arXiv subjects

Dietrich Leibfried

Publications and source records attributed to Dietrich Leibfried.

At least 19 recordsLinked to original sources

arXiv2026

Quantum signatures of proper time in optical ion clocks

Optical clocks based on atoms and ions probe relativistic effects with unprecedented sensitivity by resolving time dilation due to atom motion or different positions in the gravitational potential through frequency shifts. However, all measurements of time dilation so far can be explained effectively as the result of dynamics with respect to a classical proper time parameter. Here we show that atomic clocks can probe effects where a classical description of the proper time dynamics is insufficient. We apply a Hamiltonian formalism to derive time dilation effects in harmonically trapped clock atoms and show how second-order Doppler shifts (SODS) due to the vacuum energy (vSODS), squeezing (sqSODS) and quantum corrections to the dynamics (qSODS) arise. We also demonstrate that the entanglement between motion and clock evolution can become observable in state-of-the-art clocks when the motion of the atoms is strongly squeezed, realizing proper time interferometry. Our results show that experiments with trapped ion clocks are within reach to probe relativistic evolution of clocks for which a quantum description of proper time becomes necessary.

quant-ph↗

arXiv2026

Robust Two-Qubit Geometric Phase Gates using Amplitude and Frequency Ramping

We demonstrate a method for generating entanglement between trapped atomic ions based on adiabatically ramped state-dependent forces. By ramping both the amplitude of the state-dependent force and the motional mode frequencies, we realize an entangling operation that is robust to motional mode occupation and drifts in the mode frequencies. We measure Bell state fidelities above 0.99 across a broad range of ramp parameters and with motional occupations up to 10 phonons. This technique enables high-fidelity entangling operations without ground-state cooling, has a reduced calibration overhead, and is well suited for both quantum logic spectroscopy applications and scalable quantum computing architectures.

quant-ph↗

arXiv2025

Observation of a Topological Berry Phase with a Single Phonon in an Ion Microtrap Array

Controlled quantum mechanical motion of trapped atomic ions can be used to simulate and explore collective quantum phenomena and to process quantum information. Groups of cold atomic ions in an externally applied trapping potential self-organize into "Coulomb crystals" due to their mutual electrostatic repulsion. The motion of the ions in these crystals is strongly coupled, and the eigenmodes of motion all involve multiple ions. While this enables studies of many-body physics, it limits the flexibility and tunability of the system as a quantum platform. Here, we demonstrate an array of trapped ions in individual trapping sites whose motional modes can be controllably coupled and decoupled by tuning the local applied confining potential for each ion. We show that a single motional quantum, or phonon, can be coherently shared among two or three ions confined at the vertices of an equilateral triangle 30 $μ$m on a side. We can adiabatically tune the ion participation in the motional modes around a closed contour in configuration space, observing that the single-phonon wavefunction acquires a topological Berry phase if the contour encircles a conical intersection of motional eigenvalue surfaces. We observe this phase by single-phonon interference and study its breakdown as the motional mode tuning becomes non-adiabiatic. Our results show that precise, individual quantum control of ion motion in a two-dimensional array can provide unique access to quantum multi-body effects.

quant-ph↗

arXiv2025

High-fidelity quantum state control of a polar molecular ion in a cryogenic environment

We use a quantum-logic spectroscopy (QLS) protocol to control the quantum state of a CaH+ ion in a cryogenic environment, in which reduced thermal radiation extends rotational state lifetimes by an order of magnitude over those at room temperature. By repeatedly and adaptively probing the molecule, detecting the outcome of each probe via an atomic ion, and using a Bayesian update scheme to quantify confidence in the molecular state, we demonstrate state preparation and measurement (SPAM) in a single quantum state with infidelity less than 6x10^-3 and measure Rabi flopping between two states with greater than 99% contrast. The protocol does not require any molecule-specific lasers and the detection scheme is non-destructive.

physics.atom-ph↗

arXiv2024

Individual Addressing and State Readout of Trapped Ions Utilizing Radio-Frequency Micromotion

Excess "micromotion" of trapped ions due to the residual radio-frequency (rf) trapping field at their location is often undesirable and is usually carefully minimized. Here, we induce precise amounts of excess micromotion on individual ions by adjusting the local static electric field they experience. Micromotion modulates the coupling of an ion to laser fields, ideally tuning it from its maximum value to zero as the ion is moved away from the trap's rf null. We use tunable micromotion to vary the Rabi frequency of stimulated Raman transitions over two orders of magnitude, and to individually control the rates of resonant fluorescence from three ions under global laser illumination without any changes to the driving light fields. The technique is amenable to situations where addressing individual ions with focused laser beams is challenging, such as tightly packed linear ion strings or two-dimensional ion arrays illuminated from the side.

physics.atom-ph↗

arXiv2024

Quantum state tracking and control of a single molecular ion in a thermal environment

Understanding molecular state evolution is central to many disciplines, including molecular dynamics, precision measurement, and molecule-based quantum technology. Details of the evolution are obscured when observing a statistical ensemble of molecules. Here, we reported real-time observations of thermal radiation-driven transitions between individual states ("jumps") of a single molecule. We reversed these "jumps" through microwave-driven transitions, resulting in a twentyfold improvement in the time the molecule dwells in a chosen state. The measured transition rates showed anisotropy in the thermal environment, pointing to the possibility of using single molecules as in-situ probes for the strengths of ambient fields. Our approaches for state detection and manipulation could apply to a wide range of species, facilitating their uses in fields including quantum science, molecular physics, and ion-neutral chemistry.

physics.atom-ph↗

arXiv2024

Coherent coupling and non-destructive measurement of trapped-ion mechanical oscillators

Precise quantum control and measurement of several harmonic oscillators, such as the modes of the electromagnetic field in a cavity or of mechanical motion, are key for their use as quantum platforms. The motional modes of trapped ions can be individually controlled and have good coherence properties. However, achieving high-fidelity two-mode operations and nondestructive measurements of the motional state has been challenging. Here we demonstrate the coherent exchange of single motional quanta between spectrally separated harmonic motional modes of a trapped-ion crystal. The timing, strength, and phase of the coupling are controlled through an oscillating electric potential with suitable spatial variation. Coupling rates that are much larger than decoherence rates enable demonstrations of high fidelity quantum state transfer and beamsplitter operations, entanglement of motional modes, and Hong-Ou-Mandel-type interference. Additionally, we use the motional coupling to enable repeated non-destructive projective measurement of a trapped-ion motional state. Our work enhances the suitability of trapped-ion motion for continuous-variable quantum computing and error correction and may provide opportunities to improve the performance of motional cooling and motion-mediated entangling interactions.

quant-ph↗

arXiv2024

Fast Ground State to Ground State Separation of Small Ion Crystals

Rapid separation of linear crystals of trapped ions into different subsets is critical for realizing trapped ion quantum computing architectures where ions are rearranged in trap arrays to achieve all-to-all connectivity between qubits. We introduce a general theoretical framework that can be used to describe the separation of same-species and mixed-species crystals into smaller subsets. The framework relies on an efficient description of the evolution of Gaussian motional states under quadratic Hamiltonians that only requires a special solution of the classical equations of motion of the ions to describe their quantum evolution under the influence of a time-dependent applied potential and the ions' mutual Coulomb repulsion. We provide time-dependent applied potentials suitable for separation of a mixed species three-ion crystal on timescales similar to that of free expansion driven by Coulomb repulsion, with all modes along the crystal axis starting and ending close to their ground states. Three separately-confined mixed species ions can be combined into a crystal held in a single well without energy gain by time-reversal of this separation process.

quant-ph↗

arXiv2024

Indirect Cooling of Weakly Coupled Trapped-Ion Mechanical Oscillators

Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool due to weak or zero interaction between the modes and the cooling radiation, typically laser beams. We overcome this challenge by coupling a mode with weak cooling radiation interaction to one with strong cooling radiation interaction using parametric modulation of the trapping potential, thereby enabling indirect cooling of the former. In this way, we demonstrate near-ground-state cooling of motional modes with weak or zero cooling radiation interaction in multi-ion crystals of the same and mixed ion species, specifically $^9$Be$^+$-$^9$Be$^+$, $^9$Be$^+$-$^{25}$Mg$^+$, and $^9$Be$^+$-$^{25}$Mg$^+$-$^9$Be$^+$ crystals. This approach can be generally applied to any Coulomb crystal where certain motional modes cannot be directly cooled efficiently, including crystals containing molecular ions, highly-charged ions, charged fundamental particles, or charged macroscopic objects.

quant-ph↗

arXiv2023

Optimized experiment design and analysis for fully randomized benchmarking

Randomized benchmarking (RB) is a widely used strategy to assess the quality of available quantum gates in a computational context. RB involves applying known random sequences of gates to an initial state and using the statistics of a final measurement step to determine an effective depolarizing error per step of the sequence, which is a metric of gate quality. Here we investigate the advantages of fully randomized benchmarking, where a new random sequence is drawn for each experimental trial. The advantages of full randomization include smaller confidence intervals on the inferred step error, the ability to use maximum likelihood analysis without heuristics, straightforward optimization of the sequence lengths, and the ability to model and measure behaviors that go beyond the typical assumption of time-independent error rates. We discuss models of time-dependent or non-Markovian errors that generalize the basic RB model of a single exponential decay of the success probability. For any of these models, we implement a concrete protocol to minimize the uncertainty of the estimated parameters given a fixed time constraint on the complete experiment, and we implement a maximum likelihood analysis. We consider several previously published experiments and determine the potential for improvements with optimized full randomization. We experimentally observe such improvements in Clifford randomized benchmarking experiments on a single trapped ion qubit at the National Institute of Standards and Technology (NIST). For an experiment with uniform lengths and intentionally repeated sequences the step error was $2.42^{+0.30}_{-0.22}\times 10^{-5}$, and for an optimized fully randomized experiment of the same total duration the step error was $2.57^{+0.07}_{-0.06}\times 10^{-5}$. We find a substantial decrease in the uncertainty of the step error as a result of optimized fully randomized benchmarking.

quant-ph↗

arXiv2023

Trap-Integrated Superconducting Nanowire Single-Photon Detectors with Improved RF Tolerance for Trapped-Ion Qubit State Readout

State readout of trapped-ion qubits with trap-integrated detectors can address important challenges for scalable quantum computing, but the strong rf electric fields used for trapping can impact detector performance. Here, we report on NbTiN superconducting nanowire single-photon detectors (SNSPDs) employing grounded aluminum mirrors as electrical shielding that are integrated into linear surface-electrode rf ion traps. The shielded SNSPDs can be successfully operated at applied rf trapping potentials of up to $\mathrm{54\,V_{peak}}$ at $\mathrm{70\,MHz}$ and temperatures of up to $\mathrm{6\,K}$, with a maximum system detection efficiency of $\mathrm{68\,\%}$. This performance should be sufficient to enable parallel high-fidelity state readout of a wide range of trapped ion species in typical cryogenic apparatus.

quant-ph↗

arXiv2022

Rotational spectroscopy of a single molecular ion at sub part-per-trillion resolution

We use quantum-logic spectroscopy (QLS) and interrogate rotational transitions of a single CaH+ ion with a highly coherent frequency comb, achieving a fractional statistical uncertainty for a transition line center of 4 x 10^-13. We also improve the resolution in measurement of the Stark effect due to the radio-frequency (rf) electric field experienced by a molecular ion in an rf Paul trap, which we characterize and model. This allows us to determine the electric dipole moment of CaH+ by systematically displacing the ion to sample different known rf electric fields and measuring the resultant shifts in transition frequency.

physics.atom-ph↗

arXiv2021

High-fidelity indirect readout of trapped-ion hyperfine qubits

We propose and demonstrate a protocol for high-fidelity indirect readout of trapped ion hyperfine qubits, where the state of a $^9\text{Be}^+$ qubit ion is mapped to a $^{25}\text{Mg}^+$ readout ion using laser-driven Raman transitions. By partitioning the $^9\text{Be}^+$ ground state hyperfine manifold into two subspaces representing the two qubit states and choosing appropriate laser parameters, the protocol can be made robust to spontaneous photon scattering errors on the Raman transitions, enabling repetition for increased readout fidelity. We demonstrate combined readout and back-action errors for the two subspaces of $1.2^{+1.1}_{-0.6} \times 10^{-4}$ and $0^{+1.9}_{-0} \times 10^{-5}$ with 68% confidence while avoiding decoherence of spectator qubits due to stray resonant light that is inherent to direct fluorescence detection.

quant-ph↗

arXiv2021

Feasibility study of quantum computing using trapped electrons

We investigate the feasibility of using electrons in a linear Paul trap as qubits in a future quantum computer. We discuss the necessary experimental steps to realize such a device through a concrete design proposal, including trapping, cooling, electronic detection, spin readout and single and multi-qubit gate operations. Numeric simulations indicate that two-qubit Bell-state fidelities of order 99.99% can be achieved assuming reasonable experimental parameters.

quant-ph↗

arXiv2021

Measurement of electric-field noise from interchangeable samples with a trapped-ion sensor

We demonstrate the use of a single trapped ion as a sensor to probe electric-field noise from interchangeable test surfaces. As proof of principle, we measure the magnitude and distance dependence of electric-field noise from two ion-trap-like samples with patterned Au electrodes. This trapped-ion sensor could be combined with other surface characterization tools to help elucidate the mechanisms that give rise to electric-field noise from ion-trap surfaces. Such noise presents a significant hurdle for performing large-scale trapped-ion quantum computations.

physics.atom-ph↗

arXiv2021

Resource-efficient dissipative entanglement of two trapped-ion qubits

We demonstrate a simplified method for dissipative generation of an entangled state of two trapped-ion qubits. Our implementation produces its target state faster and with higher fidelity than previous demonstrations of dissipative entanglement generation and eliminates the need for auxiliary ions. The entangled singlet state is generated in $\sim$7 ms with a fidelity of 0.949(4). The dominant source of infidelity is photon scattering. We discuss this error source and strategies for its mitigation.

quant-ph↗

arXiv2021

Quantum harmonic oscillator spectrum analyzers

Characterization and suppression of noise are essential for the control of harmonic oscillators in the quantum regime. We measure the noise spectrum of a quantum harmonic oscillator from low frequency to near the oscillator resonance by sensing its response to amplitude modulated periodic drives with a qubit. Using the motion of a trapped ion, we experimentally demonstrate two different implementations with combined sensitivity to noise from 500 Hz to 600 kHz. We apply our method to measure the intrinsic noise spectrum of an ion trap potential in a previously unaccessed frequency range.

quant-ph↗

arXiv2021

Dissipative preparation of W states in trapped ion systems

We present protocols for dissipative entanglement of three trapped-ion qubits and discuss a scheme that uses sympathetic cooling as the dissipation mechanism. This scheme relies on tailored destructive interference to generate any one of six entangled W states in a three-ion qubit space. Using a beryllium-magnesium ion crystal as an example system, we theoretically investigate the protocol's performance and the effects of likely error sources, including thermal secular motion of the ion crystal, calibration imperfections, and spontaneous photon scattering. We estimate that a fidelity of $\sim$ 98 % may be achieved in typical trapped ion experiments with $\sim$ 1 ms interaction time. These protocols avoid timescale hierarchies for faster preparation of entangled states.

quant-ph↗