arXiv subjects

E. Somorjai

Publications and source records attributed to E. Somorjai.

At least 37 records · Page 2Linked to original sources

arXiv2012

First Direct Measurement of the ^{17}O(p,γ)^{18}F Reaction Cross-Section at Gamow Energies for Classical Novae

Classical novae are important contributors to the abundances of key isotopes, such as the radioactive ^{18}F, whose observation by satellite missions could provide constraints on nucleosynthesis models in novae. The ^{17}O(p,γ)^{18}F reaction plays a critical role in the synthesis of both oxygen and fluorine isotopes but its reaction rate is not well determined because of the lack of experimental data at energies relevant to novae explosions. In this study, the reaction cross section has been measured directly for the first time in a wide energy range Ecm = 200 - 370 keV appropriate to hydrogen burning in classical novae. In addition, the E=183 keV resonance strength, ωγ=1.67\pm0.12 \mueV, has been measured with the highest precision to date. The uncertainty on the ^{17}O(p,γ)^{18}F reaction rate has been reduced by a factor of 4, thus leading to firmer constraints on accurate models of novae nucleosynthesis.

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arXiv2012

Preparation and characterisation of isotopically enriched Ta$_2$O$_5$ targets for nuclear astrophysics studies

The direct measurement of reaction cross sections at astrophysical energies often requires the use of solid targets of known thickness, isotopic composition, and stoichiometry that are able to withstand high beam currents for extended periods of time. Here, we report on the production and characterisation of isotopically enriched Ta$_2$O$_5$ targets for the study of proton-induced reactions at the Laboratory for Underground Nuclear Astrophysics facility of the Laboratori Nazionali del Gran Sasso. The targets were prepared by anodisation of tantalum backings in enriched water (up to 66% in $^{17}$O and up to 96% in $^{18}$O). Special care was devoted to minimising the presence of any contaminants that could induce unwanted background reactions with the beam in the energy region of astrophysical interest. Results from target characterisation measurements are reported, and the conclusions for proton capture measurements with these targets are drawn.

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arXiv2012

Relation between total cross sections from elastic scattering and alpha-induced reactions: the example of 64Zn

The total reaction cross section is related to the elastic scattering angular distribution by a basic quantum-mechanical relation. We present new experimental data for alpha-induced reaction cross sections on 64Zn which allow for the first time the experimental verification of this simple relation at low energies by comparison of the new experimental reaction data to the result obtained from 64Zn(alpha,alpha)64Zn elastic scattering.

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arXiv2012

Investigation of alpha-induced reactions on 127I for the astrophysical gamma process

(Shorten version of the PRC abstract) Alpha-induced reactions on 127I have been studied using the activation technique in order to provide cross section data for the modeling of the astrophysical gamma process. The relative intensity of the 536.1 keV gamma transition was measured precisely, its uncertainty was reduced from 13% to 4%. By measuring the yield of the characteristic X-rays, the cross sections of the 127I(alpha,gamma)131Cs reaction have been determined for the first time close to the astrophysically relevant energy region, at energies 9.50 < Ec.m. < 15.15$ MeV. The 127I(alpha,n)130Cs reaction was studied in the range 9.62 < Ec.m. < 15.15 MeV by measuring the yield of the 536.1 keV gamma-ray and at the lower part of this energy range by counting the characteristic X-rays. A comparison of the resulting cross sections to predictions of statistical model calculations confirmed the predictions of the astrophysically relevant averaged alpha width. Nevertheless, the newly derived stellar reaction rates at gamma process temperatures for 127I(alpha,gamma)131$Cs and its reverse reaction are factors 4-10 faster than previous calculations, due to improvements in the reaction model.

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arXiv2012

Astrophysical analysis of the measurement of (alpha,gamma) and (alpha,n) cross sections of 169Tm

Reaction cross sections of 169Tm(alpha,gamma)173Lu and 169Tm(alpha,n)172Lu have been measured in the energy range 12.6<=E_alpha<=17.5 MeV and 11.5<=E_alpha<=17.5 MeV, respectively, using the recently introduced method of combining activation with X-ray counting. Improved shielding allowed to measure the (alpha,gamma) to lower energy than previously possible. The combination of (alpha,gamma) and (alpha,n) data made it possible to study the energy dependence of the alpha width. While absolute value and energy dependence are perfectly reproduced by theory at energies above 14 MeV, the observed change in energy dependence at energies below 14 MeV requires a modification of the predicted alpha width. Using an effective, energy-dependent, local optical alpha+nucleus potential it is possible to reproduce the data but the astrophysical rate is still not well constrained at gamma-process temperatures. The additional uncertainty stemming from a possible modification of the compound formation cross section is discussed. Including the remaining uncertainties, the recommended range of astrophysical reaction rate values at 2 GK is higher than the previously used values by factors of 2-37.

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arXiv2012

Investigation of alpha-induced reactions on 130Ba and 132Ba and their importance for the synthesis of heavy p nuclei

Captures of alpha particles on the proton-richest Barium isotope, 130Ba, have been studied in order to provide cross section data for the modeling of the astrophysical gamma process. The cross sections of the 130Ba(alpha,gamma)134Ce and 130Ba(alpha,n)133Ce reactions have been measured with the activation technique in the center-of mass energy range between 11.6 and 16 MeV, close above the astrophysically relevant energies. As a side result, the cross section of the 132Ba(alpha,n)135Ce reaction has also been measured. The results are compared with the prediction of statistical model calculations, using different input parameters such as alpha+nucleus optical potentials. It is found that the (alpha,n) data can be reproduced employing the standard alpha+nucleus optical potential widely used in astrophysical applications. Assuming its validity also in the astrophysically relevant energy window, we present new stellar reaction rates for 130Ba(alpha,gamma)134Ce and 132Ba(alpha,gamma)136Ce and their inverse reactions calculated with the SMARAGD statistical model code. The highly increased 136Ce(gamma,alpha)132Ba rate implies that the p nucleus 130Ba cannot directly receive contributions from the Ce isotopic chain. Further measurements are required to better constrain this result.

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arXiv2011

The 25Mg(p,g)Al reaction at low astrophysical energies

In the present work we report on a new measurement of resonance strengths in the reaction 25Mg(p,gamma)26Al at E_cm= 92 and 189 keV. This study was performed at the LUNA facility in the Gran Sasso underground laboratory using a 4pi BGO summing crystal. For the first time the 92 keV resonance was directly observed and a resonance strength omega-gamma=(2.9+/-0.6)x10E-10 eV was determined. Additionally, the gamma-ray branchings and strength of the 189 keV resonance were studied with a high resolution HPGe detector yielding an omega-gamma value in agreement with the BGO measurement, but 20% larger compared to previous works.

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arXiv2011

Experimental study of alpha-induced reactions on 64Zn for the astrophysical gamma-process

For the synthesis of the heavy, proton rich isotopes in the astrophysical gamma-process the precise knowledge of alpha-induced cross sections is of high importance. We have initiated a comprehensive study of the 64Zn+alpha system involving the cross section measurement of different reaction channels as well as the elastic scattering at low, astrophysically relevant energies. In this paper the experimental technique and some preliminary results of the 64Zn(alpha,p)67Ga cross section measurement are presented.

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arXiv2011

Revision of the 15N(p,γ)16O reaction rate and oxygen abundance in H-burning zones

The NO cycle takes place in the deepest layer of a H-burning core or shell, when the temperature exceeds T {\simeq} 30 {\cdot} 106 K. The O depletion observed in some globular cluster giant stars, always associated with a Na enhancement, may be due to either a deep mixing during the RGB (red giant branch) phase of the star or to the pollution of the primordial gas by an early population of massive AGB (asymptotic giant branch) stars, whose chemical composition was modified by the hot bottom burning. In both cases, the NO cycle is responsible for the O depletion. The activation of this cycle depends on the rate of the 15N(p,γ)16O reaction. A precise evaluation of this reaction rate at temperatures as low as experienced in H-burning zones in stellar interiors is mandatory to understand the observed O abundances. We present a new measurement of the 15N(p,γ)16O reaction performed at LUNA covering for the first time the center of mass energy range 70-370 keV, which corresponds to stellar temperatures between 65 {\cdot} 106 K and 780 {\cdot}106 K. This range includes the 15N(p,γ)16O Gamow-peak energy of explosive H-burning taking place in the external layer of a nova and the one of the hot bottom burning (HBB) nucleosynthesis occurring in massive AGB stars. With the present data, we are also able to confirm the result of the previous R-matrix extrapolation. In particular, in the temperature range of astrophysical interest, the new rate is about a factor of 2 smaller than reported in the widely adopted compilation of reaction rates (NACRE or CF88) and the uncertainty is now reduced down to the 10% level.

astro-ph.SR↗

arXiv2011

The 14N(p,gamma)15O reaction studied with a composite germanium detector

The rate of the carbon-nitrogen-oxygen (CNO) cycle of hydrogen burning is controlled by the 14N(p,gamma)15O reaction. The reaction proceeds by capture to the ground states and several excited states in O-15. In order to obtain a reliable extrapolation of the excitation curve to astrophysical energy, fits in the R-matrix framework are needed. In an energy range that sensitively tests such fits, new cross section data are reported here for the four major transitions in the 14N(p,gamma)15O reaction. The experiment has been performed at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400 kV accelerator placed deep underground in the Gran Sasso facility in Italy. Using a composite germanium detector, summing corrections have been considerably reduced with respect to previous studies. The cross sections for capture to the ground state and to the 5181, 6172, and 6792 keV excited states in O-15 have been determined at 359, 380, and 399 keV beam energy. In addition, the branching ratios for the decay of the 278 keV resonance have been remeasured.

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arXiv2011

Target characterization for the 130Ba(alpha,gamma)134Ce gamma-process experiment

In order to extend the available experimental database for the astrophysical gamma-process, the cross section measurement of the 130Ba(alpha,gamma)134Ce and 130Ba(alpha,n)133Ce reactions is in progress. The measurements are carried out using thin layers of evaporated BaCO3 as target. Since the target thickness enters directly into the calculation of the cross sections, the reliability of its determination is of crucial importance. Three different methods have been used to determine the target thickness. Details of these experiments and the obtained results are presented.

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arXiv2010

High precision $^{89}$Y($α$,$α$)$^{89}$Y scattering at low energies

Elastic scattering cross sections of the $^{89}$Y($α$,$α$)$^{89}$Y reaction have been measured at energies E$_{c.m.}$ = 15.51 and 18.63 MeV. The high precision data for the semi-magic $N = 50$ nucleus $^{89}$Y are used to derive a local potential and to evaluate the predictions of global and regional $α$-nucleus potentials. The variation of the elastic alpha scattering cross sections along the $N = 50$ isotonic chain is investigated by a study of the ratios of angular distributions for $^{89}$Y($α$,$α$)$^{89}$Y and $^{92}$Mo($α$,$α$)$^{92}$Mo at E$_{c.m.} \approx$ 15.51 and 18.63 MeV. This ratio is a very sensitive probe at energies close to the Coulomb barrier, where scattering data alone is usually not enough to characterize the different potentials. Furthermore, $α$-cluster states in $^{93}$Nb = $^{89}$Y $\otimes$ $α$ are investigated.

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arXiv2010

Determining reaction cross sections via characteristic X-ray detection: α-induced reactions on 169Tm for the astrophysical γ -process

The cross sections of the 169Tm(α, γ)173Lu and 169Tm(α,n)172Lu reactions have been measured first time using a new method, by detecting the characteristic X-ray radiation following the electron capturedecay of 172,173Lu. Despite the relatively long half-life of the reaction products (T1/2 = 500 and 6.7 days, respectively) it was possible to measure the cross section of the 169Tm(α,γ)173Lu reaction close to the Gamow window (T9 = 3.5 GK), between Ec.m. = 13.16 and 17.08 MeV. The 169Tm(α,n)172Lu reaction cross section was measured from Ec.m. = 11.21 MeV up to Ec.m. = 17.08 MeV. The experimental results have been compared to theoretical predictions

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arXiv2010

Constraining the S factor of 15N(p,g)16O at Astrophysical Energies

The 15N(p,g)16O reaction represents a break out reaction linking the first and second cycle of the CNO cycles redistributing the carbon and nitrogen abundances into the oxygen range. The reaction is dominated by two broad resonances at Ep = 338 keV and 1028 keV and a Direct Capture contribution to the ground state of 16O. Interference effects between these contributions in both the low energy region (Ep < 338 keV) and in between the two resonances (338 <Ep < 1028 keV) can dramatically effect the extrapolation to energies of astrophysical interest. To facilitate a reliable extrapolation the 15N(p,g)16O reaction has been remeasured covering the energy range from Ep=1800 keV down to 130 keV. The results have been analyzed in the framework of a multi-level R-matrix theory and a S(0) value of 39.6 keV b has been found.

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arXiv2010

Total reaction cross sections from elastic alpha-nucleus scattering angular distributions around the Coulomb barrier

The total reaction cross section $σ_{\rm{reac}}$ is a valuable measure for the prediction of $α$-induced reaction cross sections within the statistical model and for the comparison of scattering of tightly bound projectiles to weakly bound and exotic projectiles. Here we provide the total reaction cross sections $σ_{\rm{reac}}$ derived from our previously published angular distributions of $α$-elastic scattering on $^{89}$Y, $^{92}$Mo, $^{112,124}$Sn, and $^{144}$Sm at energies around the Coulomb barrier.

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arXiv2010

Alpha-induced reaction cross section measurements on 151Eu for the astrophysical gamma-process

In order to extend the experimental database relevant for the astrophysical gamma-process towards the unexplored heavier mass region, the cross sections of the 151Eu(alpha,gamma)155Tb and 151Eu(alpha,n)154Tb reactions have been measured at low energies between 12 and 17 MeV using the activation technique. The results are compared with the predictions of statistical model calculations and it is found that the calculations overestimate the cross sections by about a factor of two. A sensitivity analysis shows that this discrepancy is caused by the inadequate description of the alpha+nucleus channel. A factor of two reduction of the reaction rate of 151Eu(alpha,gamma)155Tb in gamma-process network calculations with respect to theoretical rates using the optical potential by McFadden and Satchler (1966) is recommended.

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arXiv2010

New experimental study of low-energy (p,gamma) resonances in magnesium isotopes

Proton captures on Mg isotopes play an important role in the Mg-Al cycle active in stellar H shell burning. In particular, the strengths of low-energy resonances with E < 200 keV in 25Mg(p,gamma)26Al determine the production of 26Al and a precise knowledge of these nuclear data is highly desirable. Absolute measurements at such low-energies are often very difficult and hampered by gamma-ray background as well as changing target stoichiometry during the measurements. The latter problem can be partly avoided using higher energy resonances of the same reaction as a normalization reference. Hence the parameters of suitable resonances have to be studied with adequate precision. In the present work we report on new measurements of the resonance strengths omega_gamma of the E = 214, 304, and 326 keV resonances in the reactions 24Mg(p,gamma)25Al, 25Mg(p,gamma)26Al, and 26Mg(p,gamma)27Al, respectively. These studies were performed at the LUNA facility in the Gran Sasso underground laboratory using multiple experimental techniques and provided results with a higher accuracy than previously achieved.

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arXiv2010

An actively vetoed Clover gamma-detector for nuclear astrophysics at LUNA

An escape-suppressed, composite high-purity germanium detector of the Clover type has been installed at the Laboratory for Underground Nuclear Astrophysics (LUNA) facility, deep underground in the Gran Sasso Laboratory, Italy. The laboratory gamma-ray background of the Clover detector has been studied underground at LUNA and, for comparison, also in an overground laboratory. Spectra have been recorded both for the single segments and for the virtual detector formed by online addition of all four segments. The effect of the escape-suppression shield has been studied as well. Despite their generally higher intrinsic background, escape-suppressed detectors are found to be well suited for underground nuclear astrophysics studies. As an example for the advantage of using a composite detector deep underground, the weak ground state branching of the Ep = 223 keV resonance in the 24Mg(p,gamma)25Al reaction is determined with improved precision.

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