arXiv subjects

E. Arimondo

Publications and source records attributed to E. Arimondo.

At least 19 recordsLinked to original sources

arXiv2025

Reversing adiabatic state preparation in few-level quantum systems

We present a detailed study of an adiabatic state preparation in an effective three-level quantum system. States can be prepared with high speed and fidelity by adding a counterdiabatic (CD) quantum control protocol. As a second step, we invert the preparation protocol to get back to the initial state. This describes an overall cyclic evolution in state space. Using counterdiabatic terms, the resulting composed fast evolution can be repeated many times. We then analyze the control of Berry's phase along the adiabatic cyclic path and show that Berry's phase can act as a sensitive detector of non-perfect state transfer.

quant-ph↗

arXiv2023

Engineering quantum control with twisted-light fields induced optical transitions

A novel form of quantum control is proposed by applying twisted-light also known as optical vortex beams to drive ultra-narrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg and Cd bosonic isotopes. This innovative all-optical spectroscopic method introduces spatially tailored electric and magnetic fields to fully rewrite atomic selection rules reducing simultaneously probe-induced frequency-shifts and additional action of external ac and dc field distortions. A twisted-light focused probe beam produces strong longitudinal electric and magnetic fields along the laser propagation axis which opens the 1S0-3P0 doubly forbidden clock transition with a high E1M1 two-photon excitation rate. This long-lived clock transition is thus immune to nonscalar electromagnetic perturbations. Zeeman components of the M2 magnetic quadrupole 1S0-3P2 transition considered for quantum computation and simulation are now selectively driven by transverse or longitudinal field gradients with vanishing electric fields. These field gradients are manipulated by the mutual action of orbital and spin angular momentum of the light beam and are used in presence of tunable vector and tensor polarizabilities. A combination of these two different twisted-light induced clock transitions within a single quantum system, at the same magic wavelength and in presence of a common thermal environment significantly reduces systematic uncertainties. Furthermore, it generates an optical synthetic frequency which efficiently limits the blackbody radiation shift and its variations at room temperature. Engineering light-matter interaction by optical vortices will benefit to experimental atomic and molecular platforms targeting an optimal coherent control of quantum states, reliant quantum simulation, novel approach to atomic interferometry and precision tests of fundamental theories in physics and high-accuracy optical metrology.

physics.atom-ph↗

arXiv2022

Survey of hyperfine structure measurements in alkali atoms

The spectroscopic hyperfine constants for all the alkali atoms are reported. For atoms from lithium to cesium, only the long lived atomic isotopes are examined. For francium, the measured data for nuclear ground states of all available isotopes are listed. All results obtained since the beginning of laser investigations are presented, while for previous works the data of Arimondo {\it et. al.} Rev. Mod. Phys. 49, 31 (1977) are recalled. Global analyses based on the scaling laws and on the hyperfine anomalies are performed.

physics.atom-ph↗

arXiv2019

Measurements of individual and ensemble lifetimes of high-lying Rb Rydberg states

We demonstrate a hybrid method based on field ionization and state-selective de-excitation capable of measuring the lifetimes of high-lying Rydberg states. For nS Rydberg states of Rb atoms with principal quantum number $60\leq n\leq88$, we measure both the individual target state lifetimes and those of the ensemble of Rydberg states populated via black-body radiation-induced transitions. We find good overall agreement with numerical calculations of the expected lifetimes in both cases. However, for the target state lifetimes, we find a local deviation towards shorter lifetimes for states around $n=72$, which we interpret as a signature of a modified black-body spectrum in the finite volume in which our experiments take place.

quant-ph↗

arXiv2017

Optical spectroscopy of a microsized Rb vapour sample in magnetic fields up to 58 tesla

We use a magnetometer probe based on the Zeeman shift of the rubidium resonant optical transition to explore the atomic magnetic response for a wide range of field values. We record optical spectra for fields from few tesla up to 60 tesla, the limit of the coil producing the magnetic field. The atomic absorption is detected by the fluorescence emissions from a very small region with a submillimiter size. We investigate a wide range of magnetic interactions from the hyperfine Paschen-Back regime to the fine one, and the transitions between them. The magnetic field measurement is based on the rubidium absorption itself. The rubidium spectroscopic constants were previously measured with high precision, except the excited state Landé $g$-factor that we derive from the position of the absorption lines in the transition to the fine Paschen-Back regime. Our spectroscopic investigation, even if limited by the Doppler broadening of the absorption lines, measures the field with a 20 ppm uncertainty at the explored high magnetic fields. Its accuracy is limited to 75 ppm by the excited state Landé $g$-factor determination.

physics.atom-ph↗

arXiv2017

De-excitation spectroscopy of strongly interacting Rydberg gases

We present experimental results on the controlled de-excitation of Rydberg states in a cold gas of Rb atoms. The effect of the van der Waals interactions between the Rydberg atoms is clearly seen in the de-excitation spectrum and dynamics. Our observations are confirmed by numerical simulations. In particular, for off-resonant (facilitated) excitation we find that the de-excitation spectrum reflects the spatial arrangement of the atoms in the quasi one-dimensional geometry of our experiment. We discuss future applications of this technique and implications for detection and controlled dissipation schemes.

physics.atom-ph↗

arXiv2015

Experimental observation of controllable kinetic constraints in a cold atomic gas

Many-body systems relaxing to equilibrium can exhibit complex dynamics even if their steady state is trivial. At low temperatures or high densities their evolution is often dominated by steric hindrances affecting particle motion [1,2,3]. Local rearrangements are highly constrained, giving rise to collective - and often slow - relaxation.This dynamics can be difficult to analyse from first principles, but the essential physical ingredients are captured by idealized lattice models with so- called kinetic constraints [4]. Here we experimentally realize a many-body system exhibiting manifest kinetic constraints and measure its dynamical properties. In the cold Rydberg gas used in our experiments, the nature of the constraints can be tailored through the detuning of the excitation lasers from resonance [5,6,7,8], which controls whether the system undergoes correlated or anti- correlated dynamics. Our results confirm recent theoretical predictions [5,6], and highlight the analogy between the dynamics of interacting Rydberg gases and that of soft-matter systems.

cond-mat.stat-mech↗

arXiv2015

Van der Waals explosion of cold Rydberg clusters

We report on the direct measurement in real space of the effect of the van der Waals forces between individual Rydberg atoms on their external degrees of freedom. Clusters of Rydberg atoms with inter-particle distances of around 5 μm are created by first generating a small number of seed excitations in a magneto-optical trap, followed by off-resonant excitation that leads to a chain of facilitated excitation events. After a variable expansion time the Rydberg atoms are field ionized, and from the arrival time distributions the size of the Rydberg cluster after expansion is calculated. Our experimental results agree well with a numerical simulation of the van der Waals explosion.

physics.atom-ph↗

arXiv2014

Quantum engineering of atomic phase-shifts in optical clocks

Quantum engineering of time-separated Raman laser pulses in three-level systems is presented to produce an ultra-narrow optical transition in bosonic alkali-earth clocks free from light shifts and with a significantly reduced sensitivity to laser parameter fluctuations. Based on a quantum artificial complex-wave-function analytical model, and supported by a full density matrix simulation including a possible residual effect of spontaneous emission from the intermediate state, atomic phase-shifts associated to Ramsey and Hyper-Ramsey two-photon spectroscopy in optical clocks are derived. Various common-mode Raman frequency detunings are found where the frequency shifts from off-resonant states are canceled, while strongly reducing their uncertainties at the 10$^{-18}$ level of accuracy.

physics.atom-ph↗

arXiv2013

Full counting statistics and phase diagram of a dissipative Rydberg gas

Ultra-cold gases excited to strongly interacting Rydberg states are a promising system for quantum simulations of many-body systems. For off-resonant excitation of such systems in the dissipative regime, highly correlated many-body states exhibiting, among other characteristics, intermittency and multi-modal counting distributions are expected to be created. So far, experiments with Rydberg atoms have been carried out in the resonant, non-dissipative regime. Here we realize a dissipative gas of rubidium Rydberg atoms and measure its full counting statistics for both resonant and off-resonant excitation. We find strongly bimodal counting distributions in the off-resonant regime that are compatible with intermittency due to the coexistence of dynamical phases. Moreover, we measure the phase diagram of the system and find good agreement with recent theoretical predictions. Our results pave the way towards detailed studies of many-body effects in Rydberg gases.

cond-mat.quant-gas↗

arXiv2013

Rydberg tomography of an ultra-cold atomic cloud

One of the most striking features of the strong interactions between Rydberg atoms is the dipole blockade effect, which allows only a single excitation to the Rydberg state within the volume of the blockade sphere. Here we present a method that spatially visualizes this phenomenon in an inhomogeneous gas of ultra-cold rubidium atoms. In our experiment we scan the position of one of the excitation lasers across the cold cloud and determine the number of Rydberg excitations detected as a function of position. Comparing this distribution to the one obtained for the number of ions created by a two-photon ionization process via the intermediate 5P level, we demonstrate that the blockade effect modifies the width of the Rydberg excitation profile. Furthermore, we study the dynamics of the Rydberg excitation and find that the timescale for the excitation depends on the atomic density at the beam position.

cond-mat.quant-gas↗

arXiv2012

Quantum driving protocols for a two level system: from generalized Landau-Zener sweeps to superadiabatic control

We present experimental results on the preparation of a desired quantum state in a two-level system with the maximum possible fidelity using driving protocols ranging from generalizations of the linear Landau-Zener protocol to transitionless driving protocols that ensure perfect following of the instantaneous adiabatic ground state. We also study the minimum time needed to achieve a target fidelity and explore and compare the robustness of some of the protocols against parameter variations simulating a possible experimental uncertainty. In our experiments, we realize a two-level model system using Bose-Einstein condensates inside optical lattices, but the results of our investigation should hold for any quantum system that can be approximated by a two-level system.

quant-ph↗

arXiv2012

Rydberg excitation of a Bose-Einstein condensate

We have performed two-photon excitation via the 6P3/2 state to n=50-80 S or D Rydberg state in Bose-Einstein condensates of rubidium atoms. The Rydberg excitation was performed in a quartz cell, where electric fields generated by plates external to the cell created electric charges on the cell walls. Avoiding accumulation of the charges and realizing good control over the applied electric field was obtained when the fields were applied only for a short time, typically a few microseconds. Rydberg excitations of the Bose-Einstein condensates loaded into quasi one-dimensional traps and in optical lattices have been investigated. The results for condensates expanded to different sizes in the one-dimensional trap agree well with the intuitive picture of a chain of Rydberg excitations controlled by the dipole-dipole interaction. The optical lattice applied along the one-dimensional geometry produces localized, collective Rydberg excitations controlled by the nearest-neighbour blockade.

physics.atom-ph↗

arXiv2012

Effect of photoions on the line shapes of the Förster resonance and microwave transitions in cold rubidium Rydberg atoms

Experiments on the spectroscopy of the Förster resonance Rb(37P)+Rb(37P) -> Rb(37S)+Rb(38S) and microwave transitions nP -> n'S, n'D between Rydberg states of cold Rb atoms in a magneto-optical trap have been performed. Under ordinary conditions, all spectra exhibited a 2-3 MHz line width independently of the interaction time of atoms with each other or with microwave radiation, although the ultimate resonance width should be defined by the inverse interaction time. Analysis of the experimental conditions has shown that the main source of the line broadening was the inhomogeneous electric field of cold photoions appeared at the excitation of initial Rydberg nP states by broadband pulsed laser radiation. Using an additional pulse of the electric field, which rapidly removed the photoions after the laser pulse, lead to a substantial narrowing of the microwave and Förster resonances. An analysis of various sources of the line broadening in cold Rydberg atoms has been conducted.

physics.atom-ph↗

arXiv2012

Wave Function Renormalization Effects in Resonantly Enhanced Tunneling

We study the time evolution of ultra-cold atoms in an accelerated optical lattice. For a Bose- Einstein condensate with a narrow quasi-momentum distribution in a shallow optical lattice the decay of the survival probability in the ground band has a step-like structure. In this regime we establish a connection between the wave function renormalization parameter Z introduced in [Phys. Rev. Lett. 86, 2699 (2001)] to characterize non-exponential decay and the phenomenon of resonantly enhanced tunneling, where the decay rate is peaked for particular values of the lattice depth and the accelerating force.

quant-ph↗

arXiv2011

Rydberg atoms in one-dimensional optical lattices

We experimentally realize Rydberg excitations in Bose-Einstein condensates of rubidium atoms loaded into quasi one-dimensional traps and in optical lattices. Our results for condensates expanded to different sizes in the one-dimensional trap agree well with the intuitive picture of a chain of Rydberg excitations. We also find that the Rydberg excitations in the optical lattice do not destroy the phase coherence of the condensate, and our results in that system agree with the picture of localized collective Rydberg excitations including nearest-neighbour blockade.

cond-mat.quant-gas↗

arXiv2010

Observation of Stückelberg oscillations in accelerated optical lattices

We report the experimental observation of Stückelberg oscillations of matter waves in optical lattices. Extending previous work on Landau-Zener tunneling of Bose-Einstein condensates in optical lattices, we study the effects of the accumulated phase between two successive crossings of the Brillouin zone edge. Our results agree well with a simple model for multiple Landau-Zener tunneling events taking into account the band structure of the optical lattice.

cond-mat.quant-gas↗

arXiv2010

Stimulated Raman adiabatic passage into continuum

We propose a technique which produces nearly complete ionization of the population of a discrete state coupled to a continuum by a two-photon transition via a lossy intermediate state whose lifetime is much shorter than the interaction duration. We show that using counterintuitively ordered pulses, as in stimulated Raman adiabatic passage (STIRAP), wherein the pulse coupling the intermediate state to the continuum precedes and partly overlaps the pulse coupling the initial and intermediate states, greatly increases the ionization signal and strongly reduces the population loss due to spontaneous emission through the lossy state. For strong spontaneous emission from that state, however, the ionization is never complete because the dark state required for STIRAP does not exist. We demonstrate that this drawback can be eliminated almost completely by creating a laser-induced continuum structure (LICS) by embedding a third discrete state into the continuum with a third control laser. This LICS introduces some coherence into the continuum, which enables a STIRAP-like population transfer into the continuum. A highly accurate analytic description is developed and numerical results are presented for Gaussian pulse shapes.

quant-ph↗