arXiv subjects

F. Ji

Publications and source records attributed to F. Ji.

11 recordsLinked to original sources

arXiv2023

Relativistic ultrafast electron diffraction at high repetition rates

The ability to resolve the dynamics of matter on its native temporal and spatial scales constitutes a key challenge and convergent theme across chemistry, biology, and materials science. The last couple of decades have witnessed ultrafast electron diffraction (UED) emerge as one of the forefront techniques with the sensitivity to resolve atomic motions. Increasingly sophisticated UED instruments are being developed that are aimed at increasing the beam brightness in order to observe structural signatures, but so far they have been limited to low average current beams. Here we present the technical design and capabilities of the HiRES (High Repetition Rate Electron Scattering) instrument, which blends relativistic electrons and high repetition rates to achieve orders of magnitude improvement in average beam current compared to the existing state-of-the-art UED instruments. The setup utilizes a novel electron source to deliver femtosecond duration electron pulses at up to MHz repetition rates for UED experiments. We provide example cases of diffraction measurements on solid-state and gas-phase samples, including both micro- and nanodiffraction modes, which showcase the potential of the instrument for novel UED experiments.

physics.ins-det↗

arXiv2021

Peta-electron volt gamma-ray emission from the Crab Nebula

The Crab pulsar and the surrounding nebula powered by the pulsar's rotational energy through the formation and termination of a relativistic electron-positron wind is a bright source of gamma-rays carrying crucial information about this complex conglomerate. We report the detection of $\gamma$-rays with a spectrum showing gradual steepening over three energy decades, from $5\times 10^{-4}$ to $1.1$ petaelectronvolt (PeV). The ultra-high-energy photons exhibit the presence of a PeV electron accelerator (a pevatron) with an acceleration rate exceeding 15% of the absolute theoretical limit. Assuming that unpulsed $\gamma$-rays are produced at the termination of the pulsar's wind, we constrain the pevatron's size, between $0.025$ and $0.1$ pc, and the magnetic field $\approx 110 \mu$G. The production rate of PeV electrons, $2.5 \times 10^{36}$ erg $\rm s^{-1}$, constitutes 0.5% of the pulsar's spin-down luminosity, although we do not exclude a non-negligible contribution of PeV protons to the production of the highest energy $\gamma$-rays.

astro-ph.HE↗

arXiv2021

Conformer-specific Chemistry Imaged in Real Space and Time

Conformational isomers or conformers of molecules play a decisive role in chemistry and biology. However, experimental methods to investigate chemical reaction dynamics are typically not conformer-sensitive. Here, we report on a gas-phase megaelectronvolt ultrafast electron diffraction investigation of {\alpha}-phellandrene undergoing an electrocyclic ring-opening reaction. We directly image the evolution of a specific set of {\alpha}-phellandrene conformers into the product isomer predicted by the Woodward-Hoffmann rules in real space and time. Our experimental results are in quantitative agreement with nonadiabatic quantum molecular dynamics simulations, which provide unprecedented detail of how conformation influences time scale and quantum efficiency of photoinduced ring-opening reactions. Due to the prevalence of large numbers of conformers in organic chemistry, our findings impact our general understanding of reaction dynamics in chemistry and biology.

physics.chem-ph↗

arXiv2021

Discovery of a new $\gamma$-ray source LHAASO J0341+5258 with emission up to 200TeV

We report the discovery of a new unidentified extended $\gamma$-ray source in the Galactic plane named LHAASO J0341+5258 with a pre-trial significance of 8.2 standard deviations above 25 TeV. The best fit position is R.A.$=55.34^{\circ}\pm0.11^{\circ}$ and Dec$=52.97^{\circ}\pm0.07^{\circ}$. The angular size of LHAASO J0341+5258 is $0.29^\circ \pm 0.06^\circ_{stat} \pm0.02^\circ_{sys}$. The flux above 25 TeV is about $20\%$ of the flux of Crab Nebula. Although a power-law fit of the spectrum from 10 TeV to 200 TeV with the photon index $\alpha=2.98 \pm 0.19_{stat} \pm 0.02_{sys}$ is not excluded, the LHAASO data together with the flux upper limit at 10 GeV set by the Fermi LAT observation, indicate a noticeable steepening of an initially hard power-law spectrum %($\alpha \leq 1.75$) spectrum with a cutoff at $\approx 50$ TeV. We briefly discuss the origin of UHE gamma-rays. The lack of an energetic pulsar and a young SNR inside or in the vicinity of LHAASO J0341+5258 challenge, but do not exclude both the leptonic and hadronic scenarios of gamma-ray production.

astro-ph.HE↗

arXiv2021

Exploring Lorentz Invariance Violation from Ultra-high-energy Gamma Rays Observed by LHAASO

Recently the LHAASO Collaboration published the detection of 12 ultra-high-energy gamma-ray sources above 100 TeV, with the highest energy photon reaching 1.4 PeV. The first detection of PeV gamma rays from astrophysical sources may provide a very sensitive probe of the effect of the Lorentz invariance violation (LIV), which results in decay of high-energy gamma rays in the superluminal scenario and hence a sharp cutoff of the energy spectrum. Two highest energy sources are studied in this work. No signature of the existence of LIV is found in their energy spectra, and the lower limits on the LIV energy scale are derived. Our results show that the first-order LIV energy scale should be higher than about 10^5 times the Planck scale M_{pl} and that the second-order LIV scale is >10^{-3}M_{pl}. Both limits improve by at least one order of magnitude the previous results.

astro-ph.HE↗

arXiv2021

Discovery of the Ultra-high energy gamma-ray source LHAASO J2108+5157

We report the discovery of a UHE gamma-ray source, LHAASO J2108+5157, by analyzing the LHAASO-KM2A data of 308.33 live days. Significant excess of gamma-ray induced showers is observed in both energy bands of 25-100 TeV and $\gt$100 TeV with 9.5 sigma and 8.5 sigma, respectively. This source is not significantly favored as an extensive source with the angular extension smaller than the point-spread function of KM2A. The measured energy spectrum from 20 to 200 TeV can be approximately described by a power-law function with an index of -2.83$\pm$ 0.18stat. A harder spectrum is demanded at lower energies considering the flux upper limit set by Fermi-LAT observations. The position of the gamma-ray emission is correlated with a giant molecular cloud, which favors a hadronic origin. No obvious counterparts have been found, deeper multiwavelength observations will help to shed new light on this intriguing UHE source.

astro-ph.HE↗

arXiv2021

Discerning the painter's hand: machine learning on surface topography

Attribution of paintings is a critical problem in art history. This study extends machine learning analysis to surface topography of painted works. A controlled study of positive attribution was designed with paintings produced by a class of art students. The paintings were scanned using a confocal optical profilometer to produce surface data. The surface data were divided into virtual patches and used to train an ensemble of convolutional neural networks (CNNs) for attribution. Over a range of patch sizes from 0.5 to 60 mm, the resulting attribution was found to be 60 to 96% accurate, and, when comparing regions of different color, was nearly twice as accurate as CNNs using color images of the paintings. Remarkably, short length scales, as small as twice a bristle diameter, were the key to reliably distinguishing among artists. These results show promise for real-world attribution, particularly in the case of workshop practice.

cs.CV↗

arXiv2021

Calibration of the Air Shower Energy Scale of the Water and Air Cherenkov Techniques in the LHAASO experiment

The Wide Field-of-View Cherenkov Telescope Array (WFCTA) and the Water Cherenkov Detector Arrays (WCDA) of LHAASO are designed to work in combination for measuring the energy spectra of various cosmic ray species over a very wide energy range from a few TeV to 10 PeV. The energy calibration of WCDA can be achieved with a proven technique of measuring the westward shift of the Moon shadow of galactic cosmic rays due to the geomagnetic field. This deflection angle $\Delta$ is inversely proportional to the energy of the cosmic rays. The precise measurements of the shifts by WCDA allows us to calibrate its energy scale for energies as high as 35 TeV. The energy scale measured by WCDA can be used to cross calibrate the energy reconstructed by WFCTA, which spans the whole energy range up to 10 PeV. In this work, we will demonstrate the feasibility of the method using the data collected from April 2019 to January 2020 by the WFCTA array and WCDA-1 detector, the first of the three water Cherenkov ponds, already commissioned at LHAASO site.

astro-ph.IM↗

arXiv2020

Construction and On-site Performance of the LHAASO WFCTA Camera

The focal plane camera is the core component of the Wide Field-of-view Cherenkov/fluorescence Telescope Array (WFCTA) of the Large High-Altitude Air Shower Observatory (LHAASO). Because of the capability of working under moonlight without aging, silicon photomultipliers (SiPM) have been proven to be not only an alternative but also an improvement to conventional photomultiplier tubes (PMT) in this application. Eighteen SiPM-based cameras with square light funnels have been built for WFCTA. The telescopes have collected more than 100 million cosmic ray events and preliminary results indicate that these cameras are capable of working under moonlight. The characteristics of the light funnels and SiPMs pose challenges (e.g. dynamic range, dark count rate, assembly techniques). In this paper, we present the design features, manufacturing techniques and performances of these cameras. Finally, the test facilities, the test methods and results of SiPMs in the cameras are reported here.

physics.ins-det↗

arXiv2020

The observation of the Crab Nebula with LHAASO-KM2A for the performance study

As a sub-array of the Large High Altitude Air Shower Observatory (LHAASO), KM2A is mainly designed to cover a large fraction of the northern sky to hunt for gamma-ray sources at energies above 10 TeV. Even though the detector construction is still underway, a half of the KM2A array has been operating stably since the end of 2019. In this paper, we present the pipeline of KM2A data analysis and the first observation on the Crab Nebula, a standard candle in very high energy gamma-ray astronomy. We detect gamma-ray signals from the Crab Nebula in both energy ranges of 10$-$100 TeV and $>$100 TeV with high significance, by analyzing the KM2A data of 136 live days between December 2019 and May 2020. With the observations, we test the detector performance including angular resolution, pointing accuracy and cosmic ray background rejection power. The energy spectrum of the Crab Nebula in the energy range 10-250 TeV fits well with a single power-law function dN/dE =(1.13$\pm$0.05$_{stat}$$\pm$0.08$_{sys}$)$\times$10$^{-14}$$\cdot$(E/20TeV)$^{-3.09\pm0.06_{stat}\pm0.02_{sys}}$ cm$^{-2}$ s$^{-1}$ TeV$^{-1}$. It is consistent with previous measurements by other experiments. This opens a new window of gamma-ray astronomy above 0.1 PeV through which ultrahigh-energy gamma-ray new phenomena, such as cosmic PeVatrons, might be discovered.

astro-ph.HE↗

arXiv2017

Influence of Spin Orbit Coupling in the Iron-Based Superconductors

We report on the influence of spin-orbit coupling (SOC) in the Fe-based superconductors (FeSCs) via application of circularly-polarized spin and angle-resolved photoemission spectroscopy. We combine this technique in representative members of both the Fe-pnictides and Fe-chalcogenides with ab initio density functional theory and tight-binding calculations to establish an ubiquitous modification of the electronic structure in these materials imbued by SOC. The influence of SOC is found to be concentrated on the hole pockets where the superconducting gap is generally found to be largest. This result contests descriptions of superconductivity in these materials in terms of pure spin-singlet eigenstates, raising questions regarding the possible pairing mechanisms and role of SOC therein.

cond-mat.supr-con↗