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Dominique Delande

Publications and source records attributed to Dominique Delande.

At least 91 records · Page 5Linked to original sources

Light transport in cold atoms and thermal decoherence

By using the coherent backscattering interference effect, we investigate experimentally and theoretically how coherent transport of light inside a cold atomic vapour is affected by the residual motion of atomic scatterers. As the temperature of the atomic cloud increases, the interference contrast dramatically decreases emphazising the role of motion-induced decoherence for resonant scatterers even in the sub-Doppler regime of temperature. We derive analytical expressions for the corresponding coherence time.

quant-ph↗

Multiple scattering of photons by atomic hyperfine multiplets

Mesoscopic interference effects in multiple scattering of photons depend crucially on the internal structure of the scatterers. In the present article, we develop the analytical theory of multiple photon scattering by cold atoms with arbitrary internal hyperfine multiplets. For a specific application, we calculate the enhancement factor of elastic coherent backscattering as a function of detuning from an entire hyperfine multiplet of neighboring resonances that cannot be considered isolated. Our theory permits to understand why atoms behave differently from classical Rayleigh point-dipole scatterers, and how the classical description is recovered for larger but still microscopic objects like molecules or clusters.

physics.atom-ph↗

Coherent Backscattering of Light with Nonlinear Atomic Scatterers

We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear refractive index) and the scattering events. Using a perturbative approach, the nonlinear effects arise from inelastic two-photon scattering processes. We present a detailed diagrammatic derivation of the elastic and inelastic components of the backscattering signal both for scalar and vectorial photons. Especially, we show that the coherent backscattering phenomenon originates in some cases from the interference between three different scattering amplitudes. This is in marked contrast with the linear regime where it is due to the interference between two different scattering amplitudes. In particular we show that, if elastically scattered photons are filtered out from the photo-detection signal, the nonlinear backscattering enhancement factor exceeds the linear barrier two, consistently with a three-amplitude interference effect.

quant-ph↗

Reversible Destruction of Dynamical Localization

Dynamical localization is a localization phenomenon taking place, for example, in the quantum periodically-driven kicked rotor. It is due to subtle quantum destructive interferences and is thus of intrinsic quantum origin. It has been shown that deviation from strict periodicity in the driving rapidly destroys dynamical localization. We report experimental results showing that this destruction is partially reversible when the deterministic perturbation that destroyed it is slowly reversed. We also provide an explanation for the partial character of the reversibility.

physics.atom-ph↗

Magnetic Field Enhanced Coherence Length in Cold Atomic Gases

We study the effect of an external magnetic field on coherent backscattering of light from a cool rubidium vapor. We observe that the backscattering enhancement factor can be {\it increased} with $B$. This surprising behavior shows that the coherence length of the system can be increased by applying a magnetic field, in sharp contrast with ususal situations. This is mainly due to the lifting of the degeneracy between Zeeman sublevels. We find good agreement between our experimental data and a full Monte-Carlosimulation, taking into account the magneto-optical effects and the geometry of the atomic cloud.

cond-mat.mes-hall↗

Coherent backscattering in nonlinear atomic media: quantum Langevin approach

In this theoretical paper, we investigate coherence properties of the near-resonant light scattered by two atoms exposed to a strong monochromatic field. To properly incorporate saturation effects, we use a quantum Langevin approach. In contrast to the standard optical Bloch equations, this method naturally provides the inelastic spectrum of the radiated light induced by the quantum electromagnetic vacuum fluctuations. However, to get the right spectral properties of the scattered light, it is essential to correctly describe the statistical properties of these vacuum fluctuations. Because of the presence of the two atoms, these statistical properties are not Gaussian : (i) the spatial two-points correlation function displays a speckle-like behavior and (ii) the three-points correlation function does not vanish. We also explain how to incorporate in a simple way propagation with a frequency-dependent scattering mean-free path, meaning that the two atoms are embedded in an average scattering dispersive medium. Finally we show that saturation-induced nonlinearities strongly modify the atomic scattering properties and, as a consequence, provide a source of decoherence in multiple scattering. This is exemplified by considering the coherent backscattering configuration where interference effects are blurred by this decoherence mechanism. This leads to a decrease of the so-called coherent backscattering enhancement factor.

quant-ph↗

Quantum diffusion in the quasiperiodic kicked rotor

We study the mechanisms responsible for quantum diffusion in the quasiperiodic kicked rotor. We report experimental measurements of the diffusion constant on the atomic version of the system and develop a theoretical approach (based on the Floquet theorem) explaining the observations, especially the ``sub-Fourier'' character of the resonances observed in the vicinity of exact periodicity, i.e. the ability of the system to distinguish two neighboring driving frequencies in a time shorter than the inverse of the difference of the two frequencies.

quant-ph↗

Analysis of dynamical tunnelling experiments with a Bose-Einstein condensate

Dynamical tunnelling is a quantum phenomenon where a classically forbidden process occurs, that is prohibited not by energy but by another constant of motion. The phenomenon of dynamical tunnelling has been recently observed in a sodium Bose-Einstein condensate. We present a detailed analysis of these experiments using numerical solutions of the three dimensional Gross-Pitaevskii equation and the corresponding Floquet theory. We explore the parameter dependency of the tunnelling oscillations and we move the quantum system towards the classical limit in the experimentally accessible regime.

nlin.CD↗

Mechanism and Lineshapes of Sub-Fourier Resonances

Subtle internal interference effects allow quantum-chaotic systems to display "sub-Fourier" resonances, i.e. to distinguish two neighboring driving frequencies in a time shorter than the inverse of the difference of the two frequencies. We report experiments on the atomic version of the kicked rotor showing the unusual properties of the sub-Fourier resonances, and develop a theoretical approach (based on the Floquet theorem) explaining these properties, and correctly predicting the widths and lineshapes.

quant-ph↗

A new vibrational level of the H$_2^+$ molecular ion

A new state of the H$_2^+$ molecular ion with binding energy of 1.09$\times10^{-9}$ a.u. below the first dissociation limit is predicted, using highly accurate numerical nonrelativistic quantum calculations. It is the first L=0 excited state, antisymmetric with respect to the exchange of the two protons. It manifests itself as a huge p-H scattering length of $a=750\pm 5$ Bohr radii.

physics.atom-ph↗

A realistic example of chaotic tunneling: The hydrogen atom in parallel static electric and magnetic fields

Statistics of tunneling rates in the presence of chaotic classical dynamics is discussed on a realistic example: a hydrogen atom placed in parallel uniform static electric and magnetic fields, where tunneling is followed by ionization along the fields direction. Depending on the magnetic quantum number, one may observe either a standard Porter-Thomas distribution of tunneling rates or, for strong scarring by a periodic orbit parallel to the external fields, strong deviations from it. For the latter case, a simple model based on random matrix theory gives the correct distribution.

nlin.CD↗

Signatures of chaotic tunnelling

Recent experiments with cold atoms provide a significant step toward a better understanding of tunnelling when irregular dynamics is present at the classical level. In this paper, we lay out numerical studies which shed light on the previous experiments, help to clarify the underlying physics and have the ambition to be guidelines for future experiments.

nlin.CD↗

Coherent backscattering of light by cold atoms: theory meets experiment

Coherent backscattering (CBS) of quasi-resonant light by cold atoms presents some specific features due to the internal structure of the atomic scatterers. We present the first quantitative comparison between the experimentally observed CBS cones and Monte-Carlo calculations which take into account the shape of the atomic cloud as well as the internal atomic structure.

physics.atom-ph↗

Non-dispersive wave packets in periodically driven quantum systems

With the exception of the harmonic oscillator, quantum wave-packets usually spread as time evolves. We show here that, using the nonlinear resonance between an internal frequency of a system and an external periodic driving, it is possible to overcome this spreading and build non-dispersive (or non-spreading) wave-packets which are well localized and follow a classical periodic orbit without spreading. From the quantum mechanical point of view, the non-dispersive wave-packets are time periodic eigenstates of the Floquet Hamiltonian, localized in the nonlinear resonance island. We discuss the general mechanism which produces the non-dispersive wave-packets, with emphasis on simple realization in the electronic motion of a Rydberg electron driven by a microwave field. We show the robustness of such wavepackets for a model one-dimensional as well as for realistic three dimensional atoms. We consider their essential properties such as the stability versus ionization, the characteristic energy spectrum and long lifetimes. The requirements for experiments aimed at observing such non-dispersive wave-packets are also considered. We also discuss other related phenomena in atomic and molecular physics as well as possible further extensions of the theory.

quant-ph↗

Observation of sub-Fourier resonances in a quantum-chaotic system

We experimentally show that the response of a quantum-chaotic system can display resonance lines sharper than the inverse of the excitation duration. This allows us to discriminate two neighboring frequencies with a resolution nearly 40 times better than the limit set by the Fourier inequality. Furthermore, numerical studies indicate that there is no limit, but the loss of signal, to this resolution, opening ways for the development of sub-Fourier quantum-chaotic signal processing.

quant-ph↗

Manipulating the shape of electronic non-dispersive wave-packets in the hydrogen atom: numerical tests in realistic experimental conditions

We show that combination of a linearly polarized resonant microwave field and a parallel static electric field may be used to create a non-dispersive electronic wavepacket in Rydberg atoms. The static electric field allows for manipulation of the shape of the elliptical trajectory the wavepacket is propagating on. Exact quantum numerical calculations for realistic experimental parameters show that the wavepacket evolving on a linear orbit can be very easily prepared in a laboratory either by a direct optical excitation or by preparing an atom in an extremal Stark state and then slowly switching on the microwave field. The latter scheme seems to be very resistant to experimental imperfections. Once the wavepacket on the linear orbit is excited, the static field may be used to manipulate the shape of the orbit.

quant-ph↗

Weak localization of light by cold atoms: the impact of quantum internal structure

Since the work of Anderson on localization, interference effects for the propagation of a wave in the presence of disorder have been extensively studied, as exemplified in coherent backscattering (CBS) of light. In the multiple scattering of light by a disordered sample of thermal atoms, interference effects are usually washed out by the fast atomic motion. This is no longer true for cold atoms where CBS has recently been observed. However, the internal structure of the atoms strongly influences the interference properties. In this paper, we consider light scattering by an atomic dipole transition with arbitrary degeneracy and study its impact on coherent backscattering. We show that the interference contrast is strongly reduced. Assuming a uniform statistical distribution over internal degrees of freedom, we compute analytically the single and double scattering contributions to the intensity in the weak localization regime. The so-called ladder and crossed diagrams are generalized to the case of atoms and permit to calculate enhancement factors and backscattering intensity profiles for polarized light and any closed atomic dipole transition.

quant-ph↗

Multiple scattering of light by atoms in the weak localization regime

Coherent backscattering is a multiple scattering interference effect which enhances the diffuse reflection off a disordered sample in the backward direction. Classically, the enhanced intensity is twice the average background under well chosen experimental conditions. We show how the quantum internal structure of atomic scatterers leads to a significantly smaller enhancement. Theoretical results for double scattering in the weak localization regime are presented which confirm recent experimental observations.

physics.atom-ph↗