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Ethan G. Arnault

Publications and source records attributed to Ethan G. Arnault.

17 recordsLinked to original sources

Evidence for a low-gap component in compressively stressed niobium thin films

We investigate the microwave response of sputtered Nb films as a function of biaxial film stress. Although transport measurements show nearly identical superconducting transition temperatures ($9.0\pm 0.2$K) and residual resistance ratios across the stress series, microwave resonators fabricated from highly compressive films exhibit enhanced temperature-dependent loss and larger frequency shifts. A conventional single-phase Mattis--Bardeen description yields an effective critical temperature of $2.4\pm0.2$K, approximately a factor of four below the value obtained from transport measurements. We show that the data are instead consistent with the presence of an additional low-gap component whose contribution increases with compressive stress. These results show that conventional transport measurements can overlook stress-dependent low-energy excitations that strongly influence microwave performance.

quant-ph↗

Full-Stack High-Volume Quantum Networking Architecture based on Photonic-Integrated Tin Vacancy Centers in Diamond

Solid state quantum emitters are a leading platform for photonic quantum networking with memory nodes. However, the inhomogeneous distribution of quantum emitters, as well as several environmental factors (i.e. strain and electric fields) spread the frequency spectrum of the qubits, making them distinguishable and therefore not a reliable resource for distributed quantum entanglement. In this paper, we demonstrate a full-stack approach to integrating nearly indistinguishable tin vacancy (SnV$^-$) quantum emitters on a frequency-tunable photonic interposer that overcomes the native distribution and static variation of quantum emitters for an indistinguishable photonic quantum networking platform. We demonstrate a silicon nitride-on-insulator photonic integrated circuit (PIC) with accompanying multiphysics digital twin (MPhDT) that guides discovery of SnV$^-$ strain-tuning parameters and informs construction of a multi-channel quantum repeater node. On this node, we achieve the first simultaneous demonstration of spectral tuning of the zero phonon line (ZPL) at GHz scale; coherent electron spin control with gate times of $<80$ ns; strongly- and weakly-coupled nuclear spin detection; and commercial fiber array-coupled readout of a SnV$^-$ center. Finally, we propose and simulate improvements to the architecture that achieve 99.96% connectivity of $ N \sim 1000$ emitters spanning the inhomogeneous distribution of SnV$^-$ centers in strained diamond, where distributed quantum entanglement may be realized.

quant-ph↗

Crystalline superconductor-semiconductor Josephson junctions for compact superconducting qubits

The narrow bandgap of semiconductors allows for thick, uniform Josephson junction barriers, potentially enabling reproducible, stable, and compact superconducting qubits. We study vertically stacked van der Waals Josephson junctions with semiconducting weak links, whose crystalline structures and clean interfaces offer a promising platform for quantum devices. We observe robust Josephson coupling across 2--12 nm (3--18 atomic layers) of semiconducting WSe$_2$ and, notably, a crossover from proximity- to tunneling-type behavior with increasing weak link thickness. Building on these results, we fabricate a prototype all-crystalline merged-element transmon qubit with transmon frequency and anharmonicity closely matching design parameters. We demonstrate dispersive coupling between this transmon and a microwave resonator, highlighting the potential of crystalline superconductor-semiconductor structures for compact, tailored superconducting quantum devices.

cond-mat.mes-hall↗

Electrostatic control of quantum phases in KTaO3-based planar constrictions

Two-dimensional electron gases (2DEGs) formed at complex oxide interfaces offer a unique platform to engineer quantum nanostructures. However, scalable fabrication of locally addressable devices in these materials remains challenging. Here, we demonstrate an efficient fabrication approach by patterning narrow constrictions in a superconducting KTaO3-based heterostructure. The constrictions are individually tunable via the coplanar side gates formed within the same 2DEG plane. Our technique leverages the high dielectric permittivity of KTaO3 (epsilon_r ~ 5000) to achieve strong electrostatic modulation of the superconducting 2DEG. Transport measurements through the constriction reveal a range of transport regimes: Within the superconducting state, we demonstrate efficient modulation of the critical current and Berezinskii Kosterlitz Thouless (BKT) transition temperature at the weak link. Further tuning of the gate voltage reveals an unexpectedly regular Coulomb blockade pattern. All of these states are achievable with a side gate voltage |V_SG| < 1 V. The fabrication process is scalable and versatile, enabling a platform both to make superconducting field-effect transistors and to study a wide array of physical phenomena present at complex oxide interfaces.

cond-mat.supr-con↗

Microwave single-photon detection using a hybrid spin-optomechanical quantum interface

Semiconductor single-photon detectors cannot be straightforwardly adapted for the microwave regime, primarily because microwave photons carry far less energy and thus require cryogenic temperatures and specialized architectures. Here, we propose a hybrid spin-optomechanical interface to detect single microwave photons where the microwave photons are coupled to a phononic resonator via piezoelectric actuation. This phononic cavity also acts as a photonic cavity with either a single embedded Silicon-Vacancy (SiV) center in diamond or an ensemble of these centers, bridging optical single-photon detection protocols into the microwave domain. We model the detection process as a communication channel whose capacity is quantified by the mutual information \(I(A;B)\) between the true photon occupancy (A) and the detector outcome (B). Depending on experimentally achievable parameters, simulations predict \(I(A;B)\) in the range \(0.57\,\ln(2)\) to \(0.67\,\ln(2)\), corresponding to true-positive (detection) probabilities above 90\% and false-positive (dark count) probabilities below 10\% per detection interval. These results suggest a viable path to low-noise, high-efficiency single-photon detection at microwave frequencies.

quant-ph↗

Graphene calorimetric single-photon detector

Single photon detectors (SPDs) are essential technology in quantum science, quantum network, biology, and advanced imaging. To detect the small quantum of energy carried in a photon, conventional SPDs rely on energy excitation across either a semiconductor bandgap or superconducting gap. While the energy gap suppresses the false-positive error, it also sets an energy scale that can limit the detection efficiency of lower energy photons and spectral bandwidth of the SPD. Here, we demonstrate an orthogonal approach to detect single near-infrared photons using graphene calorimeters. By exploiting the extremely low heat capacity of the pseudo-relativistic electrons in graphene near its charge neutrality point, we observe an electron temperature rise up to ~2 K using a hybrid Josephson junction. In this proof-of-principle experiment, we achieve an intrinsic quantum efficiency of 87% (75%) with dark count < 1 per second (per hour) at operation temperatures as high as 1.2 K. Our results highlight the potential of electron calorimetric SPDs for detecting lower-energy photons from the mid-IR to microwave regimes, opening pathways to study space science in far-infrared regime, to search for dark matter axions, and to advance quantum technologies across a broader electromagnetic spectrum.

cond-mat.mes-hall↗

Multiplet Supercurrents in a Josephson Circuit

Multiterminal Josephson junctions are a promising platform to host synthetic topological phases of matter and Floquet states. However, the energy scales governing topological protection in these devices are on the order of the spacing between Andreev bound states. Recent theories suggest that similar phenomena may instead be explored in circuits composed of two-terminal Josephson junctions, allowing for the topological protection to be controlled by the comparatively large Josephson energy. Here, we explore a Josephson circuit, in which three superconducting electrodes are connected through Josephson junctions to a common superconducting island. We demonstrate the dynamic generation of multiplet resonances, which have previously been observed in multiterminal Josephson junctions. The multiplets are found to be robust to elevated temperatures and are confirmed by exhibiting the expected Shapiro step quantization under a microwave drive. We also find an unexpected novel supercurrent, which couples a pair of contacts that are both voltage-biased with respect to the common superconducting island. We show that this supercurrent results from synchronization of the phase dynamics and pose the question whether it should also carry a topological contribution.

cond-mat.mes-hall↗

Noise-induced stabilization of dynamical states with broken time-reversal symmetry

Under a high frequency drive, Josephson junctions demonstrate "Shapiro steps" of quantized voltage. These are dynamically stabilized states, in which the phase across the junction locks to the external drive. We explore the stochastic switching between two symmetric steps at $\frac{\hbarω}{2e}$ and $-\frac{\hbarω}{2e}$. Surprisingly, the switching rate exhibits a pronounced non-monotonicity as a function of temperature, violating the general expectation that transitions should become faster with temperature. We explain this behavior by realizing that the system retains memory of the dynamic state from which it is switching, thereby breaking the conventional simplifying assumptions about separations of time scales.

cond-mat.mes-hall↗

Non-local transport measurements in hybrid quantum Hall - superconducting devices

There has been a growing interest in hybrid quantum Hall (QH) superconductor devices, driven by the prospect to realize exotic ground states and excitations with non-abelian exchange statistics. While the existing experiments clearly demonstrate Andreev coupling between the edge states and the superconductors, the question remains whether the quantum coherence could propagate between several superconducting contacts via chiral channels. To answer this question, we have first extended the Landauer-Büttiker (LB) formalism to samples with one superconducting contact and found a remarkable agreement within a series of measurements related to each other via LB-type formulae. We have then switched to the case of multiple superconducting contacts, and found that we can describe the measurements self-consistently if we neglect the superconducting phase coherence between multiple contacts. We interpret this result as a negative answer to the question posed above: the phase correlations between multiple superconducting contacts are not established via micron-long quantum Hall edge states. Looking forward, our approach may find applications in the broader field of topological superconductivity and proximal structures. Possible violations of the self-consistency tests presented here may be used as an indication that superconducting phase coherence is induced in the quantum Hall edges.

cond-mat.supr-con↗

Performance limits due to thermal transport in graphene single-photon bolometers

In high-sensitivity bolometers and calorimeters, the photon absorption often occurs at a finite distance from the temperature sensor to accommodate antennas or avoid the degradation of superconducting circuitry exposed to radiation. As a result, thermal propagation from the input to the temperature readout can critically affect detector performance. In this report we model the performance of a graphene bolometer, accounting for electronic thermal diffusion and dissipation via electron-phonon coupling at low temperatures in three regimes: clean, supercollision, and resonant scattering. Our results affirm the feasibility of a superconducting readout without Cooper-pair breaking by mid- and near-infrared photons, and provide a recipe for designing graphene absorbers for calorimetric single-photon detectors. We investigate the tradeoff between the input-readout distance and detector efficiency, and predict an intrinsic timing jitter of ~2.7 ps. Based on our result, we propose a spatial-mode-resolving photon detector to increase communication bandwidth.

cond-mat.mes-hall↗

Graphene-based quantum Hall interferometer with self-aligned side gates

The vanishing band gap of graphene has long presented challenges for making high-quality quantum point contacts (QPCs) -- the partially transparent p-n interfaces introduced by conventional split-gates tend to short the QPC. This complication has hindered the fabrication of graphene quantum Hall Fabry-Pérot interferometers, until recent advances have allowed split-gate QPCs to operate utilizing the highly resistive $ν=0$ state. Here, we present a simple recipe to fabricate QPCs by etching a narrow trench in the graphene sheet to separate the conducting channel from self-aligned graphene side gates. We demonstrate operation of the individual QPCs in the quantum Hall regime, and further utilize these QPCs to create and study a quantum Hall interferometer.

cond-mat.mes-hall↗

Interference of chiral Andreev edge states

The search for topological excitations such as Majorana fermions has spurred interest in the boundaries between distinct quantum states. Here, we explore an interface between two prototypical phases of electrons with conceptually different ground states: the integer quantum Hall insulator and the s-wave superconductor. We find clear signatures of hybridized electron and hole states similar to chiral Majorana fermions, to which we refer as chiral Andreev edge states (CAES). They propagate along the interface in the direction determined by magnetic field and their interference can turn an incoming electron into an outgoing electron or a hole, depending on the phase accumulated by the CAES along their path. Our results demonstrate that these excitations can propagate and interfere over a significant length, opening future possibilities for their coherent manipulation.

cond-mat.mes-hall↗

Loss and decoherence at the quantum Hall - superconductor interface

We perform a systematic study of Andreev conversion at the interface between a superconductor and graphene in the quantum Hall (QH) regime. We find that the probability of Andreev conversion from electrons to holes follows an unexpected but clear trend: the dependencies on temperature and magnetic field are nearly decoupled. We discuss these trends and the role of the superconducting vortices, whose normal cores could both absorb and dephase the individual electrons in a QH edge. Our study may pave the road to engineering future generation of hybrid devices for exploiting superconductivity proximity in chiral channels.

cond-mat.mes-hall↗

Non-Reciprocal Supercurrents in a Field-Free Graphene Josephson Triode

Superconducting diodes are proposed non-reciprocal circuit elements that should exhibit non-dissipative transport in one direction while being resistive in the opposite direction. Multiple examples of such devices have emerged in the past couple of years, however their efficiency is typically limited, and most of them require magnetic field to function. Here we present a device achieving efficiencies upwards of 90% while operating at zero field. Our samples consist of a network of three graphene Josephson junctions linked by a common superconducting island, to which we refer as a Josephson triode. The triode is tuned by applying a control current to one of the contacts, thereby breaking the time-reversal symmetry of the current flow. The triode's utility is demonstrated by rectifying a small (tens of nA amplitude) applied square wave. We speculate that devices of this type could be realistically employed in the modern quantum circuits.

cond-mat.mes-hall↗

Dynamical Stabilization of Multiplet Supercurrents in Multi-terminal Josephson Junctions

The dynamical properties of multi-terminal Josephson junctions have recently attracted interest, driven by the promise of new insights into synthetic topological phases of matter and Floquet states. This effort has culminated in the discovery of Cooper multiplets, in which the splitting of a Cooper pair is enabled via a series of Andreev reflections that entangle four (or more) electrons. In this text, we show conclusively that multiplet resonances can also emerge as a consequence of the three terminal circuit model. The supercurrent appears due to the correlated phase dynamics at values that correspond to the multiplet condition $nV_1 = -mV_2$ of applied bias. The emergence of multiplet resonances is seen in i) a nanofabricated three-terminal graphene Josephson junction, ii) an analog three terminal Josephson junction circuit, and iii) a circuit simulation. The mechanism which stabilizes the state of the system under those conditions is purely dynamical, and a close analog to Kapitza's inverted pendulum problem. We describe parameter considerations that best optimize the detection of the multiplet lines both for design of future devices. Further, these supercurrents have a classically robust $\cos2ϕ$ energy contribution, which can be used to engineer qubits based on higher harmonics.

cond-mat.mes-hall↗

The Multi-terminal Inverse AC Josephson Effect

When a Josephson junction is exposed to microwave radiation, it undergoes the inverse AC Josephson effect - the phase of the junction locks to the drive frequency. As a result, the I-V curves of the junction acquire "Shapiro steps" of quantized voltage. If the junction has three or more superconducting contacts, coupling between different pairs of terminals must be taken into account and the state of the junction evolves in a phase space of higher dimensionality. Here, we study the multi-terminal inverse AC Josephson effect in a graphene sample with three superconducting terminals. We observe robust fractional Shapiro steps and correlated switching events, which can only be explained by considering the device as a completely connected Josephson network. We successfully simulate the observed behaviors using a modified two-dimensional RCSJ model. Our results suggest multi-terminal Josephson junctions are a playground to study highly-connected nonlinear networks with novel topologies.

cond-mat.mes-hall↗

Full control of quantum Hall supercurrent in a side gated graphene Josephson junction

We present a study of a graphene-based Josephson junction with dedicated side gates carved from the same sheet of graphene as the junction itself. These side gates are highly efficient, and allow us to modulate carrier density along either edge of the junction in a wide range. In particular, in magnetic fields in the $1-2$ Tesla range, we are able to populate the next Landau level, resulting in Hall plateaus with conductance that differs from the bulk filling factor. When counter-propagating quantum Hall edge states are introduced along either edge, we observe supercurrent localized along that edge of the junction. Here we study these supercurrents as a function of magnetic field and carrier density.

cond-mat.mes-hall↗