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Dieter Koelle

Publications and source records attributed to Dieter Koelle.

At least 55 records · Page 3Linked to original sources

Improving superconducting resonators in magnetic fields by reduced field-focussing and engineered flux screening

We experimentally investigate superconducting coplanar waveguide resonators in external magnetic fields and present two strategies to reduce field-induced dissipation channels and resonance frequency shifts. One of our approaches is to significantly reduce the superconducting ground-plane areas, which leads to reduced magnetic field-focussing and thus to lower effective magnetic fields inside the waveguide cavity. By this measure, the field-induced losses can be reduced by more than one order of magnitude in mT out-of-plane magnetic fields. When these resonators are additionally coupled inductively instead of capacitively to the microwave feedlines, an intrinsic closed superconducting loop is effectively shielding the heart of the resonator from magnetic fields by means of flux conservation. In total, we achieve a reduction of the field-induced resonance frequency shift by up to two orders of magnitude. We combine systematic parameter variations on the experimental side with numerical magnetic field calculations to explain the effects of our approaches and to support our conclusions. The presented results are relevant for all areas, where high-performance superconducting resonators need to be operated in magnetic fields, e.g. for quantum hybrid devices with superconducting circuits or electron spin resonance detectors based on coplanar waveguide cavities.

cond-mat.supr-con↗

Current-phase relation of ballistic graphene Josephson junctions

The current-phase relation (CPR) of a Josephson junction (JJ) determines how the supercurrent evolves with the superconducting phase difference across the junction. Knowledge of the CPR is essential in order to understand the response of a JJ to various external parameters. Despite the rising interest in ultra-clean encapsulated graphene JJs, the CPR of such junctions remains unknown. Here, we use a fully gate-tunable graphene superconducting quantum intereference device (SQUID) to determine the CPR of ballistic graphene JJs. Each of the two JJs in the SQUID is made with graphene encapsulated in hexagonal boron nitride. By independently controlling the critical current of the JJs, we can operate the SQUID either in a symmetric or asymmetric configuration. The highly asymmetric SQUID allows us to phase-bias one of the JJs and thereby directly obtain its CPR. The CPR is found to be skewed, deviating significantly from a sinusoidal form. The skewness can be tuned with the gate voltage and oscillates in anti-phase with Fabry-Pérot resistance oscillations of the ballistic graphene cavity. We compare our experiments with tight-binding calculations which include realistic graphene-superconductor interfaces and find a good qualitative agreement.

cond-mat.mes-hall↗

Metallic coplanar resonators optimized for low-temperature measurements

Metallic coplanar microwave resonators are widely employed at room temperature, but their low-temperature performance has received little attention so far. We characterize compact copper coplanar resonators with multiple modes from 2.5 to 20 GHz at temperatures as low as 5 K. We investigate the influence of center conductor width (20 to 100 μm) and coupling gap size (10 to 50 μm), and we observe a strong increase of quality factor (Q) for wider center conductors, reaching values up to 470. The magnetic-field dependence of the resonators is weak, with a maximum change in Q of 3.5% for an applied field of 7 T. This makes these metallic resonators well suitable for magnetic resonance studies, as we document with electron spin resonance (ESR) measurements at multiple resonance frequencies.

cond-mat.mes-hall↗

Quantum interference in an interfacial superconductor

The two-dimensional superconductor formed at the interface between the complex oxides, lanthanum aluminate (LAO) and strontium titanate (STO) has several intriguing properties that set it apart from conventional superconductors. Most notably, an electric field can be used to tune its critical temperature (T$_c$), revealing a dome-shaped phase diagram reminiscent of high T$_c$ superconductors. So far, experiments with oxide interfaces have measured quantities which probe only the magnitude of the superconducting order parameter and are not sensitive to its phase. Here, we perform phase-sensitive measurements by realizing the first superconducting quantum interference devices (SQUIDs) at the LAO/STO interface. Furthermore, we develop a new paradigm for the creation of superconducting circuit elements, where local gates enable in-situ creation and control of Josephson junctions. These gate-defined SQUIDs are unique in that the entire device is made from a single superconductor with purely electrostatic interfaces between the superconducting reservoir and the weak link. We complement our experiments with numerical simulations and show that the low superfluid density of this interfacial superconductor results in a large, gate-controllable kinetic inductance of the SQUID. Our observation of robust quantum interference opens up a new pathway to understand the nature of superconductivity at oxide interfaces.

cond-mat.mes-hall↗

3D simulations of the electrothermal and THz emission properties of Bi$_2$Sr$_2$CaCu$_2$O$_8$ intrinsic Josephson junction stacks

We used 2D coupled sine-Gordon equations combined with 3D heat diffusion equations to numerically investigate the thermal and electromagnetic properties of a $250 \times 70\,μ\mathrm{m}^2$ intrinsic Josephson junction stack. The 700 junctions are grouped to 20 segments; we assume that in a segment all junctions behave identically. At large input power a hot spot forms in the stack. Resonant electromagnetic modes, oscillating either along the length ((0, $n$) modes) or the width (($m$, 0) modes) of the stack or having a more complex structure, can be excited both with and without a hot spot. At fixed bath temperature and bias current several cavity modes can coexist in the absence of a magnetic field. The (1, 0) mode, considered to be the most favorable mode for THz emission, can be stabilized by applying a small magnetic field along the length of the stack. A strong field-induced enhancement of the emission power is also found in experiment, for an applied field around 5.9 mT.

cond-mat.supr-con↗

Quantitative nanoscale vortex-imaging using a cryogenic quantum magnetometer

Microscopic studies of superconductors and their vortices play a pivotal role in our understanding of the mechanisms underlying superconductivity. Local measurements of penetration depths or magnetic stray-fields enable access to fundamental aspects of superconductors such as nanoscale variations of superfluid densities or the symmetry of their order parameter. However, experimental tools, which offer quantitative, nanoscale magnetometry and operate over the large range of temperature and magnetic fields relevant to address many outstanding questions in superconductivity, are still missing. Here, we demonstrate quantitative, nanoscale magnetic imaging of Pearl vortices in the cuprate superconductor YBCO, using a scanning quantum sensor in form of a single Nitrogen-Vacancy (NV) electronic spin in diamond. The sensor-to-sample distance of ~10nm we achieve allows us to observe striking deviations from the prevalent monopole approximation in our vortex stray-field images, while we find excellent quantitative agreement with Pearl's analytic model. Our experiments yield a non-invasive and unambiguous determination of the system's local London penetration depth, and are readily extended to higher temperatures and magnetic fields. These results demonstrate the potential of quantitative quantum sensors in benchmarking microscopic models of complex electronic systems and open the door for further exploration of strongly correlated electron physics using scanning NV magnetometry.

cond-mat.mes-hall↗

Observing electron spin resonance between 0.1 and 67 GHz at temperatures between 50 mK and 300 K using broadband metallic coplanar waveguides

We describe a fully broadband approach for electron spin resonance (ESR) experiments where it is possible to not only tune the magnetic field but also the frequency continuously over wide ranges. Here a metallic coplanar transmission line acts as compact and versatile microwave probe that can easily be implemented in different cryogenic setups. We perform ESR measurements at frequencies between 0.1 and 67 GHz and at temperatures between 50 mK and room temperature. Three different types of samples (Cr3+ ions in ruby, organic radicals of the nitronyl-nitroxide family, and the doped semiconductor Si:P) represent different possible fields of application for the technique. We demonstrate that an extremely large phase space in temperature, magnetic field, and frequency for ESR measurements, substantially exceeding the range of conventional ESR setups, is accessible with metallic coplanar lines.

cond-mat.mes-hall↗

Low-Noise YBa$_2$Cu$_3$O$_7$ NanoSQUIDs for Performing Magnetization-Reversal Measurements on Magnetic Nanoparticles

We fabricated YBa$_2$Cu$_3$O$_7$ (YBCO) direct current (dc) nano superconducting quantum interference devices (nanoSQUIDs) based on grain boundary Josephson junctions by focused ion beam patterning. Characterization of electric transport and noise properties at 4.2$\,$K in magnetically shielded environment yields a very small inductance $L$ of a few pH for an optimized device geometry. This in turn results in very low values of flux noise $<50\,{\rm n}Φ_0/{\rm Hz}^{1/2}$ in the thermal white noise limit, which yields spin sensitivities of a few $μ_{\rm B}/{\rm Hz}^{1/2}$ ($Φ_0$ is the magnetic flux quantum and $μ_{\rm B}$ is the Bohr magneton). We observe frequency-dependent excess noise up to 7$\,$MHz, which can only partially be eliminated by bias reversal readout. This indicates the presence of fluctuators of unknown origin, possibly related to defect-induced spins in the SrTiO$_3$ substrate. We demonstrate the potential of using YBCO nanoSQUIDs for the investigation of small spin systems, by placing a 39$\,$nm diameter Fe nanowire, encapsulated in a carbon nanotube, on top of a non-optimized YBCO nanoSQUID and by measuring the magnetization reversal of the Fe nanowire via the change of magnetic flux coupled to the nanoSQUID. The measured flux signals upon magnetization reversal of the Fe nanowire are in very good agreement with estimated values, and the determined switching fields indicate magnetization reversal of the nanowire via curling mode.

cond-mat.supr-con↗

Electrical-transport characteristics of as-grown and oxygen-reduced La$_{0.7}$Ce$_{0.3}$MnO$_3$ films: calculation of hopping energies, Mn valences, and carrier localization lengths

Presently, cerium-doped LaMnO$_3$ is vividly discussed as an electron-doped counterpart prototype to the well-established hole-doped mixed-valence manganites. Here, La$_{0.7}$Ce$_{0.3}$MnO$_3$ thin films of different thicknesses, degrees of CeO$_2$ phase segregation, and oxygen deficiency, grown on SrTiO$_3$ single crystal substrates, are compared with respect to their resistance-vs.-temperature (R vs. T) behavior from 300~K down to 90~K. While the variation of the film thickness (and thus the degree of epitaxial strain) in the range between 10~nm and 100~nm has only a weak impact on the electrical transport, the degree of oxygen deficiency as well as the existence of CeO$_2$ clusters can completely change the type of hopping mechanism. This is shown by fitting the respective \textit{R-T} curves with three different transport models (adiabatic polaron hopping, Mott variable-range hopping, Efros-Shklovskii variable-range hopping), which are commonly used for the mixed-valence manganites. Several characteristic transport parameters, such as the hopping energies, the carrier localization lengths, as well as the Mn valences are derived from the fitting procedures.

cond-mat.mtrl-sci↗

Conductivity and magnetoresistance of La$_{0.7}$Ce$_{0.3}$MnO$_3$ thin films under photoexcitation

La$_{0.7}$Ce$_{0.3}$MnO$_3$ thin films of different thicknesses, degrees of CeO$_2$-phase segregation and oxygen deficiency, grown on SrTiO$_3$ single crystal substrates, were comparatively investigated with respect to both their spectral and temperature-dependent photoconductivity (PC) and their magnetoresistance (MR) behaviour under photoexcitation. While as-grown films were insensitive to optical excitation, oxygen reduction appeared to be an effective way to decrease the film resistance, but the film thickness was found to play a minor role. However, from the evaluation of the spectral behaviour of the PC and the comparison of the MR of the LCeMO/substrate-samples with a bare substrate under illumination we find that the photoconductivity data reflects not only contributions from (i) photogenerated charge carriers in the film and (ii) carriers injected from the photoconductive substrate (as concluded from earlier works), but also (iii) a decisive parallel photoconduction in the SrTiO$_3$ substrate. Furthermore -- also by analyzing the MR characteristics -- the unexpected occurence of a strong electroresistive effect in the sample with the highest degree of CeO$_2$ segregation and oxygen deficiency could be attributed to the electroresistance of the SrTiO$_3$ substrate as well. The results suggest a critical reconsideration and possibly a reinterpretation of several previous photoconductivity and electroresistance investigations of manganite thin films on SrTiO$_3$.

cond-mat.mtrl-sci↗

Niobium stripline resonators for microwave studies on superconductors

Microwave spectroscopy is a powerful experimental tool to reveal information on the intrinsic properties of superconductors. Superconducting stripline resonators, where the material under study constitutes one of the ground planes, offer a high sensitivity to investigate superconducting bulk samples. In order to improve this measurement technique, we have studied stripline resonators made of niobium, and we compare the results to lead stripline resonators. With this technique we are able to determine the temperature dependence of the complex conductivity of niobium and the energy gap $Δ(0)=2.1$ meV. Finally we show measurements at the superconducting transition of a tantalum bulk sample using niobium stripline resonators.

cond-mat.supr-con↗

Optimizing the spin sensitivity of grain boundary junction nanoSQUIDs -- towards detection of small spin systems with single-spin resolution

We present an optimization study of the spin sensitivity of nanoSQUIDs based on resistively shunted grain boundary Josephson junctions. In addition the dc SQUIDs contain a narrow constriction onto which a small magnetic particle can be placed (with its magnetic moment in the plane of the SQUID loop and perpendicular to the grain boundary) for efficient coupling of its stray magnetic field to the SQUID loop. The separation of the location of optimum coupling from the junctions allows for an independent optimization of the coupling factor $ϕ_μ$ and junction properties. We present different methods for calculating $ϕ_μ$ (for a magnetic nanoparticle placed 10\,nm above the constriction) as a function of device geometry and show that those yield consistent results. Furthermore, by numerical simulations we obtain a general expression for the dependence of the SQUID inductance on geometrical parameters of our devices, which allows to estimate their impact on the spectral density of flux noise $S_Φ$ of the SQUIDs in the thermal white noise regime. Our analysis of the dependence of $S_Φ$ and $ϕ_μ$ on the geometric parameters of the SQUID layout yields a spin sensitivity $S_μ^{1/2}=S_Φ^{1/2}/ϕ_μ$ of a few $μ_{\rm{B}}/\rm{Hz^{1/2}}$ ($μ_B$ is the Bohr magneton) for optimized parameters, respecting technological constraints. However, by comparison with experimentally realized devices we find significantly larger values for the measured white flux noise, as compared to our theoretical predictions. Still, a spin sensitivity on the order of $10\,μ_{\rm B}/\rm{Hz^{1/2}}$ for optimized devices seems to be realistic.

cond-mat.supr-con↗

Optimizing the spin sensitivity of grain boundary junction nanoSQUIDs -- towards detection of small spin systems with single-spin resolution

We present an optimization study of the spin sensitivity of nanoSQUIDs based on resistively shunted grain boundary Josephson junctions. In addition the dc SQUIDs contain a narrow constriction onto which a small magnetic particle can be placed (with its magnetic moment in the plane of the SQUID loop and perpendicular to the grain boundary) for efficient coupling of its stray magnetic field to the SQUID loop. The separation of the location of optimum coupling from the junctions allows for an independent optimization of the coupling factor $ϕ_μ$ and junction properties. We present different methods for calculating $ϕ_μ$ (for a magnetic nanoparticle placed 10\,nm above the constriction) as a function of device geometry and show that those yield consistent results. Furthermore, by numerical simulations we obtain a general expression for the dependence of the SQUID inductance on geometrical parameters of our devices, which allows to estimate their impact on the spectral density of flux noise $S_Φ$ of the SQUIDs in the thermal white noise regime. Our analysis of the dependence of $S_Φ$ and $ϕ_μ$ on the geometric parameters of the SQUID layout yields a spin sensitivity $S_μ^{1/2}=S_Φ^{1/2}/ϕ_μ$ of a few $μ_{\rm{B}}/\rm{Hz^{1/2}}$ ($μ_B$ is the Bohr magneton) for optimized parameters, respecting technological constraints. However, by comparison with experimentally realized devices we find significantly larger values for the measured white flux noise, as compared to our theoretical predictions. Still, a spin sensitivity on the order of $10\,μ_{\rm B}/\rm{Hz^{1/2}}$ for optimized devices seems to be realistic.

cond-mat.supr-con↗

Mn$^{2+}$/Mn$^{3+}$ state of La$_{0.7}$Ce$_{0.3}$MnO$_3$ by oxygen reduction and photodoping

Films of cerium-doped LaMnO$_3$, which has been intensively discussed as an electron-doped counterpart to hole-doped mixed-valence lanthanum manganites during the past decade, were analyzed by x-ray photoemission spectroscopy with respect to their manganese valence under photoexcitation. The comparative analysis of the Mn 3s exchange splitting of La$_{0.7}$Ce$_{0.3}$MnO$_3$ (LCeMO) films in the dark and under illumination clearly shows that both oxygen reduction and illumination are able to decrease the Mn valence towards a mixed 2$+$/3$+$ state, independently of the film thickness and the degree of CeO$_2$ segregation. Charge injection from the photoconductive SrTiO$_3$ substrate into the Mn e$_g$ band with carrier lifetimes in the range of tens of seconds and intrinsic generation of electron-hole pairs within the films are discussed as two possible sources of the Mn valence shift and the subsequent electron doping.

cond-mat.mtrl-sci↗

Inductively coupled superconducting half wavelength resonators as persistent current traps for ultracold atoms

A crucial point in the experimental implementation of hybrid quantum systems consisting of superconducting circuits and atomic ensembles is bringing the two partners close enough to each other that a strong quantum coherent coupling can be established. Here, we propose to use the metallization structures of a half wavelength superconducting coplanar waveguide resonator as a persistent current trap for ultracold paramagnetic atoms. Trapping atoms with the resonator structure itself is provided by using short-ended and inductively coupled resonators instead of capacitively coupled ones as customary in circuit quantum electrodynamics.We analyze the external quality factor of short-ended coplanar waveguide resonators and show that it can be easily designed for the desired regime of quantum circuits. The magnetic field configuration at the resonator is calculated by means of numerical three-dimensional simulations of the London equations. We present a way to transport an atomic ensemble into the coplanar resonator gap where the magnetic field of the cavity mode is maximum. The configuration allows stable trapping by persistent currents and paves the route towards strong coupling between atomic clouds and the cavity mode which is required for cooperative effects and gives the interface between atoms and circuit quantum electrodynamics.

cond-mat.supr-con↗

Nb nano superconducting quantum interference devices with high spin sensitivity for operation in magnetic fields up to 0.5\,T

We investigate electric transport and noise properties of microstrip-type submicron direct current superconducting quantum interference devices (dc SQUIDs) based on Nb thin films and overdamped Josephson junctions with a HfTi barrier. The SQUIDs were designed for optimal spin sensitivity $S_μ^{1/2}$ upon operation in intermediate magnetic fields $B$ (tens of mT), applied perpendicular to the substrate plane. Our so far best SQUID can be continuously operated in fields up to $B\approx\pm50\,\rm{mT}$ with rms flux noise $S_{Φ,\rm w}^{1/2}\leq250\,\rm{nΦ_0/Hz^{1/2}}$ in the white noise regime and spin sensitivity $S_μ^{1/2}\leq29\,\rm{μ_B/Hz^{1/2}}$. Furthermore, we demonstrate operation in $B=0.5\,\rm{T}$ with high sensitivity in flux $S_{Φ,\rm w}^{1/2}\approx680\,\rm{nΦ_0/Hz^{1/2}}$ and in electron spin $S_μ^{1/2}\approx79\,\rm{μ_B/Hz^{1/2}}$. We discuss strategies to further improve the nanoSQUID performance.

cond-mat.supr-con↗

The phase boundary of superconducting niobium thin films with antidot arrays fabricated with microsphere photolithography

The experimental investigation of the $I_c(B)$--$T_c(B)$ phase boundary of superconducting niobium films with large area quasihexagonal hole arrays is reported. The hole arrays were patterned with microsphere photolithography. We investigate the perforated niobium films by means of electrical directed current transport measurements close to the transition temperature $T_c$ in perpendicularly applied magnetic fields. We find pronounced modulations of the critcal current with applied magnetic field, which we interpret as a consequence of commensurable states between the Abrikosov vortex lattice and the quasihexagonal pinning array. Furthermore, we observe Little-Parks oscillations in the critical temperature vs magnetic field.

cond-mat.supr-con↗

Magnetic hysteresis effects in superconducting coplanar microwave resonators

We performed transmission spectroscopy experiments on coplanar half wavelength niobium resonators at a temperature T=4.2 K. We observe not only a strong dependence of the quality factor Q and the resonance frequency f_res on an externally applied magnetic field but also on the magnetic history of our resonators, i.e. on the spatial distribution of trapped Abrikosov vortices in the device. We find these results to be valid for a broad range of frequencies and angles between the resonator plane and the magnetic field direction as well as for resonators with and without antidots near the edges of the center conductor and the ground planes. In a detailed analysis we show, that characteristic features of the experimental data can only be reproduced in calculations, if a highly inhomogeneous rf-current density and a flux density gradient with maxima at the edges of the superconductor is assumed. We furthermore demonstrate, that the hysteretic behaviour of the resonator properties can be used to considerably reduce the vortex induced losses and to fine-tune the resonance frequency by the proper way of cycling to a desired magnetic field.

cond-mat.supr-con↗