arXiv subjects

E. Somorjai

Publications and source records attributed to E. Somorjai.

At least 19 recordsLinked to original sources

arXiv2019

High precision half-life measurement of $^{125}$Cs and $^{125}$Xe with γ-spectroscopy

In order to provide data for the simulation of the astrophysical $γ$-process, the cross section measurement of the $^{124}$Xe(p,$γ$)$^{125}$Cs reaction is in progress at MTA Atomki using the activation technique. Precise information on the decay characteristics of the reaction products is of crucial importance for measurements carried out using this method. The half-lives of the produced $^{125}$Cs and its daughter $^{125}$Xe are published in previous works, but with large uncertainties and ambiguous values. To make these nuclear parameters more precise, the half-lives have been re-measured with high precision using $γ$-spectroscopy. The obtained new half-life values are t$_{1/2}$ = 44.35 $\pm$ 0.29 minutes for $^{125}$Cs and t$_{1/2}$ = 16.87 $\pm$ 0.08 hours for $^{125}$Xe.

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arXiv2018

Investigation of $α$-induced reactions on Sb isotopes relevant to the astrophysical $γ$-process

The aim of the present work is to measure the $^{121}$Sb($α,γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reaction cross sections. The $α$-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The ($α$,$γ$) cross sections of $^{121}$Sb were measured and are reported for first time. To determine the cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reactions, the yields of $γ$-rays following the $β$-decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic X-rays were counted with a LEPS (Low Energy Photon Spectrometer) detector. The cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I and $^{123}$Sb($α$,n)$^{126}$I reactions were measured with high precision in an energy range between 9.74 MeV to 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The ($α$,n) data show that the $α$ widths are predicted well for these reactions. The ($α$,$γ$) results are overestimated by the calculations but this is due to the applied neutron- and $γ$ widths. Relevant for the astrophysical reaction rate is the $α$ width used in the calculations.While for other reactions the $α$ widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.

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arXiv2016

$α$-scattering and $α$-induced reaction cross sections of $^{64}$Zn at low energies

Background: alpha-nucleus potentials play an essential role for the calculation of alpha-induced reaction cross sections at low energies in the statistical model... Purpose: The present work studies the total reaction cross section sigma_reac of alpha-induced reactions at low energies which can be determined from the elastic scattering angular distribution or from the sum over the cross sections of all open non-elastic channels. Method: Elastic and inelastic 64Zn(a,a)64Zn angular distributions were measured at two energies around the Coulomb barrier at 12.1 MeV and 16.1 MeV. Reaction cross sections of the (a,g), (a,n), and (a,p) reactions were measured at the same energies using the activation technique. The contributions of missing non-elastic channels were estimated from statistical model calculations. Results: The total reaction cross sections from elastic scattering and from the sum of the cross sections over all open non-elastic channels agree well within the uncertainties. This finding confirms the consistency of the experimental data. At the higher energy of 16.1 MeV, the predicted significant contribution of compound-inelastic scattering to the total reaction cross section is confirmed experimentally. As a by-product it is found that most recent global alpha-nucleus potentials are able to describe the reaction cross sections for 64Zn around the Coulomb barrier. Conclusions: Total reaction cross sections of alpha-induced reactions can be well determined from elastic scattering angular distributions. The present study proves experimentally that the total cross section from elastic scattering is identical to the sum of non-elastic reaction cross sections. Thus, the statistical model can reliably be used to distribute the total reaction cross section among the different open channels.

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arXiv2016

Improved Direct Measurement of the 64.5 keV Resonance Strength in the 17O(p,a)14N Reaction at LUNA

The $^{17}$O(p,$α$)$^{14}$N reaction plays a key role in various astrophysical scenarios, from asymptotic giant branch stars to classical novae. It affects the synthesis of rare isotopes such as $^{17}$O and $^{18}$F, which can provide constraints on astrophysical models. A new direct determination of the $E_{\rm R}~=~64.5$~keV resonance strength performed at the Laboratory for Underground Nuclear Astrophysics accelerator has led to the most accurate value to date, $ωγ= 10.0 \pm 1.4_{\rm stat} \pm 0.7_{\rm syst}$~neV, thanks to a significant background reduction underground and generally improved experimental conditions. The (bare) proton partial width of the corresponding state at $E_{\rm x} = 5672$~keV in $^{18}$F is $Γ_{\rm p} = 35 \pm 5_{\rm stat} \pm 3_{\rm syst}$~neV. This width is about a factor of 2 higher than previously estimated thus leading to a factor of 2 increase in the $^{17}$O(p,$α$)$^{14}$N reaction rate at astrophysical temperatures relevant to shell hydrogen-burning in red giant and asymptotic giant branch stars. The new rate implies lower $^{17}$O/$^{16}$O ratios, with important implications on the interpretation of astrophysical observables from these stars.

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arXiv2016

Experimental study of the astrophysical gamma-process reaction 124Xe(alpha,gamma)128Ba

The synthesis of heavy, proton rich isotopes in the astrophysical gamma-process proceeds through photodisintegration reactions. For the improved understanding of the process, the rates of the involved nuclear reactions must be known. The reaction 128Ba(g,a)124Xe was found to affect the abundance of the p nucleus 124Xe. Since the stellar rate for this reaction cannot be determined by a measurement directly, the aim of the present work was to measure the cross section of the inverse 124Xe(a,g)128Ba reaction and to compare the results with statistical model predictions. Of great importance is the fact that data below the (a,n) threshold was obtained. Studying simultaneously the 124Xe(a,n)127Ba reaction channel at higher energy allowed to further identify the source of a discrepancy between data and prediction. The 124Xe + alpha cross sections were measured with the activation method using a thin window 124Xe gas cell. The studied energy range was between E = 11 and 15 MeV close above the astrophysically relevant energy range. The obtained cross sections are compared with statistical model calculations. The experimental cross sections are smaller than standard predictions previously used in astrophysical calculations. As dominating source of the difference, the theoretical alpha width was identified. The experimental data suggest an alpha width lower by at least a factor of 0.125 in the astrophysical energy range. An upper limit for the 128Ba(g,a)124Xe stellar rate was inferred from our measurement. The impact of this rate was studied in two different models for core-collapse supernova explosions of 25 solar mass stars. A significant contribution to the 124Xe abundance via this reaction path would only be possible when the rate was increased above the previous standard value. Since the experimental data rule this out, they also demonstrate the closure of this production path.

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arXiv2015

Three new low-energy resonances in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle affects the synthesis of the elements between $^{20}$Ne and $^{27}$Al in asymptotic giant branch stars and novae. The $^{22}$Ne(p,$γ$)$^{23}$Na reaction rate is very uncertain because of a large number of unobserved resonances lying in the Gamow window. At proton energies below 400\,keV, only upper limits exist in the literature for the resonance strengths. Previous reaction rate evaluations differ by large factors. In the present work, the first direct observations of the $^{22}$Ne(p,$γ$)$^{23}$Na resonances at 156.2, 189.5, and 259.7\,keV are reported. Their resonance strengths have been derived with 2-7\% uncertainty. In addition, upper limits for three other resonances have been greatly reduced. Data were taken using a windowless $^{22}$Ne gas target and high-purity germanium detectors at the Laboratory for Underground Nuclear Astrophysics in the Gran Sasso laboratory of the National Institute for Nuclear Physics, Italy, taking advantage of the ultra-low background observed deep underground. The new reaction rate is a factor of 5 higher than the recent evaluation at temperatures relevant to novae and asymptotic giant branch stars nucleosynthesis.

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arXiv2015

Measurements of $^{152}$Gd(p,$γ$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reaction cross sections for the astrophysical $γ$ process

The total cross sections for the $^{152}$Gd(p,$γ$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reactions have been measured by the activation method at effective center-of-mass energies \mbox{$3.47 \leq E_\mathrm{c.m.}^\mathrm{eff}\leq 7.94$ MeV} and \mbox{$4.96 \leq E_\mathrm{c.m.}^\mathrm{eff} \leq 7.94$ MeV}, respectively. The targets were prepared by evaporation of 30.6\% isotopically enriched $^{152}$Gd oxide on aluminum backing foils, and bombarded with proton beams provided by a cyclotron accelerator. The cross sections were deduced from the observed $γ$-ray activity, which was detected off-line by a HPGe detector in a low background environment. The results are presented and compared with predictions of statistical model calculations. This comparison supports a modified optical proton+$^{152}$Gd potential suggested earlier.

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arXiv2015

The 106Cd(alpha,alpha)106Cd elastic scattering in a wide energy range for gamma-process studies

Alpha elastic scattering angular distributions of the 106Cd(alpha,alpha)106Cd reaction were measured at three energies around the Coulomb barrier to provide a sensitive test for the alpha + nucleus optical potential parameter sets. Furthermore, the new high precision angular distributions, together with the data available from the literature were used to study the energy dependence of the locally optimized α+nucleus optical potential in a wide energy region ranging from E_Lab = 27.0 MeV down to 16.1 MeV. The potentials under study are a basic prerequisite for the prediction of alpha-induced reaction cross sections and thus, for the calculation of stellar reaction rates used for the astrophysical gamma process. Therefore, statistical model predictions using as input the optical potentials discussed in the present work are compared to the available 106Cd + alpha cross section data.

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arXiv2015

Test of statistical model cross section calculations for $α$-induced reactions on $^{107}$Ag at energies of astrophysical interest

Astrophysical reaction rates, which are mostly derived from theoretical cross sections, are necessary input to nuclear reaction network simulations for studying the origin of $p$ nuclei. Past experiments have found a considerable difference between theoretical and experimental cross sections in some cases, especially for ($α$,$γ$) reactions at low energy. Therefore, it is important to experimentally test theoretical cross section predictions at low, astrophysically relevant energies. The aim is to measure reaction cross sections of $^{107}$Ag($α$,$γ$)$^{111}$In and $^{107}$Ag($α$,n)$^{110}$In at low energies in order to extend the experimental database for astrophysical reactions involving $α$ particles towards lower mass numbers. Reaction rate predictions are very sensitive to the optical model parameters and this introduces a large uncertainty into theoretical rates involving $α$ particles at low energy. We have also used Hauser-Feshbach statistical model calculations to study the origin of possible discrepancies between prediction and data. An activation technique has been used to measure the reaction cross sections at effective center of mass energies between 7.79 MeV and 12.50 MeV. Isomeric and ground state cross sections of the ($α$,n) reaction were determined separately. The measured cross sections were found to be lower than theoretical predictions for the ($α$,$γ$) reaction. Varying the calculated averaged widths in the Hauser-Feshbach model, it became evident that the data for the ($α$,$γ$) and ($α$,n) reactions can only be simultaneously reproduced when rescaling the ratio of $γ$- to neutron width and using an energy-dependent imaginary part in the optical $α$+$^{107}$Ag potential.......

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arXiv2014

A new study of the $^{22}$Ne(p,$γ$)$^{23}$Na reaction deep underground: Feasibility, setup, and first observation of the 186 keV resonance

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle is active in asymptotic giant branch stars as well as in novae and contributes to the nucleosythesis of neon and sodium isotopes. In order to reduce the uncertainties in the predicted nucleosynthesis yields, new experimental efforts to measure the $^{22}$Ne(p,$γ$)$^{23}$Na cross section directly at the astrophysically relevant energies are needed. In the present work, a feasibility study for a $^{22}$Ne(p,$γ$)$^{23}$Na experiment at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400\,kV accelerator deep underground in the Gran Sasso laboratory, Italy, is reported. The ion beam induced $γ$-ray background has been studied. The feasibility study led to the first observation of the $E_{\rm p}$ = 186\,keV resonance in a direct experiment. An experimental lower limit of 0.12\,$\times$\,10$^{-6}$\,eV has been obtained for the resonance strength. Informed by the feasibility study, a dedicated experimental setup for the $^{22}$Ne(p,$γ$)$^{23}$Na experiment has been developed. The new setup has been characterized by a study of the temperature and pressure profiles. The beam heating effect that reduces the effective neon gas density due to the heating by the incident proton beam has been studied using the resonance scan technique, and the size of this effect has been determined for a neon gas target.

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arXiv2014

Alpha induced reaction cross section measurements on 162Er for the astrophysical gamma process

The cross sections of the 162Er(a,g,)166Yb and 162Er(a,n)165Yb reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m. = 16.09 down to Ec.m. = 11.21 MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The 162Er(a,n)165Yb reaction was studied above the reaction threshold between Ec.m. = 12.19 and 16.09 MeV. The fact that the 162Er(a,g)166Yb cross sections were measured below the (a,n) threshold at first time in this mass region opens the opportunity to study directly the a-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted.

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arXiv2013

Cross section and reaction rate of 92Mo(p,gamma)93Tc determined from thick target yield measurements

For the better understanding of the astrophysical gamma-process the experimental determination of low energy proton- and alpha-capture cross sections on heavy isotopes is required. The existing data for the 92Mo(p,gamma)93Tc reaction are contradictory and strong fluctuation of the cross section is observed which cannot be explained by the statistical model. In this paper a new determination of the 92Mo(p,gamma)93Tc and 98Mo(p,gamma)99mTc cross sections based on thick target yield measurements are presented and the results are compared with existing data and model calculations. Reaction rates of 92Mo(p,gamma)93Tc at temperatures relevant for the gamma-process are derived directly from the measured thick target yields. The obtained rates are a factor of 2 lower than the ones used in astrophysical network calculations. It is argued that in the case of fluctuating cross sections the thick target yield measurement can be more suited for a reliable reaction rate determination.

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arXiv2013

$^{110,116}$Cd($α,α$)$^{110,116}$Cd elastic scattering and systematic investigation of elastic $α$ scattering cross sections along the $Z$ = 48 isotopic and $N$ = 62 isotonic chains

The elastic scattering cross sections for the reactions $^{110,116}$Cd($α,α$)$^{110,116}$Cd at energies above and below the Coulomb barrier are presented to provide a sensitive test for the alpha-nucleus optical potential parameter sets. Additional constraints for the optical potential are taken from the analysis of elastic scattering excitation functions at backward angles which are available in literature. Moreover, the variation of the elastic alpha scattering cross sections along the $Z = 48$ isotopic and $N = 62$ isotonic chain is investigated by the study of the ratios of the of $^{106,110,116}$Cd($α,α$)$^{106,110,116}$Cd scattering cross sections at E$_{c.m.} \approx$ 15.6 and 18.8 MeV and the ratio of the $^{110}$Cd($α,α$)$^{110}$Cd and $^{112}$Sn($α,α$)$^{112}$Sn reaction cross sections at E$_{c.m.} \approx$ 18.8 MeV, respectively. These ratios are sensitive probes for the alpha-nucleus optical potential parameterizations. The potentials under study are a basic prerequisite for the prediction of $α$-induced reaction cross sections, e.g.\ for the calculation of stellar reaction rates in the astrophysical $p$- or $γ$-process.

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arXiv2013

High precision $^{113}$In($α,α$)$^{113}$In elastic scattering at energies around the Coulomb barrier for the astrophysical $γ$ process

The $γ$ process in supernova explosions is thought to explain the origin of proton-rich isotopes between Se and Hg, the so-called $p$ nuclei. The majority of the reaction rates for $γ$ process reaction network studies has to be predicted in Hauser-Feshbach statistical model calculations using global optical potential parameterizations. While the nucleon+nucleus optical potential is fairly known, for the $α$+nucleus optical potential several different parameterizations exist and large deviations are found between the predictions calculated using different parameter sets. By the measurement of elastic $α$-scattering angular distributions at energies around the Coulomb barrier a comprehensive test for the different global $α$+nucleus optical potential parameter sets is provided. Between 20$^{\circ}$ and 175$^{\circ}$ complete elastic alpha scattering angular distributions were measured on the $^{113}$In \textit{p} nucleus with high precision at E$_{c.m.}$ = 15.59 and 18.82 MeV. The elastic scattering cross sections of the $^{113}$In($α$,$α$)$^{113}$In reaction were measured for the first time at energies close to the astrophysically relevant energy region. The high precision experimental data were used to evaluate the predictions of the recent global and regional $α$+nucleus optical potentials. Parameters for a local $α$+nucleus optical potential were derived from the measured angular distributions. Predictions for the reaction cross sections of $^{113}$In($α,γ$)$^{117}$Sb and $^{113}$In($α$,n)$^{116}$Sb at astrophysically relevant energies were given using the global and local optical potential parameterizations.

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arXiv2013

Activation measurement of the 3He(a,g)7Be reaction cross section at high energies

The astrophysically important 3He(a,g)7Be reaction was studied at high energies where the available experimental data are in contradiction. A thin window 3He gas cell was used and the cross section was measured with the activation method. The obtained cross sections at energies between Ec.m. = 1.5 and 2.5 MeV are compared with the available data and theoretical calculations. The present results support the validity of the high energy cross section energy dependence observed by recent experiments.

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arXiv2013

Neutron-induced background by an alpha-beam incident on a deuterium gas target and its implications for the study of the 2H(alpha,gamma)6Li reaction at LUNA

The production of the stable isotope Li-6 in standard Big Bang nucleosynthesis has recently attracted much interest. Recent observations in metal-poor stars suggest that a cosmological Li-6 plateau may exist. If true, this plateau would come in addition to the well-known Spite plateau of Li-7 abundances and would point to a predominantly primordial origin of Li-6, contrary to the results of standard Big Bang nucleosynthesis calculations. Therefore, the nuclear physics underlying Big Bang Li-6 production must be revisited. The main production channel for Li-6 in the Big Bang is the 2H(alpha,gamma)6Li reaction. The present work reports on neutron-induced effects in a high-purity germanium detector that were encountered in a new study of this reaction. In the experiment, an α-beam from the underground accelerator LUNA in Gran Sasso, Italy, and a windowless deuterium gas target are used. A low neutron flux is induced by energetic deuterons from elastic scattering and, subsequently, the 2H(d,n)3He reaction. Due to the ultra-low laboratory neutron background at LUNA, the effect of this weak flux of 2-3 MeV neutrons on well-shielded high-purity germanium detectors has been studied in detail. Data have been taken at 280 and 400 keV alpha-beam energy and for comparison also using an americium-beryllium neutron source.

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arXiv2012

Elastic alpha scattering experiments and the alpha-nucleus optical potential at low energies

High precision angular distribution data of ($α$,$α$) elastic scattering are presented for the nuclei $^{89}$Y, $^{92}$Mo, $^{106,110,116}$Cd, $^{112,124}$Sn, and $^{144}$Sm at energies around the Coulomb barrier. Such data with small experimental uncertainties over the full angular range (20-170 degrees) are the indispensable prerequisite for the extraction of local optical potentials and for the determination of the total reaction cross section $σ_{\rm{reac}}$. A systematic fitting procedure was applied to the presented experimental scattering data to obtain comprehensive local potential parameter sets which are composed of a real folding potential and an imaginary potential of Woods-Saxon surface type. The obtained potential parameters were used in turn to construct a new systematic $α$-nucleus potential with very few parameters. Although this new potential cannot reproduce the angular distributions with the same small deviations as the local potential, the new potential is able to predict the total reaction cross sections for all cases under study.

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arXiv2012

Impact of a revised $^{25}$Mg(p,$γ$)$^{26}$Al reaction rate on the operation of the Mg-Al cycle

Proton captures on Mg isotopes play an important role in the Mg-Al cycle active in stellar H-burning regions. In particular, low-energy nuclear resonances in the $^{25}$Mg(p,$γ$)$^{26}$Al reaction affect the production of radioactive $^{26}$Al$^{gs}$ as well as the resulting Mg/Al abundance ratio. Reliable estimations of these quantities require precise measurements of the strengths of low-energy resonances. Based on a new experimental study performed at LUNA, we provide revised rates of the $^{25}$Mg(p,$γ$)$^{26}$Al$^{gs}$ and the $^{25}$Mg(p,$γ$)$^{26}$Al$^{m}$ reactions with corresponding uncertainties. In the temperature range 50 to 150 MK, the new recommended rate of the $^{26}$Al$^{m}$ production is up to 5 times higher than previously assumed. In addition, at T$=100$ MK, the revised total reaction rate is a factor of 2 higher. Note that this is the range of temperature at which the Mg-Al cycle operates in an H-burning zone. The effects of this revision are discussed. Due to the significantly larger $^{25}$Mg(p,$γ$)$^{26}$Al$^{m}$ rate, the estimated production of $^{26}$Al$^{gs}$ in H-burning regions is less efficient than previously obtained. As a result, the new rates should imply a smaller contribution from Wolf-Rayet stars to the galactic $^{26}$Al budget. Similarly, we show that the AGB extra-mixing scenario does not appear able to explain the most extreme values of $^{26}$Al/$^{27}$Al, i.e. $>10^{-2}$, found in some O-rich presolar grains. Finally, the substantial increase of the total reaction rate makes the hypothesis of a self-pollution by massive AGBs a more robust explanation for the Mg-Al anticorrelation observed in Globular-Cluster stars.

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