arXiv subjects

Dapeng Yu

Publications and source records attributed to Dapeng Yu.

At least 109 records · Page 6Linked to original sources

arXiv2020

Core-level x-ray photoemission and Raman spectroscopy studies on electronic structures in Mott-Hubbard type nickelate oxide NdNiO$_2$

We perform core-level X-ray photoemission spectroscopy (XPS) and electronic Raman scattering studies of electronic structures and spin fluctuations in the bulk samples of the nickelate oxide NdNiO$_2$. According to Nd $3d$ and O $1s$ XPS spectra, we conclude that NdNiO$_2$ has a large transfer energy. From the analysis of the main line of the Ni $2p_{3/2}$ XPS, we confirm the NiO$_2$ planes in NdNiO$_2$ are of Mott-Hubbard type in the Zaanen-Sawatzky-Allen scheme. The two-magnon peak in the Raman scattering provides direct evidence for the strong spin-fluctuation in NdNiO$_2$. The peak position determines the antiferromagnetic exchange $J=25$~meV. Our experimental results agree well with our previous theoretical results.

cond-mat.supr-con↗

arXiv2020

Observation of a thermoelectric Hall plateau in the extreme quantum limit

The thermoelectric Hall effect is the generation of a transverse heat current upon applying an electric field in the presence of a magnetic field. Here we demonstrate that the thermoelectric Hall conductivity $α_{xy}$ in the three-dimensional Dirac semimetal ZrTe$_5$ acquires a robust plateau in the extreme quantum limit of magnetic field. The plateau value is independent of the field strength, disorder strength, carrier concentration, or carrier sign. We explain this plateau theoretically and show that it is a unique signature of three-dimensional Dirac or Weyl electrons in the extreme quantum limit. We further find that other thermoelectric coefficients, such as the thermopower and Nernst coefficient, are greatly enhanced over their zero-field values even at relatively low fields.

cond-mat.mtrl-sci↗

arXiv2020

Quantum Control via Stimulated Raman User-defined Passage

Stimulated Raman adiabatic passage (STIRAP) is a widely-used technique of coherent state-to-state manipulation for many applications in physics, chemistry, and beyond. The adiabatic evolution of the state involved in STIRAP, called adiabatic passage, guarantees its robustness against control errors, but also leads to problems of low efficiency and decoherence. Here we propose and experimentally demonstrate an alternative approach, termed stimulated Raman "user-defined" passage (STIRUP), where a parameterized state is employed for constructing desired evolutions to replace the adiabatic passage in STIRAP. The user-defined passages can be flexibly designed for optimizing different objectives for different tasks, e.g. minimizing leakage error. To experimentally benchmark its performance, we apply STIRUP to the task of coherent state transfer in a superconducting Xmon qutrit. We found that STIRUP completed the transfer more then four times faster than STIRAP with enhanced robustness, and achieved a fidelity of 99.5%, which is the highest among all recent experiments based on STIRAP and its variants. In practice, STIRUP differs from STIRAP only in the design of driving pulses; therefore, most existing applications of STIRAP can be readily implemented with STIRUP.

quant-ph↗

arXiv2020

Realization and detection of non-ergodic critical phases in optical Raman lattice

The critical phases, being delocalized but non-ergodic, are fundamental phases which are different from both the many-body localization and ergodic extended quantum phases, and have so far not been realized in experiment. Here we propose to realize such critical phases with and without interaction based on a topological optical Raman lattice scheme, which possesses one-dimensional spin-orbit coupling and an incommensurate Zeeman potential. We demonstrate the existence of both the noninteracting and many-body critical phases, which can coexist with the topological phase, and show that the critical-localization transition coincides with the topological phase boundary in noninteracting regime. The dynamical detection of the critical phases is proposed and studied in detail. Finally, we demonstrate how the proposed critical phases can be achieved based on the current cold atom experiments. This work paves the way to observe the novel critical phases.

cond-mat.str-el↗

arXiv2019

Chiral spin-wave velocities induced by all-garnet interfacial Dzyaloshinskii-Moriya interaction in ultrathin yttrium iron garnet films

Spin waves can probe the Dzyaloshinskii-Moriya interaction (DMI) which gives rise to topological spin textures, such as skyrmions. However, the DMI has not yet been reported in yttrium iron garnet (YIG) with arguably the lowest damping for spin waves. In this work, we experimentally evidence the interfacial DMI in a 7~nm-thick YIG film by measuring the nonreciprocal spin wave propagation in terms of frequency, amplitude and most importantly group velocities using all electrical spin-wave spectroscopy. The velocities of propagating spin waves show chirality among three vectors, i.e. the film normal direction, applied field and spin-wave wavevector. By measuring the asymmetric group velocities, we extract a DMI constant of 16~$μ$J/m$^{2}$ which we independently confirm by Brillouin light scattering. Thickness-dependent measurements reveal that the DMI originates from the oxide interface between the YIG and garnet substrate. The interfacial DMI discovered in the ultrathin YIG films is of key importance for functional chiral magnonics as ultra-low spin-wave damping can be achieved.

cond-mat.mtrl-sci↗

arXiv2019

Correlating the Electronic Structures of Metallic/Semiconductor MoTe2 Interface to its Atomic Structures

Contact interface properties are important in determining the performances of devices based on atomically thin two-dimensional (2D) materials, especially those with short channels. Understanding the contact interface is therefore quite important to design better devices. Herein, we use scanning transmission electron microscopy, electron energy loss spectroscopy, and first-principles calculations to reveal the electronic structures within the metallic (1T')-semiconducting (2H) MoTe2 coplanar phase boundary across a wide spectral range and correlate its properties and atomic structure. We find that the 2H-MoTe2 excitonic peaks cross the phase boundary into the 1T' phase within a range of approximately 150 nm. The 1T'-MoTe2 crystal field can penetrate the boundary and extend into the 2H phase by approximately two unit cells. The plasmonic oscillations exhibit strong angle dependence, i.e., a red-shift (approximately 0.3 eV-1.2 eV) occurs within 4 nm at 1T'/2H-MoTe2 boundaries with large tilt angles, but there is no shift at zero-tilted boundaries. These atomic-scale measurements reveal the structure-property relationships of 1T'/2H-MoTe2 boundary, providing useful information for phase boundary engineering and device development based on 2D materials.

cond-mat.mtrl-sci↗

arXiv2019

Atomic Origin of Spin-Valve Magnetoresistance at the SrRuO3 Grain Boundary

Defects ubiquitously exist in crystal materials and usually exhibit a very different nature than the bulk matrix, and hence, their presence can have significant impacts on the properties of devices. Although it is well accepted that the properties of defects are determined by their unique atomic environments, the precise knowledge of such relationships is far from clear for most oxides due to the complexity of defects and difficulties in characterization. Here, we fabricate a 36.8° SrRuO3 grain boundary of which the transport measurements show a spin-valve magnetoresistance. We identify its atomic arrangement, including oxygen, using scanning transmission electron microscopy and spectroscopy. Based on the as-obtained atomic structure, the density functional theory calculations suggest that the spin-valve magnetoresistance is because of the dramatically reduced magnetic moments at the boundary. The ability to manipulate magnetic properties at the nanometer scale via defect control allows new strategies to design magnetic/electronic devices with low-dimensional magnetic order.

cond-mat.mtrl-sci↗

arXiv2019

Magnetic Raman continuum in single crystalline H$_3$LiIr$_2$O$_6$

Recently H$_3$LiIr$_2$O$_6$ has been reported as a spin-orbital entangled quantum spin liquid (QSL) [K. Kitagawa et al., Nature {\bf 554}, 341 (2018)], albeit its connection to Kitaev QSL has not been yet identified. To unveil the related Kitaev physics, we perform the first Raman spectroscopy studies on single crystalline H$_3$LiIr$_2$O$_6$ samples. We implement a soft chemical replacement of Li$^+$ with H$^+$ from $α$-Li$_2$IrO$_3$ single crystals to synthesize the single crystal samples of the iridate second generation H$_3$LiIr$_2$O$_6$. The Raman spectroscopy can be used to diagnose the QSL state since the magnetic Raman continuum arises from a process involving pairs of fractionalized Majorana fermionic excitation in a pure Kitaev model. We observe a broad dome-shaped magnetic continuum in H$_3$LiIr$_2$O$_6$, in line with theoretical expectations for the two-spin process in the Kitaev QSL. Our results establish the close connection to the Kitaev QSL physics in H$_3$LiIr$_2$O$_6$.

cond-mat.str-el↗

arXiv2019

Interfacial superconductivity induced by single-quintuple-layer Bi$_2$Te$_3$ on top of FeTe forming van-der-Waals heterostructure

We report the first clear observation of interfacial superconductivity on top of FeTe(FT) covered by one quintuple-layer Bi$_2$Te$_3$(BT) forming van-der-Waals heterojunction. Both transport and scanning tunneling spectroscopy measurements confirm the occurrence of superconductivity at a transition temperature T$_c$ = 13~K, when a single-quintuple-layer BT is deposited on the non-superconducting FT surface. The superconductivity gap decays exponentially with the thickness of BT, suggesting it occurs at the BT-FT interface and the proximity length is above 5-6~nm. We also measure the work function's dependence on the thickness of BT, implying a charge transfer may occur at the BT/FT interface to introduce hole doping into the FT layer, which may serve as a possible candidate for the superconducting mechanism. Our BT/FT heterojunction provides a clean system to study the unconventional interfacial superconductivity.

cond-mat.supr-con↗

arXiv2019

Topological Hall effect in bulk ferromagnet Cr$_2$Te$_3$ embedded with black-phosphorus-like bismuth nanosheets

We implement the molecular beam epitaxy method to embed the black-phosphorus-like bismuth nanosheets into the bulk ferromagnet Cr$_2$Te$_3$. As a typical surfactant, bismuth lowers the surface tensions and mediates the layer-by-layer growth of Cr$_2$Te$_3$. Meanwhile, the bismuth atoms precipitate into black-phosphorus-like nanosheets with the lateral size of several tens of nanometers. In Cr$_2$Te$_3$ embedded with Bi-nanosheets, we observe simultaneously a large topological Hall effect together with the magnetic susceptibility plateau and magnetoresistivity anomaly. As a control experiment, none of these signals is observed in the pristine Cr$_2$Te$_3$ samples. Therefore, the Bi-nanosheets serve as seeds of topological Hall effect induced by non-coplanar magnetic textures planted into Cr$_2$Te$_3$. Our experiments demonstrate a new method to generates a large topological Hall effect by planting strong spin-orbit couplings into the traditional ferromagnet, which may have potential applications in spintronics.

cond-mat.mtrl-sci↗

arXiv2019

Experimental Realization of Nonadiabatic Shortcut to Non-Abelian Geometric Gates

When a quantum system is driven adiabatically through a parametric cycle in a degenerate Hilbert space, the state would acquire a non-Abelian geometric phase, which is stable and forms the foundation for holonomic quantum computation (HQC). However, in the adiabatic limit, the environmental decoherence becomes a significant source of errors. Recently, various non-adiabatic HQC schemes have been proposed, but all at the price of increased sensitivity to control errors. Alternatively, there exist theoretical proposals for speeding up HQC by the technique of "shortcut to adiabaticity" (STA), but no experimental demonstration has been reported so far, as these proprosals involve a complicated control of four energy levels simultaneously. Here we propose and experimentally demonstrate that HQC via shortcut to adiabaticity can be constructed with only three energy levels, using a superconducting qubit in a scalable architecture. With this scheme, all holonomic single-qubit operations can be realized non-adiabatically through a single cycle of state evolution. As a result, we are able to experimentally benchmark the stability of STA+HQC against NHQC in the same platform. The flexibility and simplicity of our scheme makes it also implementable on other systems, such as nitrogen-vacancy center, quantum dots, and nuclear magnetic resonance.

quant-ph↗

arXiv2018

Towards the growth of single-crystal boron nitride monolayer on Cu

Atom-layered hexagonal boron nitride (hBN), with excellent stability, flat surface and large bandgap, has been reported to be the best 2D insulator to open up the great possibilities for exciting potential applications in electronics, optoelectronics and photovoltaics. The ability to grow high-quality large single crystals of hBN is at the heart for those applications, but the size of single-crystal 2D BN is less than a millimetre till now. Here, we report the first epitaxial growth of a 10*10 cm2 single-crystal hBN monolayer on a low symmetry Cu(110) "vicinal surface". The growth kinetics, unidirectional alignment and seamless stitching of hBN domains are unambiguously illustrated using centimetre- to the atomic-scale characterization techniques. The findings in this work are expected to significantly boost the massive applications of 2D materials-based devices, and also pave the way for the epitaxial growth of broad non-centrosymmetric 2D materials.

cond-mat.mtrl-sci↗

arXiv2018

Probing lattice vibration at surface and interface of SiO$_2$/Si with nanometer resolution

Recent advances in monochromatic aberration corrected electron microscopy make it possible to detect the lattice vibration with both high-energy resolution and high spatial resolution. Here, we use sub-10 meV electron energy loss spectroscopy to investigate the local vibrational properties at surface and interface of an amorphous SiO$_2$ (a-SiO$_2$) thin film on Si substrate. We find that each optical mode splits into three sub-modes, i.e., surface mode, bulk mode and interface mode, which can be measured from different locations. The pure surface modes can be measured in the vacuum near the surface, and the pure interface modes are expected to be obtained either at the interface location or in the Si, while inside the SiO$_2$ the measured signal is a mixture of bulk, surface, and interface modes. The bulk mode has the largest vibration energy and surface mode has the lowest. The energy of surface mode is thickness dependent, showing a blue-shift as z-thickness (parallel to fast electron beam) of SiO$_2$ film increases, while the bulk and interface modes have constant vibration energy. The intensity of bulk mode linearly increases with thickness being increased, and it drops steeply to zero near the surface and interface (within a few nanometers). The surface modes decay slowly in the vacuum following a Bessel function. The mechanism of the observed spatially dependent vibration behavior is discussed and quantitatively compared with dielectric response theory analysis. Our nanometer scale measurements of vibrations properties provide useful information about the bonding conditions at the surface and interface and thus may help to design better silicon-based electronic devices via surface and interface treatments

cond-mat.mtrl-sci↗

arXiv2018

V$_5$S$_8$: a Kondo lattice based on intercalation of van der Waals layered transition metal dichalcogenide

Since the discovery of graphene, a tremendous amount of two dimensional (2D) materials have surfaced. Their electronic properties can usually be well understood without considering correlations between electrons. On the other hand, strong electronic correlations are known to give rise to a variety of exotic properties and new quantum phases, for instance, high temperature superconductivity, heavy fermions and quantum spin liquids. The study of these phenomena has been one of the main focuses of condensed matter physics. There is a strong incentive to introduce electronic correlations into 2D materials. Via intercalating a van der Waals layered compound VS$_2$, we show an emergence of a Kondo lattice, an extensively studied strongly correlated system, by magnetic, specific heat, electrical and thermoelectric transport studies. In particular, an exceptionally large Sommerfeld coefficient, 440 mJ$\cdot$K$^{-2}\cdot$mol$^{-1}$, indicates a strong electron correlation. The obtained Kadowaki-Woods ratio, $2.7\times 10^{-6}$ $μΩ\cdot$cm$\cdot$mol$^2\cdot$K$^2\cdot$mJ$^{-2}$, also supports the strong electron-electron interaction. The temperature dependence of the resistivity and thermopower corroborate the Kondo lattice picture. The intercalated compound is one of a few rare examples of $d$-electron Kondo lattices. We further show that the Kondo physics persists in ultra-thin films. This work thus demonstrates a route to generate strong correlations in 2D materials.

cond-mat.mtrl-sci↗

arXiv2018

Quantum carpets from Gaussian sum theory

In many closed quantum systems, an interesting phenomenon, called quantum carpet, can be observed, where the evolution of wave function exhibits a carpet-like pattern. The mechanism of quantum carpet is similar to the classical interference pattern of light. Although the origin of quantum carpets has been studied previously, there are still many interesting details worth exploring. Here, we presented a unified framework for a simultaneous analyzing on three features of quantum carpets, namely full revival, fractional revival and diagonal canal. For fractional revival, a complete formula is presented to explain its generation through "Gaussian sum theory", in which all the essential features, including the phases and amplitudes, of this phenomenon could be captured analytically. Moreover, we also revealed the relations between the interference terms of the diagonal canals and their geometric interpretations, providing a better understanding in the formation of diagonal canals.

quant-ph↗

arXiv2018

Raman evidence for dimerization and Mott collapse in $α$-RuCl$_3$ under pressures

We perform Raman spectroscopy studies on $α$-RuCl$_3$ at room temperature to explore its phase transitions of magnetism and chemical bonding under pressures. The Raman measurements resolve two critical pressures, about $p_1=1.1$~GPa and $p_2=1.7$~GPa, involving very different intertwining behaviors between the structural and magnetic excitations. With increasing pressures, a stacking order phase transition of $α$-RuCl$_3$ layers develops at $p_1=1.1$~GPa, indicated by the new Raman phonon modes and the modest Raman magnetic susceptibility adjustment. The abnormal softening and splitting of the Ru in-plane Raman mode provide direct evidence of the in-plane dimerization of the Ru-Ru bonds at $p_2=1.7$~GPa. The Raman susceptibility is greatly enhanced with pressure increasing and sharply suppressed after the dimerization. We propose that the system undergoes Mott collapse at $p_2=1.7$~GPa and turns into a dimerized correlated band insulator. Our studies demonstrate competitions between Kitaev physics, magnetism, and chemical bondings in Kitaev compounds.

cond-mat.str-el↗

arXiv2018

Imaging nanoscale spatial modulation of a relativistic electron beam with a MeV ultrafast electron microscope

Accelerator-based MeV ultrafast electron microscope (MUEM) has been proposed as a promising tool to study structural dynamics at the nanometer spatial scale and picosecond temporal scale. Here we report experimental tests of a prototype MUEM where high quality images with nanoscale fine structures were recorded with a pulsed 3 MeV picosecond electron beam. The temporal and spatial resolution of the MUEM operating in single-shot mode is about 4 ps (FWHM) and 100 nm (FWHM), corresponding to a temporal-spatial resolution of 4e-19 s*m, about 2 orders of magnitude higher than that achieved with state-of-the-art single-shot keV UEM. Using this instrument we offer the demonstration of visualizing the nanoscale periodic spatial modulation of an electron beam, which may be converted into longitudinal density modulation through emittance exchange to enable production of high-power coherent radiation at short wavelengths. Our results mark a great step towards single-shot nanometer-resolution MUEMs and compact intense x-ray sources that may have wide applications in many areas of science.

physics.acc-ph↗

arXiv2018

Atomic-scale structure and chemistry of YIG/GGG Interface

Y3Fe5O12 (YIG) is a promising candidate for spin wave devices. In the thin film devices, the interface between YIG and substrate may play important roles in determining the device properties. Here, we use spherical aberration-corrected scanning electron microscopy and spectroscopy to study the atomic arrangement, chemistry and electronic structure of the YIG/Gd3Ga5O12 (GGG) interface. We find that the chemical bonding of the interface is FeO-GdGaO and the interface remains sharp in both atomic and electronic structures. These results provide necessary information for understanding the properties of interface and also for atomistic calculation.

cond-mat.mtrl-sci↗