arXiv subjects

E. Brambrink

Publications and source records attributed to E. Brambrink.

7 recordsLinked to original sources

arXiv2026

Nanosecond timescale plasticity in shock-compressed polycrystalline MgO: evidence for transition in mechanism above 100 GPa

The mechanical properties of ceramics under extreme conditions directly impact applications ranging from shielding spacecrafts, designing plasma facing materials in nuclear fusion to understanding the rheology of deep planetary interiors. Here, we use polycrystalline MgO as a model ceramic to understand the high-pressure-temperature mechanical behaviour of such materials under extreme strain rates. We use laser-driven shock compression up to 175(15) GPa on the principal Hugoniot along with ultrafast diagnostics at the European X-ray Free Electron Laser to probe the dominant deformation mechanisms with changing P -T conditions. These near-instantaneous time-resolved snapshots, coupled with elasto-viscoplastic self-consistent (EVPSC) simulations, strongly suggest that MgO attains plastic regime in the nanoseconds scale accompanied by a pressure-mediated change in dominant slip system between 95 and 175 GPa. This work provides a new direct window into the deformation dynamics of polycrystalline ceramics under high-velocity impacts.

cond-mat.mtrl-sci↗

arXiv2026

Volume Collapse Without a Structural Transition in Shock-Compressed FeO

We report x-ray diffraction and emission spectroscopy of FeO under laser-driven shock compression between 31-199 GPa. FeO retains the B1 (rocksalt) structure along the Hugoniot to the melt boundary at 191 GPa. While the phase and volume are broadly consistent with results from static compression, we observe an anomalous 7-10% volume collapse around 60 GPa absent in static experiments. We identify this as an isostructural high-spin to low-spin metallic transition in FeO. The low-spin state is directly evidenced by x-ray emission spectroscopy at 180 GPa.

cond-mat.mtrl-sci↗

arXiv2025

Scaling of thin wire cylindrical compression after 100 fs Joule surface heating with material, diameter and laser energy

We present the first systematic experimental validation of return-current-driven implosion scaling in micrometer-sized wires irradiated by femtosecond laser pulses. Employing XFEL-based imaging with sub-micrometer spatial and femtosecond temporal resolution, supported by hydrodynamic and particle-in-cell simulations, we reveal how return current density depends precisely on wire diameter, material properties, and incident laser energy. We identify deviations from simple theoretical predictions due to geometrically influenced electron escape dynamics. These results refine and confirm the scaling laws essential for predictive modeling in high-energy-density physics and inertial fusion research.

physics.plasm-ph↗

arXiv2025

Shake-off in XFEL heated solid density plasma

In atoms undergoing ionisation, an abrupt re-arrangement of free and bound electrons can lead to the ejection of another bound electron (shake-off). The spectroscopic signatures of shake-off have been predicted and observed in atoms and solids. Here, we present the first observation of this process in a solid-density plasma heated by an x-ray free electron laser. The results show that shake-off of L-shell electrons persists up to temperatures of 10 eV at solid density, and follow the probability predicted for solids. This work shows that shake-off should be included in plasma models for the correct interpretation of emission spectra.

physics.plasm-ph↗

arXiv2024

Plasma screening in mid-charged ions observed by K-shell line emission

Dense plasma environment affects the electronic structure of ions via variations of the microscopic electrical fields, also known as plasma screening. This effect can be either estimated by simplified analytical models, or by computationally expensive and to date unverified numerical calculations. We have experimentally quantified plasma screening from the energy shifts of the bound-bound transitions in matter driven by the x-ray free electron laser (XFEL). This was enabled by identification of detailed electronic configurations of the observed K{\alpha}, K\b{eta} and K{\gamma} lines. This work paves the way for improving plasma screening models including connected effects like ionization potential depression and continuum lowering, which will advance the understanding of atomic physics in Warm Dense Matter regime.

physics.plasm-ph↗

arXiv2018

Characterising equation of state and optical properties of dynamically pre-compressed materials

Characterising materials at pressures of several megabar and temperatures of a few thousand Kelvin is critical for the understanding of the Warm Dense Matter regime and to improve planetary models as these conditions are typical of planets' interiors. Today, laser-driven shock compression is the only technique to achieve multimegabar pressures, but the associated temperatures are too high to be representative of planetary states. Double-shock compression represents an alternative to explore lower temperatures. Here we present a method to create well-controlled double-shocked states and measure their thermodynamic state and optical reflectivity using standard optical diagnostics (Doppler velocimetry and optical pyrometry) in a laser-driven shock experiment. This method, which does not require the support of hydrodynamical simulations, is based on the application of generalised Rankine-Hugoniot relations together with a self impedance mismatch technique. A validation experiment has been performed at the LULI2000 facility (École Polytechnique, France) on a sample of $α$-quartz. A temperature $60 \%$ lower than along the principal Hugoniot has been obtained at 7.5 Mbar.

physics.plasm-ph↗

arXiv2018

Equation of state and optical properties of shock-compressed C:H:N:O molecular mixtures

Water, ethanol, and ammonia are the key components of the mantles of Uranus and Neptune. To improve structure and evolution models and give an explanation of the magnetic fields and luminosities of the icy giants, those components need to be characterised at planetary conditions (some Mbar and a few $10^3$ K). Those conditions are typical of the Warm Dense Matter regime, which exhibits a rich phase diagram, with the coexistence of many states of matter and a large variety of chemical processes. H$_2$O, C:H:O, and C:H:N:O mixtures have been compressed up to 2.8 Mbar along the principal Hugoniot using laser-driven decaying shocks. The experiments were performed at the GEKKO XII and LULI 2000 laser facilities using standard optical diagnostics (Doppler velocimetry and pyrometry) to characterise equation of state and optical reflectivity of the shocked states. The results show that H$_2$O and the C:H:N:O mixture share the same equation of state with a density scaling, while the reflectivity behaves differently by what concerns both the onset pressures and the saturation values. The reflectivity measurement at two frequencies allows to estimate the conductivity and the complex refractive index using a Drude model.

astro-ph.EP↗