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E. Caden

Publications and source records attributed to E. Caden.

At least 19 recordsLinked to original sources

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det

Cosmogenic Neutron Production in Water at SNO+

Accurate measurement of the cosmogenic muon-induced neutron yield is crucial for constraining a significant background in a wide range of low-energy physics searches. Although previous underground experiments have measured this yield across various cosmogenic muon energies, SNO+ is uniquely positioned due to its exposure to one of the highest average cosmogenic muon energies at $364\,\text{GeV}$. Using ultra-pure water, we have determined a neutron yield of $Y_{n}=(3.38^{+0.23}_{-0.30})\times10^{-4}\,\text{cm}^{2}\text{g}^{-1}μ^{-1}$ at SNO+. Comparison with simulations demonstrates clear agreement with the FLUKA neutron production model, highlighting discrepancies with the widely used GEANT4 model. Furthermore, this measurement reveals a lower cosmogenic neutron yield than that observed by the SNO experiment, which used heavy water under identical muon flux conditions. This result provides new evidence that nuclear structure and target material composition significantly influence neutron production by cosmogenic muons, offering fresh insight with important implications for the design and background modelling of future underground experiments.

hep-ex

Characterization of CRYO ASIC for charge readout in the nEXO experiment

nEXO is a proposed next-generation experiment searching for the neutrinoless double beta decay of $^{136}$Xe using a tonne-scale liquid xenon (LXe) time projection chamber (TPC). To image the ionization signals from events in the liquid xenon, the detector will employ metallized fused-silica charge collection tiles instrumented with cryogenic application-specific integrated circuits (ASICs), referred to as CRYO ASIC, which are designed to operate directly in LXe to minimize input capacitance and pick-up noise. Here we present the performance of the CRYO ASIC mounted on an auxiliary printed circuit board and evaluated both in a cryogenic environmental chamber and in a dedicated LXe test stand. We demonstrate that the ASICs achieve the desired performance at liquid xenon temperatures, showing a gain stability better than 0.2% over 24-hour operation and reliable in-situ calibration using an on-chip pulser. In the LXe test stand, we show that boiling caused by the chip heat dissipation can be mitigated by operating the system above ~0.1 MPa. The in-LXe noise measured agrees with simulation, which indicates it the $150~e^-$ design requirement can be satisfied. These results establish CRYO ASIC as a viable low-noise in-LXe charge readout solution for nEXO.

physics.ins-det

Measurement of reactor antineutrino oscillations with 1.46 ktonne-years of data at SNO+

The SNO+ Collaboration reports new results on reactor antineutrino oscillations using data acquired from May 2022 through July 2025. The spectral analysis of a flux dominated by nuclear reactors at 240, 350, and 355 kilometers yields the mass-squared difference $\Delta m^2_{21}=(7.93^{+0.21}_{-0.24})\times 10^{-5}$ eV$^2$. This result is compatible with and approaches the precision of the only other long-baseline reactor antineutrino measurement, by KamLAND. Combining these measurements, along with those from solar neutrino experiments, the global values of the neutrino mixing parameters become: $\Delta m^2_{21}$ = $(7.63\pm0.17)\times 10^{-5}$ eV$^2$ and $\sin^2{\theta_{12}}=0.310\pm0.012$. The analysis of geoneutrinos at SNO+ is also improved, with a measured signal of 49$^{+13}_{-12}$ TNU.

hep-ex

First Evidence of Solar Neutrino Interactions on $^{13}$C

The SNO+ Collaboration reports the first evidence of $^{8}\text{B}$ solar neutrinos interacting on $^{13}\text{C}$ nuclei. The charged current interaction proceeds through $^{13}\text{C} + ν_e \rightarrow {}^{13}\text{N} + e^-$ which is followed, with a 10 minute half-life, by ${}^{13}\text{N} \rightarrow {}^{13}\text{C} + e^+ +ν_e .$ The detection strategy is based on the delayed coincidence between the electron and the positron. Evidence for the charged current signal is presented with a significance of 4.2$σ$. Using the natural abundance of $^{13}\text{C}$ present in the scintillator, 5.7 tonnes of $^{13}\text{C}$ over 231 days of data were used in this analysis. The 5.6$^{+3.0}_{-2.3}$ observed events in the data set are consistent with the expectation of 4.7$^{+0.6}_{-1.3}$ events. This result is the second real-time measurement of CC interactions of $^{8}\text{B}$ neutrinos with nuclei and constitutes the lowest energy observation of neutrino interactions on $^{13}\text{C}$ generally. This enables the first direct measurement of the CC $ν_e$ reaction to the ground state of ${}^{13}\text{N}$, yielding an average cross section of $(16.1 ^{+8.5}_{-6.7} (\text{stat.}) ^{+1.6}_{-2.7} (\text{syst.}) )\times 10^{-43}$ cm$^{2}$ over the relevant $^{8}\text{B}$ solar neutrino energies.

nucl-ex

Measurement of reactor antineutrino oscillation at SNO+

The SNO+ collaboration reports its second spectral analysis of reactor antineutrino oscillation using 286 tonne-years of new data. The measured energies of reactor antineutrino candidates were fitted to obtain the second-most precise determination of the neutrino mass-squared difference $Δm^2_{21}$ = ($7.96^{+0.48}_{-0.42}$) $\times$ 10$^{-5}$ eV$^2$. Constraining $Δm^2_{21}$ and $\sin^2θ_{12}$ with measurements from long-baseline reactor antineutrino and solar neutrino experiments yields $Δm^2_{21}$ = ($7.58^{+0.18}_{-0.17}$) $\times$ 10$^{-5}$ eV$^2$ and $\sin^2θ_{12} = 0.308 \pm 0.013$. This fit also yields a first measurement of the flux of geoneutrinos in the Western Hemisphere, with $73^{+47}_{-43}$ TNU at SNO+.

hep-ex

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Community Report from the 2025 SNOLAB Future Projects Workshop

SNOLAB hosts a biannual Future Projects Workshop (FPW) with the goal of encouraging future project stakeholders to present ideas, concepts, and needs for experiments or programs that could one day be hosted at SNOLAB. The 2025 FPW was held in the larger context of a 15-year planning exercise requested by the Canada Foundation for Innovation. This report collects input from the community, including both contributions to the workshop and contributions that could not be scheduled in the workshop but nonetheless are important to the community.

hep-ex

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $μ$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

Sensitivity of nEXO to $^{136}$Xe Charged-Current Interactions: Background-free Searches for Solar Neutrinos and Fermionic Dark Matter

We study the sensitivity of nEXO to solar neutrino charged-current interactions, $ν_e + ^{136}$Xe$\rightarrow ^{136}$Cs$^* + e^-$, as well as analogous interactions predicted by models of fermionic dark matter. Due to the recently observed low-lying isomeric states of $^{136}$Cs, these interactions will create a time-delayed coincident signal observable in the scintillation channel. Here we develop a detailed Monte Carlo of scintillation emission, propagation, and detection in the nEXO detector to model these signals under different assumptions about the timing resolution of the photosensor readout. We show this correlated signal can be used to achieve background discrimination on the order of $10^{-9}$, enabling nEXO to make background-free measurements of solar neutrinos above the reaction threshold of 0.668 MeV. We project that nEXO could measure the flux of CNO solar neutrinos with a statistical uncertainty of 25%, thus contributing a novel and competitive measurement towards addressing the solar metallicity problem. Additionally, nEXO could measure the mean energy of the $^7$Be neutrinos with a precision of $σ\leq 1.5$ keV and could determine the survival probability of $^{7}$Be and $pep$ solar $ν_e$ with precision comparable to state-of-the-art. These quantities are sensitive to the Sun's core temperature and to non-standard neutrino interactions, respectively. Furthermore, the strong background suppression would allow nEXO to search for for charged-current interactions of fermionic dark matter in the mass range $m_χ$ = $0.668$-$7$ MeV with a sensitivity up to three orders of magnitude better than current limits.

nucl-ex

Initial measurement of reactor antineutrino oscillation at SNO+

The SNO+ collaboration reports its first spectral analysis of long-baseline reactor antineutrino oscillation using 114 tonne-years of data. Fitting the neutrino oscillation probability to the observed energy spectrum yields constraints on the neutrino mass-squared difference $Δm^2_{21}$. In the ranges allowed by previous measurements, the best-fit $Δm^2_{21}$ is (8.85$^{+1.10}_{-1.33}$) $\times$ 10$^{-5}$ eV$^2$. This measurement is continuing in the next phases of SNO+ and is expected to surpass the present global precision on $Δm^2_{21}$ with about three years of data.

hep-ex

Measurement of the $^8$B Solar Neutrino Flux Using the Full SNO+ Water Phase Dataset

The SNO+ detector operated initially as a water Cherenkov detector. The implementation of a sealed covergas system midway through water data taking resulted in a significant reduction in the activity of $^{222}$Rn daughters in the detector and allowed the lowest background to the solar electron scattering signal above 5 MeV achieved to date. This paper reports an updated SNO+ water phase $^8$B solar neutrino analysis with a total livetime of 282.4 days and an analysis threshold of 3.5 MeV. The $^8$B solar neutrino flux is found to be $\left(2.32^{+0.18}_{-0.17}\text{(stat.)}^{+0.07}_{-0.05}\text{(syst.)}\right)\times10^{6}$ cm$^{-2}$s$^{-1}$ assuming no neutrino oscillations, or $\left(5.36^{+0.41}_{-0.39}\text{(stat.)}^{+0.17}_{-0.16}\text{(syst.)} \right)\times10^{6}$ cm$^{-2}$s$^{-1}$ assuming standard neutrino oscillation parameters, in good agreement with both previous measurements and Standard Solar Model Calculations. The electron recoil spectrum is presented above 3.5 MeV.

hep-ex

Supernova electron-neutrino interactions with xenon in the nEXO detector

Electron-neutrino charged-current interactions with xenon nuclei were modeled in the nEXO neutrinoless double-$β$ decay detector (~5 metric ton, 90% ${}^{136}$Xe, 10% ${}^{134}$Xe) to evaluate its sensitivity to supernova neutrinos. Predictions for event rates and detectable signatures were modeled using the Model of Argon Reaction Low Energy Yields (MARLEY) event generator. We find good agreement between MARLEY's predictions and existing theoretical calculations of the inclusive cross sections at supernova neutrino energies. The interactions modeled by MARLEY were simulated within the nEXO simulation framework and were run through an example reconstruction algorithm to determine the detector's efficiency for reconstructing these events. The simulated data, incorporating the detector response, were used to study the ability of nEXO to reconstruct the incident electron-neutrino spectrum and these results were extended to a larger xenon detector of the same isotope enrichment. We estimate that nEXO will be able to observe electron-neutrino interactions with xenon from supernovae as far as 5-8 kpc from Earth, while the ability to reconstruct incident electron-neutrino spectrum parameters from observed interactions in nEXO is limited to closer supernovae.

hep-ph

Imaging of single barium atoms in a second matrix site in solid xenon for barium tagging in a $^{136}$Xe double beta decay experiment

Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is $^{136}$Xe, which would double beta decay into $^{136}$Ba. Detecting the single $^{136}$Ba daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon.

physics.atom-ph

Event-by-Event Direction Reconstruction of Solar Neutrinos in a High Light-Yield Liquid Scintillator

The direction of individual $^8$B solar neutrinos has been reconstructed using the SNO+ liquid scintillator detector. Prompt, directional Cherenkov light was separated from the slower, isotropic scintillation light using time information, and a maximum likelihood method was used to reconstruct the direction of individual scattered electrons. A clear directional signal was observed, correlated with the solar angle. The observation was aided by a period of low primary fluor concentration that resulted in a slower scintillator decay time. This is the first time that event-by-event direction reconstruction in high light-yield liquid scintillator has been demonstrated in a large-scale detector.

hep-ex

An integrated online radioassay data storage and analytics tool for nEXO

Large-scale low-background detectors are increasingly used in rare-event searches as experimental collaborations push for enhanced sensitivity. However, building such detectors, in practice, creates an abundance of radioassay data especially during the conceptual phase of an experiment when hundreds of materials are screened for radiopurity. A tool is needed to manage and make use of the radioassay screening data to quantitatively assess detector design options. We have developed a Materials Database Application for the nEXO experiment to serve this purpose. This paper describes this database, explains how it functions, and discusses how it streamlines the design of the experiment.

physics.ins-det

Evidence of Antineutrinos from Distant Reactors using Pure Water at SNO+

The SNO+ Collaboration reports the first evidence of reactor antineutrinos in a Cherenkov detector. The nearest nuclear reactors are located 240~km away in Ontario, Canada. This analysis uses events with energies lower than in any previous analysis with a large water Cherenkov detector. Two analytical methods are used to distinguish reactor antineutrinos from background events in 190 days of data and yield consistent evidence for antineutrinos with a combined significance of 3.5$σ$.

nucl-ex

Neutrinoless Double Beta Decay

This White Paper, prepared for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting related to the 2023 Nuclear Physics Long Range Plan, makes the case for double beta decay as a critical component of the future nuclear physics program. The major experimental collaborations and many theorists have endorsed this white paper.

nucl-ex