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Denis Bartolo

Publications and source records attributed to Denis Bartolo.

At least 19 recordsLinked to original sources

Order by inertia in spinning active matter: holey fluids and spin-textured crystals

Active matter sustains emergent flows at the expense of preserving structural order. The feedback between structure and viscous flows typically disrupts crystalline and liquid-crystalline organization by amplifying the very deformations they generate. Yet this destabilizing paradigm has recently been challenged by experiments showing that inertial fluid flows can stabilize few-body bound states of active spinners. Whether inertial active matter can sustain genuine cohesion and order at the many-body level, however, remains elusive. Here we investigate two-dimensional assemblies of macroscopic spinners operating at high Reynolds number and uncover two phase transitions leading to the emergence of a dilute percolating fluid and a dense spin-textured crystal. At low density, inertial flows generate two competing interactions: anisotropic attractions and transverse Magnus forces that continuously break and reconfigure bonds. Together they drive a percolation transition toward a dynamically rearranging holey liquid reminiscent of the empty-liquid states observed in equilibrium patchy colloids. At high density, the feedback between spin alignment and particle positions suppresses transverse rearrangements and yields a first-order transition toward a spin-ordered crystal. Our results demonstrate that, beyond the overdamped limit, hydrodynamic feedback can promote rather than destroy collective order, revealing a distinct regime of many-body active matter governed by inertial flows.

cond-mat.soft

Phase coherence and disorder-induced wave propagation in micromotor arrays

Machines are designed, assembled, and programmed to convert power into predetermined dynamics and functions. In contrast, living systems such as interacting cells and animal groups self-organize, synchronize, and perform complex tasks without predefined patterns. Inspired by these decentralized architectures, experiments have shown that small assemblies of elastically coupled self-propelled robots can achieve two fundamental functionalities observed in nature: collective motion and oscillatory deformations. However, biological inspiration has steered research toward translational self-propulsion, while active rotation remains an underexplored route to designing broader animate materials. Here, we study the self-organization of microscopic metamachines composed of thousands of 3D-printed rotary motors. We first demonstrate and explain how motors precessing in unspecified directions collectively arrange their dynamics into a pristine antiferromagnetic phase. Next, we elucidate the emergence of spatiotemporal order in the form of phase coherence in the rotors' precession. Finally, we show how quenched disorder initiates the free propagation of phase waves across self-organized regions with mismatched rotation speeds. Our results suggest that spinner-based metamachines could illuminate metachronal-wave formation in living systems, and signal propagation in synthetic animate materials.

cond-mat.soft

Melting of non reciprocal solids: how dislocations propel and fission in flowing crystals

When soft matter is driven out of equilibrium its constituents interact via effective interactions that escape Newton's action-reaction principle. Prominent examples include the hydrodynamic interactions between colloidal particles driven in viscous fluids, phoretic interactions between chemically active colloids, and quorum sensing interactions in bacterial colonies. Despite a recent surge of interest in non-reciprocal physics a fundamental question remains : do non-reciprocal interactions alter or strengthen the ordered phases of matter driven out of equilibrium? Here, through a combination of experiments and simulations, we show how nonreciprocal forces propel and fission dislocations formed in hydrodynamically driven Wigner crystals. We explain how dislocation motility results in the continuous reshaping of grain-boundary networks, and how their fission reaction melts driven crystals from their interfaces. Beyond the specifics of hydrodynamics, we argue theoretically that topological defects and nonreciprocal interactions should invariably conspire to deform and ultimately destroy crystals whose the elementary units defy Newton's third law

cond-mat.soft

Synthetic Quorum Sensing and Absorbing Phase Transitions in Colloidal Active Matter

Unlike biological active matter that constantly adapt to their environment, the motors of synthetic active particles are typically agnostic to their surroundings and merely operate at constant force. Here, we design colloidal active rods capable of modulating their inner activity in response to crowding, thereby enforcing a primitive form of quorum sensing interactions. Through experiments, simulations, and theory we elucidate the impact of these interactions on the phase behavior of isotropic active matter. We demonstrate that, when conditioned to density, motility regulation can either lead to an absorbing phase transition, where all particles freeze their dynamics, or to atypical phase separation, where flat interfaces supporting a net pressure drop are in mechanical equilibrium. Fully active and fully arrested particles can then form heterogeneous patterns ruled by the competition between quorum sensing and mechanical interactions. Beyond the specifics of motile colloids, we expect our findings to apply broadly to adaptive active matter assembled from living or synthetic units.

cond-mat.stat-mech

Active-hydraulic flows solve the 6-vertex model (and vice versa)

By confining colloidal active fluids in microchannel networks, we demonstrate that their degenerate flows corresponds to the configurations of the six-vertex model. We use this quantitative correspondence to control and explain the active flows that emerge in square grid networks. In particular, we show that the Lagrangian trajectories of active particles realize the Baxter-Kelland-Wu mapping and form completely packed loops, whose geometry can be exactly predicted and explained. We then go beyond the square-grid geometry and introduce a general framework for predicting the geometry of active-hydraulic flows in arbitrary networks.

cond-mat.soft

Interpreting neural operators: how nonlinear waves propagate in non-reciprocal solids

We present a data-driven pipeline for model building that combines interpretable machine learning, hydrodynamic theories, and microscopic models. The goal is to uncover the underlying processes governing nonlinear dynamics experiments. We exemplify our method with data from microfluidic experiments where crystals of streaming droplets support the propagation of nonlinear waves absent in passive crystals. By combining physics-inspired neural networks, known as neural operators, with symbolic regression tools, we generate the solution, as well as the mathematical form, of a nonlinear dynamical system that accurately models the experimental data. Finally, we interpret this continuum model from fundamental physics principles. Informed by machine learning, we coarse grain a microscopic model of interacting droplets and discover that non-reciprocal hydrodynamic interactions stabilise and promote nonlinear wave propagation.

cond-mat.soft

Curvature heterogeneities act as singular perturbations to smooth Laplacian fields: a fluid mechanics demonstration

In this Letter, we use a model fluid mechanics experiment to elucidate the impact of curvature heterogeneities on two-dimensional fields deriving from harmonic potential functions. This result is directly relevant to explain the smooth stationary structures in physical systems as diverse as curved liquid crystal and magnetic films, heat and Ohmic transport in wrinkled two-dimensional materials and flows in confined channels. Combining microfluidic experiments and theory, we explain how curvature heterogeneities shape confined viscous flows. We show that isotropic bumps induce local distortions to Darcy's flows whereas anisotropic curvature heterogeneities disturb them algebraically over system-spanning scales. Thanks to an electrostatic analogy, we gain insight into this singular geometric perturbation, and quantitatively explain it using both conformal mapping and numerical simulations. Altogether our findings establish the robustness of our experimental observations and their broad relevance to all Laplacian problems beyond the specifics of our fluid mechanics experiment.

cond-mat.soft

Active hydraulics laws from frustration principles

Viscous flows are laminar and deterministic. Robust linear laws accurately predict their streamlines in structures as complex as blood vessels, porous media and pipe networks. However, biological and synthetic active fluids defy these fundamental laws. Irrespective of their microscopic origin, confined active flows are intrinsically bistable, and therefore non-linear. As a consequence, their emergent patterns in channel networks are out of reach of available theories, and lack quantitative experiments. Here, we lay out the basic laws of active hydraulics. We show that active hydraulic flows are non-deterministic and yield degenerate streamline patterns ruled by frustration at nodes with an odd coordination number. More precisely, colloidal-roller experiments in trivalent networks reveal how active-hydraulic flows realize dynamical spin ices. The resulting streamline patterns split into two distinct classes of self-similar loops, which reflect the fractionalization of topological defects at the subchannel scales. Informed by our measurements, we formulate the laws of active hydraulics as a double spin model. A series of mappings on loop O(n) models then allow us to exactly predict the geometry of the degenerate streamlines. We expect our fundamental understanding to provide robust design rules for active microfluidic devices, and to offer unanticipated avenues to understand the motion of living cells and organisms in complex habitats.

cond-mat.soft

Model-free characterization of topological edge and corner states in mechanical networks

Topological materials can host edge and corner states that are protected from disorder and material imperfections. In particular, the topological edge states of mechanical structures present unmatched opportunities for achieving robust responses in wave guiding, sensing, computation, and filtering. However, determining whether a mechanical structure is topologically nontrivial and features topologically-protected modes has hitherto relied on theoretical models. This strong requirement has limited the experimental and practical significance of topological mechanics to laboratory demonstrations. Here, we introduce and validate an experimental method to detect the topologically protected zero modes of mechanical structures without resorting to any modeling step. Our practical method is based on a simple electrostatic analogy: topological zero modes are akin to electric charges. To detect them, we identify elementary mechanical molecules and measure their chiral polarization, a recently introduced marker of topology in chiral phases. Topological zero modes are then identified as singularities of the polarization field. Our method readily applies to any mechanical structure and effectively detects the edge and corner states of regular and higher-order topological insulators. Our findings extend the reach of chiral topological phases beyond designer materials, and allow their direct experimental investigation.

cond-mat.mtrl-sci

Non-orientable order and non-Abelian response in frustrated metamaterials

From atomic crystals to bird flocks, most forms of order are captured by the concept of spontaneous symmetry breaking. This paradigm was challenged by the discovery of topological order, in materials where the number of accessible states is not solely determined by the number of broken symmetries, but also by space topology. Until now however, the concept of topological order has been linked to quantum entanglement and has therefore remained out of reach in classical systems. Here, we show that classical systems whose global geometry frustrates the emergence of homogeneous order realise an unanticipated form of topological order defined by non-orientable order-parameter bundles: non-orientable order. We validate experimentally and theoretically this concept by designing frustrated mechanical metamaterials that spontaneously break a discrete symmetry under homogeneous load. While conventional order leads to a discrete ground-state degeneracy, we show that non-orientable order implies an extensive ground-state degeneracy -- in the form of topologically protected zero-nodes and zero-lines. Our metamaterials escape the traditional classification of order by symmetry breaking. Considering more general stress distributions, we leverage non-orientable order to engineer robust mechanical memory and achieve non-Abelian mechanical responses that carry an imprint of the braiding of local loads. We envision this principle to open the way to designer materials that can robustly process information across multiple areas of physics, from mechanics to photonics and magnetism.

cond-mat.soft

When soft crystals defy Newton's third law: Non-reciprocal mechanics and dislocation motility

The effective interactions between the constituents of driven soft matter generically defy Newton's third law. Combining theory and numerical simulations, we establish that six classes of mechanics with no counterparts in equilibrium systems emerge in elastic crystals challenged by nonreciprocal interactions. Going beyond linear deformations, we reveal that interactions violating Newton's third law generically turn otherwise quiescent dislocations into motile singularities which steadily glide though periodic lattices.

cond-mat.soft

Topology-driven ordering of flocking matter

When interacting motile units self-organize into flocks, they realize one of the most robust ordered state found in nature. However, after twenty five years of intense research, the very mechanism controlling the ordering dynamics of both living and artificial flocks has remained unsettled. Here, combining active-colloid experiments, numerical simulations and analytical work, we explain how flocking liquids heal their spontaneous flows initially plagued by collections of topological defects to achieve long-ranged polar order even in two dimensions. We demonstrate that the self-similar ordering of flocking matter is ruled by a living network of domain walls linking all $\pm 1$ vortices, and guiding their annihilation dynamics. Crucially, this singular orientational structure echoes the formation of extended density patterns in the shape of interconnected bow ties. We establish that this double structure emerges from the interplay between self-advection and density gradients dressing each $-1$ topological charges with four orientation walls. We then explain how active Magnus forces link all topological charges with extended domain walls, while elastic interactions drive their attraction along the resulting filamentous network of polarization singularities. Taken together our experimental, numerical and analytical results illuminate the suppression of all flow singularities, and the emergence of pristine unidirectional order in flocking matter.

cond-mat.soft

Motile dislocations knead odd crystals into whorls

The competition between thermal fluctuations and potential forces is the foundation of our understanding of phase transitions and matter in equilibrium. Driving matter out of equilibrium allows for a new class of interactions which are neither attractive nor repulsive but transverse. The existence of such transverse forces immediately raises the question of how they interfere with basic principles of material self-organization. Despite a recent surge of interest, this question remains open. Here, we show that activating transverse forces by homogeneous rotation of colloidal units generically turns otherwise quiescent solids into a crystal whorl state dynamically shaped by self-propelled dislocations. Simulations of both a minimal model and a full hydrodynamics model establish the generic nature of the chaotic dynamics of these self-kneading polycrystals. Using a continuum theory, we explain how odd and Hall stresses conspire to destabilize chiral crystals from within. This chiral instability produces dislocations that are unbound by their self-propulsion. Their proliferation eventually leads to a crystalline whorl state out of reach of equilibrium matter.

cond-mat.soft

Emergence of dynamic vortex glasses in disordered polar active fluids

In equilibrium, disorder conspires with topological defects to redefine the ordered states of matter in systems as diverse as crystals, superconductors and liquid crystals. Far from equilibrium, however, the consequences of quenched disorder on active condensed matter remain virtually uncharted. Here, we reveal a state of strongly disordered active matter with no counterparts in equilibrium: a dynamical vortex glass. Combining high-content microfluidic experiments and theory, we show how colloidal flocks collectively cruise through disorder without relaxing the topological singularities of their flows. The resulting state is highly dynamical but the flow patterns, shaped by a finite density of frozen vortices, are stationary and exponentially degenerated. Quenched isotropic disorder acts as a random gauge field turning active liquids into dynamical vortex glasses. We argue that this robust mechanism should shape the collective dynamics of a broad class of disordered active matter, from synthetic active nematics to collections of living cells exploring heterogeneous media.

cond-mat.soft

Flowing emulsions through disorder: Critical depinning and smectic rivers

During the past sixty minutes only, oil companies have extracted six trillions liters of oil from the ground, i.e. the volume of about two hundreds Olympic swimming pools. This phenomenal number gives a striking illustration of the impact of multiphase flows on the world economy and environment. From a fundamental perspective, we now clearly understand the large-scale patterns formed when liquid interfaces are driven through heterogeneous environments. In stark contrast, the displacement of fragmented fluids through disordered media remains limited to isolated droplets and bubbles. Here, we elucidate the collective dynamics of emulsions hydrodynamically driven through disordered environments. Advecting hundreds of thousands of microfluidic droplets through random lattices of pinning sites, we establish that the mobilization of confined emulsions is a critical dynamical transition. Unlike contact-line depinning, emulsion mobilization is not triggered by large-scale avalanches but merely requires the coordinated motion of small groups of particles. Criticality arises from the correlations of seemingly erratic depinning events over system-spanning scales along smectic river networks. We elucidate the microscopic origin of these self-organized flow patterns: contact interactions and hydrodynamic focusing conspire to mobilize emulsion out of disorder. We close our article commenting on the similarities (and profound differences) with the plastic depinning transitions of driven flux lines in high-$T_{\rm c}$ superconductors, and grain transport in eroded sand beds.

cond-mat.soft

Colloidal transport in bacteria suspensions: from bacteria scattering to anomalous and enhanced diffusion

Colloids coupled to a bath of swimming cells generically display enhanced diffusion. This transport dynamics stems from a subtle interplay between the active and passive particles that still resists our understanding despite decades of intense research. Here, we tackle the root of the problem by providing a quantitative characterisation of the single scattering events between a colloid and a bacterium. Based on our experiments, we build a minimal model that quantitatively predicts the geometry of the scattering trajectories, and enhanced colloidal diffusion at long times. This quantitative confrontation between theory and experiments elucidates the microscopic origin of enhanced transport. Collisions are solely ruled by stochastic contact interactions responsible both for genuine anomalous diffusion at short times and enhanced diffusion at long times with no ballistic regime at any scale.

cond-mat.soft

Geometry and Topology Tango in Ordered and Amorphous Chiral Matter

Systems as diverse as mechanical structures assembled from elastic components, and photonic metamaterials enjoy a common geometrical feature: a sublattice symmetry. This property realizes a chiral symmetry first introduced to characterize a number of electronic insulators in the vicinity of their energy gaps. In this article, we introduce a generic framework to elucidate and design zero-energy topological boundary modes in all systems enjoying a chiral symmetry, whether crystalline or amorphous. We first show how to distinguish chiral insulators from one another by a real-space measure: their chiral polarization. In crystals, we use it to redefine the very concept of bulk-boundary correspondence, and resolve long-standing ambiguities in its application to chiral insulators. In amorphous metamaterials, we use it to lay out generic geometrical rules to locate topologically distinct phases, and explain how to engineer localized zero-mode wave guides even more robust than in periodic structures.

cond-mat.str-el

Topological elasticity of non-orientable ribbons

In this article, we unravel an intimate relationship between two seemingly unrelated concepts: elasticity, that defines the local relations between stress and strain of deformable bodies, and topology that classifies their global shape. Focusing on Moebius strips, we establish that the elastic response of surfaces with non-orientable topology is: non-additive, non-reciprocal and contingent on stress-history. Investigating the elastic instabilities of non-orientable ribbons, we then challenge the very concept of bulk-boundary-correspondence of topological phases. We establish a quantitative connection between the modes found at the interface between inequivalent topological insulators and solitonic bending excitations that freely propagate through the bulk non-orientable ribbons. Beyond the specifics of mechanics, we argue that non-orientability offers a versatile platform to tailor the response of systems as diverse as liquid crystals, photonic and electronic matter.

cond-mat.soft