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E. A. Muljarov

Publications and source records attributed to E. A. Muljarov.

At least 37 records · Page 2Linked to original sources

Resonant-state expansion for open optical systems: Generalization to magnetic, chiral, and bi-anisotropic materials

The resonant-state expansion, a recently developed powerful method in electrodynamics, is generalized here for open optical systems containing magnetic, chiral, or bi-anisotropic materials. It is shown that the key matrix eigenvalue equation of the method remains the same, but the matrix elements of the perturbation now contain variations of the permittivity, permeability, and bi-anisotropy tensors. A general normalization of resonant states in terms of the electric and magnetic fields is presented.

physics.optics↗

Optimizing the Drude-Lorentz model for material permittivity - method, program, and examples for gold, silver, and copper

Approximating the frequency dispersion of the permittivity of materials with simple analytical functions is of fundamental importance for understanding and modeling the optical response of materials and resulting structures. In the generalized Drude-Lorentz model, the permittivity is described in the complex frequency plane by a number of simple poles having complex weights, which is a physically relevant and mathematically simple approach: By construction, it respects causality represents physical resonances of the material, and can be implemented easily in numerical simulations. We report here an efficient method of optimizing the fit of measured data with the Drude-Lorentz model having an arbitrary number of poles. We show examples of such optimizations for gold, silver, and copper, for different frequency ranges and up to four pairs of Lorentz poles taken into account. We also provide a program implementing the method for general use.

physics.optics↗

Resonant-state expansion of light propagation in non-uniform waveguides

A new rigorous approach for precise and efficient calculation of light propagation along non-uniform waveguides is presented. Resonant states of a uniform waveguide, which satisfy outgoing-wave boundary conditions, form a natural basis for expansion of the local electromagnetic field. Using such an expansion at fixed frequency, we convert the wave equation for light propagation in a non-uniform waveguide into an ordinary second-order matrix differential equation for the expansion coefficients depending on the coordinate along the waveguide. We illustrate the method on several examples of non-uniform planar waveguides and evaluate its efficiency compared to the aperiodic Fourier modal method and the finite element method, showing improvements of one to four orders of magnitude. A similar improvement can be expected also for applications in other fields of physics showing wave phenomena, such as acoustics and quantum mechanics.

physics.optics↗

Dipolar polaritons in microcavity-embedded coupled quantum wells in electric and magnetic fields

We present a precise calculation of spatially-indirect exciton states in semiconductor coupled quantum wells and polaritons formed from their coupling to the optical mode of a microcavity. We include the presence of electric and magnetic fields applied perpendicular to the quantum well plane. Our model predicts the existence of polaritons which are in the strong coupling regime and at the same time possess a large static dipole moment. We demonstrate, in particular, that a magnetic field can compensate for the reduction in light-matter coupling that occurs when an electric field impresses a dipole moment on the polariton.

cond-mat.mes-hall↗

Comment on "Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators"

Recently, Kristensen, Ge and Hughes have compared [Phys. Rev. A 92, 053810 (2015)] three different methods for normalization of quasinormal modes in open optical systems, and concluded that they all provide the same result. We show here that this conclusion is incorrect and illustrate that the normalization of [Opt. Lett. 37, 1649 (2012)] is divergent for any optical mode having a finite quality factor, and that the Silver-Mueller radiation condition is not fulfilled for quasinormal modes.

cond-mat.mes-hall↗

Exciton effective mass enhancement in coupled quantum wells in electric and magnetic fields

We present a calculation of exciton states in semiconductor coupled quantum wells (CQWs) in the presence of electric and magnetic fields applied perpendicular to the QW plane. The exciton Schrödinger equation is solved in real space in three dimensions to obtain the Landau levels of both direct and indirect excitons. Calculation of the exciton energy levels and oscillator strengths enables mapping of the electric and magnetic field dependence of the exciton absorption spectrum. For the ground state of the system, we evaluate the Bohr radius, optical lifetime, binding energy and dipole moment. The exciton mass renormalization due to the magnetic field is calculated using a perturbative approach. We predict a non-monotonous dependence of the exciton ground state effective mass on magnetic field. Such a trend is explained in a classical picture, in terms of the ground state tending from an indirect to a direct exciton with increasing magnetic field.

cond-mat.mes-hall↗

Exact mode volume and Purcell factor of open optical systems

The Purcell factor quantifies the change of the radiative decay of a dipole in an electromagnetic environment relative to free space. Designing this factor is at the heart of photonics technology, striving to develop ever smaller or less lossy optical resonators. The Purcell factor can be expressed using the electromagnetic eigenmodes of the resonators, introducing the notion of a mode volume for each mode. This approach allows to use an analytic treatment, consisting only of sums over eigenmode resonances, a so-called spectral representation. We show in the present work that the expressions for the mode volumes known and used in literature are only approximately valid for modes of high quality factor, while in general they are incorrect. We rectify this issue, introducing the exact normalization of modes. We present an analytic theory of the Purcell effect based on the exact mode normalization and resulting effective mode volume. We use a homogeneous dielectric sphere in vacuum, which is analytically solvable, to exemplify these findings.

cond-mat.mes-hall↗

Controlled strong coupling and absence of dark polaritons in microcavities with double quantum wells

We demonstrate an efficient switching between strong and weak exciton-photon coupling regimes in microcavity-embedded asymmetric double quantum wells, controlled by an applied electric field. We show that a fine tuning of the electric field leads to drastic changes in the polariton properties, with the polariton ground state being red-shifted by a few meV and having acquired prominent features of a spatially indirect dipolar exciton. We study the properties of dipolar exciton polaritons, called dipolaritons, on a microscopic level and show that, unlike recent findings, they are not dark polaritons but, owing to the finite size of the excition, are mixed states with comparable contribution of the cavity photon, bright direct, and long-living indirect exciton modes.

cond-mat.mes-hall↗

Resonant-state expansion of dispersive open optical systems

A resonant-state expansion (RSE) for open optical systems with a general frequency dispersion of the relative permittivity, described by a finite number of simple poles, is presented. As in the non-dispersive case, the RSE of dispersive systems converts Maxwell's wave equation into a linear matrix eigenvalue problem in the basis of unperturbed resonant states, in this way numerically exactly determining all relevant eigenmodes of the optical system. This dispersive RSE is verified by application to the analytically solvable system of a sphere in vacuum, with a dispersion of the dielectric constant described by the Drude and Drude-Lorentz models. We calculate the change of the optical modes when converting the sphere material from gold to non-dispersive silica and back to gold, and evaluate the accuracy using the exact solutions.

cond-mat.mes-hall↗

Resonant-state expansion for a simple dispersive medium

The resonant-state expansion (RSE), a rigorous perturbative method developed in electrodynamics for non-dispersive optical systems is applied to media with an Ohm's law dispersion, in which the frequency dependent part of the permittivity scales inversely with the frequency, corresponding to a frequency-independent conductivity. This dispersion has only a single pole at zero frequency, which is already present in the non-dispersive RSE, allowing to maintain not only the linearity of the eigenvalue problem of the RSE but also its size. Media which can be described by this dispersion over the relevant frequency range, such as optical glass or doped semiconductors, can be treated in the RSE without additional complexity. Results are presented using analytically solvable homogeneous spheres, for doped silicon and BK7 glass, both for a perturbation of the system going from non-dispersive to dispersive media and the reverse, from dispersive to non-dispersive media.

physics.optics↗

Resonant state expansion applied to three-dimensional open optical systems

The resonant state expansion (RSE), a rigorous perturbative method in electrodynamics, is developed for three-dimensional open optical systems. Results are presented using the analytically solvable homogeneous dielectric sphere as unperturbed system. Since any perturbation which breaks the spherical symmetry mixes transverse electric (TE) and transverse magnetic (TM) modes, the RSE is extended here to include TM modes and a zero-frequency pole of the Green's function. We demonstrate the validity of the RSE for TM modes by verifying its convergence towards the exact result for a homogeneous perturbation of the sphere. We then apply the RSE to calculate the modes for a selection of perturbations sequentially reducing the remaining symmetry, given by a change of the dielectric constant of half-sphere and quarter-sphere shape. Since no exact solutions are known for these perturbations, we verify the RSE results by comparing them with the results of state of the art finite element method (FEM) and finite difference in time domain (FDTD) solvers. We find that for the selected perturbations, the RSE provides a significantly higher accuracy than the FEM and FDTD for a given computational effort, demonstrating its potential to supersede presently used methods. We furthermore show that in contrast to presently used methods, the RSE is able to determine the perturbation of a selected group of modes by using a limited basis local to these modes, which can further reduce the computational effort by orders of magnitude.

physics.optics↗

Resonant state expansion applied to planar waveguides

The resonant state expansion, a recently developed method in electrodynamics, is generalized here to planar open optical systems with non-normal incidence of light. The method is illustrated and verified on exactly solvable examples, such as a dielectric slab and a Bragg reflector microcavity, for which explicit analytic formulas are developed. This comparison demonstrates the accuracy and convergence of the method. Interestingly, the spectral analysis of a dielectric slab in terms of resonant states reveals an influence of waveguide modes in the transmission. These modes, which on resonance do not couple to external light, surprisingly do couple to external light for off-resonant excitation.

physics.optics↗

Resonant state expansion applied to two-dimensional open optical systems

The resonant state expansion (RSE), a rigorous perturbative method in electrodynamics, is applied to two-dimensional open optical systems. The analytically solvable homogeneous dielectric cylinder is used as unperturbed system, and its Green's function is shown to contain a cut in the complex frequency plane, which is included in the RSE basis. The complex eigenfrequencies of modes are calculated using the RSE for a selection of perturbations which mix unperturbed modes of different orbital momentum, such as half-cylinder, thin-film and thin-wire perturbation, demonstrating the accuracy and convergency of the method. The resonant states for the thin-wire perturbation are shown to reproduce an approximative analytical solution.

physics.optics↗

Drift-diffusion model of the fragmentation of the external ring structure in the photoluminescence pattern of indirect excitons in coupled quantum wells

Under optical excitation, coupled quantum wells are known to reveal fascinating features in the photoluminescence pattern originating from dipole orientated indirect excitons. The appearance of an external ring has been attributed to macroscopic charge separation in the quantum well plane. We present a classical model of non-linear diffusion to account for the observed fragmentation of the external ring into a periodic array of islands. The model incorporates the Coulomb interactions between electrons, holes and indirect excitons. At low temperatures, these interactions lead to pattern formation similar to the experimentally observed ring fragmentation. The fragmentation is found to persist to temperatures above the quantum degeneracy temperature of indirect excitons.

cond-mat.mes-hall↗

Microcavity controlled coupling of excitonic qubits

Controlled non-local energy and coherence transfer enables light harvesting in photosynthesis and non-local logical operations in quantum computing. The most relevant mechanism of coherent coupling of distant qubits is coupling via the electromagnetic field. Here, we demonstrate the controlled coherent coupling of spatially separated excitonic qubits via the photon mode of a solid state microresonator. This is revealed by two-dimensional spectroscopy of the sample's coherent response, a sensitive and selective probe of the coherent coupling. The experimental results are quantitatively described by a rigorous theory of the cavity mediated coupling within a cluster of quantum dots excitons. Having demonstrated this mechanism, it can be used in extended coupling channels - sculptured, for instance, in photonic crystal cavities - to enable a long-range, non-local wiring up of individual emitters in solids.

quant-ph↗

Hydrogen supersymmetry: A new method in perturbation theory

The O(4) supersymmetry of the hydrogen atom is utilized to construct a complete basis using only the bound state wave functions. For a large class of perturbations, an expansion of the electron (exciton) wave function into such a complete set reduces the perturbed Schroedinger equation to a standard eigenvalue problem with an equidistant unperturbed spectrum. A high-order polarizability of the ground state of the hydrogen atom in a static electric field is calculated via Rayleigh-Schroedinger perturbation theory for illustration of the new method.

math-ph↗

Hyperspherical theory of anisotropic exciton

A new approach to the theory of anisotropic exciton based on Fock transformation, i.e., on a stereographic projection of the momentum to the unit 4-dimensional (4D) sphere, is developed. Hyperspherical functions are used as a basis of the perturbation theory. The binding energies, wave functions and oscillator strengths of elongated as well as flattened excitons are obtained numerically. It is shown that with an increase of the anisotropy degree the oscillator strengths are markedly redistributed between optically active and formerly inactive states, making the latter optically active. An approximate analytical solution of the anisotropic exciton problem taking into account the angular momentum conserving terms is obtained. This solution gives the binding energies of moderately anisotropic exciton with a good accuracy and provides a useful qualitative description of the energy level evolution.

math-ph↗

Resonant acousto-optics in the terahertz range: TO-phonon polaritons driven by an ultrasonic wave

The resonant acousto-optic effect is studied both analytically and numerically in the terahertz range where the transverse-optical (TO) phonons play the role of a mediator which strongly couples the ultrasound and light fields. A propagating acoustic wave interacts with the TO phonons via anharmonic channels and opens band gaps in the TO-phonon polariton energy dispersion that results in pronounced Bragg scattering and reflection of the incoming light. The separation in frequency of different Bragg replicas, which is at the heart of acousto-optics, allows us to study the resonant acousto-optic effect in the most simple and efficient geometry of collinear propagation of electromagnetic and ultrasonic waves. The acoustically induced energy gaps, Bragg reflection spectra, and the spatial distribution of the electric field and polarization are calculated for CuCl parameters, in a wide range of frequencies and intensities of the pumping acoustic wave. Our results show drastic changes in terahertz spectra of semiconductor crystals that opens the way for efficient and accessible manipulation of their infrared properties, by tuning the parameters of the acoustic wave.

cond-mat.other↗