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Eugene Demler

Publications and source records attributed to Eugene Demler.

At least 37 records · Page 2Linked to original sources

Giant Resonant Enhancement of Photoinduced Dynamical Cooper Pairing, far above $T_c$

Pump-probe experiments performed on $\mathrm{K}_3\mathrm{C}_{60}$ have unveiled both optical and transport signatures of metastable light-induced superconductivity up to room temperature, far above $T_c$. Recent experiments have uncovered that excitation in the vicinity of $50 ~\textrm{meV}$ enables the observation of high temperature light-induced superconductivity at significantly lower fluences. Inspired by these experiments we develop a mechanism which can explain such a giant resonant enhancement of light-induced superconductivity. Within a minimal non-linear Holstein model, we show that resonantly driving optical Raman modes leads to a time-dependent electron-phonon coupling. Such a coupling then modulates the effective electron-electron attraction, with the strongest modulations occurring when the drive is resonant with the phonon frequency. These dynamical modulations of the pairing interactions lead to Floquet-BCS instabilities at temperatures far exceeding equilibrium $T_c$, as observed in experiments. We conclude by discussing the implications of our general analysis on the $\mathrm{K}_3\mathrm{C}_{60}$ experiments specifically and suggesting experimental signatures of our mechanism.

cond-mat.supr-con↗

Optical Detection and Manipulation of Pseudospin Orders in Wigner Crystals

In Wigner-crystal states of two-dimensional electrons, the spin ordering remains poorly understood. The small energy differences between candidate spin orders make theoretical studies less reliable, and probing magnetic order at a nonzero wave vector is experimentally challenging. In modern realizations of Wigner crystals, the electronic spin degree of freedom is often replaced by a valley pseudospin associated with nonzero Berry curvature. The resulting anomalous velocity couples the electrons' pseudospin texture to their orbital vibration. We show that this mechanism enables optical detection of pseudospin orders in Wigner crystals by producing sharp signatures in the terahertz optical conductivity. For example, antiferromagnetic pseudospin order enables light to excite collective electronic vibrations at the ordering wave vector, generating a characteristic absorption peak. Based on the same principle, we further show that a strong optical drive generates an effective potential that reshapes the pseudospin energy landscape, inducing phase transitions to stripe antiferromagnetic states. These results point to a route for optical detection and control of spin order via its coupling to orbital motion.

cond-mat.str-el↗

Magnon Nesting in Driven Two-Dimensional Quantum Magnets

We uncover a new class of dynamical quantum instability in driven magnets leading to emergent enhancement of antiferromagnetic correlations even for purely ferromagnetic microscopic couplings. A primary parametric amplification creates a frequency-tuned nested magnon distribution in momentum space, which seeds a secondary instability marked by the emergence of enhanced antiferromagnetic correlations, mirroring the instability of nested Fermi surfaces in electronic systems. In sharp contrast to the fermionic case, however, the magnon-driven instability is intrinsically non-equilibrium and fundamentally inaccessible in thermal physics. Its quantum mechanical origin sets it apart from classical instabilities such as Faraday and modulation instabilities, which underlie several instances of dynamical behavior observed in magnetic and cold-atom systems.

cond-mat.mtrl-sci↗

Connecting single-layer $t$-$J$ to Kondo lattice models: Exploration with cold atoms

The Kondo effect, a hallmark of many-body physics, emerges from the antiferromagnetic coupling between localized spins and conduction fermions, leading to a correlated many-body singlet state. Here we propose to use the mixed-dimensional (mixD) bilayer Hubbard geometry as a platform to study Kondo lattice physics with current ultracold atom experiments. At experimentally feasible temperatures, we predict that key features of the Kondo effect can be observed, including formation of the Kondo cloud around a single impurity and the competition of singlet formation with Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions for multiple impurities, summarized in the Doniach phase diagram. Moreover, we show that the mixD platform provides a natural bridge between the Doniach phase diagram of the Kondo lattice model, relevant to heavy-fermion materials, and the phase diagram of cuprate superconductors as described by a single-layer Zhang-Rice type $t$-$J$ model: It is possible to continuously tune between the two regimes by changing the interlayer Kondo coupling. Our findings demonstrate that the direct connection between high-temperature superconductivity and heavy-fermion physics can be experimentally studied using currently available quantum simulation platforms.

cond-mat.quant-gas↗

Casimir Stabilization of Fluctuating Electronic Nematic Order

Vacuum cavity control of quantum materials is the engineering of quantum materials systems through electromagnetic zero-point fluctuations. In this work we articulate a generic mechanism for vacuum optical control of correlated electronic order: Casimir control, where the zero-point energy of the electromagnetic continuum, the Casimir energy, depends on the properties of the material system. To assess the experimental viability of this mechanism we focus on the Casimir stabilization of fluctuating nematic order. In nematic Fermi liquids, different orientations of the electronic order are often energetically degenerate. Thus, while local domains of fixed orientation may form, thermal disordering inhibits long range order. By engineering the electromagnetic environment of the electronic system, however, we show that the Casimir energy can be used as a tool to preferentially stabilize particular orientations of the nematic order. As a concrete example, we examine the interplay between a birefringent crystal -- which sources an anisotropic electromagnetic environment -- and a quantum Hall stripe system, an archetypal nematic Fermi fluid. We show that for experimentally feasible setups, the anisotropy induced by the orientation dependent Casimir energy can be $10^4$ times larger than other mechanisms known to stabilize quantum Hall stripes. This finding convincingly implies that our setting may be realized with currently available experimental technology. Having demonstrated that the Casimir energy can be used to stabilize fluctuating nematic order, we close by discussing the implications for recent terahertz cavity experiments on quantum Hall stripes, as well as pave the road towards broader Casimir control of competing correlated electronic phases.

cond-mat.str-el↗

Superconductivity in Substitutional Ga-Hyperdoped Ge Epitaxial Thin Films

Doping-induced superconductivity in group IV elements may enable quantum functionalities in material systems accessible with well-established semiconductor technologies. Non-equilibrium hyperdoping of group III atoms into C, Si, or Ge can yield superconductivity; however, its origin is obscured by structural disorder and dopant clustering. Here, we report the epitaxial growth of hyperdoped Ga:Ge films and trilayer heterostructures by molecular beam epitaxy with extreme hole concentrations ($n_\textup{h} = 4.15 \times 10^{21}$~cm$^{-3}$, ~17.9\% Ga substitution) that yield superconductivity with a critical temperature of $T_{\textup{c}} = 3.5$~K and an out-of-plane critical field of 1~T at 270~mK. Synchrotron-based X-ray absorption and scattering methods reveal that Ga dopants are substitutionally incorporated within the Ge lattice, introducing a tetragonal distortion to the crystal unit cell. Our findings, corroborated by first-principles calculations, suggest that the structural order of Ga dopants creates a narrow band for the emergence of superconductivity in Ge, establishing hyperdoped Ga:Ge as a low-disorder, epitaxial superconductor-semiconductor platform.

cond-mat.mes-hall↗

Role of Phase Fluctuation in Dynamic Competition Between Charge Order and Superconductivity in Cuprates

Phase fluctuations are a key factor distinguishing nonthermal (ultrafast) and thermal phase transitions. Charge order in cuprates is characterized by short-range coherence while competing with superconductivity, and as such, it provides a representative case to study the role of phase fluctuation in coupled order parameter dynamics. In this work, we investigated the intertwined evolution of charge order and superconductivity in cuprate/manganite heterostructures using time-resolved resonant X-ray scattering. The resulting dynamics are analyzed within a space- and time-dependent nonperturbative model capturing both amplitude and phase dynamics. At low fluence, photo-induced suppression of superconductivity results in a nonthermal enhancement of charge order, underscoring the dynamic competition between charge order and superconductivity. With increasing fluence, the slowing down of melting and recovery dynamics is observed, indicating a critical role of phase fluctuations. At high fluence, both charge order and superconductivity remain suppressed for an extended time window due to decoupling between amplitude and phase dynamics and the delayed recovery of phase coherence. Our work underscores the importance of phase fluctuation for understanding the dynamic competition between order parameters in cuprates.

cond-mat.str-el↗

Kinetically-induced bound states in a frustrated Rydberg tweezer array

Understanding how particles bind into composite objects is a ubiquitous theme in physics, from the formation of molecules to hadrons in quantum chromodynamics and the pairing of charge carriers in superconductors. The formation of bound states usually originates from attractive interactions between particles. However, the binding can also arise purely from the motion of dopants due to kinetic frustration, which is potentially related to unconventional pairing in moiré materials. Here, we report the first direct observation of kinetically-induced bound states between holes and magnons using a Rydberg atom array quantum simulator of the bosonic $t$-$J$ model in frustrated ladders and 2D lattices. First, we demonstrate the formation of mobile one-hole-one-magnon bound states. We then construct three-particle one-hole-two-magnon bound states and reveal the underlying binding mechanism by observing kinetically-induced singlet correlations. Finally, we investigate how mobile dopants structure their magnetic environment in a spin-balanced 2D triangular lattice, showing that a hole induces $120^\circ$ antiferromagnetic order, while a doublon dopant generates in-plane ferromagnetic correlations. Our results demonstrates compelling evidence of kinetically-induced binding, opening a new avenue to understand novel pairing mechanisms in correlated quantum materials like superconductors in moiré superlattices.

quant-ph↗

Momentum-resolved two-dimensional spectroscopy as a probe of nonlinear quantum field dynamics

Emergent collective excitations constitute a hallmark of interacting quantum many-body systems, yet in solid-state platforms their study has been largely limited by the constraints of linear-response probes and by finite momentum resolution. We propose to overcome these limitations by combining the spatial resolution of ultracold atomic systems with the nonlinear probing capabilities of two-dimensional spectroscopy (2DS). As a concrete illustration, we analyze momentum-resolved 2DS of the quantum sine-Gordon model describing the low energy dynamics of two weakly coupled one-dimensional Bose-Einstein condensates. This approach reveals distinctive many-body signatures, most notably asymmetric cross-peaks reflecting the interplay between isolated ($B_2$ breather) and continuum ($B_1$ pair) modes. The protocol further enables direct characterization of anharmonicity and disorder, establishing momentum-resolved 2DS as both a powerful diagnostic for quantum simulators and a versatile probe of correlated quantum matter.

cond-mat.quant-gas↗

Gap Inhomogeneity in Cuprates: a view from Two-Dimensional Josephson Echo Spectroscopy

Novel theoretical developments have allowed to connect microscopic disorder in bosonic collective excitations to the signatures in two-dimensional terahertz spectroscopy (Gómez Salvador et al. 2025). Here, we employ this framework to analyze the recently measured Josepshon echoes in optimally doped La$_{2-x}$Sr$_x$CuO$_4$ (Liu et al. 2024). We consider the spatial gap inhomogeneities -- observed in scanning tunneling microscopy -- as input for the disorder in the superfluid density, and compute the resulting echo peaks. The excellent agreement supports the interpretation that the gap inhomogeneity arises solely from pairing gap fluctuations, with no evidence for non-superconducting competing local orders. Finally, we study the microscopic origin of the inelastic processes, contributing to the damping of the Josephson plasmon at low temperatures, and conclude that it can be attributed to nodal quasiparticles.

cond-mat.supr-con↗

Optimal Calibration of Qubit Detuning and Crosstalk

Characterizing and calibrating physical qubits is essential for maintaining the performance of quantum processors. A key challenge in this process is the presence of crosstalk that complicates the estimation of individual qubit detunings. In this work, we derive optimal strategies for estimating detuning and crosstalk parameters by optimizing Ramsey interference experiments using Fisher information and the Cramer-Rao bound. We compare several calibration protocols, including measurements of a single quadrature at multiple times and of two quadratures at a single time, for a fixed number of total measurements. Our results predict that the latter approach yields the highest precision and robustness in both cases of isolated and coupled qubits. We validate experimentally our approach using a single NV center as well as superconducting transmons. Our approach enables accurate parameter extraction with significantly fewer measurements, resulting in up to a 50% reduction in calibration time while maintaining estimation accuracy.

quant-ph↗

Two-dimensional spectroscopy of bosonic collective excitations in disordered many-body systems

We present a novel theoretical approach for computing and analyzing two-dimensional spectroscopy of bosonic collective excitations in disordered many-body systems. Specifically, we employ the Keldysh formalism to derive, within a non-pertubative treatment of disorder effects, the third-order nonlinear response and obtain two-dimensional spectroscopy maps. In the weak nonlinear regime of our formalism, we demonstrate the ability of the echo peak to distinguish between elastic and inelastic scattering processes, in perfect agreement with the intuition developed in isolated two-level systems. Furthermore, we discuss unique many-body effects on the echo peak signature arising from interaction induced quantum fluctuations. In particular, we show that these quantum fluctuations induce a finite nonrephasable broadening and examine how the echo peak is influenced by the attractive or repulsive nature of the collective excitations.

cond-mat.str-el↗

Dissipative realization of Kondo models

We demonstrate that the Kondo effect can be induced through non-linear dissipative channels, without requiring any coherent interaction on the impurity site. Specifically, we consider a reservoir of noninteracting fermions that can hop on a few impurity sites that are subjected to strong two-body losses. In the simplest case of a single lossy site, we recover the Anderson impurity model in the regime of infinite repulsion, with a small residual dissipation as a perturbation. While the Anderson model gives rise to the Kondo effect, this residual dissipation competes with it, offering an instance of a nonlinear dissipative impurity where the interplay between coherent and incoherent dynamics emerges from the same underlying physical process. We further outline how this dissipative engineering scheme can be extended to two or more lossy sites, realizing generalizations of the Kondo model with spin 1 or higher. Our results suggest alternative implementations of Kondo models using ultracold atoms in transport experiments, where localized dissipation can be naturally introduced, and the Kondo effect observed through conductance measurements.

cond-mat.quant-gas↗

Variational approach to the dynamics of dissipative quantum impurity models

Recent experiments with quantum simulators using ultracold atoms and superconducting qubits have demonstrated the potential of controlled dissipation as a versatile tool for realizing correlated many-body states. However, determining the dynamics of dissipative quantum many-body systems remains a significant analytical and numerical challenge. In this work, we focus on a dissipative impurity problem as a testbed for new methodological developments. We introduce an efficient non-perturbative framework that combines the superposition of Gaussian states (SGS) variational ansatz with the quantum trajectory approach to simulate open systems featuring a dissipative impurity. Applying this method to a spinful impurity subject to two-body losses and embedded in a bath of noninteracting fermions, we explore the full crossover from weak to strong dissipation regimes. The non-perturbative nature of the SGS ansatz allows us to thoroughly examine this crossover, providing comprehensive insights into the system's behavior. In the strong dissipation regime, our approach reproduces the finding that localized two-body losses can induce the Kondo effect [arXiv:2406.03527], characterized by a slowdown of spin relaxation and an enhancement of charge conductance. Furthermore, we reveal an exotic ``negative conductance" phenomenon at zero potential bias -- a counter-intuitive single-body effect resulting from intermediate dissipation and finite bandwidth. Finally, we investigate the formation of ferromagnetic domains and propose an extension to realize a higher-spin Kondo model using localized dissipation.

cond-mat.quant-gas↗

Subgap pumping of antiferromagnetic Mott insulators: photoexcitation mechanisms and applications

We study the behavior of the 2D repulsive Hubbard model on a square lattice at half filling, under strong driving with ac electric fields, by employing a time-dependent Gaussian variational approach. Within the same theoretical framework, we analytically obtain the conventional Keldysh crossover between multiphoton and tunneling photoexcitation mechanisms, as well as two new regimes beyond the Keldysh paradigm. We discuss how dynamical renormalization of the Mott-Hubbard gap feeds back into the photoexcitation process, modulating the carrier generation rate in real time. The momentum distribution of quasiparticle excitations immediately after the drive is calculated, and shown to contain valuable information about the generation mechanism. Finally, we discuss experimental probing of the pump-induced nonequilibrium electronic state.

cond-mat.str-el↗

Observation of Nagaoka Polarons in a Fermi-Hubbard Quantum Simulator

Quantum interference can deeply alter the nature of many-body phases of matter. In the paradigmatic case of the Hubbard model, Nagaoka famously proved that introducing a single itinerant charge can transform a paramagnetic insulator into a ferromagnet through path interference. However, a microscopic observation of such kinetic magnetism induced by individually imaged dopants has been so far elusive. Here we demonstrate the emergence of Nagaoka polarons in a Hubbard system realized with strongly interacting fermions in a triangular optical lattice. Using quantum gas microscopy, we reveal these polarons as extended ferromagnetic bubbles around particle dopants arising from the local interplay of coherent dopant motion and spin exchange. In contrast, kinetic frustration due to the triangular geometry promotes antiferromagnetic polarons around hole dopants, as proposed by Haerter and Shastry. Our work augurs the exploration of exotic quantum phases driven by charge motion in strongly correlated systems and over sizes that are challenging for numerical simulation.

cond-mat.quant-gas↗

Wideband covariance magnetometry below the diffraction limit

We experimentally demonstrate a method for measuring correlations of wideband magnetic signals with spatial resolution below the optical diffraction limit. Our technique employs two nitrogen-vacancy (NV) centers in diamond as nanoscale magnetometers, spectrally resolved by inhomogeneous optical transitions. Using high-fidelity optical readout and long spin coherence time, we probe correlated MHz-range noise with sensitivity of 15 nT Hz$^{-1/4}$. In addition, we use this system for correlated $T_1$ relaxometry, enabling correlation measurements of GHz-range noise. Under such externally applied noise, while individual NV centers exhibit featureless relaxation, their correlation displays rich coherent and incoherent dynamics reminiscent of superradiance physics. This capability to probe high-frequency correlations provides a powerful tool for investigating a variety of condensed-matter phenomena characterized by nonlocal correlations.

quant-ph↗

Magnon hydrodynamics in an atomically-thin ferromagnet

Strong interactions between particles can lead to emergent collective excitations. These phenomena have been extensively established in electronic systems, but are also expected to occur for gases of neutral particles like magnons, i.e. spin waves, in magnets. In a hydrodynamic regime where magnons are strongly interacting, they can form a slow collective density mode -- in analogy to sound waves in water -- with characteristic low-frequency signatures. While such a mode has been predicted in theory, its signatures have yet to be observed experimentally. In this work, we isolate exfoliated sheets of CrCl$_3$ where magnon interactions are strong, and develop a technique to measure its collective magnon dynamics via the quantum coherence of nearby Nitrogen-Vacancy (NV) centers in diamond. We find that the thermal magnetic fluctuations generated by monolayer CrCl$_3$ exhibit an anomalous temperature dependence, whereby fluctuations increase upon decreasing temperature. Our analysis suggests that this anomalous trend is a consequence of the damping rate of a low-energy magnon sound mode which sharpens as magnon interactions increase with increasing temperature. By measuring the magnetic fluctuations emitted by thin multilayer CrCl$_{3}$ in the presence of a variable-frequency drive field, we observe spectroscopic evidence for this two-dimensional magnon sound mode.

cond-mat.mes-hall↗