arXiv subjects

Dietrich Leibfried

Publications and source records attributed to Dietrich Leibfried.

At least 37 records · Page 2Linked to original sources

arXiv2020

Quantum entanglement between an atom and a molecule

Conventional information processors freely convert information between different physical carriers to process, store, or transmit information. It seems plausible that quantum information will also be held by different physical carriers in applications such as tests of fundamental physics, quantum-enhanced sensors, and quantum information processing. Quantum-controlled molecules in particular could transduce quantum information across a wide range of quantum-bit (qubit) frequencies, from a few kHz for transitions within the same rotational manifold, a few GHz for hyperfine transitions, up to a few THz for rotational transitions, to hundreds of THz for fundamental and overtone vibrational and electronic transitions, possibly all within the same molecule. Here, we report the first demonstration of entanglement between states of the rotation of a $\rm^{40}CaH^+$ molecular ion and internal states of a $\rm^{40}Ca^+$ atomic ion. The qubit addressed in the molecule has a frequency of either 13.4 kHz or 855 GHz, highlighting the versatility of molecular qubits. This work demonstrates how molecules can transduce quantum information between qubits with different frequencies to enable hybrid quantum systems. We anticipate that quantum control and measurement of molecules as demonstrated here will create opportunities for quantum information science, quantum sensors, fundamental and applied physics, and controlled quantum chemistry.

quant-ph↗

arXiv2019

Precision frequency-comb terahertz spectroscopy on pure quantum states of a single molecular ion

Spectroscopy is a powerful tool for studying molecules and is commonly performed on large thermal molecular ensembles that are perturbed by motional shifts and interactions with the environment and one another, resulting in convoluted spectra and limited resolution. Here, we use generally applicable quantum-logic techniques to prepare a trapped molecular ion in a single quantum state, drive terahertz rotational transitions with an optical frequency comb, and read out the final state non-destructively, leaving the molecule ready for further manipulation. We resolve rotational transitions to 11 significant digits and derive the rotational constant of CaH+ to be B_R = 142501777.9(1.7) kHz. Our approach suits a wide range of molecular ions, including polyatomics and species relevant for tests of fundamental physics, chemistry, and astrophysics.

physics.atom-ph↗

arXiv2019

Quantum gate teleportation between separated qubits in a trapped-ion processor

Large-scale quantum computers will require quantum gate operations between widely separated qubits. A method for implementing such operations, known as quantum gate teleportation (QGT), requires only local operations, classical communication, and shared entanglement. We demonstrate QGT in a scalable architecture by deterministically teleporting a controlled-NOT (CNOT) gate between two qubits in spatially separated locations in an ion trap. The entanglement fidelity of our teleported CNOT is in the interval [0.845, 0.872] at the 95% confidence level. The implementation combines ion shuttling with individually-addressed single-qubit rotations and detections, same- and mixedspecies two-qubit gates, and real-time conditional operations, thereby demonstrating essential tools for scaling trapped-ion quantum computers combined in a single device.

quant-ph↗

arXiv2019

Quantum-enhanced sensing of a mechanical oscillator

The use of special quantum states to achieve sensitivities below the limits established by classically behaving states has enjoyed immense success since its inception. In bosonic interferometers, squeezed states, number states and cat states have been implemented on various platforms and have demonstrated improved measurement precision over interferometers based on coherent states. Another metrologically useful state is an equal superposition of two eigenstates with maximally different energies; this state ideally reaches the full interferometric sensitivity allowed by quantum mechanics. By leveraging improvements to our apparatus made primarily to reach higher operation fidelities in quantum information processing, we extend a technique to create number states up to $n=100$ and to generate superpositions of a harmonic oscillator ground state and a number state of the form $\textstyle{\frac{1}{\sqrt{2}}}(\lvert 0\rangle+\lvert n\rangle)$ with $n$ up to 18 in the motion of a single trapped ion. While experimental imperfections prevent us from reaching the ideal Heisenberg limit, we observe enhanced sensitivity to changes in the oscillator frequency that initially increases linearly with $n$, with maximal value at $n=12$ where we observe 3.2(2) dB higher sensitivity compared to an ideal measurement on a coherent state with the same average occupation number. The quantum advantage from using number-state superpositions can be leveraged towards precision measurements on any harmonic oscillator system; here it enables us to track the average fractional frequency of oscillation of a single trapped ion to approximately 2.6 $\times$ 10$^{-6}$ in 5 s. Such measurements should provide improved characterization of imperfections and noise on trapping potentials, which can lead to motional decoherence, a leading source of error in quantum information processing with trapped ions.

physics.atom-ph↗

arXiv2018

Quantum optimal control of the dissipative production of a maximally entangled state

Entanglement generation can be robust against noise in approaches that deliberately incorporate dissipation into the system dynamics. The presence of additional dissipation channels may, however, limit fidelity and speed of the process. Here we show how quantum optimal control techniques can be used to both speed up the entanglement generation and increase the fidelity in a realistic setup, whilst respecting typical experimental limitations. For the example of entangling two trapped ion qubits [Lin et al., Nature 504, 415 (2013)], we find an improved fidelity by simply optimizing the polarization of the laser beams utilized in the experiment. More significantly, an alternate combination of transitions between internal states of the ions, when combined with optimized polarization, enables faster entanglement and decreases the error by an order of magnitude.

quant-ph↗

arXiv2018

Coherently displaced oscillator quantum states of a single trapped atom

Coherently displaced harmonic oscillator number states of a harmonically bound ion can be coupled to two internal states of the ion by a laser-induced motional sideband interaction. The internal states can subsequently be read out in a projective measurement via state-dependent fluorescence, with near-unit fidelity. This leads to a rich set of line shapes when recording the internal-state excitation probability after a sideband excitation, as a function of the frequency detuning of the displacement drive with respect to the ion's motional frequency. We precisely characterize the coherent displacement based on the resulting line shapes, which exhibit sharp features that are useful for oscillator frequency determination from the single quantum regime up to very large coherent states with average occupation numbers of several hundred. We also introduce a technique based on multiple coherent displacements and free precession for characterizing noise on the trapping potential in the frequency range of 500 Hz to 400 kHz. Signals from the ion are directly used to find and eliminate sources of technical noise in this typically unaccessed part of the spectrum.

physics.atom-ph↗

arXiv2017

Preparation and coherent manipulation of pure quantum states of a single molecular ion

Laser cooling and trapping of atoms and atomic ions has led to numerous advances including the observation of exotic phases of matter, development of exquisite sensors and state-of-the-art atomic clocks. The same level of control in molecules could also lead to profound developments such as controlled chemical reactions and sensitive probes of fundamental theories, but the vibrational and rotational degrees of freedom in molecules pose a formidable challenge for controlling their quantum mechanical states. Here, we use quantum-logic spectroscopy (QLS) for preparation and nondestructive detection of quantum mechanical states in molecular ions. We develop a general technique to enable optical pumping and preparation of the molecule into a pure initial state. This allows for the observation of high-resolution spectra in a single ion (here CaH+) and coherent phenomena such as Rabi flopping and Ramsey fringes. The protocol requires a single, far-off resonant laser, which is not specific to the molecule, so that many other molecular ions, including polyatomic species, could be treated with the same methods in the same apparatus by changing the molecular source. Combined with long interrogation times afforded by ion traps, a broad range of molecular ions could be studied with unprecedented control and precision, representing a critical step towards proposed applications, such as precision molecular spectroscopy, stringent tests of fundamental physics, quantum computing, and precision control of molecular dynamics.

physics.atom-ph↗

arXiv2016

Hybrid quantum systems with trapped charged particles

We study theoretically the possibilities of coupling the quantum mechanical motion of a trapped charged particle (e.g. ion or electron) to quantum degrees of freedom of superconducting devices, nano-mechanical resonators and quartz bulk acoustic wave resonators. For each case, we estimate the coupling rate between the charged particle and its macroscopic counterpart and compare it to the decoherence rate, i.e. the rate at which quantum superposition decays. A hybrid system can only be considered quantum if the coupling rate significantly exceeds all decoherence rates. Our approach is to examine specific examples, using parameters that are experimentally attainable in the foreseeable future. We conclude that those hybrid quantum system considered involving an atomic ion are unfavorable, compared to using an electron, since the coupling rates between the charged particle and its counterpart are slower than the expected decoherence rates. A system based on trapped electrons, on the other hand, might have coupling rates which significantly exceed decoherence rates. Moreover it might have appealing properties such as fast entangling gates, long coherence and flexible electron interconnectivity topology. Realizing such a system, however, is technologically challenging, since it requires accommodating both trapping technology and superconducting circuitry in a compatible manner. We review some of the challenges involved, such as the required trap parameters, electron sources, electrical circuitry and cooling schemes in order to promote further investigations towards the realization of such a hybrid system.

quant-ph↗

arXiv2016

VECSEL systems for generation and manipulation of trapped magnesium ions

Experiments in atomic, molecular, and optical (AMO) physics rely on lasers at many different wavelengths and with varying requirements on spectral linewidth, power, and intensity stability. Vertical external-cavity surface-emitting lasers (VECSELs), when combined with nonlinear frequency conversion, can potentially replace many of the laser systems currently in use. Here we present and characterize VECSEL systems that can perform all laser-based tasks for quantum information processing experiments with trapped magnesium ions. For photoionization of neutral magnesium, 570.6$\,$nm light is generated with an intracavity frequency-doubled VECSEL containing a lithium triborate (LBO) crystal for second harmonic generation. External frequency doubling produces 285.3$\,$nm light for resonant interaction with the $^{1}S_{0}\leftrightarrow$ $^{1}P_{1}$ transition of neutral Mg. Using an externally frequency-quadrupled VECSEL, we implement Doppler cooling of $^{25}$Mg$^{+}$ on the 279.6$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{3/2}$ cycling transition, repumping on the 280.4$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{1/2}$ transition, coherent state manipulation, and resolved sideband cooling close to the motional ground state. Our systems serve as prototypes for applications in AMO requiring single-frequency, power-scalable laser sources at multiple wavelengths.

physics.atom-ph↗

arXiv2015

Freely configurable quantum simulator based on a two-dimensional array of individually trapped ions

A custom-built and precisely controlled quantum system may offer access to a fundamental understanding of another, less accessible system of interest. A universal quantum computer is currently out of reach, but an analog quantum simulator that makes the relevant observables, interactions, and states of a quantum model accessible could permit experimental insight into complex quantum dynamics that are intractable on conventional computers. Several platforms have been suggested and proof-of-principle experiments have been conducted. Here we characterise two-dimensional arrays of three ions trapped by radio-frequency fields in individually controlled harmonic wells forming equilateral triangles with side lengths 40 and 80 micrometer. In our approach, which is scalable to arbitrary two dimensional lattices, we demonstrate individual control of the electronic and motional degrees of freedom, preparation of a fiducial initial state with ion motion close to the ground state, as well as tuning of crucial couplings between ions within experimental sequences. Our work paves the way towards an analog quantum simulator of two-dimensional systems designed at will.

quant-ph↗

arXiv2015

Dissipative quantum control of a spin chain

A protocol is discussed for preparing a spin chain in a generic many-body state in the asymptotic limit of tailored non-unitary dynamics. The dynamics require the spectral resolution of the target state, optimized coherent pulses, engineered dissipation, and feedback. As an example, we discuss the preparation of an entangled antiferromagnetic state, and argue that the procedure can be applied to chains of trapped ions or Rydberg atoms.

quant-ph↗

arXiv2014

Single-mode optical fiber for high-power, low-loss UV transmission

We report large-mode-area solid-core photonic crystal fibers made from fused silica that resist ultraviolet (UV) solarization even at relatively high optical powers. Using a process of hydrogen loading and UV irradiation of the fibers, we demonstrate stable single-mode transmission over hundreds of hours for fiber output powers of 10 mW at 280 nm and 125 mW at 313 nm (limited only by the available laser power). Fiber attenuation ranges from 0.9 dB/m to 0.13 dB/m at these wavelengths, and is unaffected by bending for radii above 50 mm.

quant-ph↗

arXiv2014

Tunable spin-spin interactions and entanglement of ions in separate wells

Quantum simulation - the use of one quantum system to simulate a less controllable one - may provide an understanding of the many quantum systems which cannot be modeled using classical computers. Impressive progress on control and manipulation has been achieved for various quantum systems, but one of the remaining challenges is the implementation of scalable devices. In this regard, individual ions trapped in separate tunable potential wells are promising. Here we implement the basic features of this approach and demonstrate deterministic tuning of the Coulomb interaction between two ions, independently controlling their local wells. The scheme is suitable for emulating a range of spin-spin interactions, but to characterize the performance of our setup we select one that entangles the internal states of the two ions with 0.82(1) fidelity. Extension of this building-block to a 2D-network, which ion-trap micro-fabrication processes enable, may provide a new quantum simulator architecture with broad flexibility in designing and scaling the arrangement of ions and their mutual interactions. To perform useful quantum simulations, including those of intriguing condensed-matter phenomena such as the fractional quantum Hall effect, an array of tens of ions might be sufficient.

quant-ph↗

arXiv2014

Decoherence-assisted spectroscopy of a single Mg$^+$ ion

We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly at rest are recorded efficiently with high signal-to-noise ratios. Spectra display symmetric line shapes without stray-light background from spectroscopy probes. We employ this method on a $^{25}$Mg$^+$ ion to measure one, two, and three-photon transition frequencies from the 3S ground state to the 3P, 3D, and 4P excited states, respectively. Our results are relevant for astrophysics and searches for drifts of fundamental constants. Furthermore, the method can be extended to other transitions, isotopes, and species. The currently achieved fractional frequency uncertainty of $5 \times 10^{-9}$ is not limited by the method.

physics.atom-ph↗

arXiv2011

Quantum simulation of the hexagonal Kitaev model with trapped ions

We present a detailed study of quantum simulations of coupled spin systems in surface-electrode ion-trap arrays, and illustrate our findings with a proposed implementation of the hexagonal Kitaev model [A. Kitaev, Annals of Physics 321,2 (2006)]. The effective (pseudo)spin interactions making up such quantum simulators are found to be proportional to the dipole-dipole interaction between the trapped ions, and are mediated by motion which can be driven by state-dependent forces. The precise forms of the trapping potentials and the interactions are derived in the presence of a surface electrode and a cover electrode. These results are the starting point to derive an optimized surface-electrode geometry for trapping ions in the desired honeycomb lattice of Kitaev's model, where we design the dipole-dipole interactions in a way that allows for coupling all three bond types of the model simultaneously, without the need for time discretization. Finally we propose a simple wire structure that can be incorporated in a microfabricated chip to generate localized state-dependent forces which drive the couplings prescribed by this particular model; such a wire structure should be adaptable to many other situations.

quant-ph↗

arXiv2011

A 750 mW, continuous-wave, solid-state laser source at 313 nm for cooling and manipulating trapped 9Be+ ions

We present a solid-state laser system that generates 750 mW of continuous-wave single-frequency output at 313 nm. Sum-frequency generation with fiber lasers at 1550 nm and 1051 nm produces up to 2 W at 626 nm. This visible light is then converted to UV by cavity-enhanced second-harmonic generation. The laser output can be tuned over a 495 GHz range, which includes the 9Be+ laser cooling and repumping transitions. This is the first report of a narrow-linewidth laser system with sufficient power to perform fault-tolerant quantum-gate operations with trapped 9Be+ ions by use of stimulated Raman transitions.

quant-ph↗

arXiv2010

Optimized magnetic lattices for ultracold atomic ensembles

We introduce a general method for designing tailored lattices of magnetic microtraps for ultracold atoms, on the basis of patterned permanently magnetized films. A fast numerical algorithm is used to automatically generate patterns which provide optimal atom confinement while respecting desired lattice symmetries and trap parameters. The algorithm can produce finite and infinite lattices of any plane symmetry; we focus specifically on square and triangular lattices which are of interest to future experiments. Typical trap parameters are discussed as well as the impact of realistic imperfections such as finite lithographic resolution and magnetic inhomogeneity. The presented designer lattices open new avenues for quantum simulation and quantum information processing with ultracold atoms on atom chips.

quant-ph↗

arXiv2009

Quantum walk on a line for a trapped ion

We show that a multi-step quantum walk can be realized for a single trapped ion with interpolation between quantum and random walk achieved by randomizing the generalized Hadamard coin flip phase. The signature of the quantum walk is manifested not only in the ion's position but also its phonon number, which makes an ion trap implementation of the quantum walk feasible.

quant-ph↗