arXiv subjects

David A. Broadway

Publications and source records attributed to David A. Broadway.

At least 19 recordsLinked to original sources

arXiv2026

Magnetic Communication with an Acoustically Actuated Magnetoelectric Resonator and a Quantum Diamond Magnetometer

Wireless communication via propagating magnetic fields is a communication modality that has recently garnered significant interest for short-to-medium range communication in conductive mediums, such as underwater and underground, where existing approaches utilizing electric fields are highly inefficient. Typical implementations of magnetic communication make use of loop antennas as both the transmitter and receiver, with the sensitivity and frequency response scaling with and inversely with the loop cross-sectional area, respectively. Here, we explore an alternative hybrid magnetic communication system consisting of an highly radiation efficient and compact acoustically actuated magnetoelectric resonator as the transmitter, and a highly sensitive micrometer scale quantum magnetometer based on nitrogen-vacancy centers in diamond as the receiver, with their core properties unconstrained by size. We demonstrate amplitude and phase-encoded transmission and reception of AC magnetic fields at $f_{\mathrm{AC}}$ = 20 kHz, achieving a sensitivity of 50 pT/$\sqrt{\mathrm{Hz}}$ and 1.2 mrad/$\sqrt{\mathrm{Hz}}$, respectively. This work establishes the use of hybrid magnetoelectric resonator and quantum diamond magnetometer communication system as a viable alternative to existing loop-based approaches.

cond-mat.mes-hall↗

arXiv2026

Power sensitivity of broadband radiofrequency detectors based on quantum diamond spins

Nitrogen-vacancy (NV) centres in diamond can be used to detect radiofrequency (RF) signals through coupling of the RF magnetic field with the NV spins, combined with optical readout of the spin state. The sensitivity of such RF detectors has so far been mainly studied in terms of magnetic field sensitivity, which is relevant when the RF signal is generated by a near-field source. However, for applications where the RF input is delivered externally, a more relevant quantity is the sensitivity in terms of the input RF power. Here we theoretically analyse the power sensitivity of NV-based RF detectors as a function of the RF-spin interface geometry. We derive scaling laws of the power sensitivity for both slope-detection and variance-detection RF sensing protocols, and for various noise regimes. We find that, in most scenarios, the power sensitivity scales inversely with the characteristic physical dimension of the RF-spin interface, for instance the width of a coplanar waveguide or the diameter of a loop antenna. In other words, the smaller the structure and the probed NV volume, the better the power sensitivity, which is contrary to the case of magnetic field sensitivity. Lastly, we numerically estimate that photon shot noise limited sensitivities of 10^{-20} W Hz^{-1} (slope) and 10^{-12} W Hz^{-1/2} (variance) are achievable. This work lays the groundwork for further optimisation of NV-based RF detectors.

quant-ph↗

arXiv2026

Optical spin defect pairs in cubic boron nitride

Room-temperature optically active solid-state spin defects are widely known to be useful in quantum sensing applications, however, only a select range of materials have been found to host such systems. Recent measurements in the van der Waals material hexagonal boron nitride (hBN) have shown optically detected magnetic resonance (ODMR) with spin-1/2-like signatures can be explained by a charge transfer mechanism where charges move between adjacent defects forming weakly coupled spin pairs. Interestingly, these ODMR signatures have been reported in a variety of materials aside from hBN, suggesting the spin pair model provides a potentially material agnostic approach for enabling ODMR. Here, we test whether the charge transfer mechanism is supported in a different crystal phase, and report on ODMR signatures in cubic boron nitride (cBN), showing all the characteristic properties identified in hBN are preserved. We consider a selection of different cBN samples of varying size and observe ODMR from a single sub-micron cBN particle, paving the way towards sensing applications. This work further expands understanding of the ubiquity of optical spin defect pairs, and establishes the potential for exploring quantum technologies with a wider range of materials.

cond-mat.mes-hall↗

arXiv2026

Real-time Amplitude and Phase Estimation of AC Fields with Diamond Spins

Nitrogen-vacancy centers in diamond have been shown to be capable of detecting AC magnetic fields with high sensitivity, spectral resolution, and spatial resolution. However, most studies so far have focused on the regime of time-averaged or time-correlated measurements, while little attention has been paid to the single-shot regime. Here we show that the amplitude and phase of an AC field can be retrieved from a single pair of two consecutive measurements. We demonstrate this concept by measuring a 4 MHz AC field with a per-shot amplitude and phase sensitivity of 78 nT and 63 mrad, respectively, at a temporal resolution of 320 us. We also investigate the effects and quantify the errors resulting from probe frequency detunings, as well as operating in the strong field regime. Moreover, we showcase the ability of the measurement protocol to dynamically change the probe frequency in real-time. This work advances the use of NV centers for real-time measurements of AC magnetic fields.

cond-mat.mes-hall↗

arXiv2026

Omnidirectional magnetic imaging of magnetic anisotropy and phase transitions

Micron scale imaging of magnetic fields is an important tool for understanding the evolution of magnetism through phase transitions and as a result of interactions inside of heterostructures. However, most imaging platforms, like the nitrogen-vacancy (NV) centre in diamond, are restricted to applying magnetic fields along the quantisation axis of the quantum sensor. This greatly restricts the utility of these systems for exploring materials that emit strong fields or exhibit variable response with respect to the applied field direction. Here we explore an alternative approach using weakly coupled spin-pairs in hBN that exhibit a spin-1/2-like behaviour and an isotropic response to magnetic field. We demonstrate that the spin-pair system can operate in the presence of strong fields from a thin film magnet which were incompatible with NV diamond imaging even with applied fields along the quantisation axis. Further, we demonstrate that using this platform allows for imaging with an arbitrary applied magnetic field direction, allowing us to probe the anisotropy and spin-reorientation transition in the ferrimagnet TbMn$_6$Sn$_6$. Finally, we propose an improved geometry for imaging small anisotropy contributions such as crystalline anisotropy. These results demonstrate how this or similar spin-1/2 systems might be used for imaging magnetic materials that are incompatible with other techniques despite the reduction in sensitivity compared with NV in diamond imaging.

cond-mat.mes-hall↗

arXiv2026

Efficient and Robust p-type Transistor based on Ultra-wide-bandgap Semiconductor

The p-type transistor is an indispensable component of semiconductor technology, enabling complementary operation with n-channel transistors for computation, storage, and communication. Achieving both high robustness and high efficiency is highly desirable but challenging for p-type transistors due to limited semiconductors with reliable hole transport and their high activation energies. Here, we achieved a robust yet efficient p-type transistor by heterogeneously integrating an ultra-wide-bandgap semiconductor and a high-k dielectric layer through van der Waals integration. The p-type transistor employs a two-dimensional hole channel on hydrogenated diamond (bandgap 5.6 eV) combined with a high-k (30.5) SrTiO3 perovskite membrane. At room temperature, the transistor exhibits stable operation with a high on-current (~200 mA/mm), low subthreshold swing (70 mV/dec), high hole mobility (566 cm^2/Vs to 572 cm^2/Vs) and high on-off ratio (~10^9). Furthermore, tuning annealing temperature allows operation in either enhancement or depletion mode. The robust p-type transistor with high efficiency holds great potential for future power electronics, UV optoelectronics, and harsh-environment electronic applications.

cond-mat.mtrl-sci↗

arXiv2025

Spin-dependent photoluminescence in carbon-based quantum dots

The ability to modulate the photoluminescence (PL) of nanomaterials via spin-related effects is vital for many emerging quantum technologies, with nanoscale quantum sensing and imaging being particular areas of focus. Carbon-based quantum dots (CQDs) are among the most common forms of luminescent nanomaterials, appealing due to their ease of synthesis, tunability through organic chemistry, high brightness, and natural biocompatibility. However, the observation of room temperature, spin-dependent PL has remained elusive. Here we report on the observation of PL modulation of CQDs by magnetic fields ($\sim 10$ mT) under ambient conditions. We synthesize a series of CQDs using 19 different amino acids, which have a range of PL emission spectra and exhibit a clear magneto-PL effect (up to $\sim 1$% change). Furthermore, an electron spin resonance is detected in the PL with a g-factor of g $\approx$ 2, suggesting a process similar to the radical pair mechanism is responsible. Finally, we show that the magneto-PL contrast decreases in the presence of paramagnetic species, which we attribute to an increase in magnetic noise-induced spin relaxation in the CQDs. Our work brings new functionalities to these commonly used and biocompatible luminescent nanoparticles, opening new opportunities for in situ quantum sensing and imaging of biological samples.

cond-mat.mes-hall↗

arXiv2025

A scalable method for cavity-enhanced solid-state quantum sensors

Photoluminescent color centers in diamond and hexagonal boron nitride (hBN) are powerful nanoscale solid-state quantum sensors that are explored in a plethora of quantum technologies. Methods for integrating them into macroscopic structures that improve their sensitivity and enable their large-scale deployment are highly sought after. Here, we demonstrate cavity-enhanced photoluminescence (PL) of fluorescent nanodiamonds (FNDs) and hBN nanoparticles (NPs) embedded in polymer-based thin-film optical cavities on the centimeter scale. The cavity resonances efficiently modulate the spectral PL peak position of nitrogen-vacancy (NV) centers in FNDs across the NV PL spectrum and lead to an up to 2.9-fold Purcell-enhancement of the NV PL decay rate. The brightness of hBN NPs increases by up to a factor of three and the PL decay rate is enhanced by up to 13-fold inside the cavities. Finally, we find a 4.8 times improved magnetic field sensitivity of 20 nm FNDs in thin-film cavities due to cavity-enhanced optically detected magnetic resonance contrast and PL brightness. Our study demonstrates a low-cost and scalable method for the fabrication of quantum sensor-doped thin-film cavities, which is an important step toward the development of advanced quantum sensing technologies.

physics.optics↗

arXiv2025

Self-assembled fluorescent nanodiamond layers for quantum imaging

The nitrogen-vacancy (NV) center in diamond is emerging as a powerful tool for imaging magnetic and electric signals at the microscale and below. However, most imaging demonstrations thus far have relied on costly, millimeter-sized bulk diamond substrates, which cannot be easily scaled or integrated with other materials. Here, we report a scalable method for fabricating NV-containing dense and homogenous fluorescent nanodiamond (FND) layers through electrostatic self-assembly and demonstrate the utility of the FND layers for magnetic imaging. We investigate the effect of FND concentration in suspension, substrate immersion time, and solvent pH on the FND density on the substrate. We identify optimized self-assembly conditions that maximize the FND density while minimizing aggregation. Using FND layers on a quartz substrate, we demonstrate magnetic field and magnetic noise imaging at the microscale, based on NV optically detected magnetic resonance magnetometry and T$_1$ relaxometry, respectively. Our results provide a direction for the development of cost-effective and scalable FND layers and surface coatings. This paves the way for on-demand quantum sensing and imaging on a broad range of surfaces based on NV centers and other diamond quantum emitters.

cond-mat.mes-hall↗

arXiv2025

Lateral Exchange Bias for Néel-Vector Control in Atomically Thin Antiferromagnets

Atomically thin van der Waals (vdW) magnets have emerged as a fascinating platform for the exploration of novel physical phenomena arising from their reduced dimensionality and exceptional material properties. Their single-crystalline nature and ultimate miniaturization position them as leading candidates for next-generation spintronic applications. Antiferromagnetic (AF) vdW magnets are of particular interest, as they combine the advantages of vdW magnets with the functionality of AF spintronics, offering unique opportunities for ultrafast and robust spintronic devices. However, the lack of approaches to locally and deterministically manipulate their order parameter -- the Néel-vector -- remains a key limitation. Here, we introduce a fundamentally new paradigm in nanomagnetism, which we term lateral exchange bias (LEB), to achieve Néel vector control in bilayers of the vdW AF CrSBr. We exploit the single-crystalline registry formed by terraced CrSBr samples, where the bilayer Néel vector is controlled by LEB from neighboring, odd-layered flakes, whose nonzero magnetization we manipulate using magnetic fields. Using this control, we achieve nonvolatile manipulation of magnetic domains and domain walls (DWs) in AF CrSBr bilayers, establishing a powerful toolkit for controlling atomically thin AFs at the nanoscale. Our results challenge conventional views on exchange bias and provide a previously unexplored mechanism for achieving atomic-scale control of AFic order. Our findings pave the way for the development of advanced spintronic architectures and quantum technologies based on vdW magnets.

cond-mat.mtrl-sci↗

arXiv2025

A charge transfer mechanism for optically addressable solid-state spin pairs

Optically detected magnetic resonance (ODMR) with no resolvable zero-field splitting has been observed from emitters in hexagonal boron nitride across a broad range of wavelengths, but so far an understanding of their microscopic structure and the physical origin of ODMR has been lacking. Here we perform comprehensive measurements and modelling of the spin-resolved photodynamics of ensembles and single emitters, and uncover a universal model that accounts, and provides an intuitive physical explanation, for all key experimental features. The model, inspired by the radical-pair mechanism from spin chemistry, assumes a pair of nearby point defects -- a primary optically active defect and a secondary defect. Charge transfer between the two defects creates a metastable weakly coupled spin pair with ODMR naturally arising from selection rules. Using first-principle calculations, we show that simple defect pairs made of common carbon defects provide a plausible microscopic explanation. Our optical-spin defect pair (OSDP) model resolves several previously open questions including the asymmetric envelope of the Rabi oscillations, the large variability in ODMR contrast amplitude and sign, and the wide spread in emission wavelength. It may also explain similar phenomena observed in other wide bandgap semiconductors such as GaN. The presented framework will be instrumental in guiding future theoretical and experimental efforts to study and engineer solid-state spin pairs.

cond-mat.mes-hall↗

arXiv2025

Magnetic field imaging with an optical microscope using a quantum diamond sensor add-on

Widefield magnetic imaging using ensembles of nitrogen-vacancy (NV) centres in diamond has emerged as a useful technique for studying the microscopic magnetic properties of materials. Thus far, this technique has mainly been implemented on custom-made optical microscopes. We have developed an add-on for a standard laboratory optical microscope that integrates the NV-diamond sensor and necessary light source, microwave antenna, and bias magnet, enabling NV-based magnetic imaging while retaining the typical optical measurements modes of the microscope. We demonstrate our retrofitted quantum diamond microscope by imaging a magnetic particle sample using brightfield, darkfield, and magnetic imaging modes. Furthermore, we employ an iso-magnetic field imaging technique to visualise the magnetic field of the sample within seconds, and finally demonstrate three-dimensional stray field imaging. Retrofitting existing microscopes exploits the stability and high quality of traditional optical microscope systems while reducing the cost and space requirements of establishing a standalone magnetic imaging system.

cond-mat.mtrl-sci↗

arXiv2024

Reconstruction of non-trivial magnetization textures from magnetic field images using neural networks

Spatial imaging of magnetic stray fields from magnetic materials is a useful tool for identifying the underlying magnetic configurations of the material. However, transforming the magnetic image into a magnetization image is an ill-poised problem, which can result in artefacts that limit the inferences that can be made on the material under investigation. In this work, we develop a neural network fitting approach that approximates this transformation, reducing these artefacts. Additionally, we demonstrate that this approach allows the inclusion of additional models and bounds that are not possible with traditional reconstruction methods. These advantages allow for the reconstruction of non-trivial magnetization textures with varying magnetization directions in thin-film magnets, which was not possible previously. We demonstrate this new capability by performing magnetization reconstructions on a variety of topological spin textures.

cond-mat.mes-hall↗

arXiv2024

Optimized Current Density Reconstruction from Widefield Quantum Diamond Magnetic Field Maps

Quantum Diamond Microscopy using Nitrogen-Vacancy (NV) defects in diamond crystals has enabled the magnetic field imaging of a wide variety of nanoscale current profiles. Intimately linked with the imaging process is the problem of reconstructing the current density, which provides critical insight into the structure under study. This manifests as a non-trivial inverse problem of current reconstruction from noisy data, typically conducted via Fourier-based approaches. Learning algorithms and Bayesian methods have been proposed as novel alternatives for inference-based reconstructions. We study the applicability of Fourier-based and Bayesian methods for reconstructing two-dimensional current density maps from magnetic field images obtained from NV imaging. We discuss extensive numerical simulations to elucidate the performance of the reconstruction algorithms in various parameter regimes, and further validate our analysis via performing reconstructions on experimental data. Finally, we examine parameter regimes that favor specific reconstruction algorithms and provide an empirical approach for selecting regularization in Bayesian methods.

cond-mat.mes-hall↗

arXiv2024

Radiofrequency receiver based on isotropic solid-state spins

Optically addressable solid-state spins have been proposed as robust radiofrequency (RF)-optical transducers sensitive to a specific RF frequency tuned by an external static magnetic field, but often require precise field alignment with the system's symmetry axis. Here we introduce an isotropic solid-state spin system, namely weakly coupled spin pairs in hexagonal boron nitride (hBN), which acts as an RF-optical transducer independent of the direction of the tuning magnetic field, allowing greatly simplified experimental design. Using this platform, we first demonstrate a single-frequency RF receiver with frequency tunability from 0.1 to 19 GHz. We next demonstrate an instantaneous wideband RF spectrum analyser by applying a magnetic field gradient to encode RF frequency into spatial position. Finally, we utilise the spectrum analyser to detect free-space-transmitted RF signals matching the strength and frequency of typical Wi-Fi signals. This work exemplifies the unique capabilities of isotropic spins in hBN to operate as RF sensors, while circumventing the challenging requirement of precisely aligned magnetic fields facing conventional solid-state spins.

cond-mat.mes-hall↗

arXiv2024

Violet to near-infrared optical addressing of spin pairs in hexagonal boron nitride

Optically addressable solid-state spins are an important platform for practical quantum technologies. Van der Waals material hexagonal boron nitride (hBN) is a promising host as it contains a wide variety of optical emitters, but thus far observations of addressable spins have been sparse, and most of them lacked a demonstration of coherent spin control. Here we demonstrate robust optical readout of spin pairs in hBN with emission wavelengths spanning from violet to the near-infrared. We find these broadband spin pairs exist naturally in a variety of hBN samples from bulk crystals to powders to epitaxial films, and can be coherently controlled across the entire wavelength range. Furthermore, we identify the optimal wavelengths for independent readout of spin pairs and boron vacancy spin defects co-existing in the same sample. Our results establish the ubiquity of the optically addressable spin pair system in hBN across a broad parameter space, making it a versatile playground for spin-based quantum technologies.

cond-mat.mes-hall↗

arXiv2024

Imaging strain-controlled magnetic reversal in thin CrSBr

Two-dimensional materials are extraordinarily sensitive to external stimuli, making them ideal for studying fundamental properties and for engineering devices with new functionalities. One such stimulus, strain, affects the magnetic properties of the layered magnetic semiconductor CrSBr to such a degree that it can induce a reversible antiferromagnetic-to-ferromagnetic phase transition. Given the pervasiveness of non-uniform strain in exfoliated two-dimensional magnets, it is crucial to understand its impact on their magnetic behavior. Using scanning SQUID-on-lever microscopy, we directly image the effects of spatially inhomogeneous strain on the magnetization of layered CrSBr as it is polarized by a field applied along its easy axis. The evolution of this magnetization and the formation of domains is reproduced by a micromagnetic model, which incorporates the spatially varying strain and the corresponding changes in the local interlayer exchange stiffness. The observed sensitivity to small strain gradients along with similar images of a nominally unstrained CrSBr sample suggest that unintentional strain inhomogeneity influences the magnetic behavior of exfoliated samples and must be considered in the design of future devices.

cond-mat.mes-hall↗

arXiv2024

Current Induced Hidden States in Josephson Junctions

Josephson junctions enable dissipation-less electrical current through metals and insulators below a critical current. Despite being central to quantum technology based on superconducting quantum bits and fundamental research into self-conjugate quasiparticles, the spatial distribution of super current flow at the junction and its predicted evolution with current bias and external magnetic field remain experimentally elusive. Revealing the hidden current flow, featureless in electrical resistance, helps understanding unconventional phenomena such as the nonreciprocal critical current, i.e., Josephson diode effect. Here we introduce a platform to visualize super current flow at the nanoscale. Utilizing a scanning magnetometer based on nitrogen vacancy centers in diamond, we uncover competing ground states electrically switchable within the zero-resistance regime. The competition results from the superconducting phase re-configuration induced by the Josephson current and kinetic inductance of thin-film superconductors. We further identify a new mechanism for the Josephson diode effect involving the Josephson current induced phase. The nanoscale super current flow emerges as a new experimental observable for elucidating unconventional superconductivity, and optimizing quantum computation and energy-efficient devices.

cond-mat.mes-hall↗