arXiv subjects

F. M. Araujo-Moreira

Publications and source records attributed to F. M. Araujo-Moreira.

At least 37 records · Page 2Linked to original sources

arXiv2007

Probing pairing symmetry of Sm_{1.85}Ce_{0.15}CuO_4 via highly-sensitive voltage measurements: Evidence for strong impurity scattering

Using a highly-sensitive home-made mutual-inductance technique, temperature profiles of the magnetic penetration depth $λ(T)$ in the optimally-doped $Sm_{1.85}Ce_{0.15}CuO_4$ thin films have been extracted. The low-temperature behavior of $λ(T)$ is found to be best-fitted by linear $Δλ(T)/λ(0)= \ln(2)k_BT/Δ_0$ and quadratic $Δλ(T)/λ(0)=Γ^{-1/2}Δ_0^{-3/2}T^2$ laws above and below $T=0.22T_C$, respectively, which clearly indicates the presence of d-wave pairing mechanism dominated by strong paramagnetic scattering at the lowest temperatures. The best fits produce $Δ_0/k_BT_C=2.07$ and $Γ/T_C=0.25(T_C/Δ_0)^3$ for the estimates of the nodal gap parameter and impurity scattering rate.

cond-mat.supr-con↗

arXiv2007

On the origin of unusual transport properties observed in densely packed polycrystalline CaAl_{2}

A possible origin of unusual temperature behavior of transport coefficients observed in densely packed polycrystalline CaAl_{2} compound [M. Ausloos et al., J. Appl. Phys. 96, 7338 (2004)] is discussed, including a power-like dependence of resistivity with $ρ\propto T^{-3/4}$ and N-like form of the thermopower. All these features are found to be in good agreement with the Shklovskii-Efros localization scenario assuming polaron-mediated hopping processes controlled by the Debye energy.

cond-mat.mtrl-sci↗

arXiv2007

Thermal expansion of Josephson junctions as an elastic response to an effective stress field

By introducing a concept of thermal expansion (TE) of a Josephson junction as an elastic response to an effective stress field, we study (both analytically and numerically) the temperature and magnetic field dependence of TE coefficient $α$ in a single small junction and in a square array. In particular, we found that in addition to {\it field} oscillations due to Fraunhofer-like dependence of the critical current, $α$ of a small single junction also exhibits strong flux driven {\it temperature} oscillations near $T_C$. We also numerically simulated stress induced response of a closed loop with finite self-inductance (a prototype of an array) and found that $α$ of a $5\times 5$ array may still exhibit temperature oscillations provided the applied magnetic field is strong enough to compensate for the screening induced effects.

cond-mat.supr-con↗

arXiv2005

Magnetic properties of artificially prepared ordered two-dimensional shunted and unshunted Nb-AlO_x-Nb Josephson Junction Arrays

In this Chapter, we present our latest experimental results (along with their theoretical interpretation) related to some unusual magnetic properties of artificially prepared ordered two-dimensional Josephson junction arrays (of both shunted and unshunted Nb-AlO_x-Nb tunnel junctions). Namely, we address the following topics: (i) influence of non-uniform critical current density profile on magnetic field behavior of AC susceptibility, (ii) origin of the so-called dynamic reentrance phenomenon, and (iii) manifestation of novel geometric quantization effects in temperature behavior of AC magnetic response.

cond-mat.supr-con↗

arXiv2005

Elastic properties of polycrystalline YBa_2Cu_3O_7: Evidence for granularity induced martensitic behavior

In this work we present the study of the elastic properties of polycrystalline samples of superconducting YBa_2Cu_3O_7 prepared by the sol-gel method. The quality of all samples was checked by x-ray diffraction and scanning electronic microscopy while their physical properties were verified by transport and magnetic measurements. The elastic study was performed using the standard pulse-echo technique through measuring the phase velocity and the attenuation of ultrasonic waves (in the range of a few MHz) as a function of temperature. We have focused this study on the low temperatures interval (T < 200K). The obtained results show a strong hysteretic behavior in the ultrasonic attenuation (in addition to usually observed hysteretic behavior for the velocity) which strongly supports the existence of a martensitic-like phase above the superconducting critical temperature T_C. We argue that this peculiar behavior can be attributed to the granularity present in the samples.

cond-mat.supr-con↗

arXiv2005

On the origin of reentrance in 2D Josephson Junction Arrays

A comparative study of the magnetic properties of shunted and unshunted two-dimensional Josephson junction arrays (2D-JJA) is presented. Using a single-plaquette approximation of the 2D-JJA model, we were able to successfully fit all our experimental data (for the temperature, AC and DC field dependencies of susceptibility) and demonstrate that the dynamic reentrance of AC susceptibility is directly linked to the value of the Stewart-McCumber parameter β_C. Based on extensive numerical simulations, a phase diagram β_C vs β_L is plotted which demarcates the border between the reentrant and non-reentrant behavior in the arrays.

cond-mat.supr-con↗

arXiv2005

Influence of nonuniform critical current density profile on magnetic field behavior of AC susceptibility in 2D Josephson Junction Arrays

Employing mutual-inductance measurements we study the magnetic field dependence of complex AC susceptibility of artificially prepared highly ordered (periodic) two-dimensional Josephson junction arrays of unshunted Nb-AlO_x-Nb junctions. The observed behavior can be explained assuming single-plaquette approximation of the overdamped model with an inhomogeneous critical current distribution within a single junction.

cond-mat.supr-con↗

arXiv2005

Manifestation of geometric quantization effects in temperature behavior of AC magnetic response of Josephson Junction Arrays

By improving resolution of home-made mutual-inductance measurements technique, a pronounced step-like structure (with the number of steps n=4 for all AC fields) has been observed in the temperature dependence of AC susceptibility in artificially prepared two-dimensional Josephson Junction Arrays (2D-JJA) of unshunted Nb-AlO_x-Nb junctions with β_L(4.2K)=30. Using a single-plaquette approximation of the overdamped 2D-JJA model, we were able to successfully fit our data assuming that steps are related to the geometric properties of the plaquette. The number of steps n corresponds to the number of flux quanta that can be screened by the maximum critical current of the junctions. The steps are predicted to manifest themselves in arrays with the inductance related parameter β_L(T) matching a "quantization" condition β_L(0)=2π(n+1).

cond-mat.supr-con↗

arXiv2005

Magnetic and superconducting properties of RuSr2 Gd1.5Ce0.5Cu2O10-x samples: dependence on the oxygen content and ageing effects

The magnetic and superconducting properties of RuSr2Gd1.5Ce0.5Cu2O10-x polycrystalline samples with different oxygen doping level are presented. A strong suppression of the superconducting temperature (Tc), as well as a reduction in the superconducting fraction, occurs as the oxygen content is reduced by annealing the samples in oxygen deprived atmospheres. Drastic changes in the electrical resistivity are observed above Tc, possibly associated with oxygen removal mainly from grain boundaries. However, the magnetic ordering is relatively less affected by the changes in oxygen content of the samples. The spin glass transition is enhanced and shifted to higher temperatures with the reduction in oxygen content. This could be correlated with an increase in the spins disorder and frustration for the oxygen depleted samples. Also, the same oxygen vacancy induced disorder could explain the reduction in the fraction of the sample showing antiferromagnetic order. We also report significant changes in the measured properties of the samples as a function of time.

cond-mat.supr-con↗

arXiv2004

Fabrication and physical properties of stable room temperature bulk ferromagnetic graphite

The search for macroscopic magnetic ordering phenomena in organic materials, in particular in pure graphite, has been one of the more exciting scientific activities working in the frontiers of physics, chemistry, and materials science. In this Letter we report on a novel chemical route leading to undoubtedly obtain macroscopic quantities of magnetic graphite. This material has a stable and strong ferromagnetic response even at room temperature where it can be attracted by a commercial magnet. We have obtained this magnetic graphite by a vapor reaction consisting of a controlled etching on the graphite structure. This behavior has been previously predicted and postulated to be associated to micro-structural characteristics breaking the continuity of the delocalized p-electron clouds of the graphitic material, thus allowing the existence of magnetic centers related to the topology.

cond-mat.mtrl-sci↗

arXiv2004

Stable room temperature magnetic graphite

Carbon materials are attracting increasing attention due to the novelty of the associated physical properties and the potential applications in high-tech devices. The possibility to achieve outstanding properties in macroscopic carbon materials opens up a profusion of new striking applications. Magnetic properties induced by defects on graphite structures, such as pores, edges of the planes and topological defects, have been theoretically predicted. The possible coexistence of sp3 and sp2 bonds have been also invoked to predict this behavior (for a review, see ref. 1). Some reports have proved the existence of weak ferromagnetic-like magnetization loops in highly-oriented pyrolytic graphite (HOPG) (ref. 2-3). Very recently two reports showed that the existence of ferromagnetism in pure carbon is unambiguously possible (ref. 4-5). Here we report on a novel and inexpensive chemical route consistent in a controlled etching on the graphite structure to obtain macroscopic amounts of magnetic pure graphite. This material has a strong magnetic response even at room temperature where it can be attracted by a commercial magnet and would be the experimental confirmation for the defect induced magnetism previously predicted.

cond-mat.mtrl-sci↗

arXiv2004

Comparative study of specific heat measurements in LaMnO3, La1.35Sr1.65Mn2O7, La1.5Sr0.5NiO4 and La1.5Sr0.5CoO4

We present the temperature dependence of the specific heat, without external magnetic field and with H= 9 T, for LaMnO3, La1.35Sr1.65Mn2O7, La1.5Sr0.5NiO4 and La1.5Sr0.5CoO4 single crystals. We found that spin-wave excitations in the ferromagnetic and bilayer-structure La1.35Sr1.65Mn2O7 were suppressed by the 9 T magnetic field. On the other hand, the external magnetic field had no effect in the specific heat of the other three antiferromagnetic samples. Also, the electronic part of the interactions were removed at very low temperatures in the La1.5Sr0.5NiO4 single crystal, even with a zero applied magnetic field. Below 4 K, we found that the specific heat data for La1.35Sr1.65Mn2O7 and La1.5Sr0.5NiO4 crystals could be fitted to an exponential decay law. Detailed magnetization measurements in this low temperature interval showed the existence of a peak close to 2 K. Both results, magnetizations and specific heat suggest the existence of an anisotropy gap in the energy spectrum of La1.35Sr1.65Mn2O7 and La1.5Sr0.5NiO4 compounds.

cond-mat.mtrl-sci↗

arXiv2003

Physical properties of single-crystalline fibers of the colossal-magnetoresistance manganite La0.7Ca0.3MnO3

We have grown high-quality single crystals of the colossal-magnetoresistance (CMR) material La0.7Ca0.3MnO3 by using the laser heated pedestal growth (LHPG) method. Samples were grown as fibers of different diameters, and with lengths of the order of centimeters. Their composition and structure were verified through X-ray diffraction, scanning electron microcopy with EDX (Energy Dispersive X-ray Analysis) and by Rietveld analysis. The quality of the crystalline fibers was confirmed by Laue and EBSD (Electron Backscatter Diffraction) patterns. Rocking curves performed along the fiber axis revealed a half-height width of 0.073 degrees. The CMR behavior was confirmed by electrical resistivity and magnetization measurements as a function of temperature.

cond-mat.mtrl-sci↗

arXiv2003

Spin Glass Behavior in the Ru-1222 and Ru-1212 rutheno-cuprate families: a comparative study

Strong evidences of a spin glass phase on polycrystalline RuSr2Ln1.5Ce0.5Cu2O10-x (LnRu-1222, Ln = Y, Ho and Dy) is provided by ac susceptibility and dc magnetization measurements. The fingerprint of a spin glass transition, the frequency-dependent cusp in ac susceptibility vs. T measurements at low magnetic field, is observed for all LnRu-1222 samples. The strong supression of the cusp in the ac susceptibility measurement in the presence of magnetic fields as low as 500 Oe, and the results of thermoremanent magnetization (TRM) and isothermal remanent magnetization (IRM) measurements are also evidences of a spin glass behavior. By comparing these results with measurements on a YRu-1212 sample we conclude that the glassy behavior is characteristic of the Ru-1222 phase, not being observed for the studied YRu-1212 sample. We suggest that the spin glass transition occur only in the Ru-1222 phase possibly due to the larger number of oxygen vacancies present in these compounds.

cond-mat.supr-con↗

arXiv2002

Spin Glass Behavior in RuSr2Gd1.5Ce0.5Cu2O10

The dynamics of the magnetic properties of polycrystalline RuSr2Gd1.5Ce0.5Cu2O10 (Ru-1222) have been studied by ac susceptibility and dc magnetization measurements, including relaxation and ageing studies. Ru-1222 is a reported magneto-superconductor with Ru spins magnetic ordering at temperatures near 100 K and superconductivity in Cu-O2 planes below Tc ~ 40 K. The exact nature of Ru spins magnetic ordering is still debated and no conclusion has been reached yet. In this work, a frequency-dependent cusp was observed in ac susceptibility vs. T measurements, which is interpreted as a spin glass transition. The change in the cusp position with frequency follows the Vogel-Fulcher law, which is commonly accepted to describe a spin glass with magnetically interacting clusters. Such interpretation is supported by themoremanaent magnetization (TRM) measurements at T = 60 K. TRM relaxations are well described by a stretched exponential relation, and present significant ageing effects.

cond-mat.supr-con↗

arXiv2002

Specific heat and magnetic measurements in Nd0.5Sr0.5MnO3, Nd0.5Ca0.5MnO3 and Ho0.5Ca0.5MnO3 samples

We studied the magnetization as a function of temperature and magnetic field in the compounds Nd0.5Sr0.5MnO3, Nd0.5Ca0.5MnO3 and Ho0.5Ca0.5MnO3. It allowed us to identify the ferromagnetic, antiferromagnetic and charge ordering phases in each case. The intrinsic magnetic moments of Nd3+ and Ho3+ ions experienced a short range order at low temperatures. We also did specific heat measurements with applied magnetic fields between 0 and 9 T and temperatures between 2 and 300 K in all three samples. Close to the charge ordering and ferromagnetic transition temperatures the specific heat curves showed peaks superposed to the characteristic response of the lattice oscillations. Below 10 K the specific heat measurements evidenced a Schottky-like anomaly for all samples. However, we could not successfully fit the curves to either a two level nor a distribution of two-level Schottky anomaly. Our results indicated that the peak temperature of the Schottky anomaly was higher in the compounds with narrower conduction band.

cond-mat↗

arXiv2001

Study of magnetic and specific heat measurements at low temperatures in Nd0.5Sr0.5MnO3 and Nd0.5Ca0.5MnO3

The magnetization at low temperatures for Nd0.5Sr0.5MnO3 and Nd0.5Ca0.5MnO3 samples showed a rapid increase with decreasing temperatures, contrary to a La0.5Ca0.5MnO3 sample. Specific heat measurement at low temperatures showed a Schottky-like anomaly for the first two samples. However, there is not a straight forward correlation between the intrinsic magnetic moment of the Nd3+ ions and the Schottky-like anomaly.

cond-mat.str-el↗

arXiv2001

Unusual magnetic relaxation behavior in La0.5Ca0.5MnO3 and Nd0.5Sr0.5MnO3

We have carried out a systematic magnetic relaxation study, measured after applying and switching off a 5 T magnetic field to polycrystalline samples of La0.5Ca0.5MnO3 and Nd0.5Sr0.5MnO3. The long time logarithmic relaxation rate (LTLRR), decreased from 10 K to 150 K and increased from 150 K to 195 K in La0.5Ca0.5MnO3. This change in behavior was found to be related to the complete suppression of the antiferromagnetic phase above 150 K and in the presence of a 5 T magnetic field. At 195 K, the magnetization first decreased, and after a few minutes increased slowly as a function of time. Moreover, between 200 K and 245 K, the magnetization increased throughout the measured time span. The change in the slope of the curves, from negative to positive at about 200 K was found to be related to the suppression of antiferromagnetic fluctuations in small magnetic fields. A similar temperature dependence of the LTLRR was found for the Nd0.5Sr0.5MnO3 sample. However, the temperature where the LTLRR reached the minimum in Nd0.5Sr0.5MnO3 was lower than that of La0.5Ca0.5MnO3. This result agrees with the stronger ferromagnetic interactions that exist in Nd0.5Sr0.5MnO3 in comparison to La0.5Ca0.5MnO3. The above measurements suggested that the general temperature dependence of the LTLRR and the underlying physics were mainly independent of the particular charge ordering system considered. All relaxation curves could be fitted using a logarithmic law at long times. This slow relaxation was attributed to the coexistence of ferromagnetic and antiferromagnetic interactions between Mn ions, which produced a distribution of energy barriers.

cond-mat.str-el↗