-talk.

quant-ph↗