arXiv subjects

Domenico Montemurro

Publications and source records attributed to Domenico Montemurro.

At least 19 recordsLinked to original sources

arXiv2025

Quantifying Twist Angles in Cuprate Heterostructures with Anisotropic Raman Signatures

Artificially engineered twisted van der Waals (vdW) heterostructures have unlocked new pathways for exploring emergent quantum phenomena and strongly correlated electronic states. Many of these phenomena are highly sensitive to the twist angle, which can be deliberately tuned to tailor the interlayer interactions. This makes the twist angle a critical tunable parameter, emphasizing the need for precise control and accurate characterization during device fabrication. In particular, twisted cuprate heterostructures based on Bi2Sr2CaCu2O8+x have demonstrated angle-dependent superconducting properties, positioning the twist angle as a key tunable parameter. However, the twisted interface is highly unstable under ambient conditions and vulnerable to damage from conventional characterization tools such as electron microscopy or scanning probe techniques. In this work, we introduce a fully non-invasive, polarization-resolved Raman spectroscopy approach for determining twist angles in artificially stacked BSCCO heterostructures. By analyzing twist-dependent anisotropic vibrational Raman modes, particularly utilizing the out-of-plane A1g vibrational mode of Bi/Sr at 116 cm-1, we identify clear optical fingerprints of the rotational misalignment between cuprate layers. Our high-resolution confocal Raman setup, equipped with polarization control and RayShield filtering down to 10 cm-1, allows for reliable and reproducible measurements without compromising the material's structural integrity.

cond-mat.supr-con↗

arXiv2025

Preserving the Josephson Coupling of Twisted Cuprate Junctions via Tailored Silicon Nitride Circuits Boards

Controlled fabrication of twisted van der Waals heterostructures is essential to unlock the full potential of moire materials. However, achieving reproducibility remains a major challenge, particularly for air-sensitive materials such as $Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}$ (BSCCO), where it is crucial to preserve the intrinsic and delicate superconducting properties of the interface throughout the entire fabrication process. Here, we present a dry, inert and cryogenic assembly method that combines silicon nitride nanomembranes (NMBs) with pre-patterned electrodes and the cryogenic stacking technique (CST) to fabricate high-quality twisted BSCCO Josephson junctions (JJs). This protocol prevents thermal and chemical degradation during both interface formation and electrical contact integration. We also find that asymmetric membrane designs, such as a double cantilever, effectively suppress vibration-induced disorder due to wire bonding, resulting in sharp and hysteretic current-voltage characteristics. The junctions exhibit a twist-angle-dependent Josephson coupling with magnitudes comparable to the highest-performing devices reported to date, but achieved through a straightforward and versatile contact method, offering a scalable and adaptable platform for future applications. These findings highlight the importance of both interface and contact engineering in addressing reproducibility in superconducting van der Waals heterostructures.

cond-mat.supr-con↗

arXiv2025

Cuprate Twistronics for Quantum Hardware

Recent advances in the manipulation of complex oxide layers, particularly the fabrication of atomically thin cuprate superconducting films via molecular beam epitaxy, have revealed new ways in which nanoscale engineering can govern superconductivity and its interwoven electronic orders. In parallel, the creation of twisted cuprate heterostructures through cryogenic stacking techniques marks a pivotal step forward, exploiting cuprate superconductors to deepen our understanding of exotic quantum states and propel next-generation quantum technologies. This review explores over three decades of research in the emerging field of cuprate twistronics, examining both experimental breakthroughs and theoretical progress. It also highlights the methodologies poised to surmount the outstanding challenges in leveraging these complex quantum materials, underscoring their potential to expand the frontiers of quantum science and technology.

cond-mat.supr-con↗

arXiv2025

Implementation and readout of maximally entangled two-qubit gates quantum circuits in a superconducting quantum processor

Besides noticeable challenges in implementing low-error single- and two-qubit quantum gates in superconducting quantum processors, the readout technique and analysis are a key factor in determining the efficiency and performance of quantum processors. Being able to efficiently implement quantum algorithms involving entangling gates and asses their output is mandatory for quantum utility. In a transmon-based 5-qubit superconducting quantum processor, we compared the performance of quantum circuits involving an increasing level of complexity, from single-qubit circuits to maximally entangled Bell circuits. This comparison highlighted the importance of the readout analysis and helped us optimize the protocol for more advanced quantum algorithms. Here we report the results obtained from the analysis of the outputs of quantum circuits using two readout paradigms, referred to as "multiplied readout probabilities" and "conditional readout probabilities". The first method is suitable for single-qubit circuits, while the second is essential for accurately interpreting the outputs of circuits involving two-qubit gates.

quant-ph↗

arXiv2025

Nanoscale spin ordering and spin screening effects in tunnel ferromagnetic Josephson junctions

Magnetic Josephson junctions (MJJs) have emerged as a prominent playground to explore the interplay between superconductivity and ferromagnetism. A series of fascinating experiments have revealed striking phenomena at the Superconductor/Ferromagnet (S/F) interface, pointing to tunable phase transitions and to the generation of unconventional spin-triplet correlations. Here, we show that the Josephson effect, being sensitive to phase space variation on the nanoscale, allows a direct observation of the spin polarization of the S/F interface. By measuring the temperature dependence of the Josephson magnetic field patterns of tunnel MJJs with strong and thin F-layer, we demonstrate an induced nanoscale spin order in S along the superconducting coherence length at S/F interface, i.e., the inverse proximity effect, with the first evidence of full spin screening at very low temperatures, as expected by the theory. A comprehensive phase diagram for spin nanoscale ordering regimes at S/F interfaces in MJJs has been derived in terms of the magnetic moment induced in the S-layer. Our findings contribute to drive the design and the tailoring of S/F interfaces also in view of potential applications in quantum computing.

cond-mat.supr-con↗

arXiv2025

Exploring van der Waals cuprate superconductors using a hybrid microwave circuit

The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. In this study, we investigate the superconducting properties of Bi2Sr2CaCu2O8+x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor. We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.

cond-mat.supr-con↗

arXiv2024

Towards novel tunability schemes for hybrid ferromagnetic transmon qubits

Flux tuning of qubit frequencies in superconducting quantum processors is fundamental for implementing single and multi-qubit gates in quantum algorithms. Typical architectures involve the use of DC or fast RF lines. However, these lines introduce significant heat dissipation and undesirable decoherence mechanisms, leading to a severe bottleneck for scalability. Among different solutions to overcome this issue, we propose integrating tunnel Superconductor-Insulating-thin superconducting interlayer-Ferromagnet-Superconductor Josephson junctions (SIsFS JJs) into a novel transmon qubit design, the so-called ferrotransmon. SIsFS JJs provide memory properties due to the presence of ferromagnetic barriers and preserve at the same time the low-dissipative behavior of tunnel-insulating JJs, thus promoting an alternative tuning of the qubit frequency. In this work, we discuss the fundamental steps towards the implementation of this hybrid ferromagnetic transmon. We will give a special focus on the design, simulations, and preliminary experimental characterization of superconducting lines to provide in-plane magnetic fields, fundamental for an on-chip control of the qubit frequencies in the ferrotransmon.

cond-mat.supr-con↗

arXiv2024

Evidence of the inverse proximity effect in tunnel magnetic Josephson Junctions

Magnetic Josephson Junctions (MJJs) are a special class of hybrid systems where antagonistic correlations coexist, thus providing a key for advances in weak superconductivity, superconducting spintronics and quantum computation. So far, the memory properties of MJJs have been mostly investigated in view of digital electronics and for spintronic devices at liquid-helium temperature. At the operating temperature of quantum circuits, a magnetic order can rise in a Superconductor (S) at the S/Ferromagnet (F) interface, i.e., the inverse proximity effect (IPE), thus leading to a significant modification of the magnetic field patterns in MJJs. In this work, we have carried out a comparative investigation of the magnetic behavior of tunnel MJJs with a strong ferromagnetic layer inserted in the layout of both Nb and Al JJs, respectively. The comparative analysis validates the crucial role of the temperature, the fundamental scaling energies of S/F coupling systems, and the transparency of the S/F interface. This investigation points out that the IPE is a key aspect to consider when designing tunnel MJJs operating well below 4 K and thus in the perspective of hybrid superconducting quantum architectures.

cond-mat.supr-con↗

arXiv2024

Phase dynamics of tunnel Al-based ferromagnetic Josephson junctions

By measuring the current-voltage characteristics and the switching current distributions as a function of temperature, we have investigated the phase dynamics of Al tunnel ferromagnetic Josephson junctions (JJs), designed to fall in the typical range of parameters of state-of-the-art transmons, providing evidence of phase diffusion processes. The comparison with the experimental outcomes on non-magnetic JJs with nominally the same electrodynamical parameters demonstrates that the introduction of ferromagnetic barriers does not cause any sizeable detrimental effect, and supports the notion of including tunnel ferromagnetic JJs in qubit architectures.

cond-mat.supr-con↗

arXiv2024

Twisted cuprate van der Waals heterostructures with controlled Josephson coupling

Twisted van der Waals (vdW) heterostructures offer a unique platform for engineering the efficient Josephson coupling between cuprate thin crystals harboring the nodal superconducting order parameter. Preparing vdW heterostructures-based Josephson junction comprising stacked cuprates requires maintaining an ordered interface with preserved surface superconductivity. Here, we report the preparation of the Josephson junction out of the stacked Bi2Sr2CuCa2O8+d crystals using the cryogenic dry transfer technique and encapsulating the junction with an insulating layer, that protects the interface during the electrical contacts evaporation at the 10-6 mbar base pressure. We find that the Josephson critical current Ic has a maximum at low twist angles, comparable to that of the bulk intrinsic Josephson junctions, and is reduced by two orders of magnitude at twist angles close to 45°. The reduction of Ic occurs due to a mismatch between superconducting d-wave order parameters, which suppresses the direct Cooper pair tunneling.

cond-mat.supr-con↗

arXiv2024

Mitigating Errors on Superconducting Quantum Processors through Fuzzy Clustering

Quantum utility has been severely limited in superconducting quantum hardware until now by the modest number of qubits and the relatively high level of control and readout errors, due to the intentional coupling with the external environment required for manipulation and readout of the qubit states. Practical applications in the Noisy Intermediate Scale Quantum (NISQ) era rely on Quantum Error Mitigation (QEM) techniques, which are able to improve the accuracy of the expectation values of quantum observables by implementing classical post-processing analysis from an ensemble of repeated noisy quantum circuit runs. In this work, we focus on a recent QEM technique that uses Fuzzy C-Means (FCM) clustering to specifically identify measurement error patterns. For the first time, we report a proof-of-principle validation of the technique on a 2-qubit register, obtained as a subset of a real NISQ 5-qubit superconducting quantum processor based on transmon qubits. We demonstrate that the FCM-based QEM technique allows for reasonable improvement of the expectation values of single- and two-qubit gates based quantum circuits, without necessarily invoking state-of-the-art coherence, gate, and readout fidelities.

quant-ph↗

arXiv2023

Hall-effect in the MnBi_2Te_4 crystal using silicon nitride nanomembrane via contacts

Utilizing an interplay between band topology and intrinsic magnetism, the two-dimensional van der Waals (vdW) system MnBi_2Te_4 provides an ideal platform for realizing exotic quantum phenomena and offers great opportunities in the emerging field of antiferromagnetic spintronic technology. Yet, the fabrication of MnBi_2Te_4-based nanodevices is hindered by the high sensitivity of this material, which quickly degrades when exposed to air or to elevated temperatures. Here, we demonstrate an alternative route of fabricating vdW-MnBi_2Te_4-based electronic devices using the cryogenic dry transfer of a printable circuit embedded in an inorganic silicon nitride membrane. The electrical connections between the thin crystal and the top surface of the membrane are established through via contacts. Our magnetotransport study reveals that this innovative via contact approach enables exploring the MnBi_2Te_4-like sensitive 2D materials and engineering synthetic heterostructures as well as complex circuits based on the two-dimensional vdW systems.

cond-mat.mtrl-sci↗

arXiv2023

2D high temperature superconductor integration in contact printed circuit boards

Inherent properties of superconducting Bi2Sr2CaCu2O8+x films, such as the high superconducting transition temperature Tc, efficient Josephson coupling between neighboring CuO layers, and fast quasiparticle relaxation dynamics, make them a promising platform for advances in quantum computing and communication technologies. However, preserving two-dimensional superconductivity during device fabrication is an outstanding experimental challenge because of the fast degradation of the superconducting properties of two-dimensional flakes when they are exposed to moisture, organic sol vents, and heat. Here, to realize superconducting devices utilizing two-dimensional superconducting films, we develop a novel fabrication technique relying on the cryogenic dry transfer of printable circuits embedded into a silicon nitride membrane. This approach separates the circuit fabrication stage requiring chemically reactive substances and ionizing physical processes from the creation of the thin superconducting structures. Apart from providing electrical contacts in a single transfer step, the membrane encapsulates the surface of the crystal shielding it from the environment. The fabricated atomically thin Bi2Sr2CaCu2O8+x-based devices show high superconducting transition temperature Tc ~ 91 K close to that of the bulk crystal and demonstrate stable super conducting properties

cond-mat.supr-con↗

arXiv2023

Current-phase relation of a short multi-mode Bi2Se3 topological insulator nanoribbon Josephson junction with ballistic transport modes

We used the asymmetric superconducting quantum interference device (SQUID) technique to extract the current phase relation (CPR) of a Josephson junction with a 3D-topological insulator (TI) Bi2Se3 nanobelt as the barrier. The obtained CPR shows deviations from the standard sinusoidal CPR with a pronounced forward skewness. At temperatures below 200 mK, the junction skewness values are above the zero temperature limit for short diffusive junctions. Fitting of the extracted CPR shows that most of the supercurrent is carried by ballistic topological surface states (TSSs), with a small contribution of diffusive channels primarily due to the bulk. These findings are instrumental in engineering devices that can fully exploit the properties of the topologically protected surface states of 3D TIs.

cond-mat.supr-con↗

arXiv2023

Encapsulating high-temperature superconducting twisted van der Waals heterostructures blocks detrimental effects of disorder

High-temperature cuprate superconductors-based van der Waals (vdW) heterostructures hold high technological promise. One of the obstacles hindering progress is the detrimental effect of disorder on the properties of Josephson junctions (JJ) realized by the vdW devices. Here we report the new method of fabricating twisted vdW heterostructures made of Bi2Sr2CuCa2O8+d, crucially improving the JJ characteristics, pushing them up to those of the intrinsic JJs in bulk samples. The method combines a cryogenic stacking using a solvent-free stencil mask technique and covering interface by the insulating hexagonal boron nitride crystals. Despite the high-vacuum condition down to 10-6 mbar in the evaporation chamber, the interface appears to be protected from water molecules during the in-situ metal deposition only when fully encapsulated. Comparing the current-voltage curves of encapsulated and unencapsulated interfaces, we reveal that the encapsulated interfaces' characteristics are crucially improved so that the corresponding JJs demonstrate high critical currents and sharpness of the superconducting transition comparable to those of the intrinsic JJs. Finally, we show that the encapsulated heterostructures are more stable in time.

cond-mat.supr-con↗

arXiv2022

A hybrid ferromagnetic transmon qubit: circuit design, feasibility and detection protocols for magnetic fluctuations

We propose to exploit currently available tunnel ferromagnetic Josephson junctions to realize a hybrid superconducting qubit. We show that the characteristic hysteretic behavior of the ferromagnetic barrier provides an alternative and intrinsically digital tuning of the qubit frequency by means of magnetic field pulses. To illustrate functionalities and limitation of the device, we discuss the coupling to a read-out resonator and the effect of magnetic fluctuations. The possibility to use the qubit as a noise detector and its relevance to investigate the subtle interplay of magnetism and superconductivity is envisaged.

cond-mat.supr-con↗

arXiv2021

Inverse magnetic hysteresis of the Josephson supercurrent: study of the magnetic properties of thin niobium/permalloy (Fe_{20}Ni_{80}) interfaces

We propose a picture for the magnetic properties of superconductor/ferromagnet (S/F) heterostructures based on Nb and permalloy (Py: Fe_{20}Ni_{80}). By measuring the magnetic moment as a function of the temperature in S/F/S trilayers for different thicknesses of the middle F layer, we give evidence of the presence of a magnetic stray field of the F layer. For values of F-layer thickness below a threshold, we establish a correlation between the magnetic measurements of the S/F/S trilayers and the anomalous magnetic dependence of the critical current in S/insulator/thin superconducting film/F/S (SIsFS) Josephson junctions (JJs). These complementary investigations provide a self-consistent method to fully characterize S/F heterostructures and possibly demonstrate effects arising from the mutual interactions between ferromagnetism and superconductivity. A shift in the Fraunhofer critical current oscillations has been observed in the opposite direction to the one commonly observed in JJs with F barriers, as it has been recently predicted by inverse and electromagnetic proximity theories. This inverse memory effect is relevant for the design of these heterostructures as memory cells and spintronic devices.

cond-mat.supr-con↗

arXiv2020

Topological insulator nanoribbon Josephson junctions: evidence for size effect in transport properties

We have used Bi$_2$Se$_3$ nanoribbons, grown by catalyst-free Physical Vapor Deposition to fabricate high quality Josephson junctions with Al superconducting electrodes. In our devices we observe a pronounced reduction of the Josephson critical current density $J_c$ by reducing the width of the junction, which in our case corresponds to the width of the nanoribbon. Because the topological surface states extend over the entire circumference of the nanoribbon, the superconducting transport associated to them is carried by modes on both the top and bottom surfaces of the nanoribbon. We show that the $J_c$ reduction as a function of the nanoribbons width can be accounted for by assuming that only the modes travelling on the top surface contribute to the Josephson transport as we derive by geometrical consideration. This finding is of a great relevance for topological quantum circuitry schemes, since it indicates that the Josephson current is mainly carried by the topological surface states.

cond-mat.supr-con↗