arXiv subjects

Eugene Demler

Publications and source records attributed to Eugene Demler.

At least 55 records · Page 3Linked to original sources

arXiv2025

Time-domain identification of distinct mechanisms for competing charge density waves in a rare-earth tritelluride

Understanding the origin of phase transitions and the interactions between distinct phases remains a central task in condensed matter physics. Charge density wave (CDW) systems provide an ideal platform for investigating these phenomena. While the dominant CDW phases in many materials can be explained through Fermi surface nesting or electron-phonon interactions, certain CDW phase transitions remain poorly understood, challenging conventional paradigms. One notable example is rare-earth tritelluride ErTe3, which hosts two competing CDW orders. While the dominant CDW phase fits within the electron-phonon coupling framework, the formation mechanism of the subdominant CDW remains enigmatic. In this study, we combine time-and-angle-resolved photoemission spectroscopy (trARPES) with time-dependent Ginzburg-Landau (TDGL) theory to establish a time-domain approach for probing phase transitions in solid-state systems. By analyzing the distinct recovery dynamics of the two CDW orders in ErTe3 following light excitation, we reveal a novel nucleation-like growth mechanism that likely drives the secondary CDW phase transition. This work not only uncovers a previously unknown CDW formation mechanism in rare-earth tritellurides but also introduces a non-equilibrium framework for understanding phase transitions and phase competition in quantum materials.

cond-mat.str-el↗

arXiv2025

Cavity-mediated charge and pair-density waves in a unitary Fermi gas

Coherent light-matter interactions between a quantum gas and light in a high-finesse cavity can drive self-ordering phase transitions. To date, such phenomena have involved exclusively single-atom coupling to light, resulting in coupled charge-density or spin-density wave and superradiant order. In this work, we engineer simultaneous coupling of cavity photons to both single atoms and fermionic pairs, which are also mutually coupled due to strong correlations in the unitary Fermi gas. This interplay gives rise to an interference between the charge-density wave and a pair-density wave, where the short-range pair correlation function is spontaneously modulated in space. We observe this effect by tracking the onset of superradiance as the photon-pair coupling is varied in strength and sign, revealing constructive or destructive interference of the three orders with a coupling mediated by strong light-matter and atom-atom interactions. Our observations are compared with mean-field theory where the coupling strength between atomic- and pair-density waves is controlled by higher-order correlations in the Fermi gas. These results demonstrate the potential of cavity quantum electrodynamics to produce and observe exotic orders in strongly correlated matter, paving the way for the quantum simulation of complex quantum matter using ultracold atoms.

cond-mat.quant-gas↗

arXiv2025

Cavity QED Control of Quantum Hall Stripes

Controlling quantum phases of materials with vacuum field fluctuations in engineered cavities is a novel route towards the optical control of emergent phenomena. We demonstrate, using magnetotransport measurements of a high-mobility two-dimensional electron gas, striking cavity-induced anisotropies in the electronic transport, including the suppression of the longitudinal resistance well below the resistivity at zero magnetic field. Our cavity-induced effects occur at ultra-low temperatures (< 200 mK) when the magnetic field lies between quantized Hall plateaus. We interpret our results as arising from the stabilization of thermally-disordered quantum Hall stripes. Our work presents a clear demonstration of the cavity QED control of a correlated electronic phase.

cond-mat.mes-hall↗

arXiv2025

Bipolaron dynamics in the one-dimensional SSH model

Characterizing bipolaron binding, and understanding how it depends on electron-phonon interaction, is crucial to unraveling the nature of emergent many-body states in strongly interacting electron-phonon systems. So far, most studies of bipolarons have been limited to the Holstein model, in which the coupling constant is momentum-independent. The paradigmatic example of momentum-dependent electron-phonon interaction comes from the system in which phonon distortions modify electron hopping, the SSH model. Already individual polarons in the SSH model are richer than the Holstein model counterparts, and feature a phase transition into the finite momentum ground state with increasing electron-phonon interaction. In this paper, we use a variational approach to study bipolarons in the one-dimensional SSH model and discuss their ground state, dispersion, and excitation spectra. We explore the full parameter range of the system, including the adiabatic regime of slow phonons, which was inaccessible to previous theoretical studies. In agreement with earlier studies, we find that in the anti-adiabatic strongly interacting regime, bipolarons have low effective mass. By contrast, in the adiabatic case, we find that increasing electron-phonon interactions results in an exponential increase of the bipolaron mass. We establish the existence of multiple branches of bound excited states of SSH bipolaron and discuss the signatures of these bound states in dynamics. We show that in the anti-adiabatic regime, response functions obey a parity selection rule, that imposes symmetry constraints on the excitation spectra and provides a clear signature of SSH bipolarons.

cond-mat.str-el↗

arXiv2025

Directly imaging spin polarons in a kinetically frustrated Hubbard system

The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an interplay between the kinetic energy of doped charge carriers and superexchange spin interactions. However, in kinetically frustrated lattices, itinerant spin polarons - bound states of a dopant and a spin-flip - have been theoretically predicted even in the absence of superexchange coupling. Despite their important role in the theory of kinetic magnetism, a microscopic observation of these polarons is lacking. Here we directly image itinerant spin polarons in a triangular lattice Hubbard system realised with ultracold atoms, revealing enhanced antiferromagnetic correlations in the local environment of a hole dopant. In contrast, around a charge dopant, we find ferromagnetic correlations, a manifestation of the elusive Nagaoka effect. We study the evolution of these correlations with interactions and doping, and use higher-order correlation functions to further elucidate the relative contributions of superexchange and kinetic mechanisms. The robustness of itinerant spin polarons at high temperature paves the way for exploring potential mechanisms for hole pairing and superconductivity in frustrated systems. Furthermore, our work provides microscopic insights into related phenomena in triangular lattice moiré materials.

cond-mat.quant-gas↗

arXiv2025

Observation of Magnon-Polarons in the Fermi-Hubbard Model

The interplay of magnetic excitations and itinerant charge carriers is a ubiquitous phenomenon in strongly correlated electron systems. In the vicinity of magnetically ordered phases, strong interactions between itinerant quasiparticles and magnetic excitations can result in the dramatic renormalization of both. A key theoretical question is understanding the renormalization of the magnon quasiparticle, a collective spin excitation, upon doping a magnetic insulator. Here, we report the observation of a new type of quasiparticle arising from the dressing of a magnon with the doped holes of a cold atom Fermi-Hubbard system, i.e. a magnon-Fermi-polaron. Utilizing Raman excitation with controlled momentum in a doped, spin-polarized band insulator, we address the spectroscopic properties of the magnon-polaron. In an undoped system with strong interactions, photoexcitation produces magnons, whose properties are accurately described by spin wave theory. We measure the evolution of the photoexcitation spectra as we move away from this limit to produce magnon-polarons due to dressing of the magnons by charge excitations. We observe a shift in the polaron energy with doping that is strongly dependent on the injected momentum, accompanied by a reduction of spectral weight in the probed energy window. We anticipate that the technique introduced here, which is the analog of inelastic neutron scattering, will provide atomic quantum simulators access to the dynamics of a wide variety of excitations in strongly correlated phases.

cond-mat.quant-gas↗

arXiv2024

Quantum Cherenkov transition of finite momentum Bose polarons

We investigate the behavior of a finite-momentum impurity immersed in a weakly interacting three-dimensional Bose-Einstein condensate (BEC) of ultra-cold atoms, giving a detailed account of the dynamical quantum Cherenkov transition discussed in Ref. [arXiv:2101.00030]. Using a time-dependent variational approach, we identify a transition in the far-from-equilibrium dynamics of the system after the attractive short-range impurity-boson interaction is quenched on. The transition occurs as the impurity's velocity crosses an interaction-dependent critical value, and manifests in the long-time behavior of the Loschmidt echo and average impurity velocity. This behavior is also reflected in the finite momentum ground state of the system, where the group velocity of the interaction-dressed impurity loses it's dependence on the total momentum of the system as the critical point is crossed. The transition we discuss should be experimentally observable via a variety of common protocols in ultracold atomic systems such as time-of-flight imaging, RF spectroscopy, Ramsey interferometry, and absorption imaging.

cond-mat.quant-gas↗

arXiv2024

Optical signatures of interlayer electron coherence in a bilayer semiconductor

Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and electronic Wigner crystals~\cite{smolenski2021signatures,zhou2021bilayer} to the ongoing quest for exciton condensation~\cite{wang2019evidence,ma2021strongly,shi2022bilayer}. Here, we experimentally investigate the properties of indirect excitons in naturally-grown MoS$_2$-homobilayer, integrated in a dual-gate device structure allowing independent control of the electron density and out-of-plane electric field. Under conditions when electron tunneling between the layers is negligible~\cite{pisoni2019absence}, upon electron doping the sample, we observe that the two excitons with opposing dipoles hybridize, displaying unusual behavior distinct from both conventional level crossing and anti-crossing. We show that these observations can be explained by static random coupling between the excitons, which increases with electron density and decreases with temperature. We argue that this phenomenon is indicative of a spatially fluctuating order parameter in the form of interlayer electron coherence, a theoretically predicted many-body state~\cite{zheng1997exchange} that has yet to be unambiguously established experimentally outside of the quantum Hall regime~\cite{sarma2008perspectives,spielman2000resonantly,kellogg2004vanishing,kellogg2002observation,spielman2001observation,fertig1989energy,shi2022bilayer}. Implications of our findings for future experiments and quantum optics applications are discussed.

cond-mat.str-el↗

arXiv2024

Platform tailored co-design of gate-based quantum simulation

The utility of near-term quantum computers and simulators is likely to rely upon software-hardware co-design, with error-aware algorithms and protocols optimized for the platforms they are run on. Here, we show how knowledge of noise in a system can be exploited to improve the design of gate-based quantum simulation algorithms. We concretely demonstrate this co-design in the context of a trapped ion quantum simulation of the dynamics of a Heisenberg spin model. Specifically, we derive a theoretical noise model describing unitary gate errors due to heating of the ions' collective motion, finding that the temporal correlations in the noise induce an optimal gate depth. We then illustrate how tailored feedforward control can be used to mitigate unitary gate errors and improve the simulation outcome. Our results provide a practical guide to the co-design of gate-based quantum simulation algorithms.

quant-ph↗

arXiv2024

Collective flow of fermionic impurities immersed in a Bose-Einstein Condensate

Interacting mixtures of bosons and fermions are ubiquitous in nature. They form the backbone of the standard model of physics, provide a framework for understanding quantum materials and are of technological importance in helium dilution refrigerators. However, the description of their coupled thermodynamics and collective behaviour is challenging. Bose-Fermi mixtures of ultracold atoms provide a platform to investigate their properties in a highly controllable environment, where the species concentration and interaction strength can be tuned at will. Here we characterize the collective oscillations of spin-polarized fermionic impurities immersed in a Bose-Einstein condensate as a function of the interaction strength and temperature. For strong interactions, the Fermi gas perfectly mimics the superfluid hydrodynamic modes of the condensate, from low-energy quadrupole modes to high-order Faraday excitations. With an increasing number of bosonic thermal excitations, the dynamics of the impurities cross over from the collisionless to the hydrodynamic regime, reminiscent of the emergence of hydrodynamics in two-dimensional electron fluids.

cond-mat.quant-gas↗

arXiv2024

Spectroscopy of Hubbard-Mott excitons and their ro-vibrational excitations

Hubbard excitons are bound states of doublons and holes that can be experimentally probed both in real materials, such as cuprates, and in cold atom quantum simulators. Here we compare properties of a Hubbard exciton to those of a pair of distinguishable dopants in the $t-J$ model and show how insights into pair properties can be obtained through excitonic spectra. In particular, we perform large-scale numerical simulations of spectral functions and optical conductivities and obtain remarkable agreement between Hubbard excitons and pairs of distinguishable dopants. The latter can be decomposed into symmetric (bosonic) and anti-symmetric (fermionic) sectors of indistinguishable dopants, thus enabling a detailed understanding of different features observed in the excitonic spectra through comparison with a semi-analytical geometric string theory approach. We further compare theoretically computed exciton spectra in a single band Fermi-Hubbard model to resonant inelastic X-ray scattering (RIXS) studies of the parent insulating cuprate materials. We find remarkable agreement between the two spectra in both energy and momentum dependence. Our analysis suggests that multiple long-lived ro-vibrational exciton resonances have been observed in RIXS spectra. Experimentally, these features are known to persist up to optimal doping. The comparison we provide between semi-analytical theory, large-scale numerics, and experimental data thus provides an explanation of the RIXS measurements and provides new insight into the nature of pairing in cuprates.

cond-mat.str-el↗

arXiv2024

Dynamical Instabilities of Strongly Interacting Ultracold Fermions in an Optical Cavity

Recent quench experiments on ultra cold fermions in optical cavities provide a clean platform for studying how long-range interactions between fermions structure their dynamics. Motivated by these experiments, we provide a theoretical analysis of the dynamical instabilities that lead to the formation of superradiance as the hybrid system is driven across the self-organization transition. We compute the rate at which order forms and quantify the fluctuations of the pre-quench state which seed the instability. Our results quantitatively match existing experiments on free fermions and make predictions for quench experiments involving near unitary fermi gases coupled to an optical cavity. Our work suggests that the non-local nature of the photon-mediated interactions between fermions generates ordering dynamics that are qualitatively different than those observed in short-range interacting systems.

cond-mat.quant-gas↗

arXiv2024

Non-equilibrium dynamics of long-range interacting Fermions

A fundamental problem of out-of-equilibrium physics is the speed at which the order parameter grows upon crossing a phase transition. Here, we investigate the dynamics of ordering in a Fermi gas undergoing a density-wave phase transition induced by quenching of long-range, cavity-mediated interactions. We observe in real-time the exponential rise of the order parameter and track its growth over several orders of magnitude. Remarkably, the growth rate is insensitive to the contact interaction strength from the ideal gas up to the unitary limit and can exceed the Fermi energy by an order of magnitude, in quantitative agreement with a linearized instability analysis. We then generalize our results to linear interaction ramps, where deviations from the adiabatic behaviour are captured by a simple dynamical ansatz. Our study offers a paradigmatic example of the interplay between non-locality and non-equilibrium dynamics, where universal scaling behaviour emerges despite strong interactions at the microscopic level.

cond-mat.quant-gas↗

arXiv2024

Dynamic magnetic phase transition induced by parametric magnon pumping

Uncovering pathways to optically drive magnetic order-disorder transitions on ultrashort timescales can lead to the realization of novel out-of-equilibrium quantum phenomena. A long-sought pathway is to directly excite a highly non-thermal energy-momentum distribution of magnons, bypassing both charge and lattice degrees of freedom. However, this remains elusive owing to the weak coupling and large momentum mismatch between photons and magnons. Here we demonstrate strong parametric excitation of magnons across the entire Brillouin zone of the antiferromagnetic insulator Sr$_2$Cu$_3$O$_4$Cl$_2$ by periodically modulating the superexchange interaction with the electric field of light. The excitation efficiency is greatly enhanced by tuning to the van Hove singularity in the magnon spectrum, sufficient to transiently collapse the antiferromagnetic state using a pulsed laser field of 10$^9$ V/m. The order parameter recovery timescale increases by over 1000 times as a function of excitation density, reflecting a crossover from high- to low-energy magnon dominated decay dynamics. This electric-field induced parametric magnon pumping mechanism is applicable to a broad range of magnetic insulators and opens up the possibility of dynamically engineering magnon distributions by design.

cond-mat.str-el↗

arXiv2024

Probing the Berezinskii-Kosterlitz-Thouless vortex unbinding transition in two-dimensional superconductors using local noise magnetometry

The melting of quasi-long-range superconductivity in two spatial dimensions occurs through the proliferation and unbinding of vortex-antivortex pairs -- a phenomenon known as the Berezinskii-Kosterlitz-Thouless (BKT) transition. Although signatures of this transition have been observed in bulk measurements, these experiments are often complicated, ambiguous, and unable to resolve the rich physics of the vortex unbinding transition. Here we show that local noise magnetometry is a sensitive, noninvasive probe that can provide direct information about the scale-dependent vortex dynamics. In particular, by resolving the distance and temperature dependence of the magnetic noise, it may be possible to experimentally study the renormalization group flow equations of the vortex gas and track the onset of vortex unbinding in situ. Specifically, we predict i) a nonmonotonic dependence of the noise on temperature and ii) the local noise is almost independent of the sample-probe distance at the BKT transition. We also show that noise magnetometry can distinguish Gaussian superconducting order-parameter fluctuations from topological vortex fluctuations and can detect the emergence of unbound vortices. The weak distance dependence at the BKT transition can also be used to distinguish it from quasiparticle background noise. Our predictions may be within experimental reach for a number of unconventional superconductors.

cond-mat.supr-con↗

arXiv2024

Pairing dome from an emergent Feshbach resonance in a strongly repulsive bilayer model

A key to understanding unconventional superconductivity lies in unraveling the pairing mechanism of mobile charge carriers in doped antiferromagnets, yielding an effective attraction between charges even in the presence of strong repulsive Coulomb interactions. Here, we study pairing in a mixed-dimensional (mixD) $t-J$ model, featuring robust binding energies -- despite dominant repulsive interactions -- that are strongly enhanced in the finite doping regime. The single and coupled mixD ladders we study, corresponding to bilayers of width $w\leq 2$, feature a crossover from tightly bound pairs of holes (closed channel) at small repulsion, to more spatially extended, correlated pairs of individual holes (open channel) at large repulsion. We derive an effective model for the latter, in which the attraction is mediated by the closed channel, in analogy to atomic Feshbach resonances. Using density matrix renormalization group (DMRG) simulations we reveal a dome of large binding energies at around $30\%$ doping, accompanied by a change of the Fermi surface volume and a crossover from extended to tightly bound hole pairs. Our work provides a microscopic theory of pairing in the doped mixD system with dominant repulsion, closely related to bilayer, Ni-based superconductors, and our predictions can be tested in state-of-the-art quantum simulators.

cond-mat.str-el↗

arXiv2024

New opportunities in condensed matter physics for nanoscale quantum sensors

Nitrogen vacancy (NV) centre quantum sensors provide unique opportunities in studying condensed matter systems: they are quantitative, noninvasive, physically robust, offer nanoscale resolution, and may be used across a wide range of temperatures. These properties have been exploited in recent years to obtain nanoscale resolution measurements of static magnetic fields arising from spin order and current flow in condensed matter systems. Compared with other nanoscale magnetic-field sensors, NV centres have the unique advantage that they can probe quantities that go beyond average magnetic fields. Leveraging techniques from magnetic resonance, NV centres can perform high precision noise sensing, and have given access to diverse systems, such as fluctuating electrical currents in simple metals and graphene, as well as magnetic dynamics in yttrium iron garnet. In this review we summarise unique opportunities in condensed matter sensing by focusing on the connections between specific NV measurements and previously established physical characteristics that are more readily understood in the condensed matter community, such as correlation functions and order parameters that are inaccessible by other techniques, and we describe the technical frontier enabled by NV centre sensing.

cond-mat.mes-hall↗

arXiv2024

Terahertz amplification and lasing in pump-probe experiments with hyperbolic polaritons in h-BN

We discuss terahertz pump-probe experiments in hBN from the perspective of Floquet optical materials and photonic time crystals. Anisotropic nature of this material results in a large separation of frequencies of in-plane and out-of-plane optical phonons and leads to several branches of phonon-polariton excitations. We consider a slab of finite thickness pumped at the frequency of middle polaritons, around 25 THz. We theoretically analyze properties of the pump induced state and identify several interesting features, including possible light amplification and parametric instability at 2 THz. We relate these features to resonant pair scattering processes of polaritons excited by the pump pulse. We show that amplification/instability frequency ranges depend on both the pump intensity and the slab thickness. We point out that this setup can be used utilized to strongly enhance optical nonlinearities at terahertz frequencies. Richness and tunability of this system suggests that it holds promise for practical applications in terahertz technology.

physics.optics↗