arXiv subjects

Emmanuel Flurin

Publications and source records attributed to Emmanuel Flurin.

At least 19 recordsLinked to original sources

arXiv2026

Superconducting Parallel-Plate Resonators for the Detection of Single Electron Spins

We introduce a multilayer superconducting microwave resonator with sub-Ohm impedance optimized for high coupling strength to single electron spins. The design minimizes the magnetic far-field and therefore achieves a Purcell factor $F_P > 10^{15}$. We show several ways to fabricate this type of resonator and present resonators with an intrinsic $Q$-factor exceeding $2 \cdot 10^4$ at the single-photon level. We further characterize these resonators in magnetic fields up to $500 \, \text{mT}$. Finally, we evaluate the impact of the achievable Purcell factor on single-spin detection through photon counting and dispersive readout.

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arXiv2025

Probing the quantum motion of a macroscopic mechanical oscillator with a radio-frequency superconducting qubit

Long-lived mechanical resonators like drums oscillating at MHz frequencies and operating in the quantum regime are a powerful platform for quantum technologies and tests of fundamental physics. Yet, quantum control of such systems remains challenging, owing to their low energy scale and the difficulty of achieving efficient coupling to other well-controlled quantum devices. Here, we demonstrate repeated coherent interactions between a 4 MHz suspended silicon nitride membrane and a resonant superconducting heavy-fluxonium qubit. The qubit is initialized at an effective temperature of $21~\mathrm{\mu K}$ and read out with 77% single-shot fidelity. During the $6~\mathrm{ms}$ lifetime of the membrane the two systems swap excitations more than 300 times. After each interaction, a state-selective qubit detection is performed, implementing a stroboscopic series of weak measurements that provide information about the mechanical state. The accumulated records reconstruct the position noise spectrum of the membrane, revealing both its thermal occupation $n_\mathrm{th}\approx47$ at $10~\mathrm{mK}$ and the qubit-induced back-action. By preparing the qubit either in its ground or excited state before each interaction, we observe an imbalance between the emission and absorption spectra, proportional to $n_\mathrm{th}$ and $n_\mathrm{th}+1$, respectively-a hallmark of the non-commutation of phonon creation and annihilation operators. Since the predicted Di\'osi-Penrose gravitational collapse time is comparable to the measured mechanical decoherence time, our architecture enters a regime where gravity-induced decoherence could be tested directly.

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arXiv2025

Hyperinductance based on stacked Josephson junctions

Superinductances are superconducting circuit elements that combine a large inductance with a low parasitic capacitance to ground, resulting in a characteristic impedance exceeding the resistance quantum $R_Q = h/(2e)^2 \simeq 6.45 \mathrm{k}\Omega$. In recent years, these components have become key enablers for emerging quantum circuit architectures. However, achieving high characteristic impedance while maintaining scalability and fabrication robustness remains a major challenge. In this work, we present two fabrication techniques for realizing superinductances based on vertically stacked Josephson junctions. Using a multi-angle Manhattan (MAM) process and a zero-angle (ZA) evaporation technique -- in which junction stacks are connected pairwise using airbridges -- we fabricate one-dimensional chains of stacks that act as high-impedance superconducting transmission lines. Two-tone microwave spectroscopy reveals the expected $\sqrt{n}$ scaling of the impedance with the number of junctions per stack. The chain fabricated using the ZA process, with nine junctions per stack, achieves a characteristic impedance of $\sim 16 \mathrm{k}\Omega$, a total inductance of $5.9 \mathrm{\mu H}$, and a maximum frequency-dependent impedance of $50 \mathrm{k}\Omega$ at 1.4 GHz. Our results establish junction stacking as a scalable, robust, and flexible platform for next-generation quantum circuits requiring ultra-high impedance environments.

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arXiv2025

Noise Mitigation in Single Microwave Photon Counting by Cascaded Quantum Measurements

While single-photon counting is routinely achieved in the optical domain, operational single microwave photon detectors (SMPDs) have only recently been demonstrated. SMPDs are critical for sensing weak signals from incoherent emitters, with applications ranging from the detection of individual electron spins and dark-matter candidates to advancements in hybrid quantum devices and superconducting quantum computing. These detectors offer a substantial advantage over quantum-limited amplification schemes by bypassing the standard quantum limit for power detection, therefore further reductions in their intrinsic noise are essential for advancing quantum sensing at microwave frequencies. Several SMPD designs utilize the state of a superconducting qubit to encode the detection of an itinerant photon, and rely on a non-destructive photon-qubit interaction. Here, we leverage this Quantum-Non-Demolition feature by repeatedly measuring the impinging photon with cascaded Four-Wave-Mixing processes and encoding the detection on several qubits. This cascaded detector mitigates the intrinsic local noise of individual qubits, achieving a two-order-of-magnitude reduction in intrinsic detector noise at the cost of halving the efficiency. We report an intrinsic sensitivity of $8(1)\times10^{-24}\text{W}/\sqrt{\text{Hz}}$, with an operational sensitivity of $5.9(6)\times 10^{-23}\text{W}/\sqrt{\text{Hz}}$ limited by thermal photons in the input line.

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arXiv2025

Enhancing the sensitivity of single microwave photon detection with bandwidth tunability

We report on the characteristics of a microwave photon counter device based on a superconducting transmon qubit. Its design is similar to [arXiv:2307.03614], with an additional bandwidth tuning circuit that allows optimizing the device efficiency and noise. Owing to this new feature and to improvements in device fabrication, a power sensitivity of $3 \cdot 10^{-23} \mathrm{W}/\sqrt{\mathrm{Hz}}$ is reached. We confirm the high performance of the device by measuring single spin microwave fluorescence.

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arXiv2024

Incoherent Measurement of Sub-10 kHz Optical Linewidths

Quantum state lifetimes $T_2$, or equivalently homogeneous linewidths $\Gamma_h = 1/\pi T_2$, are a key parameter for understanding decoherence processes in quantum systems and assessing their potential for applications in quantum technologies. The most common tool for measuring narrow optical homogeneous linewidths, i.e. long $T_2$, is the measurement of coherent photon echo emissions, which however gives very weak signal when the number of emitters is small. This strongly hampers the development of nano-materials, such as those based on rare earth ions, for quantum communication and processing. In this work we propose, and demonstrate in an erbium doped crystal, a measurement of photon echoes based on incoherent fluorescence detection and its variance analysis. It gives access to $T_2$ through a much larger signal than direct photon echo detection, and, importantly, without the need for a highly coherent laser. Our results thus open the way to efficiently assess the properties of a broad range of emitters and materials for applications in quantum nano-photonics.

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arXiv2024

Individual solid-state nuclear spin qubits with coherence exceeding seconds

The ability to coherently control and read out qubits with long coherence times in a scalable system is a crucial requirement for any quantum processor. Nuclear spins in the solid state have shown great promise as long-lived qubits. Control and readout of individual nuclear spin qubit registers has made major progress in the recent years using individual electron spin ancilla addressed either electrically or optically. Here, we present a new platform for quantum information processing, consisting of $^{183}$W nuclear spin qubits adjacent to an Er$^{3+}$ impurity in a CaWO$_4$ crystal, interfaced via a superconducting resonator and detected using a microwave photon counter at 10mK. We study two nuclear spin qubits with $T_2^*$ of $0.8(2)~$s and $1.2(3)~$s, $T_2$ of $3.4(4)~$s and $4.4(6)~$ s, respectively. We demonstrate single-shot quantum non-demolition readout of each nuclear spin qubit using the Er$^{3+}$ spin as an ancilla. We introduce a new scheme for all-microwave single- and two-qubit gates, based on stimulated Raman driving of the coupled electron-nuclear spin system. We realize single- and two-qubit gates on a timescale of a few milliseconds, and prepare a decoherence-protected Bell state with 88% fidelity and $T_2^*$ of $1.7(2)~$s. Our results are a proof-of-principle demonstrating the potential of solid-state nuclear spin qubits as a promising platform for quantum information processing. With the potential to scale to tens or hundreds of qubits, this platform has prospects for the development of scalable quantum processors with long-lived qubits.

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arXiv2024

Month-long-lifetime microwave spectral holes in an erbium-doped scheelite crystal at millikelvin temperature

Rare-earth-ion (REI) ensembles in crystals have remarkable optical and spin properties characterized by narrow homogeneous linewidths relative to the inhomogeneous ensemble broadening. This makes it possible to precisely tailor the ensemble spectral density and therefore the absorption profile by applying narrow-linewidth radiation to transfer population into auxiliary levels, a process broadly known as spectral hole burning (SHB). REI-doped crystals find applications in information processing, both classical (pattern recognition, filtering, spectral analysis) and quantum (photon storage), all protocols requiring suitable ensemble preparation by SHB as a first step. In Er$^{3+}$-doped materials, the longest reported hole lifetime is one minute, and longer lifetimes are desirable. Here, we report SHB and accumulated echo measurements in a scheelite crystal of CaWO$_4$ by pumping the electron spin transition of Er$^{3+}$ ions at microwave frequencies and millikelvin temperatures, with nuclear spin states of neighboring $^{183}$W atoms serving as the auxiliary levels. The lifetime of the holes and accumulated echoes rises steeply as the sample temperature is decreased, exceeding a month at 10 mK. Our results demonstrate that millikelvin temperatures can be beneficial for signal processing applications requiring long spectral hole lifetimes.

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arXiv2024

Opto-RF transduction in Er$^{3+}$:CaWO$_4$

We use an erbium doped CaWO$_4$ crystal as a resonant transducer between the RF and optical domains at 12 GHz and 1532 nm respectively. We employ a RF resonator to enhance the spin coupling but keep a single-pass (non-resonant) optical setup. The overall efficiency is low but we carefully characterize the transduction process and show that the performance can be described by two different metrics that we define and distinguish: the electro-optics and the quantum efficiencies. We reach an electro-optics efficiency of -84 dB for 15.7 dBm RF power. The corresponding quantum efficiency is -142 dB for 0.4 dBm optical power. We develop the Schrödinger-Maxwell formalism, well-known to describe light-matter interactions in atomic systems, in order to model the conversion process. We explicitly make the connection with the cavity quantum electrodynamics (cavity QED) approach that are generally used to describe quantum transduction.

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arXiv2024

Cyclically operated Single Microwave Photon Counter with $10^\mathrm{-22}$ $\mathrm{W/\sqrt{Hz}}$ sensitivity

Single photon detection played an important role in the development of quantum optics. Its implementation in the microwave domain is challenging because the photon energy is 5 orders of magnitude smaller. In recent years, significant progress has been made in developing single microwave photon detectors (SMPDs) based on superconducting quantum bits or bolometers. In this paper we present a practical SMPD based on the irreversible transfer of an incoming photon to the excited state of a transmon qubit by a four-wave mixing process. This device achieves a detection efficiency $η= 0.43$ and an operational dark count rate $α= 85$ $\mathrm{s^{-1}}$, mainly due to the out-of-equilibrium microwave photons in the input line. The corresponding power sensitivity is $\mathcal{S} = 10^{-22}$ $\mathrm{W/\sqrt{Hz}}$, one order of magnitude lower than the state of the art. The detector operates continuously over hour timescales with a duty cycle $η_\mathrm{D}=0.84$, and offers frequency tunability of at least 50 MHz around 7 GHz.

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arXiv2023

Single electron-spin-resonance detection by microwave photon counting

Electron spin resonance (ESR) spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing, but it gives access only to ensemble-averaged quantities due to its limited signal-to-noise ratio. Single-electron-spin sensitivity has however been reached using spin-dependent photoluminescence, transport measurements, and scanning-probe techniques. These methods are system-specific or sensitive only in a small detection volume, so that practical single spin detection remains an open challenge. Here, we demonstrate single electron magnetic resonance by spin fluorescence detection, using a microwave photon counter at cryogenic temperatures. We detect individual paramagnetic erbium ions in a scheelite crystal coupled to a high-quality factor planar superconducting resonator to enhance their radiative decay rate, with a signal-to-noise ratio of 1.9 in one second integration time. The fluorescence signal shows anti-bunching, proving that it comes from individual emitters. Coherence times up to 3 ms are measured, limited by the spin radiative lifetime. The method has the potential to apply to arbitrary paramagnetic species with long enough non-radiative relaxation time, and allows single-spin detection in a volume as large as the resonator magnetic mode volume ( 10 um^3 in the present experiment), orders of magnitude larger than other single-spin detection techniques. As such, it may find applications in magnetic resonance and quantum computing.

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arXiv2023

A Multi-Qubit Quantum Gate Using the Zeno Effect

The Zeno effect, in which repeated observation freezes the dynamics of a quantum system, stands as an iconic oddity of quantum mechanics. When a measurement is unable to distinguish between states in a subspace, the dynamics within that subspace can be profoundly altered, leading to non-trivial behavior. Here we show that such a measurement can turn a non-interacting system with only single-qubit control into a two- or multi-qubit entangling gate, which we call a Zeno gate. The gate works by imparting a geometric phase on the system, conditioned on it lying within a particular nonlocal subspace. We derive simple closed-form expressions for the gate fidelity under a number of non-idealities and show that the gate is viable for implementation in circuit and cavity QED systems. More specifically, we illustrate the functioning of the gate via dispersive readout in both the Markovian and non-Markovian readout regimes, and derive conditions for longitudinal readout to ideally realize the gate.

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arXiv2022

Microwave fluorescence detection of spin echoes

Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance (EPR) spectroscopy, enabled by the development of operational Single Microwave Photon Detectors (SMPD) at millikelvin temperature. Here, we report the detection of spin echoes in the spin fluorescence signal. The echo manifests itself as a coherent modulation of the number of photons spontaneously emitted after a $π/2_X - τ- π_Y - τ- π/2_Φ$ sequence, dependent on the relative phase $Φ$. We demonstrate experimentally this detection method using an ensemble of $\mathrm{Er}^{3+}$ ion spins in a scheelite crystal of $\mathrm{CaWO}_4$. We use fluorescence-detected echoes to measure the erbium spin coherence time, as well as the echo envelope modulation due to the coupling to the $^{183}\mathrm{W}$ nuclear spins surrounding each ion. We finally compare the signal-to-noise ratio of inductively-detected and fluorescence-detected echoes, and show that it is larger with the fluorescence method.

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arXiv2022

Electron-spin spectral diffusion in an erbium doped crystal at millikelvin temperatures

Erbium-doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically-sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for many quantum applications, however, strong magnetic interactions of the electron-spin bath lead to excess spectral diffusion and rapid decoherence. Here we lithographically fabricate a 4.4 GHz superconducting planar micro-resonator on a $\text{CaWO}_{4}$ crystal doped with Er ions at a concentration of twenty parts per million relative to Ca. Using the microwave resonator, we characterize the spectral diffusion processes that limit the electron-spin coherence of Er ions at millikelvin temperatures by applying 2- and 3-pulse echo sequences. The coherence time shows a strong temperature dependence, reaching 1.3 ms at 23 mK for an electron-spin transition of $^{167}\text{Er}$.

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arXiv2021

Experimental demonstration of continuous quantum error correction

The storage and processing of quantum information are susceptible to external noise, resulting in computational errors that are inherently continuous A powerful method to suppress these effects is to use quantum error correction. Typically, quantum error correction is executed in discrete rounds where errors are digitized and detected by projective multi-qubit parity measurements. These stabilizer measurements are traditionally realized with entangling gates and projective measurement on ancillary qubits to complete a round of error correction. However, their gate structure makes them vulnerable to errors occurring at specific times in the code and errors on the ancilla qubits. Here we use direct parity measurements to implement a continuous quantum bit-flip correction code in a resource-efficient manner, eliminating entangling gates, ancilla qubits, and their associated errors. The continuous measurements are monitored by an FPGA controller that actively corrects errors as they are detected. Using this method, we achieve an average bit-flip detection efficiency of up to 91%. Furthermore, we use the protocol to increase the relaxation time of the protected logical qubit by a factor of 2.7 over the relaxation times of the bare comprising qubits. Our results showcase resource-efficient stabilizer measurements in a multi-qubit architecture and demonstrate how continuous error correction codes can address challenges in realizing a fault-tolerant system.

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arXiv2021

Twenty-three millisecond electron spin coherence of erbium ions in a natural-abundance crystal

Erbium ions doped into crystals have unique properties for quantum information processing, because of their optical transition at 1.5 $μ$m and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most applications of erbium require however long electron spin coherence times, and this has so far been missing. Here, by selecting a host matrix with a low nuclear-spin density (CaWO$_4$) and by quenching the spectral diffusion due to residual paramagnetic impurities at millikelvin temperatures, we obtain an Er$^{3+}$ electron spin coherence time of 23 ms. This is the longest electron spin coherence time measured in a material with a natural abundance of nuclear spins and on a magnetically-sensitive transition. Our results establish Er$^{3+}$:CaWO$_4$ as a leading platform for quantum networks.

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arXiv2021

Detecting spins with a microwave photon counter

Quantum emitters respond to resonant illumination by radiating electromagnetic fields. A component of these fields is phase-coherent with the driving tone, while another one is incoherent, consisting of spontaneously emitted photons and forming the fluorescence signal. Atoms and molecules are routinely detected by their fluorescence at optical frequencies, with important applications in quantum technology and microscopy. Spins, on the other hand, are usually detected by {their coherent response} at radio- or microwave frequencies, either in continuous-wave or pulsed magnetic resonance. Indeed, fluorescence detection of spins is hampered {by their low spontaneous emission rate} and by the lack of single-photon detectors in this frequency range. Here, using superconducting quantum devices, we demonstrate the detection of a small ensemble of donor spins in silicon by their fluorescence at microwave frequency and millikelvin temperatures. We enhance the spin radiative decay rate by coupling them to a high-quality-factor and small-mode-volume superconducting resonator, and we connect the device output to a newly-developed microwave single-photon counter based on a superconducting qubit. We discuss the potential of fluorescence detection as a novel method for magnetic resonance spectroscopy of small numbers of spins.

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arXiv2019

Probing a two-level system bath via the frequency shift of an off-resonantly-driven cavity

Although the main loss channel of planar microwave superconducting resonators has been identified to be related to an external coupling to a two-level system (TLS) bath, the behavior of such a cavity in the presence of an off-resonant pump has yet to be fully understood. Here a semi-classical model that predicts a power-dependent frequency shift besides the well-known TLS-induced damping is derived. The model is validated experimentally by performing a two-tone spectroscopy of several resonators fabricated on various substrates. Together with the provided analytic formulas, the technique proposed here is a simple, yet powerful, tool to characterize various properties of the TLS bath, such as their average dephasing rate.

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