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E. Martinez

Publications and source records attributed to E. Martinez.

At least 19 recordsLinked to original sources

Current-induced magnetization control in dipolar-coupled nanomagnet pairs and artificial spin ice

Exploiting current-induced spin-orbit torques (SOTs) to manipulate the magnetic state of dipolar-coupled nanomagnet systems with in-plane magnetic anisotropy, such as artificial spin ices, provides a route to local, electrically-programmable control of the magnetization, with relevance for applications including neuromorphic computing. Here, we demonstrate how the orientation of a nanomagnet relative to the direction of an applied electrical current impacts the threshold current density needed for all-electrical magnetization switching, and how dipolar coupling between the nanomagnets influences the switching of interacting pairs and ensembles of nanomagnets. Using a material system designed to generate SOTs in response to electrical currents, we find that the current required to switch the magnetization of isolated nanomagnets varies non-monotonically as the angle between the nanomagnet long axis and the current increases. In small artificial spin ice systems, we observe similar angular dependence of the switching current, which can be used to control the magnetization orientation of specific subsets of nanomagnets. These experimental results are supported by micromagnetic modeling, which illustrates how the various current induced torques can be exploited to control magnetization switching in nanomagnetic systems. These results establish SOT switching as a practical method for programmable manipulation of dipolar nanomagnetic systems.

cond-mat.mes-hall

Laser Annealing of Transparent ZnO Thin Films: A Route to Improve Electrical Conductivity and Oxygen Sensing Capabilities

The chemical deposition of high-performance Zinc Oxide (ZnO) thin films is challenging, thus significant efforts have been devoted during the past decades to develop cost-effective, scalable fabrication methods in gas phase. This work demonstrates how ultra-short-pulse Laser Beam Scanning (LBS) can be used to modulate electrical conductivity in ZnO thin films deposited on soda-lime glass by Spatial Atomic Layer Deposition (SALD), a high-throughput, low-temperature deposition technique suitable for large-area applications. By systematically optimizing laser parameters, including pulse energy and hatching distance, significant improvements in the electrical performance of 90 nm-thick ZnO films were achieved. The optimization of the laser annealing parameters, 0.21 uJ/pulse energy and a 1 micron hatching distance, yielded ZnO films with an electrical resistivity of (9 +- 2) 10-2 Ohm cm, 3 orders of magnitude lower than as deposited films. This result suggests that laser post-deposition-processing can play an important role in tailoring the properties of ZnO thin films. Excessive laser intensity can compromise structural integrity of the films, however, degrading their electrical transport properties. Notably, the electrical resistance of laser-annealed ZnO films exhibited high sensitivity to oxygen concentration in the surrounding atmosphere, suggesting exciting prospects for application in devices based on transparent oxygen sensors. This study thus positions ultra-short pulsed laser annealing as a versatile post-deposition method for fine-tuning the properties of ZnO thin films, enabling their use in advanced optoelectronic and gas-sensing technologies, particularly on temperature-sensitive substrates.

physics.app-ph

Enhancing Irradiation Resistance in Refractory Medium Entropy Alloys with Simplified Chemistry

Refractory High-Entropy Alloys (RHEAs) hold promising potential to be used as structural materials in future nuclear fusion reactors, where W and its alloys are currently leading candidates. Fusion materials must be able to withstand extreme conditions, such as (i) severe radiation-damage arising from highly-energetic neutrons, (ii) embrittlement caused by implantation of H and He ions, and (iii) exposure to extreme high-temperatures and thermal gradients. Recent research demonstrated that two RHEAs - the WTaCrV and WTaCrVHf - can outperform both coarse-grained and nanocrystalline W in terms of its radiation response and microstructural stability. Chemical complexity and nanocrystallinity enhance the radiation tolerance of these new RHEAs, but their multi-element nature, including low-melting Cr, complicates bulk fabrication and limits practical applications. We demonstrate that reducing the number of alloying elements and yet retain high-radiation tolerance is possible within the ternary system W-Ta-V via synthesis of two novel nanocrystalline refractory medium-entropy alloys (RMEAs): the W$_{53}$Ta$_{44}$V$_{3}$ and W$_{53}$Ta$_{42}$V$_{5}$ (in at.\%). We experimentally show that the radiation response of the W-Ta-V system can be tailored by small additions of V, and such experimental result was validated with theoretical analysis of chemical short-range orders (CSRO) from combined ab-initio atomistic Monte-Carlo modeling. It is predicted from computational analysis that a small change in V concentration has a significant effect on the Ta-V CRSO between W$_{53}$Ta$_{44}$V$_{3}$ and W$_{53}$Ta$_{42}$V$_{5}$ leading to radiation-resistant microstructures in these RMEAs from chemistry stand-point of views. We deviate from the original high-entropy alloy concept to show that high radiation resistance can be achieved in systems with simplified chemical complexity.

cond-mat.mtrl-sci

An innovative materials design protocol for the development of novel refractory high-entropy alloys for extreme environments

In the quest of new materials that can withstand severe irradiation and mechanical extremes for advanced applications (e.g. fission reactors, fusion devices, space applications, etc), design, prediction and control of advanced materials beyond current material designs become a paramount goal. Here, though a combined experimental and simulation methodology, the design of a new nanocrystalline refractory high entropy alloy (RHEA) system is established. Compositions of this alloy, assessed under extreme environments and in situ electron-microscopy, revealed both high mechanical strength and thermal stability, grain refinement under heavy ion irradiation and outstanding irradiation resistance to dual-beam irradiation and helium implantation, marked by remarkable resistance to defect generation, growth and coalescence. The experimental and modeling results, which demonstrated notable agreement, can be applied to design and rapidly assess other alloys subjected to extreme environmental conditions.

cond-mat.mtrl-sci

Local and Non-local Microwave Impedance of a Three-Terminal Hybrid Device

We report microwave impedance measurements of a superconductor-semiconductor hybrid nanowire device with three terminals (3T). Our technique makes use of transmission line resonators to acquire the nine complex scattering matrix parameters (S-parameters) of the device on fast timescales and across a spectrum of frequencies spanning 0.3 - 7 GHz. Via comparison with dc-transport measurements, we examine the utility of this technique for probing the local and non-local response of 3T devices where capacitive and inductive contributions can play a role. Such measurements require careful interpretation but may be of use in discerning true Majorana zero modes from trivial states arising from disorder.

cond-mat.mes-hall

Statistical investigation of the large-area Si(Li) detectors mass-produced for the GAPS experiment

The lithium-drifted silicon (Si(Li)) detector developed for the General Antiparticle Spectrometer (GAPS) experiment features a thick (~2.2 mm) sensitive layer, large (10 cm) diameter, and excellent energy resolution (~4 keV for 20-100 keV X-rays) at a relatively high operating temperature (approximately -40C). Mass production of GAPS Si(Li) detectors has been performed to construct a large-volume silicon tracker for GAPS. We achieved the first success of the mass production of large-area Si(Li) detectors with a high (~90%) yield rate. Valuable datasets related to detector fabrication, such as detector performance and manufacturing parameters, were recorded and collected during the mass production. This study analyzes the datasets using statistical methods with the aim of comprehensively examining the mass production and to gain valuable insight into the fabrication method. Sufficient uniformities of the performance parameters (leakage current and capacitance) between detectors and strips are found, demonstrating high-quality and stable mass production. We also search for correlations between detector performance and manufacturing parameters by using data-mining techniques. Conventional multivariate analysis (multiple regression analysis) and machine-learning techniques (regression tree analysis) are complementarily used, and it is found that the Li-drift process makes a significant contribution to the performance parameters of the finished detectors. Detailed investigation of the drift process is performed using environmental data, and physical interpretations are presented. Our results provide valuable insight into the fabrication methods for this kind of large-area Si(Li) detector, and encourages future projects that require large-volume silicon trackers.

physics.ins-det

Outstanding Radiation Resistance of Tungsten-based High Entropy Alloys

A novel W-based refractory high entropy alloy with outstanding radiation resistance has been developed. The alloy was grown as thin films showing a bimodal grain size distribution in the nanocrystalline and ultrafine regimes and a unique 4 nm lamella-like structure revealed by atom probe tomography (APT). Transmission electron microscopy (TEM) and X-ray diffraction show an underlying body-centered cubic crystalline structure with certain black spots appearing after thermal annealing at elevated temperatures. Thorough analysis based on TEM and APT correlated the black spots with second phase particles rich in Cr and V. After both in situ and ex situ irradiation, these precipitates evolve to quasi-spherical particles with no sign of irradiation-created dislocation loops even after 8 dpa at either room temperature or 1073 K. Furthermore, nanomechanical testing shows a large hardness of 14 GPa in the as-deposited samples, with a slight increase after thermal annealing and almost negligible irradiation hardening. Theoretical modeling based on ab initio methodologies combined with Monte Carlo techniques predicts the formation of Cr and V rich second phase particles and points at equal mobilities of point defects as the origin of the exceptional radiation tolerance. The fact that these alloys are suitable for bulk production coupled with the exceptional radiation and mechanical properties makes them ideal structural materials for applications requiring extreme conditions.

cond-mat.mtrl-sci

Modification of Dzyaloshinskii-Moriya interaction stabilized domain wall chirality by driving currents

We measure and analyze the chirality of the Dzyaloshinskii-Moriya interaction (DMI) stabilized spin textures in multilayers of Ta/Co$_{20}$Fe$_{60}$B$_{20}$/MgO. The effective DMI is measured experimentally using domain wall motion measurements, both in the presence (using spin orbit torques) and absence of driving currents (using magnetic fields). We observe that the current-induced domain wall motion yields a change in effective DMI magnitude and opposite domain wall chirality when compared to field-induced domain wall motion (without current). We explore this effect, which we refer to as current-induced DMI, by providing possible explanations for its emergence, and explore the possibilty of its manifestation in the framework of recent theoretical predictions of DMI modifications due to spin currents.

cond-mat.mes-hall

Study of energetics of 360° domain walls through annihilation

The Dzyaloshinskii-Moriya interaction (DMI) causes domain walls in perpendicular magnetized systems to adopt a homochiral configuration by winding in the same direction for both Up-Down and Down-Up walls. The topology of these domain walls is then distinct from the uniformly magnetized state. When two domain walls approach each other and are in close proximity they form winding pairs, stabilized by a dipolar repulsion. This can result in the formation of 360 ° stable domain walls, whose stability is directly related to the magnitude of the additional dipolar interaction resulting from the spin structure governed by the DMI. Application of an external magnetic field can overcome the dipolar repulsion of the winding pairs and result in the annihilation of the domain walls, which is studied here in a combined theoretical and experimental effort. We present an extended analytical model that studies the interaction and modification of the dipolar interaction of the domain wall pairs under the application of in-plane and out-of-plane magnetic fields. We realize the experiment in a system of Ta/Co$_{20}$Fe$_{60}$B$_{20}$/MgO and observe that the results are in agreement with the behavior predicted by the analytical model. To compare and understand these results, we perform micromagnetic calculations to gauge the validity of the analytics and also include the full dipolar interactions which are present due to the device geometry. We find that our numerical and experimental studies are in agreement and that the DMI indeed provides an additional stability mechanism against annihilation of DWs, which is potentially useful in dense memory storage applications. Beyond implications for domain walls, understanding the interaction is an important step to understand and control the interaction of many spin structures that contain domain walls, such as skyrmions.

cond-mat.mes-hall

Performance of synthetic antiferromagnetic racetrack memory: domain wall vs skyrmion

A storage scheme based on racetrack memory, where the information can be coded in a domain or a skyrmion, seems to be an alternative to conventional hard disk drive for high density storage. Here, we perform a full micromagnetic study of the performance of synthetic antiferromagnetic (SAF) racetrack memory in terms of velocity and sensitivity to defects by using experimental parameters. We find that to stabilize a SAF skyrmion, the Dzyaloshinskii-Moriya Interaction in the top and the bottom ferromagnet should have an opposite sign. The velocity of SAF skyrmion and SAF Neel domain wall are of the same order and can reach values larger than 1200 m/s if a spin-orbit torque from the spin-Hall effect with opposite sign is applied to both ferromagnets.

cond-mat.mtrl-sci

A strategy for the design of skyrmion racetrack memories

Magnetic storage based on racetrack memory is very promising for the design of ultra-dense, low-cost and low-power storage technology. Information can be coded in a magnetic region between two domain walls or, as predicted recently, in topological magnetic objects known as skyrmions. Here, we show the technological advantages and limitations of using Bloch and Neel skyrmions manipulated by spin current generated within the ferromagnet or via the spin-Hall effect arising from a non-magnetic heavy metal underlayer. We found that the Neel skyrmion moved by the spin-Hall effect is a very promising strategy for technological implementation of the next generation of skyrmion racetrack memories (zero field, high thermal stability, and ultra-dense storage). We employed micromagnetics reinforced with an analytical formulation of skyrmion dynamics that we developed from the Thiele equation. We identified that the excitation, at high currents, of a breathing mode of the skyrmion limits the maximal velocity of the memory.

cond-mat.mes-hall

Interfacial Dzyaloshinskii-Moriya interaction in Ta\Co20Fe60B20\MgO nanowires

We report current-induced domain wall motion (CIDWM) in Ta\Co20Fe60B20\MgO nanowires. Domain walls are observed to move against the electron flow when no magnetic field is applied, while a field along the nanowires strongly affects the domain wall motion direction and velocity. A symmetric effect is observed for up-down and down-up domain walls. This indicates the presence of right-handed domain walls, due to a Dzyaloshinskii-Moriya interaction (DMI) with a DMI coefficient D=+0.06 mJ/m2. The positive DMI coefficient is interpreted to be a consequence of boron diffusion into the tantalum buffer layer during annealing. In a Pt\Co68Fe22B10\MgO nanowire CIDWM along the electron flow was observed, corroborating this interpretation. The experimental results are compared to 1D-model simulations including the effects of pinning. This advanced modelling allows us to reproduce the experiment outcomes and reliably extract a spin-Hall angle θSH=-0.11 for Ta in the nanowires, showing the importance of an analysis that goes beyond the currently used model for perfect nanowires.

cond-mat.mes-hall

Chiral magnetization textures stabilized by the Dzyaloshinskii-Moriya interaction during spin-orbit torque switching

We study the effect of the Dzyaloshinskii-Moriya interaction (DMI) on current-induced magnetic switching of a perpendicularly magnetized heavy-metal/ferromagnet/oxide trilayer both experimentally and through micromagnetic simulations. We report the generation of stable helical magnetization stripes for a sufficiently large DMI strength in the switching region, giving rise to intermediate states in the magnetization confirming the essential role of the DMI on switching processes. We compare the simulation and experimental results to a macrospin model, showing the need for a micromagnetic approach. The influence of the temperature on the switching is also discussed.

cond-mat.mes-hall

Switching of a single ferromagnetic layer driven by spin Hall effect

The magnetization switching of a thin ferromagnetic layer placed on top of a heavy metal (such as Pt, Ta or W) driven by an in-plane current has been observed in recent experiments. The magnetization dynamics of these processes is studied in a full micromagnetic framework which takes into account the transfer-torque from spin Hall effect due to the spin-orbit coupling. Simulations indicate that the reversal occurs via nucleation of complex magnetization patterns. In particular, magnetic bubbles appear during the reversal of the magnetization in the perpendicular configuration while for the in-plane configuration, nucleation of vortexes are observed.

cond-mat.mtrl-sci

Simulations of decomposition kinetics of Fe-Cr solid solutions during thermal aging

The decomposition of Fe-Cr solid solutions during thermal aging is modeled by Atomistic Kinetic Monte Carlo (AKMC) simulations, using a rigid lattice approximation with composition dependant pair interactions that can reproduce the change of sign of the mixing energy with the alloy composition. The interactions are fitted on ab initio mixing energies and on the experimental phase diagram, as well as on the migration barriers in iron and chromium rich phases. Simulated kinetics is compared with 3D atom probe and neutron scattering experiments.

cond-mat.mtrl-sci

Geometric Hamilton-Jacobi Theory for Nonholonomic Dynamical Systems

The geometric formulation of Hamilton--Jacobi theory for systems with nonholonomic constraints is developed, following the ideas of the authors in previous papers. The relation between the solutions of the Hamilton--Jacobi problem with the symplectic structure defined from the Lagrangian function and the constraints is studied. The concept of complete solutions and their relationship with constants of motion, are also studied in detail. Local expressions using quasivelocities are provided. As an example, the nonholonomic free particle is considered.

math-ph

Hamilton-Jacobi theory and the evolution operator

We present a new setting of the geometric Hamilton-Jacobi theory by using the so-called time-evolution operator K. This new approach unifies both the Lagrangian and the Hamiltonian formulation of the problem developed in a previous paper [7], and can be applied to the case of singular Lagrangian dynamical systems.

math-ph

Non-holonomic Lagrangian systems on Lie algebroids

This paper presents a geometric description on Lie algebroids of Lagrangian systems subject to nonholonomic constraints. The Lie algebroid framework provides a natural generalization of classical tangent bundle geometry. We define the notion of nonholonomically constrained system, and characterize regularity conditions that guarantee the dynamics of the system can be obtained as a suitable projection of the unconstrained dynamics. The proposed novel formalism provides new insights into the geometry of nonholonomic systems, and allows us to treat in a unified way a variety of situations, including systems with symmetry, morphisms and reduction, and nonlinearly constrained systems. Various examples illustrate the results.

math-ph