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David Sarkisyan

Publications and source records attributed to David Sarkisyan.

At least 37 records · Page 2Linked to original sources

Selective reflection from a Potassium atomic layer with a thickness as small as $λ/13$

We demonstrate that a method using the derivative of the selective reflection signal from a nanocell is a convenient and robust tool for atomic laser spectroscopy, achieving a nearly Doppler-free spectral resolution. The recorded linewidth of the signal from a potassium-filled cell, whose thickness $\ell$ lies in the range $350-500$ nm, is 18 times smaller than the Doppler linewidth ($\sim 900$ MHz full width at half maximum) of potassium atoms. We also show experimentally a sign oscillation of the reflected signal's derivative with a periodicity of $λ/2$ when $\ell$ varies from 190 to 1200~nm confirming the theoretical prediction. We report the first measurement of the van der Waals atom-surface interaction coefficient $C_3 = 1.9\pm 0.3$ kHz$\cdotμ$m$^3$ of potassium $4S_{1/2} \rightarrow 4P_{3/2}$ transitions with the nanocell's sapphire windows, demonstrating the usefulness and convenience of the derivative of selective reflection technique for cell thicknesses in the range $60 -120~$nm.

physics.atom-ph↗

Dark resonance formation with magnetically-induced transitions: extension of spectral range and giant circular dichroism

Dark resonances were formed via electromagnetically induced transparency for the first time involving magnetically-induced $ΔF = \pm2$ atomic transitions of alkali metal atom, which are forbidden at zero magnetic field. The probability of these transitions undergoes rapid growth when $300 - 3000$~G magnetic field is applied, allowing formation of dark resonances, widely tunable in the GHz range. It is established that for $ΔF = +2$ ($ΔF =-2$) transition, the coupling laser tuned to $ΔF = +1$ ($ΔF =-1$) transition of the hyperfine $Λ$-system must be $σ^+$ ($σ^-$) polarized, manifesting anomalous circular dichroism.

physics.atom-ph↗

Study of EIT resonances in an anti-relaxation coated Rb vapor cell

We demonstrate---experimentally and theoretically---that resonances obtained in electromagnetically induced transparency (EIT) can be both bright and dark. The experiments are done using magnetic sublevels of a hyperfine transition in the D$_1$ line of $^{87}$Rb. The degeneracy of the sublevels is removed by having a magnetic field of value 27 G. The atoms are contained in a room-temperature vapor cell with anti-relaxation coating on the walls. Theoretical analysis based on a two-region model reproduces the experimental spectrum quite well. This ability to have both bright and dark resonances promises applications in sub- and super-luminal propagation of light, and sensitive magnetometry.

physics.atom-ph↗

Hyperfine Paschen-Back regime of Potassium D$_2$ line observed by Doppler-free spectroscopy

Selective reflection of a laser radiation from an interface formed by a dielectric window and a potassium atomic vapour confined in a nano-cell with $350~$nm gap thickness is implemented for the first time to study the atomic transitions of K D$_2$ line in external magnetic fields. In moderate $B$-fields, there are 44 individual Zeeman transitions which reduce to two groups (one formed by $σ^+$ the other one by $σ^-$ circularly-polarised light), each containing eight atomic transitions, as the magnetic field increases. Each of these groups contains one so-called "guiding" transition whose particularities are to have a probability (intensity) as well as a frequency shift slope (in MHz/G) that are constant in the whole range of $0 - 10~$kG magnetic fields. In the case of $π$-polarised laser radiation, among eight transitions two are forbidden at $B = 0$, yet their probabilities undergo a giant modification under the influence of a magnetic field. We demonstrate that for $B$-fields $> 165~$G a complete hyperfine Paschen-Back regime is observed. Other peculiarities of K D$_2$ line behaviour in magnetic field are also presented. We show a very good agreement between theoretical calculations and experiments. The recording of the hyperfine Paschen-Back regime of K D$_2$ line with high spectral resolution is demonstrated for the first time.

physics.atom-ph↗

Selective reflection from Rb layer with thickness below $λ$/12 and applications

We have studied the peculiarities of selective reflection from Rb vapor cell with thickness $L <$ 70 nm, which is over an order of magnitude smaller than the resonant wavelength for Rb atomic D$_1$ line $λ$ = 795 nm. A huge ($\approx$ 240 MHz) red shift and spectral broadening of reflection signal is recorded for $L =$ 40 nm caused by the atom-surface interaction. Also completely frequency resolved hyperfine Paschen-Back splitting of atomic transitions to four components for $^{87}$Rb and six components for $^{85}$Rb is recorded in strong magnetic field ($B >$ 2 kG).

physics.atom-ph↗

Decoupling of hyperfine structure of Cs $D_1$ line in strong magnetic field studied by selective reflection from a nanocell

Decoupling of total electronic and nuclear spin moments of Cs atoms in external magnetic field for the case of atomic $D_1$ line, leading to onset of the hyperfine Paschen-Back regime has been studied theoretically and experimentally. Selective reflection of laser radiation from an interface of dielectric window and atomic vapor confined in a nanocell with 300 nm gap thickness was implemented for the experimental studies. The real time derivative of selective reflection signal with a frequency position coinciding with atomic transitions was used in measurements, providing $\sim$ 40 MHz spectral resolution and linearity of signal response in respect to transition probability. Behavior of 28 individual Zeeman transitions in a wide range of longitudinal magnetic field (0 - 6 kG) has been tracked under excitation of Cs vapor by a low-intensity $σ^+$- polarized cw laser radiation. For $B\ge 6~$kG, only 8 transitions with nearly equal probabilities and the same frequency slope remained in the spectrum, which is a manifestation of the hyperfine Paschen-Back regime. The obtained experimental results are consistent with numerical modeling. Due to small divergence of selective reflection signal, as well as sub-wavelength thickness and sub-Doppler spectral linewidth inherent to nanocell, the employed technique can be used for distant remote sensing of magnetic field with high spatial and $B$-field resolution.

physics.atom-ph↗

Active narrowband filtering, line narrowing and gain using ladder electromagnetically induced transparency in an optically thick atomic vapour

Electromagnetically induced transparency (EIT) resonances using the $5\rm{S}_{1/2}\rightarrow5\rm{P}_{3/2}\rightarrow5\rm{D}_{5/2}$ ladder-system in optically thick Rb atomic vapour are studied. We observe a strong line narrowing effect and gain at the $5\rm{S}_{1/2}\rightarrow5\rm{P}_{3/2}$ transition wavelength due to an energy-pooling assisted frequency conversion with characteristics similar to four-wave mixing. As a result it is possible to observe tunable and switchable transparency resonances with amplitude close to $100\%$ and a linewidth of 15 MHz. In addition, the large line narrowing effect allows resolution of $^{85}$Rb $5\rm{D}_{5/2}$ hyperfine structure even in the presence of strong power broadening.

physics.atom-ph↗

Three-photon electromagnetically induced transparency using Rydberg states

We demonstrate electromagnetically induced transparency (EIT) in a four-level cascade system where the upper level is a Rydberg state. The observed spectral features are sub-Doppler and can be enhanced due to the compensation of Doppler shifts with AC Stark shifts. A theoretical description of the system is developed which agrees well with the experimental results and an expression for the optimum parameters is derived.

physics.atom-ph↗

N -resonances in a buffered micrometric Rb cell: splitting in a strong magnetic field

N -resonances excited in rubidium atoms confined in micrometric-thin cells with variable thickness from 1 μm to 2 mm are studied experimentally for the cases of a pure Rb atomic vapor and of a vapor with neon buffer gas. Good contrast and narrow linewidth were obtained for thicknesses as low as 30 μm. The higher amplitude and sharper profile of N-resonances in the case of a buffered cell was exploited to study the splitting of the 85Rb D1 N-resonance in a magnetic field of up to 2200 G. The results are fully consistent with the theory. The mechanism responsible for forming N-resonances is discussed. Possible applications are addressed.

physics.atom-ph↗

The cooperative Lamb shift in an atomic nanolayer

We present an experimental measurement of the cooperative Lamb shift and the Lorentz shift using an atomic nanolayer with tunable thickness and atomic density. The cooperative Lamb shift arises due to the exchange of virtual photons between identical atoms. The interference between the forward and backward propagating virtual fields is confirmed by the thickness dependence of the shift which has a spatial frequency equal to $2k$, i.e. twice that of the optical field. The demonstration of cooperative interactions in an easily scalable system opens the door to a new domain for non-linear optics.

physics.atom-ph↗

Optical transmission through a dipolar layer

The interaction between light and matter is fundamental to developments in quantum optics and information. Over recent years enormous progress has been made in controlling the interface between light and single emitters including ions, atoms, molecules, quantum dots and ensembles. For many systems, inter-particle interactions are typically negligible. However, if the emitters are separated by less than the emission wavelength, resonant dipole--dipole interactions modify the radiative decay rate and induce a splitting or shift of the resonance. Here we map out the transition between individual dipoles and a strongly interacting ensemble by increasing the density of atoms confined in a layer with thickness much less than the emission wavelength. We find two surprising results: whereas for a non-interacting ensemble the opacity increases linearly with atomic density, for an interacting ensemble the opacity saturates, i.e., a thin dipolar layer never becomes opaque regardless of how many scatterers are added. Secondly, the relative phase of the dipoles produces an abrupt change in the optical transmission around the thickness λ/4.

physics.atom-ph↗

High contrast D$_{1}$ line electromagnetically induced transparency in nanometric-thin rubidium vapor cell

Electromagnetically induced transparency (EIT) on atomic D$_{1}$ line of rubidium is studied using a nanometric-thin cell with atomic vapor column length in the range of L= 400 - 800 nm. It is shown that the reduction of the cell thickness by 4 orders as compared with an ordinary cm-size cell still allows to form an EIT resonance for $L= λ$ ($λ=794$ nm) with the contrast of up to 40%. Remarkable distinctions of EIT formation in nanometric-thin and ordinary cells are demonstrated. Despite the Dicke effect of strong spectral narrowing and increase of the absorption for $L=$ $λ/2$, EIT resonance is observed both in the absorption and the fluorescence spectra for relatively low intensity of the coupling laser. Well resolved splitting of the EIT resonance in moderate magnetic field for $L=$ $λ$ can be used for magnetometry with nanometric spatial resolution. The presented theoretical model well describes the observed results.

physics.atom-ph↗

Effect of buffer gas on electromagnetically induced transparency in a ladder system using thermal rubidium vapor

We report on the first observation of electromagnetically induced transparency (EIT) in a ladder system in the presence of a buffer gas. In particular we study the 5S1/2 - 5P3/2 - 5D5/2 transition in thermal rubidium vapor with a neon buffer gas at a pressure of 6 Torr. In contrast to the line narrowing effect of buffer gas on Λ-systems we show that the presence of the buffer gas leads to an additional broadening of (32 +/- 5) MHz, which suggests a cross section for Rb(5D5/2)-Ne of σ = (7 +/- 1) x 10-19 m2. However, in the limit where the coupling Rabi frequency is larger than k the collisional dephasing a strong transparency feature can still be observed.

physics.atom-ph↗

A method for the quantitative study of atomic transitions in a magnetic field based on an atomic vapor cell with L=lambda

We describe the so-called "Lambda-Zeeman method" to investigate individual hyperfine transitions between Zeeman sublevels of atoms in an external magnetic field of 0.1 mT - 0.25 T. Atoms are confined in a nanocell with thickness L = Lambda, where Lambda is the resonant wavelength (794 nm or 780 nm for D1 or D2 line of Rb). Narrow resonances in the transmission spectrum of the nanocell are split into several components in a magnetic field; their frequency positions and probabilities depend on the B-field. Possible applications are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references.

physics.atom-ph↗

Selective reflection spectroscopy of a vapour at a calcium fluoride interface

Fluoride materials exhibit surface resonances located in the thermal infrared. This makes them interesting to search for a fundamental temperature dependence of the atom-surface interaction, originating in the near-field thermal emissivity of the surface. Preliminary selective reflection experiments performed on a special Cs vapour cell that includes a CaF2 interface show a temperature dependence, yet to be analyzed

physics.atom-ph↗

Selective Reflection Spectroscopy at the Interface between a Calcium Fluoride Window and Cs Vapour

A special vapour cell has been built, that allows the measurement of the atom-surface van der Waals interaction exerted by a CaF2 window at the interface with Cs vapour. Mechanical and thermal fragility of fluoride windows make common designs of vapour cells unpractical, so that we have developed an all-sapphire sealed cell with an internal CaF2 window. Although impurities were accidentally introduced when filling-up the prototype cell, leading to a line-broadening and shift, the selective reflection spectrum on the Cs D1 line (894 nm) makes apparent the weak van der Waals surface interaction. The uncertainties introduced by the effects of these impurities in the van der Waals measurement are nearly eliminated when comparing the selective reflection signal at the CaF2 interface of interest, and at a sapphire window of the same cell. The ratio of the interaction respectively exerted by a sapphire interface and a CaF2 interface is found to be 0.55 $\pm$ 0.25, in good agreement with the theoretical evaluation of ~0.67.

physics.atom-ph↗

Exploring the van der Waals Atom-Surface attraction in the nanometric range

The van der Waals atom-surface attraction, scaling as C3 z-3 for z the atom-surface distance, is expected to be valid in the distance range 1-1000 nm, covering 8-10 orders of magnitudes in the interaction energy. A Cs vapour nanocell allows us to analyze the spectroscopic modifications induced by the atom-surface attraction on the 6P3/2->6D5/2 transition. The measured C3 value is found to be independent of the thickness in the explored range 40-130 nm, and is in agreement with an elementary theoretical prediction. We also discuss the specific interest of exploring short distances and large interaction energy.

physics.atom-ph↗

Laser spectroscopy with nanometric gas cells : distance dependence of atom-surface interaction and collisions under confinement

The high sensitivity of Laser Spectroscopy has made possible the exploration of atomic resonances in newly designed "nanometric" gas cells, whose local thickness varies from 20nm to more than 1000 nm. Following the initial observation of the optical analogous of the coherent Dicke microwave narrowing, the newest prospects include the exploration of long-range atom surface van der Waals interaction with spatial resolution in an unprecedented range of distances, modification of atom dielectric resonant coupling under the influence of the coupling between the two neighbouring dielectric media, and even the possible modification of interatomic collisions processes under the effect of confinement.

physics.atom-ph↗