arXiv · 2208.13586
Microwave fluorescence detection of spin echoes
Abstract
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance (EPR) spectroscopy, enabled by the development of operational Single Microwave Photon Detectors (SMPD) at millikelvin temperature. Here, we report the detection of spin echoes in the spin fluorescence signal. The echo manifests itself as a coherent modulation of the number of photons spontaneously emitted after a $\pi/2_X - \tau - \pi_Y - \tau - \pi/2_\Phi $ sequence, dependent on the relative phase $\Phi$. We demonstrate experimentally this detection method using an ensemble of $\mathrm{Er}^{3+}$ ion spins in a scheelite crystal of $\mathrm{CaWO}_4$. We use fluorescence-detected echoes to measure the erbium spin coherence time, as well as the echo envelope modulation due to the coupling to the $^{183}\mathrm{W}$ nuclear spins surrounding each ion. We finally compare the signal-to-noise ratio of inductively-detected and fluorescence-detected echoes, and show that it is larger with the fluorescence method.
Explore related subjects
Keep this discovery
Eric Billaud, Leo Balembois, Marianne Le Dantec, Milos Rančić, Emanuele Albertinale, Sylvain Bertaina, Thierry Chanelière, Philippe Goldner, Daniel Estève, Denis Vion, Patrice Bertet, Emmanuel Flurin. 2022-08-29. Microwave fluorescence detection of spin echoes. https://arxiv.org/abs/2208.13586
Cite the original work for its findings. Save a collection to share your selection of sources.