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Dmitry N. Krizhanovskii

Publications and source records attributed to Dmitry N. Krizhanovskii.

11 recordsLinked to original sources

All-optical nonlinear phase modulation in open semiconductor microcavities

We report a significant advancement in ultra low power light-by-light phase modulation using open semiconductor microcavities in the strong light-matter coupling regime. We achieve cross-phase modulation of up to 247$\pm$17 mrad per particle between laser beams attenuated to single-photon average intensities. This breakthrough extends the potential for quantum information processing and nonlinear quantum optics in strongly coupled light-matter systems, setting a new benchmark in the field without relying on atom-like emitters. Our findings suggest promising new avenues for scalable quantum optical technologies.

physics.optics↗

Flat-band compactons in a two-dimensional driven-dissipative Lieb lattice

We experimentally study the effect of inter-particle interactions on the flat-band states of a two-dimensional Lieb lattice with drive and dissipation. Exploiting the giant nonlinear interactions of exciton polaritons we observe compactly localised solitons (compactons) embedded within the continuum of propagating state bands -- a form of nonlinear bound state in the continuum (BIC). The driven-dissipative nature of the system leads to a sudden self-localisation into the compacton state above a threshold power. The experimental results agree well with numerical simulations. These results have implications for the physics of interacting quantum particles in flat-band systems and for generation of quantum-correlated light and spatially multiplexed coherent information transport.

cond-mat.other↗

Realization of Z$_2$ topological photonic insulators made from multilayer transition metal dichalcogenides

Monolayers of semiconducting transition metal dichalcogenides (TMDs) have long attracted interest for their intriguing optical and electronic properties. Recently TMDs in their quasi-bulk form have started to show considerable promise for nanophotonics thanks to their high refractive indices, large optical anisotropy, wide transparency windows reaching to the visible, and robust room temperature excitons promising for nonlinear optics. Adherence of TMD layers to any substrate via van der Waals forces is a further key enabler for nanofabrication of sophisticated photonic structures requiring heterointegration. Here, we capitalize on these attractive properties and realize topological spin-Hall photonic lattices made of arrays of triangular nanoholes in 50 to 100 nm thick WS$_2$ flakes exfoliated on SiO$_2$/Si substrates. High quality structures are achieved taking advantage of anisotropic dry etching dictated by the crystal axes of WS$_2$. Reflectance measurements at room temperature show a photonic gap opening in the near-infrared in trivial and topological phases. Unidirectional propagation along the domain interface is demonstrated in real space via circularly polarized laser excitation in samples with both zigzag and armchair domain boundaries. Finite-difference time-domain simulations are used to interpret optical spectroscopy results. Our work opens the way for future sophisticated nanophotonic devices based on the layered (van der Waals) materials platform.

physics.optics↗

Electrostatic control of nonlinear photonic-crystal polaritons in a monolayer semiconductor

Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of practical devices, it is crucial that the polariton excitations in the structure are easily tunable and exhibit strong nonlinear response. Here we study neutral and charged exciton-polaritons in an electrostatically gated planar photonic crystal slab with an embedded monolayer semiconductor MoSe$_2$ and experimentally demonstrate strong polariton nonlinearity, which can be tuned via gate voltage. We find that modulation of dielectric environment within the photonic crystal results in the formation of two distinct resonances with significantly different nonlinear response, which enables optical switching with ultrashort laser pulses. Our results open new avenues towards development of active polaritonic devices in a compact chip-compatible implementation.

cond-mat.mes-hall↗

Probing and control of guided exciton-polaritons in a 2D semiconductor-integrated slab waveguide

Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are characterized by long propagation distances and efficient nonlinear interaction but cannot be directly accessed from the free space. Here we demonstrate a powerful approach for probing and manipulating guided polaritons in a Ta2O5 slab integrated with a WS2 monolayer using evanescent coupling through a high-index solid immersion lens. Tuning the nanoscale lens-sample gap allows for extracting all the intrinsic parameters of the system. We also demonstrate the transition from weak to strong coupling accompanied by the onset of the motional narrowing effect: with the increase of exciton-photon coupling strength, the inhomogeneous contribution to polariton linewidth, inherited from the exciton resonance, becomes fully lifted. Our results enable the development of integrated optics employing room-temperature exciton-polaritons in 2D semiconductor-based structures.

physics.optics↗

Observation of Zitterbewegung in photonic microcavities

We present and experimentally study the effects of the photonic spin-orbit coupling on real space propagetion of polariton wavepackets in planar semiconductor microcavities and polaritonic analogs of graphene. In particular, we demonstrate the appearance of an analog Zitterbewegung effect, a term which translates as 'trembling motion' in english, which was originally proposed for relativistic Dirac electrons and consists of the oscillations of the center of mass of a wavepacket in the direction perpendicular to its propagation. For a planar microcavity we observe regular Zitterbewegung oscillations whose amplitude and period depend on the wavevector of the polaritons. We then extend these results to a honeycomb lattice of coupled microcavity resonators. Compared to the planar cavity such lattices are inherently more tuneable and versatile, allowing simulation of the Hamilitonians of a wide range of important physical systems. We observe an oscillation pattern related to the presence of the spin-split Dirac cones in the dispersion. In both cases the experimentally observed oscillations are in good agreement with theoretical modelling and independently measured bandstructure parameters, providing strong evidence for the observation of Zitterbewegung.

physics.optics↗

Photoluminescence imaging of single photon emitters within nanoscale strain profiles in monolayer WSe$_2$

Local deformation of atomically thin van der Waals materials provides a powerful approach to create site-controlled chip-compatible single-photon emitters (SPEs). However, the microscopic mechanisms underlying the formation of such strain-induced SPEs are still not fully clear, which hinders further efforts in their deterministic integration with nanophotonic structures for developing practical on-chip sources of quantum light. Here we investigate SPEs with single-photon purity up to 98% created in monolayer WSe$_2$ via nanoindentation. Using photoluminescence imaging in combination with atomic force microscopy, we locate single-photon emitting sites on a deep sub-wavelength spatial scale and reconstruct the details of the surrounding local strain potential. The obtained results suggest that the origin of the observed single-photon emission is likely related to strain-induced spectral shift of dark excitonic states and their hybridization with localized states of individual defects.

cond-mat.mes-hall↗

Polariton lasing in AlGaN microring with GaN/AlGaN quantum wells

Microcavity polaritons are strongly interacting hybrid light-matter quasiparticles, which are promising for the development of novel light sources and active photonic devices. Here, we report polariton lasing in the UV spectral range in microring resonators based on GaN/AlGaN slab waveguides, with experiments carried out from 4 K up to room temperature. Stimulated polariton relaxation into multiple ring resonator modes is observed, which exhibit threshold-like dependence of the emission intensity with pulse energy. The strong exciton-photon coupling regime is confirmed by the significant reduction of the free spectral range with energy and the blueshift of the exciton-like modes with increasing pulse energy. Importantly, the exciton emission shows no broadening with power, further confirming that lasing is observed at electron-hole densities well below the Mott transition. Overall, our work paves the way towards development of novel UV devices based on the high-speed slab waveguide polariton geometry operating up to room temperature with potential to be integrated into complex photonic circuits.

physics.optics↗

Few-photon all-optical phase rotation in a quantum-well micropillar cavity

Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be provided by optical nonlinearities in the form of cross-phase-modulation (XPM). This approach underpins many proposed applications in quantum optics and information processing, but achieving its potential requires strong single-photon-level nonlinear phase shifts and also scalable nonlinear elements. In this work we show that the required nonlinearity can be provided by exciton-polaritons in micropillars with embedded quantum wells. These combine the strong interactions of excitons with the scalability of micrometer-sized emitters. We observe XPM up to $3 \pm 1$ mrad per particle using laser beams attenuated to below single photon average intensity. With our work serving as a first stepping stone, we lay down a route for quantum information processing in polaritonic lattices.

physics.optics↗

Ultrafast-nonlinear ultraviolet pulse modulation in an AlInGaN polariton waveguide operating up to room temperature

Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on sub-picosecond timescales and on length scales suitable for integrated photonics. Currently there is no platform that can provide this for the UV spectral range where broadband spectra generated by nonlinear modulation can pave the way to new on-chip ultrafast (bio-) chemical spectroscopy devices. We demonstrate the giant nonlinearity of UV hybrid light-matter states (exciton-polaritons) up to room temperature in an AlInGaN waveguide. We experimentally measure ultrafast nonlinear spectral broadening of UV pulses in a compact 100 $μ$m long device and deduce a nonlinearity 1000 times that in common UV nonlinear materials and comparable to non-UV polariton devices. Our demonstration promises to underpin a new generation of integrated UV nonlinear light sources for advanced spectroscopy and measurement.

physics.optics↗

Logic Gates with Bright Dissipative Polariton Solitons in Bragg-Cavity Systems

Optical solitons are an ideal platform for the implementation of communication lines, since they can be packed extremely close one to another without risking partial loss of the encoded information due to their interaction. On the other hand, soliton-soliton interactions are needed to implement computations and achieve all-optical information processing. Here we study how bright dissipative polariton solitons interact and exploit their interaction to implement AND and OR gates with state of the art technology. Moreover, we show that soliton-soliton interaction can be used to determine the sign of α2, the parameter describing the interaction between polaritons with opposite spin.

cond-mat.other↗