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Dawei Shen

Publications and source records attributed to Dawei Shen.

At least 37 records · Page 2Linked to original sources

Contrasting Momentum-Selective Spin-Density-Wave Gaps in Bilayer and Trilayer Nickelates

Resolving where the density-wave gap opens in momentum space is essential for identifying the microscopic origin of the instability in layered nickelates. Using polarization-resolved electronic Raman scattering, we map the momentum selectivity of the spin-density-wave (SDW) gap in trilayer La4Ni3O10. We observe a SDW-induced redistribution of spectral weight on both the $α$ pocket at the Brillouin-zone centre and a portion of the $β$ pocket near the zone boundary, characterized by gap energies of approximately 55~meV. In contrast, no comparable spectral weight suppression is observed along the diagonal region of $β$ pockets, implying little or no gap opening. This gap topology contrasts sharply with that in La3Ni2O7, where anisotropic SDW gaps open solely on the $β$ pocket. Our results establish a distinct momentum-space gap topology between bilayer and trilayer nickelates, placing new constraints on the ordering wave vector and the mechanism of the density-wave instability relevant to superconductivity.

cond-mat.supr-con↗

Unusual Dual Flat Bands and two-dimensional Dirac-node Arc State in Kagome Metal Ni3In2S2

Kagome materials are at the frontier of condensed matter physics. An ideal kagome lattice features only one geometrically frustrated flat band spanning the entire momentum space and a single Dirac cone at the Brillouin-zone corners. However, for the first time, here we observe unusual flat-band and Dirac physics in the newly discovered "322" kagome material Ni3In2S2 by combining high-resolution synchrotron- and laser-based angle-resolved photoemission spectroscopy with a micro-focused beam, scanning tunneling microscopy, and first-principles calculations. We resolve two distinct electronic flat-band states located in close proximity to the Fermi level: a robust Topological Surface Flat Band at ~40 meV below the Fermi level on the Sulfur-terminated surface, originating from weak topological insulator states, and a kagome lattice-derived flat band at ~100 meV binding energy with an ultranarrow bandwidth (~5 meV). Instead of the single Dirac cone, the Indium-terminated surface hosts a rare two-dimensional Dirac-node arc state, where the gapless Dirac nodes extend along an open one-dimensional line crossing the Brillouin-zone boundary, exhibiting sharp linear dispersion, exceptionally high Fermi velocity, and pronounced circular dichroism. These findings establish Ni3In2S2 as a unique topological kagome metal in which multiple flat-band states of different physical origin coexist with an unusual Dirac-node arc, opening an avenue for discovering flat-band--driven and topology-enabled quantum phenomena.

cond-mat.mtrl-sci↗

Absence of magnetic order in epitaxial RuO2 revealed by X-ray linear dichroism

Recently, the topic of altermagnetism has attracted tremendous attention and RuO2 have been demonstrated to be one of the most promising altermagnetic candidates. However, disputes still remain on the existence of magnetic order in RuO2. Here in this work, we employ X-ray linear dichroism (XLD), a widely utilized technique for characterizing antiferromagnets, in conjunction with photoemission electron microscopy and multiple scattering calculation to provide clear evidence of the absence of magnetic order in epitaxial RuO2 films. The observed XLD signal is nearly invariant with temperature and independent on cooling field direction, in stark contrast to the substantial magnetic order-related XLD signal predicted by multiple scattering calculation. This finding strongly suggests a nonmagnetic origin for RuO2. Furthermore, we observed significantly distinct XLD signals at the Ru M3 and O K edges in RuO2 films grown on TiO2 substrate with different surface orientations, which can be attributed to the low-symmetry crystal field. These results unequivocally demonstrate the absence of magnetic order in RuO2 and establishes XLD measurement as a robust technique for probing the low-symmetry magnetic materials.

cond-mat.mtrl-sci↗

Cauchy Data for Formation of Multiple Black Holes with Prescribed ADM Parameters

We give a simple construction of smooth, asymptotically flat vacuum initial data modeling a relativistic collapsing $N$--body system, with independently prescribed ADM energy, linear momentum, and angular momentum for each component, subject to the timelike condition $\E>|¶|$. The initial data contain no trapped surfaces, and the future development contains multiple causally independent trapped regions that dynamically form from localized subsets of the initial slice. In particular, the maximal development of data with well-separated collapsing components and relative motion is expected to yield spacetimes containing multiple black holes.

gr-qc↗

Cauchy data for multiple collapsing boson stars

We construct Cauchy initial data for the Einstein-Maxwell-Klein-Gordon (EMKG) system, which evolves in finite time into spacetimes containing multiple trapped surfaces. From a physical perspective, this corresponds to preparing multiple well-separated boson stars, each of which collapses to form a spacelike black hole region. In particular, this extends the result of the second and third named authors on the formation of multiple trapped surfaces in vacuum to the EMKG system.

gr-qc↗

Many-body electronic structure in pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7

The pyrochlore lattice materials can exhibit geometrical frustration, while the related many-body electronic states remain elusive. In this work, we performed scanning tunneling microscopy measurements on the pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7 at 0.3 K. For the first time, we obtained atomically resolved images of their (111) surfaces, revealing a hexagonal lattice or a kagome lattice. Tunneling spectroscopy in CsBi2 reveals a nearly fully opened superconductivity gap. The ratio of 2Δ/kBTC = 4.7 suggests relatively strong coupling superconductivity, as compared with that in kagome superconductors AV3Sb5 (A = K, Rb, Cs). In contrast to the previous study categorizing CsBi2 as a type-I superconductor, the applied magnetic field induces a hexagonal vortex lattice in which each vortex core exhibits an intriguing three-fold symmetry state. In Pr2Ir2O7, we observed a spatially homogeneous Kondo-lattice resonance, which is compared with that in the kagome Kondo-lattice material CsCr6Sb6. We further discover that the Kondo resonance exhibits a spatial modulation with three-fold symmetry, and the applied magnetic field induces a Zeeman splitting of the Kondo resonance with intriguing atomic site dependence. We discuss the relations of these many-body electronic phenomena with the pyrochlore lattice geometry and its charge or spin frustration. Our systematic observations offer atomic-scale insights into the many-body electronic structures of the geometrically frustrated pyrochlore superconductors and spin liquids.

cond-mat.str-el↗

Surface reconstruction and orthogonal decoupling in SrAl4 and EuAl4

Surface-induced symmetry breaking in quantum materials can stabilize exotic electronic phases distinct from those in the bulk, yet its momentum-space manifestations remain elusive due to domain-averaging effects. Here, using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy (STM), we present a microscopic investigation of the electronic structures of SrAl4 and EuAl4, layered tetragonal intermetallic compounds that exhibit well-characterized incommensurate charge-density-wave (CDW) transitions. Below the CDW transition temperatures, we uncover linearly dispersing electronic states and pronounced unidirectional replica bands orthogonal to the bulk CDW wave vector, evidencing the emergence of an in-plane C4 symmetry-breaking electronic order that is not dictated by the bulk incommensurate CDW. STM measurements further reveal a 1 times 2 surface reconstruction with quasi-one-dimensional modulations and half-unit-cell steps, traced to ordered 50 percent Sr/Eu vacancies, which vanish irreversibly upon thermal cycling, indicating decoupled surface and bulk orders. These findings establish SrAl4 and EuAl4 as model platforms for exploring surface-confined nematicity and emergent low-dimensional phases in quantum materials.

cond-mat.mtrl-sci↗

Stability of Big Bang singularity for the Einstein-Maxwell-scalar field-Vlasov system in the full strong sub-critical regime

In $3+1$ dimensions, we study the stability of Kasner solutions for the Einstein-Maxwell-scalar field-Vlasov system. This system incorporates gravity, electromagnetic, weak and strong interactions for the initial stage of our universe. Due to the presence of the Vlasov field, various new challenges arise. By observing detailed mathematical structures and designing new delicate arguments, we identify a new strong sub-critical regime and prove the nonlinear stability with Kasner exponents lying in this full regime. This extends the result of Fournodavlos-Rodnianski-Speck [8] from the Einstein-scalar field system to the physically more complex system with the Vlasov field.

gr-qc↗

Observation of superconductivity-induced leading-edge gap in Sr-doped $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films

The discovery of high-temperature superconductivity in pressurized bulk $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ has ignited significant interest in nickelate superconductors. Unlike cuprates, where superconductivity predominantly originates from the $\mathrm{3}d_{x^2-y^2}$ orbital, nickelates exhibit additional complexities involving contributions from the $\mathrm{3}d_{z^2}$ orbital, prompting fundamental questions about their pairing mechanisms. Despite recent progress in stabilizing superconductivity in $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films at ambient pressure, direct spectroscopic evidence of the superconducting gap opening remains elusive. Here, we present an in-situ angle-resolved photoemission spectroscopy study of Sr-doped superconducting $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films. Fermi surface mapping reveals Ni-$\mathrm{3}d_{x^2-y^2}$-derived $α$ and $β$ pockets, with orbital fillings of 0.11$\pm$0.02 electrons and 0.66$\pm$0.03 holes per Ni, respectively, resulting in a total of 0.45$\pm$0.04 electrons for each Ni. These bands exhibit moderate electron correlations, characterized by a band renormalization factor of 3-4. Notably, both $α$ and $β$ bands exhibit leading-edge shifts across the superconducting transition, with gap magnitude of ~1-2 meV at Fermi momenta along the Brillouin zone diagonal and slightly away from the zone diagonal, deviating from the conventional $d_{x^2-y^2}$-wave gap structure. Additionally, the Ni-$\mathrm{3}d_{z^2}$-derived $γ$ band lies ~75 meV below the Fermi level, indicating a $\mathrm{3}d_{x^2-y^2}$-dominated fermiology in this compound.

cond-mat.supr-con↗

Formation of multiple Black Holes from Cauchy data

We construct a family of asymptotically flat Cauchy initial data for the Einstein vacuum equations that contain no trapped surfaces, yet whose future development admits multiple causally independent trapped surfaces. Assuming the weak cosmic censorship conjecture, this implies the formation of multiple black holes in finite time. The initial data are obtained by surgically modifying a vacuum geometrostatic manifold equipped with the Brill-Lindquist metric: the data agree exactly with the Brill-Lindquist metric outside a collection of balls centered at its multiple poles, and each ball is replaced by a constant-time slice of a well-prepared dynamical spacetime. The construction is based on Christodoulou's short-pulse framework, a stability analysis in the finite future of the short-pulse region, the geometry of geometrostatic manifolds with small mass and large separation, and the obstruction-free annular gluing method developed by Mao-Oh-Tao. The absence of trapped surfaces in the initial data is verified via a standard mean curvature comparison argument.

gr-qc↗

Unconventional band splitting of CeSb in the devil's staircase transition

The interplay between magnetism and electronic band structure is a central theme in condensed matter physics. CeSb, with its complex devil's staircase antiferromagnetic transition, offers a unique opportunity to explore this interplay. Using angle-resolved photoemission spectroscopy (ARPES), we investigate the electronic structure evolution across the devil's staircase transition. Upon entering the antiferromagnetic phase, we observe an intriguing band splitting of the electron pocket around the X point. The energy separation between the split bands changes abruptly with temperature, consistent with the characteristics of the first-order phase transition. However, their respective spectral weights behave gradually with temperature. Combined with our density functional theory (DFT) calculations, we suggest that this atypical behavior deviates from conventional magnetically induced band splitting and potentially arises from the intricate modulation of paramagnetic and antiferromagnetic layers within the devil's staircase transition. Our results provide insights into the complex relationship between electronic structure and magnetism in correlated electron systems.

cond-mat.str-el↗

Formation of trapped surfaces for the Einstein--Maxwell--charged scalar field system

In this paper, we prove a scale-critical trapped surface formation result for the Einstein--Maxwell--charged scalar field (EMCSF) system, without any symmetry assumptions. Specifically, we establish a scale-critical semi-global existence theorem from past null infinity and show that the focusing of gravitational waves, the concentration of electromagnetic fields, or the condensation of complex scalar fields, each individually, can lead to the formation of a trapped surface. In addition, we capture a nontrivial charging process along past null infinity, which introduces new difficulties due to the abnormal behavior of the matter fields. Nevertheless, the semi-global existence result and the formation of a trapped surface remain valid.

math.AP↗

Revealing nanoscale structural phase separation in La$_{3}$Ni$_{2}$O$_{7-δ}$ single crystal via scanning near-field optical microscopy

The discovery of superconductivity in La3Ni2O7-$δ$ under high pressure,with an onset critical temperature around 80 K, has sparked significant interest in the superconducting phases of Ruddlesden-Popper nickelates, Lan+1NinO3n+1. While La4Ni3O10 exhibits nearly 100% superconductivity with Tc~30 K under high pressure, magnetic susceptibility studies on La3Ni2O7-$δ$, however, reveal a more complex picture, indicating either filamentary superconductivity or that approximately 50% of crystal phase becomes superconducting in polycrystalline samples. In this study, we employed scattering-type scanning near-field optical microscopy to visualize nanoscale structural phase separation in La3Ni2O7-$δ$, identifying enhanced optical conductivity with stripes approximately 183 nm wide. These stripes run diagonally with respect to the Ni-O-Ni bond directions in the a-b plane, ruling out the possibility that they arise from impurity phases, like the '1313', '214' or '4310' structures. The dark regions and bright stripes exhibit optical conductivities ~ 22% and 29% of gold's, respectively. Additionally, we find that the bright stripes constitute about 38% of the total field of view, while the remainder consists of dark regions and the transitional region between dark regions and bright stripes. Our results suggest that optical conductivity stripes originate from nanoscale structural phase separation. In contrast, La4Ni3O10 exhibits uniform and higher optical conductivity with no observable evidence of phase separation. Thus, our study represents a pioneering effort to directly image nanoscale phase separation in Lan+1NinO3n+1 nickelates. This observation could provide crucial insights into the factors that limit the superconducting volume fraction of La3Ni2O7-$δ$, highlighting SNOM as a powerful probe for exploring nanoscale low-energy physics in correlated quantum materials.

cond-mat.supr-con↗

Observation of multiple surface states in naturally cleavable chiral crystal PdSbSe

Chiral multifold fermions in solids exhibit unique band structures and topological properties, making them ideal for exploring fundamental physical phenomena related to nontrivial topology, chirality, and symmetry breaking. However, the challenge of obtaining clean, flat surfaces through cleavage has hindered the investigation of their unique electronic states. In this study, we utilize high-resolution angle-resolved photoemission spectroscopy and density functional theory calculations to investigate the low-energy electronic structure of the cleavable single-crystal PdSbSe. Our combined experimental and theoretical analysis reveals the presence of multifold degenerate fermions within this chiral crystal. We also observe multiple chiral Fermi arc surface states and spin-splitting behavior in the associated bulk bands. These findings provide unique insights into chiral, multifold fermionic states in easily cleavable crystals and offer a robust platform for further research into their unique electronic properties and potential applications in novel electronic devices.

cond-mat.mtrl-sci↗

Revealing the electron-spin fluctuation coupling by photoemission in CaKFe4As4

Electron-boson coupling in unconventional superconductors is one of the key parameters in understanding the superconducting pairing symmetry. Here, we report definitive photoemission evidence of electron-spin exciton coupling in the iron-based superconductor CaKFe4As4, obtained via high-resolution ARPES. Our study identifies a distinct kink structure on the α band, observable only in the superconducting phase and closely linked with the superconductivity, indicative of strong electron-boson interactions. Notably, this kink structure corresponds to two distinct bosonic modes at 11 meV and 13 meV, aligning with spin resonance modes previously observed in inelastic neutron scattering experiments. This alignment underscores the significant role of antiferromagnetic fluctuations in the pairing mechanism of this superconductor. Furthermore, the unique momentum-dependent and orbital-selective properties of the coupling revealed by ARPES provide profound insights into the pairing symmetry, suggesting predominantly s_+- wave pairing facilitated by spin fluctuations. Our findings not only highlight the pivotal role of spin resonance in the superconductivity of CaKFe4As4 but also enhance understanding of the electron-spin exciton interactions in unconventional superconductors.

cond-mat.supr-con↗

A canonical foliation on null infinity in perturbations of Kerr

Kerr stability for small angular momentum has been proved in the series of works by Klainerman-Szeftel, Giorgi-Klainerman-Szeftel and Shen. Some of the most basic conclusions of the result, concerning various physical quantities on the future null infinity are derived in the work of Klainerman-Szeftel. Further important conclusions were later derived in An-He-Shen and Chen-Klainerman. In this paper, based on the existence and uniqueness results for GCM spheres by Klainerman-Szeftel, we establish the existence of a canonical foliation on the future null infinity for which the null energy, linear momentum, center of mass and angular momentum are well defined and satisfy the expected physical laws of gravitational radiation. The rigid character of this foliation eliminates the usual ambiguities related to these quantities in the physics literature. We also show that under the initial assumption of Klainerman-Szeftel, the center of mass of the black hole has a large deformation (recoil) after the perturbation.

gr-qc↗

Points on Rational Normal Curves and the ABCT Variety

The ABCT variety is defined as the closure of the image of $G(2,n)$ under the Veronese map. We realize the ABCT variety $V(3,n)$ as the determinantal variety of a vector bundle morphism. We use this to give a recursive formula for the fundamental class of $V(3,n)$. As an application, we show that special Schubert coefficients of this class are given by Eulerian numbers, matching a formula by Cachazo-He-Yuan. On the way to this, we prove that the variety of configuration of points on a common divisor on a smooth variety is reduced and irreducible, generalizing a result of Caminata-Moon-Schaffler.

math.AG↗

Large band-splitting in $g$-wave type altermagnet CrSb

Altermagnetism (AM), a newly discovered magnetic state, ingeniously integrates the properties of ferromagnetism and antiferromagnetism, representing a significant breakthrough in the field of magnetic materials. Despite experimental verification of some typical AM materials, such as MnTe and MnTe$_2$, the pursuit of AM materials that feature larger spin splitting and higher transition temperature is still essential. Here, our research focuses on CrSb, which possesses N{é}el temperature of up to 700K and giant spin splitting near the Fermi level ($E_F$). Utilizing high-resolution angle-resolved photoemission spectroscopy and density functional theory calculations, we meticulously map the three-dimensional electronic structure of CrSb. Our photoemission spectroscopic results on both (0001) and (10$\overline{1}$0) cleavages of CrSb collaboratively reveal unprecedented details on AM-induced band splitting, and subsequently pin down its unique bulk $g$-wave symmetry through quantitative analysis of the angular and photon-energy dependence of spin splitting. Moreover, the observed spin splitting reaches the magnitude of 0.93~eV near $E_F$, the most substantial among all confirmed AM materials. This study not only validates the nature of CrSb as a prototype $g$-wave like AM material but also underscores its pivotal role in pioneering applications in spintronics.

cond-mat.mtrl-sci↗