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Ephraim Spindler

Publications and source records attributed to Ephraim Spindler.

7 recordsLinked to original sources

Methods for traceable scanning magnetometry using single nitrogen vacancy centers in diamond: determining orientation, distance and localization

Individual, scannable nitrogen vacancy (NV) centers in single crystal diamond nanostructures enable nanoscale, quantitative imaging of magnetic stray fields. Nevertheless, important parameters like distance between the NV center and the sample and the orientation of the NV high symmetry axis are often not known precisely and enter data evaluation as free fitting parameters. We here use scanning NV imaging on micro-patterned, perpendicularly magnetized stripes and discs. From these measurements, we directly infer NV - sample distance d_NV and the NV's azimuthal orientation without the need for an external vector magnet control. We determine d_NV = 31.5 nm, while we infer the azimuthal orientation with a precision of 3{\deg}. We additionally employ commercially available silicon needles to image the apex topography of our diamond nanostructures to detect surface contamination. Simultaneously, monitoring NV fluorescence as a function of the needle's position allows us to estimate the lateral placement of the NV inside the diamond nanostructure.

cond-mat.mes-hall

Phase-dependent parametric amplification of propagating spin waves in YIG nanostructures enabled by local inhomogeneities

As magnonics evolves towards non-conventional computing, the development of phase-conserving and phase-sensitive amplification mechanisms becomes increasingly important. A particularly promising approach is non-adiabatic parametric amplification. In this work, the influence of local inhomogeneities on the parallel parametric amplification of spin waves in nano-scale Yttrium Iron Garnet waveguides is investigated. Micromagnetic simulations reveal that in larger pump regions, where only adiabatic amplification is expected, scattering centers provide additional linear momentum that enables non-adiabatic amplification of propagating spin waves. Importantly, the coherence of the process remains unaffected by the scattering and the generation of co-propagating spin waves enhance the effective amplification. Our simulations are confirmed by micro-focused Brillouin light scattering spectroscopy experiments, reproducing both the phase-dependent behavior and the characteristic features of the time-resolved dynamics. These findings demonstrate the flexibility of the parametric amplification process and provide a key mechanism for the development of large-scale spin-wave computing circuits.

cond-mat.other

Nonlinear frequency shift and bistability of magnon-polarons

We investigate the nonlinear dynamics of strongly coupled surface acoustic waves (SAWs) and spin waves (SWs) in a magnetoacoustic resonator based on a YIG/ZnO heterostructure by combining microwave reflection measurements with microfocused Brillouin light scattering spectroscopy. In the linear regime, the electrical response reveals clear hybridization between standing SAW cavity modes and finite-wave-vector SWs, resulting in pronounced avoided crossings. At elevated drive powers, the hybrid system exhibits a strongly field-dependent nonlinear response characterized by a positive frequency shift of the driven SW mode. Using the vector Hamiltonian formalism for nonlinear spin-wave dynamics, we show that this shift is dominated by a cross-shift term. In our resonator geometry, this contribution becomes significant because the standing SAW cavity mode simultaneously excites counterpropagating SWs with wave vectors $+k$ and $-k$. For suitable field detuning, the nonlinear shift drives the SW mode into resonance with the SAW excitation, leading to a strong enhancement of the magnon population, broadband nonlinear scattering, and bistable foldover behavior. Beyond the foldover threshold, both the magnon and phonon responses stabilize. These results establish SAW-driven $k \neq 0$ magnon-phonon hybrids as a promising platform for nonlinear magnetoacoustics and wave-based information processing.

cond-mat.mes-hall

Direct Laser Writing of Ferromagnetic Nickel Utilizing the Principle of Sensitized Triplet-Triplet Annihilation Upconversion

Direct laser writing of ferromagnetic microstructures is of great interest for sensing and data storage in compact three-dimensional architectures. However, reliable direct laser writing of metallic and even more so ferromagnetic materials remains a major challenge. Here, we present a novel photoresist suitable to direct laser write ferromagnetic nickel based on sensitized triplet-triplet annihilation upconversion. By combining an in-situ photochemical deoxygenation process with a sensitized triplet-triplet annihilation upconversion process as well as a photoreduction of Ni2+ ions, the deposition of metallic nickel is enabled under ambient conditions. Using this approach, nickel structures are fabricated as a proof of concept. Scanning electron microscopy and EDX analysis confirm the spatially confined deposition of nickel, while magnetic characterization by vibrating sample magnetometry and scanning NV magnetometry demonstrate the ferromagnetic nature of the printed structures. This work presents a major step forward in extending the possibilities of direct laser writing to metallic and ferromagnetic materials.

cond-mat.mtrl-sci

Nanoscale Dipolar Fields in Artificial Spin Ice Probed by Scanning NV Magnetometry

We investigate dipolar coupling fields in two square-lattice artificial spin ice (ASI) systems with different lattice constants using scanning probe microscopy based on a single nitrogen-vacancy (NV) center in diamond. This technique offers unprecedented spatial resolution, operates under ambient condition, and provides quantitative stray field measurements, making it uniquely suited for studying nanoscale magnetic textures. Our approach combines fluorescence quenching imaging and continuous-wave optically detected magnetic resonance (cODMR). A comparison of the two ASI samples, which differ in their lattice constants of 1000 nm and 910 nm respectively, reveals differences in the appearance of ice-rule violations - deviations from the lowest energy configuration in ASI vertices. We attribute these variations to varying coupling strengths dictated by the lattice constant. From the cODMR data, we extract both axial and transverse components of the local magnetic field relative to the NV axis. Micromagnetic modeling of these measurements allows for an iterative determination of the external magnetic field orientation, the detection of subtle magnetization tilts induced by weak external fields (well below the nanomagnets' switching threshold), and an estimation of the effective saturation magnetization, thereby accounting for deviations in nanomagnet dimensions. These findings provide crucial insights into the tunable magnetic interactions in ASI, paving the way for the design of advanced magnonic and spintronic devices.

cond-mat.mes-hall

Charge accumulation by Direct Magnetoelectric Effect in ScAlN/Ni Nanoscale Devices

This work investigates the direct magnetoelectric effect in thin-film lab scale composite heterostructures comprising a 100 nm thick piezoelectric Sc0.4Al0.6N (ScAlN) and a magnetostrictive Ni with 100-200 nm thickness, fabricated on Si/SiO2 substrates. The films are patterned into square pillar arrays with lateral dimensions down to 500 nm x 500 nm. Vibrating sample magnetometry (VSM) measurements reveal in-plane magnetic anisotropy in the Ni films, attributed to strain induced by the underlying ScAlN layer. Nitrogen-vacancy (NV) magnetometry imaging confirms the formation of magnetic domains at remanence in polycrystalline Ni when patterned in sub-microscale structures. Capacitance measurements reveal a ScAlN dielectric constant at the device level consistent with unpatterned thin films, confirming the preservation of electrical integrity at the sub-microscale. The direct magnetoelectric effect is demonstrated through quasi-static charge measurements under applied out-of-plane DC magnetic fields, yielding equivalent open-circuit voltages up to 1.17 mV.

physics.app-ph

Ratchet motion of magnetic skyrmions driven by surface acoustic sawtooth waves

The manipulation of skyrmions by surface acoustic waves (SAW) has garnered significant interest in the field of spintronic devices. Previous studies established that skyrmions can be generated and moved by strain pulses. In this study, we propose that sawtooth-SAWs can be used to drive a ratchet motion of magnetic skyrmions in the presence of pinning centers. This results in a net motion of the skyrmions orthogonal to the continuously applied SAW. The ratchet motion is fundamentally caused by non-vanishing pinning, so that a certain strain gradient magnitude is required to overcome pinning and start skyrmion motion. We demonstrate the feasibility of our concept by micromagnetic simulations and analytical model calculations.

cond-mat.mes-hall